The strong coupling between elementary excitations of the electromagnetic field (photons) and quantized mechanical vibrations (phonons) produces hybrid quasi-particle states, known as phonon-polaritons. Their typical signature is the avoided crossing between the eigenfrequencies of the coupled system, as paradigmatically illustrated by the Jaynes-Cummings Hamiltonian, and observed in quantum electrodynamics experiments where cavity photons are coupled to atoms, ions, excitons, spin ensambles and superconducting qubits. In this work, we demonstrate the generation of phonon-polaritons in the quantum motion of an optically-levitated nanosphere. The particle is trapped in high vacuum by an optical tweezer and strongly coupled to a single cavity mode by coherent scattering of the tweezer photons. The two-dimensional motion splits into two nearly-degenerate components that, together with the optical cavity mode, define an optomechanical system with three degrees-of-freedom. As such, when entering the strong coupling regime, we observe hybrid light-mechanical states with a dispersion law typical of tripartite quantum systems. Remarkably, the independent components of motion here identify a physical vibration direction on a plane that, similarly to the polarization of light, confers a vectorial nature to the polariton field. Our results pave the way to novel protocols for quantum information transfer between photonic and phononic components and represent a key-step towards the demonstration of optomechanical entangled states at room temperature.
We theoretically analyse the ground-state cooling of optically levitated nanosphere in unresolved- sideband regime by introducing a coupled high-quality-factor cavity. On account of the quantum interference stemming from the presence of the coupled cavity, the spectral density of the optical force exerting on the nanosphere gets changed and then the symmetry between the heating and the cooling processes is broken. Through adjusting the detuning of strong-dissipative cavity mode, one obtains an enhanced net cooling rate for the nanosphere. It is illustrated that the ground state cooling can be …
We explore entanglement generation between multiple optically levitated nanospheres interacting with a common optical cavity via the Coherent Scattering optomechanical interaction. We derive the many-particle Hamiltonian governing the unitary evolution of the system and show that it gives rise to quantum correlations among the various partitions of the setup, following a non-Markovian dynamics of entanglement birth, death and revivals. We also consider the effects of coupling the system to external environments and show that under reasonable experimental conditions entanglement between the mec…
We report on cooling the center-of-mass motion of a nanoparticle due to a purely quadratic coupling between its motion and the optical field of a high finesse cavity. The resulting interaction gives rise to a Van der Pol nonlinear damping, which is analogous to conventional parametric feedback where the cavity provides passive feedback without measurement. We show experimentally that like feedback cooling the resulting energy distribution is strongly nonthermal and can be controlled by the nonlinear damping of the cavity. As quadratic coupling has a prominent role in proposed protocols to gene…
Recently, remarkable advances have been made in coupling a number of high-Q modes of nano-mechanical systems to high-finesse optical cavities, with the goal of reaching regimes where quantum behavior can be observed and leveraged toward new applications. To reach this regime, the coupling between these systems and their thermal environments must be minimized. Here we propose a novel approach to this problem, in which optically levitating a nano-mechanical system can greatly reduce its thermal contact, while simultaneously eliminating dissipation arising from clamping. Through the long coherenc…
A phonon laser made from a levitated silica nanosphere held in a controllable optical trap offers a useful tool for studying phonon-photon interactions.
We theoretically investigate the effect of optical-force-mediated interactions onto the quantum dynamics of a pair of dielectric nanospheres optically trapped in two neighboring optical tweezers. Thanks to the interference between the tweezer beams and the elastically scattered light by the other nanosphere, the effective inter nanosphere coupling can reach the ultrastrong coupling regime. Experimentally accessible signatures of the entangled nature of the quantum ground state are highlighted, including entanglement witnesses based on position/momentum correlation functions and a sizable dynam…
Optomechanical cooling of levitated dielectric particles represents a promising new approach in the quest to cool small mechanical resonators towards their quantum ground state. We investigate two-mode cooling of levitated nanospheres in a self-trapping regime. We identify a rich structure of split sidebands (by a mechanism unrelated to usual strong-coupling effects) and strong cooling even when one mode is blue detuned. We show the best regimes occur when both optical fields cooperatively cool and trap the nanosphere, where cooling rates are over an order of magnitude faster compared to corre…
We report on the two-dimensional (2D) dynamics of a levitated nanoparticle in an optical cavity. The motion of the nanosphere is strongly coupled to the cavity field by coherent scattering and heavily cooled in the plane orthogonal to the tweezer axis. Due to the characteristics of the 2D motion and the strong optomechanical coupling, the motional sideband asymmetry that reveals the quantum nature of the dynamics is not limited to mere scale factors between Stokes and anti-Stokes peaks, as customary in quantum optomechanics, but assumes a peculiar spectral dependence. We introduce and discuss …
Collapse models postulate the existence of intrinsic noise which modifies quantum mechanics and is responsible for the emergence of macroscopic classicality. Assessing the validity of these models is extremely challenging because it is nontrivial to discriminate unambiguously their presence in experiments where other hardly controllable sources of noise compete to the overall decoherence. Here we provide a simple procedure able to probe the hypothetical presence of the collapse noise with a levitated nanosphere in a Fabry-Perot cavity. We show that the stationary state of the system is particu…
We report three-dimensional cooling of a levitated nanoparticle inside an optical cavity. The cooling mechanism is provided by cavity-enhanced coherent scattering off an optical tweezer. The observed 3D dynamics and cooling rates are as theoretically expected from the presence of both linear and quadratic terms in the interaction between the particle motion and the cavity field. By achieving nanometer-level control over the particle location we optimize the position-dependent coupling and demonstrate axial cooling by two orders of magnitude at background pressures as high as $6\times10^{-2}$ m…
In this paper we investigate cooling of a levitated nanosphere in a system of coupled cavities in the resolved sideband regime. Thanks to the presence of an extra resonance in the coupled cavity cooling system, the coupling strength can be maximized at the optimum detuning. In this fashion, the intra-cavity photon number is increased and thereby the cooling rate is enhanced and the strong coupling regime is achieved without resorting to increased driving laser power. The underlying physics of the increased cooling efficiency in the here-proposed system of coupled cavities in the resolved sideb…
The use of levitated nanospheres represents a new paradigm for the optomechanical cooling of a small mechanical oscillator, with the prospect of realising quantum oscillators with unprecedentedly high quality factors. We investigate the dynamics of this system, especially in the so-called self-trapping regimes, where one or more optical fields simultaneously trap and cool the mechanical oscillator. The determining characteristic of this regime is that both the mechanical frequency $ω_M$ and single-photon optomechanical coupling strength parameters $g$ are a function of the optical field intens…
We consider an array of optically levitated nanospheres in vacuum and investigate nontrivial phonon transports in this system. The levitated nanospheres are coupled by optical binding. Key parameters of this system, such as the interaction range, trapping frequencies and mechanical dissipation, are all highly tunable. By tuning the spacing between neighboring spheres, the mechanical dissipation and the trapping frequency of each sphere, counter-intuitive phenomena such as prethermalization and nonreciprocal phonon transport can be achieved. Our system provides a great platform to investigate n…
Einstein realised that the fluctuations of a Brownian particle can be used to ascertain properties of its environment. A large number of experiments have since exploited the Brownian motion of colloidal particles for studies of dissipative processes, providing insight into soft matter physics, and leading to applications from energy harvesting to medical imaging. Here we use optically levitated nanospheres that are heated to investigate the non-equilibrium properties of the gas surrounding them. Analysing the sphere's Brownian motion allows us to determine the temperature of the centre-of-mass…
We report on measurements of photon induced heating of silica nanospheres levitated in vacuum by a thermal light source formed by a superluminescent diode. Heating of the nanospheres motion along the three trap axes was measured as a function of gas pressure and for two particle sizes. Heating rates were also compared with the much lower reheating of the same sphere when levitated by a laser. We find the measured trap heating rates are dominated by the much larger heating rates expected from the recoil of thermal photons.
Levitated optomechanics is showing potential for precise force measurements. Here, we report a case study, to show experimentally the capacity of such a force sensor. Using an electric field as a tool to detect a Coulomb force applied onto a levitated nanosphere. We experimentally observe the spatial displacement of up to 6.6 nm of the levitated nanosphere by imposing a DC field. We further apply an AC field and demonstrate resonant enhancement of force sensing when a driving frequency, $ω_{AC}$, and the frequency of the levitated mechanical oscillator, $ω_0$, converge. We directly measure a f…
Optically trapped dielectric objects are well suited for reaching the quantum regime of their center of mass motion in an ultra-high vacuum environment. We show that ground state cooling of an optically trapped nanosphere is achievable when starting at room temperature, by sympathetic cooling of a cold atomic gas optically coupled to the nanoparticle. Unlike cavity cooling in the resolved sideband limit, this system requires only a modest cavity finesse and it allows the cooling to be turned off, permitting subsequent observation of strongly-coupled dynamics between the atoms and sphere. Nanos…
Position measurement of a levitated particle with vectorial light
Pontifical Catholic University of Rio de Janeiro（里约热内卢天主教大学）；Universidade Federal do Rio de Janeiro（里约热内卢联邦大学）；Tecnológico de Monterrey（蒙特雷理工学院）；University of Southampton（南安普顿大学）
Following the first demonstration of a levitated nanosphere cooled to the quantum ground state in 2020 [1], macroscopic quantum sensors are seemingly on the horizon. The nanosphere's large mass as compared to other quantum systems enhances the susceptibility of the nanoparticle to gravitational and inertial forces. In this viewpoint we describe the features of experiments with optically levitated nanoparticles [2] and their proposed utility for acceleration sensing. Unique to the levitated nanoparticle platform is the ability to implement not only quantum noise limited transduction, predicted …
With the purpose of controlling the steady state of a dielectric nanosphere levitated within an optical cavity, we study its conditional dynamics under simultaneous sideband cooling and additional time-continuous measurement of either the output cavity mode or the nanosphere's position. We find that the average phonon number, purity and quantum squeezing of the steady-states can all be made more non-classical through the addition of time-continuous measurement. We predict that the continuous monitoring of the system, together with Markovian feedback, allows one to stabilize the dynamics for an…
Optomechanical systems explore and exploit the coupling between light and the mechanical motion of matter. A nonlinear coupling offers access to rich new physics, in both the quantum and classical regimes. We investigate a dynamic, as opposed to the usually studied static, nonlinear optomechanical system, comprising of a nanosphere levitated and cooled in a hybrid electro-optical trap. An optical cavity offers readout of both linear-in-position and quadratic-in-position (nonlinear) light-matter coupling, whilst simultaneously cooling the nanosphere to millikelvin temperatures for indefinite pe…
We theoretically study the levitation of a single magnetic domain nanosphere in an external static magnetic field. We show that apart from the stability provided by the mechanical rotation of the nanomagnet (as in the classical Levitron), the quantum spin origin of its magnetization provides two additional mechanisms to stably levitate the system. Despite of the Earnshaw theorem, such stable phases are present even in the absence of mechanical rotation. For large magnetic fields, the Larmor precession of the quantum magnetic moment stabilizes the system in full analogy with magnetic trapping o…
Stationary entanglement of a levitated oscillator with an optical field
Università di Firenze（佛罗伦萨大学）；INFN, Sezione di Firenze（意大利国家核物理研究所佛罗伦萨分部）；CNR-INO（意大利国家研究委员会光学研究所）；European Laboratory for Non-Linear Spectroscopy (LENS)（欧洲非线性光谱学实验室）
Levitated nanospheres in optical cavities open a novel route to study many-body systems out of solution and highly isolated from the environment. We show that properly tuned optical parameters allow for the study of the non-equilibrium dynamics of composite nano-particles with non-isotropic optical friction. We find friction induced ordering and nematic transitions with non-equilibrium analogs to liquid crystal phases for ensembles of dimers.
We theoretically show that the dipole force of an ensemble of quantum emitters embedded in a dielectric nanosphere can be exploited to achieve near-field optical levitation. The key ingredient is that the polarizability from the ensemble of embedded quantum emitters can be larger than the bulk polarizability of the sphere, thereby enabling the use of repulsive optical potentials and consequently the levitation using optical near-fields. In levitated cavity quantum optomechanics, this could be used to boost the single-photon coupling by combining larger polarizability to mass ratio, larger fiel…
The strong light-matter optomechanical coupling offered by Coherent Scattering (CS) set-ups have allowed the experimental realisation of quantum ground state cavity cooling of the axial motion of a levitated nanoparticle [U. Delić et al., Science 367, 892 (2020)]. An appealing milestone is now quantum 2D cooling of the full in-plane motion, in any direction in the transverse plane. By a simple adjustment of the trap polarisation, one obtains two nearly equivalent modes, with similar frequencies $ω_{x}\simω_{y}$ and optomechanical couplings $g_{x}\simeq g_{y}$ -- in this experimental configurat…
Single-atom detection with a quantum-controlled mechanical oscillator
ETH Zürich（苏黎世联邦理工学院）；Photonics Laboratory, ETH Zürich（苏黎世联邦理工学院光子学实验室）；Quantum Center, ETH Zürich（苏黎世联邦理工学院量子中心）；Laboratory of Physical Chemistry, ETH Zürich（苏黎世联邦理工学院物理化学实验室）；Kavli Institute of Nanoscience, Department of Quantum Nanoscience, TU Delft（代尔夫特理工大学量子纳米科学系卡弗里纳米科学研究所）
We study entanglement of the motional degrees of freedom of two tethered and optically trapped microdisks inside a single cavity. By properly choosing the position of the trapped objects in the optical cavity and driving proper modes of the cavity it is possible to equip the system with linear and quadratic optomechanical couplings. We show that a parametric coupling between the fundamental vibrational modes of two tethered mircodiscs can be generated via a time modulated input laser. For a proper choice of the modulation frequency, this mechanism can drive the motion of the microdisks into an…
Nanoparticles levitated in vacuum can be set to spin at ultimate frequencies, limited only by the tensile strength of the material. At such high frequencies, drastic changes to the dynamics of solid-state quantum excitations are to be expected. Here, we theoretically describe the interaction between acoustic phonons and the rotation of a nanoparticle around its own axis, and model how the acoustic and optical properties of the nanoparticle change when it rotates at a fixed frequency. As an example, we analytically predict the scaling of the shape, the acoustic eigenmode spectrum, the permittiv…
