We theoretically show that the dipole force of an ensemble of quantum emitters embedded in a dielectric nanosphere can be exploited to achieve near-field optical levitation. The key ingredient is that the polarizability from the ensemble of embedded quantum emitters can be larger than the bulk polarizability of the sphere, thereby enabling the use of repulsive optical potentials and consequently the levitation using optical near-fields. In levitated cavity quantum optomechanics, this could be used to boost the single-photon coupling by combining larger polarizability to mass ratio, larger field gradients, and smaller cavity volumes while remaining in the resolved sideband regime and at room temperature. A case study is done with a nanodiamond containing a high-density of silicon-vacancy color centers that is optically levitated in the evanescent field of a tappered nano-fiber and coupled to a high-finesse microsphere cavity.
Electron spins of diamond nitrogen-vacancy (NV) centers are important quantum resources for nanoscale sensing and quantum information. Combining NV spins with levitated optomechanical resonators will provide a hybrid quantum system for novel applications. Here we optically levitate a nanodiamond and demonstrate electron spin control of its built-in NV centers in low vacuum. We observe that the strength of electron spin resonance (ESR) is enhanced when the air pressure is reduced. To better understand this system, we investigate the effects of trap power and measure the absolute internal temper…
We propose a scheme to realize universal quantum gates between nitrogen-vacancy (NV) centers in an optically trapped nanodiamond, through uniform magnetic field induced coupling between the NV centers and the torsional mode of the levitated nanodiamond. The gates are tolerant to the thermal noise of the torsional mode. By combining the scheme with dynamical decoupling technology, it is found that the high fidelity quantum gates are possible for the present experimental conditions. The proposed scheme is useful for NV-center-based quantum network and distributed quantum computation
Using the spin properties of nitrogen-vacancy (NV) centers in levitated diamond, we characterize the absorption of single nanodiamonds. We first calibrate the thermometry response of the NV centers embedded in our nanodiamonds. Then, using this calibration, we estimate the absorption cross-section of single levitated nanodiamonds. We show that this absorption is extrinsic and dominated by volumic effects. Our work opens the way to diamond materials optimization for levitation quantum experiments. It also demonstrates optical levitation as a unique platform to characterize material thermal prop…
There is significant interest in potential experimental tests of macroscopic quantum effects, both to test potential modifications to quantum theory and to probe the quantum nature of gravity. A proposed platform with which to generate the required macroscopic quantum spatial superposition is a nanodiamond containing a negatively charged nitrogen vacancy (${\text{NV}}^{-}$) centre. In this review, methods to fabricate nanodiamonds containing ${\text{NV}}^{-}$ suitable for these quantum applications are discussed. The proposed probes of the macroscopic limits of quantum theory are presented alo…
We propose a method to generate and detect large quantum superposition states and arbitrary Fock states for the oscillational mode of an optically levitated nanocrystal diamond. The nonlinear interaction required for the generation of non-Gaussian quantum states is enabled through the spin-mechanical coupling with a built-in nitrogen-vacancy center inside the nanodiamond. The proposed method allows the generation of large superpositions of nanoparticles with millions of atoms and the observation of the associated spatial quantum interference under reasonable experimental conditions.
The Brownian motion of a particle hotter than its environment is an iconic out-of-equilibrium system. Its study provides valuable insights into nanoscale thermal effects. Notably, it supplies an excellent diagnosis of thermal effects in optically levitated particles, a promising platform for force sensing and quantum physics tests. Thus, understanding the relevant parameters in this effect is critical. In this context, we test the role of particles' shape and material, using optically levitated nanodiamonds hosting NV centers to measure the particles' internal temperature and center-of-mass dy…
Hybrid spin-mechanical systems have great potentials in sensing, macroscopic quantum mechanics, and quantum information science. In order to induce strong coupling between an electron spin and the center-of-mass motion of a mechanical oscillator, a large magnetic gradient is usually required, which is difficult to achieve. Here we show that strong coupling between the electron spin of a nitrogen-vacancy (NV) center and the torsional vibration of an optically levitated nanodiamond can be achieved in a uniform magnetic field. Thanks to the uniform magnetic field, multiple spins can strongly coup…
We present the first evidence of nitrogen vacancy (NV) photoluminescence from a nanodiamond suspended in a free-space optical dipole trap at atmospheric pressure. The photoluminescence rates are shown to decrease with increasing trap laser power, but are inconsistent with a thermal quenching process. For a continuous-wave trap, the neutral charge state (NV$^0$) appears to be suppressed. Chopping the trap laser yields higher total count rates and results in a mixture of both NV$^0$ and the negative charge state (NV$^-$).
Nonclassical states of macroscopic objects are promising for ultrasensitive metrology as well as testing quantum mechanics. In this work, we investigate dissipative mechanical quantum state engineering in an optically levitated nanodiamond. First, we study single-mode mechanical squeezed states by magnetically coupling the mechanical motion to a dressed three-level system provided by a Nitrogen-vacancy center in the nanoparticle. Quantum coherence between the dressed levels is created via microwave fields to induce a two-phonon transition, which results in mechanical squeezing. Remarkably, we …
Levitated nanospheres in optical cavities open a novel route to study many-body systems out of solution and highly isolated from the environment. We show that properly tuned optical parameters allow for the study of the non-equilibrium dynamics of composite nano-particles with non-isotropic optical friction. We find friction induced ordering and nematic transitions with non-equilibrium analogs to liquid crystal phases for ensembles of dimers.
In recent years quantum phenomena have been experimentally demonstrated on variety of optomechanical systems ranging from micro-oscillators to photonic crystals. Since single photon couplings are quite small, most experimental approaches rely on the realization of high finesse Fabry-Perot cavities in order to enhance the effective coupling. Here we show that by exploiting a, long path, low finesse fiber Fabry-Perot interferometer ground state cooling can be achieved. We model a 100 m long cavity with a finesse of 10 and analyze the impact of additional noise sources arising from the fiber. As …
We consider feedback cooling in a cavityless levitated optomechanics setup, and we investigate the possibility to improve the feedback implementation. We apply optimal control theory to derive the optimal feedback signal both for quadratic (parametric) and linear (electric) feedback. We numerically compare optimal feedback against the typical feedback implementation used for experiments. In order to do so, we implement a tracking scheme that takes into account the modulation of the laser intensity. We show that such a tracking implementation allows us to increase the feedback strength, leading…
We theoretically explore a quantum memory using a single nanoparticle levitated in an optical dipole trap and subjected to feedback cooling. This protocol is realized by storing and retrieving a single photon quantum state from a mechanical mode in levitated cavityless optomechanics. We describe the effectiveness of the photon-phonon-photon transfer in terms of the fidelity, the Wigner function, and the zero-delay second-order autocorrelation function. For experimentally accessible parameters, our numerical results indicate robust conversion of the quantum states of the input signal photon to …
Optomechanical cooling of levitated dielectric particles represents a promising new approach in the quest to cool small mechanical resonators towards their quantum ground state. We investigate two-mode cooling of levitated nanospheres in a self-trapping regime. We identify a rich structure of split sidebands (by a mechanism unrelated to usual strong-coupling effects) and strong cooling even when one mode is blue detuned. We show the best regimes occur when both optical fields cooperatively cool and trap the nanosphere, where cooling rates are over an order of magnitude faster compared to corre…
An optically levitated nanoparticle in vacuum is a paradigm optomechanical system for sensing and studying macroscopic quantum mechanics. While its center-of-mass motion has been investigated intensively, its torsional vibration has only been studied theoretically in limited cases. Here we report the first experimental observation of the torsional vibration of an optically levitated nonspherical nanoparticle in vacuum. We achieve this by utilizing the coupling between the spin angular momentum of photons and the torsional vibration of a nonspherical nanoparticle whose polarizability is a tenso…
Optically levitated nanodiamonds with nitrogen-vacancy centers promise a high-quality hybrid spin-optomechanical system. However, the trapped nanodiamond absorbs energy form laser beams and causes thermal damage in vacuum. We propose to solve the problem by trapping a composite particle (a nanodiamond core coated with a less absorptive silica shell) at the center of strongly focused doughnut-shaped laser beams. Systematical study on the trapping stability, heat absorption, and oscillation frequency concludes that the azimuthally polarized Gaussian beam and the linearly polarized Laguerre-Gauss…
Nonclassical optomechanical correlations enable optical control of mechanical motion beyond the limitations of classical driving. Here we investigate the feasibility of using pulsed cavity-optomechanics to create and verify nonclassical phase-sensitive correlations between light and the motion of a levitated nanoparticle in a realistic scenario. We show that optomechanical two-mode squeezing can persist even at the elevated temperatures of state-of-the-art experimental setups. We introduce a detection scheme based on optical homodyning that allows revealing nonclassical correlations without fu…
We demonstrate a technique to estimate the strength of non-linearities present in the trapping potential of an optically levitated nanoparticle. By applying a brief pulsed reduction in trapping laser power of the system such as to squeeze the phase space distribution and then matching the time evolution of the shape of the phase space distribution to that of numerical simulations, one can estimate the strength of the non-linearity present in the system. We apply this technique to estimate the strength of the Duffing non-linearity present in the optical trapping potential.
Sympathetic Cooling of Levitated Optomechanics through Nonreciprocal Coupling
Center for Quantum Technology Research and Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurements (MOE), School of Physics, Beijing Institute of Technology（北京理工大学物理学院量子技术研究中心及先进光电子量子架构与测量教育部重点实验室）
We demonstrate the reconstruction of the Wigner function from marginal distributions of the motion of a single trapped particle using homodyne detection. We show that it is possible to generate quantum states of levitated optomechanical systems even under the effect of continuous measurement by the trapping laser light. We describe the opto-mechanical coupling for the case of the particle trapped by a free-space focused laser beam, explicitly for the case without an optical cavity. We use the scheme to reconstruct the Wigner function of experimental data in perfect agreement with the expected …
We investigate experimentally the dynamics of a non-spherical levitated nanoparticle in vacuum. In addition to translation and rotation motion, we observe the light torque-induced precession and nutation of the trapped particle. We provide a theoretical model, which we numerically simulate and from which we derive approximate expressions for the motional frequencies. Both, the simulation and approximate expressions, we find in good agreement with experiments. We measure a torque of $1.9 \pm 0.5 \times 10^{-23}$ Nm at $1 \times 10^{-1}$ mbar, with an estimated torque sensitivity of $3.6 \pm 1.1…
We discuss the detection of an anisotropic particle trapped by an elliptically polarized focused Gaussian laser beam. We obtain the full rotational and translational dynamics, as well as, the measured photo-current in a general-dyne detection. As an example, we discuss a toy model of homodyne detection, which captures the main features typically found in experimental setups.
We describe how to prepare an electrically levitated nanodiamond in a superposition of orientations via microwave driving of a single embedded nitrogen-vacancy (NV) center. Suitably aligning the magnetic field with the NV center can serve to reach the regime of ultrastrong coupling between the NV and the diamond rotation, enabling single-spin control of the particle's three-dimensional orientation. We derive the effective spin-oscillator Hamiltonian for small amplitude rotation about the equilibrium configuration and develop a protocol to create and observe quantum superpositions of the partic…
We report on cooling the center-of-mass motion of a nanoparticle due to a purely quadratic coupling between its motion and the optical field of a high finesse cavity. The resulting interaction gives rise to a Van der Pol nonlinear damping, which is analogous to conventional parametric feedback where the cavity provides passive feedback without measurement. We show experimentally that like feedback cooling the resulting energy distribution is strongly nonthermal and can be controlled by the nonlinear damping of the cavity. As quadratic coupling has a prominent role in proposed protocols to gene…
We demonstrate a classical analogy to the Fano anti-resonance in levitated optomechanics by applying a DC electric field. Specifically, we experimentally tune the Fano parameter by applying a DC voltage from 0~kV to 10~kV on a nearby charged needle tip. We find consistent results across negative and positive needle voltages, with the Fano line-shape feature able to exist at both higher and lower frequencies than the fundamental oscillator frequency. We can use the Fano parameter to characterize our system to be sensitive to static interactions which are ever-present. Currently, we can distingu…
Ultra-high sensitivity detection of quantum-scale displacements in cavity optomechanics optimises the combined errors from measurement back-action and imprecisions from incoming quantum noises. This sets the well-known Standard Quantum Limit (SQL). Normal quantum cavity optomechanics allows cooling and detection of a single degree of freedom, along the cavity axis. However, a recent breakthrough that allows quantum ground-state cooling of levitated nanoparticles [Delic et al, arxiv:1911.04406], is uniquely 3D in character, with coupling along the $x$, $y$ and $z$ axes. We investigate current e…
Cavity optomechanics offers quantum cooling, quantum control and measurement of small mechanical oscillators. However the optical backactions that underpin quantum control can significantly disturb the oscillator modes: mechanical frequencies are shifted by the optical spring effect and light-matter hybridisation in strong coupling regimes; mechanical modes hybridise with each other via the cavity mode. This is even more pertinent in the field of levitated optomechanics, where optical trapping fully determines the mechanical modes and their frequencies. Here, using the coherent-scattering (CS)…
We analyze magnetometry using an optically levitated nanodiamond. We consider a configuration where a magnetic field gradient couples the mechanical oscillation of the diamond with its spin degree of freedom provided by a Nitrogen vacancy center. First, we investigate measurement of the position spectrum of the mechanical oscillator. We find that conditions of ultrahigh vacuum and feedback cooling allow a magnetic field gradient sensitivity of 1 $μ$Tm$^{-1}$/$\sqrt{\mbox{Hz}}$. At high pressure and room temperature, this sensitivity degrades and can attain a value of the order of 100 $m$Tm$^{-…
Levitated optomechanical systems are rapidly becoming leading tools for precision sensing, enabling a high level of control over the sensor's center of mass motion, rotation and electric charge state. Higher-order multipole moments in the charge distribution, however, remain a major source of backgrounds. By applying controlled precessive torques to the dipole moment of a levitated microsphere in vacuum, we demonstrate cancellation of dipole-induced backgrounds by 2 orders of magnitude. We measure the dipole moments of ng-mass spheres and determine their scaling with sphere size, finding that …
Particles with electric charge 10^(-12)e in bulk mass are not excluded by present experiments. In the present letter we provide a feasible scheme to measure the millicharged particles via the optical cavity coupled to a levitated microsphere. The results show that the optical probe spectrum of the micro-oscillator presents a distinct shift due to the existence of millicharged particles. Owing to the very narrow linewidth(10^(-7) Hz) of the optical Kerr effect, this shift will be more obvious, which makes the millicharges more easy to be detectable. We propose a method to eliminate the polariza…
Levitated nanodiamonds containing nitrogen vacancy centres in high vacuum are a potential test bed for numerous phenomena in fundamental physics. However, experiments so far have been limited to low vacuum due to heating arising from optical absorption of the trapping laser. We show that milling pure diamond creates nanodiamonds that do not heat up as the optical intensity is raised above 700 GW/m$^2$ below 5 mbar of pressure. This advance now means that the level of attainable vacuum for nanodiamonds in optical dipole traps is no longer temperature limited.
Counterintuitively, experiments show that an electromagnetically levitated particle escapes from its trap when the ambient pressure is reduced below a certain level even if the particle's motion is cooled by a resonator-based or feedback-based mechanism. Here, we theoretically show that the ambient pressure must be kept well above a critical value arising from gradient force fluctuations (viz., fluctuations in part of the EM force whose Hamiltonian is quadratic in the position of the particle). Also, we consider other force fluctuations, and determine whether different realizations of feedback…
Quantum control of levitated dielectric particles is an emerging subject in quantum optomechanics. A major challenge is to efficiently measure and manipulate the particle's motion at the Heisenberg uncertainty limit. Here we present a nanophotonic interface suited to address this problem. By optically trapping a 150 nm silica particle and placing it in the near field of a photonic crystal cavity, we achieve tunable single-photon optomechanical coupling of up to $g_0/2π=9$ kHz, three orders of magnitude larger than previously reported for levitated cavity optomechanical systems. Efficient colle…
The strong light-matter optomechanical coupling offered by Coherent Scattering (CS) set-ups have allowed the experimental realisation of quantum ground state cavity cooling of the axial motion of a levitated nanoparticle [U. Delić et al., Science 367, 892 (2020)]. An appealing milestone is now quantum 2D cooling of the full in-plane motion, in any direction in the transverse plane. By a simple adjustment of the trap polarisation, one obtains two nearly equivalent modes, with similar frequencies $ω_{x}\simω_{y}$ and optomechanical couplings $g_{x}\simeq g_{y}$ -- in this experimental configurat…
Optically trapped dielectric objects are well suited for reaching the quantum regime of their center of mass motion in an ultra-high vacuum environment. We show that ground state cooling of an optically trapped nanosphere is achievable when starting at room temperature, by sympathetic cooling of a cold atomic gas optically coupled to the nanoparticle. Unlike cavity cooling in the resolved sideband limit, this system requires only a modest cavity finesse and it allows the cooling to be turned off, permitting subsequent observation of strongly-coupled dynamics between the atoms and sphere. Nanos…
We experimentally squeeze the thermal motional state of an optically levitated nanosphere, by fast switching between two trapping frequencies. The measured phase space distribution of our particle shows the typical shape of a squeezed thermal state, from which we infer up to 2.7dB of squeezing along one motional direction. The experiment features a large number of thermal excitations, therefore remaining in the classical regime. Nevertheless, we argue that the manipulation scheme described here could be used to achieve squeezing below the zero-point level, if preceded by ground state cooling o…
Recently, remarkable advances have been made in coupling a number of high-Q modes of nano-mechanical systems to high-finesse optical cavities, with the goal of reaching regimes where quantum behavior can be observed and leveraged toward new applications. To reach this regime, the coupling between these systems and their thermal environments must be minimized. Here we propose a novel approach to this problem, in which optically levitating a nano-mechanical system can greatly reduce its thermal contact, while simultaneously eliminating dissipation arising from clamping. Through the long coherenc…
We theoretically investigate the rigid body dynamics of an optically levitated nanodumbbell under parametric feedback cooling and provide a simplified model for describing the motion. Differing from previous studies, the spin of the nanoparticle about its symmetry axis is considered non-negligible. Simulations reveal that standard parametric feedback cooling can extract energy from two of the five rotational degrees of freedom when the nanoparticle is levitated using a linearly polarized laser beam. The dynamics after feedback cooling are characterized by a normal mode describing precession ab…
Levitated nanoparticles are being intensively investigated from two different perspectives: as a potential realisation of macroscopic quantum coherence; and as ultra-sensitive sensors of force, down to the zeptoNewton level, with a range of various applications, including the search for Dark Matter. A future aim is to merge these two strands, enabling the development of quantum-limited sensors. Here we propose that mechanical cross-correlation spectra $S_{xy}(ω)$ offer new possibilities: once detector misalignment errors are minimised, the spectral shape of $S_{xy}(ω)$ directly points out the …
Optomechanical systems explore and exploit the coupling between light and the mechanical motion of matter. A nonlinear coupling offers access to rich new physics, in both the quantum and classical regimes. We investigate a dynamic, as opposed to the usually studied static, nonlinear optomechanical system, comprising of a nanosphere levitated and cooled in a hybrid electro-optical trap. An optical cavity offers readout of both linear-in-position and quadratic-in-position (nonlinear) light-matter coupling, whilst simultaneously cooling the nanosphere to millikelvin temperatures for indefinite pe…
Optical levitation of nanoscale particles has emerged as a platform for precision measurement. Extremely low damping, together with optical interferometric position detection, makes possible exquisite force measurement and promises low-energy tests of fundamental physics. Essential to such measurement is an understanding of the confidence with which parameters can be inferred from spectra estimated from the indirect measurement provided by interferometry. We present an apparatus optimized for sensitivity along one motional degree of freedom, a theoretical model of the spectrum, and maximum lik…
Stationary entanglement of a levitated oscillator with an optical field
Università di Firenze（佛罗伦萨大学）；INFN, Sezione di Firenze（意大利国家核物理研究所佛罗伦萨分部）；CNR-INO（意大利国家研究委员会光学研究所）；European Laboratory for Non-Linear Spectroscopy (LENS)（欧洲非线性光谱学实验室）
We demonstrate a simple and robust geometry for optical trapping in vacuum of a single nanoparticle based on a parabolic mirror and the optical gradient force, and we demonstrate rapid parametric feedback cooling of all three motional degrees of freedom from room temperature to a few mK. A single laser at 1550nm, and a single photodiode, are used for trapping, position detection, and cooling for all three dimensions. Particles with diameters from 26nm to 160nm are trapped without feedback to 10$^{-5}$mbar and with feedback engaged the pressure is reduced to 10$^{-6}$mbar. Modifications to the …
We describe a proposal for a new type of optomechanical system based on a drop of liquid helium that is magnetically levitated in vacuum. In the proposed device, the drop would serve three roles: its optical whispering gallery modes would provide the optical cavity, its surface vibrations would constitute the mechanical element, and evaporation of He atoms from its surface would provide continuous refrigeration. We analyze the feasibility of such a system in light of previous experimental demonstrations of its essential components: magnetic levitation of mm-scale and cm-scale drops of liquid H…
A pertinent question in cavity optomechanics is whether reaching the regime of large single-photon cooperativity, where the single-photon coupling rate exceeds the geometric mean of the cavity and mechanical decay rates, can enable any new phenomena. We show that in some multimode optomechanical systems, the single-photon cooperativity can indeed be a figure of merit. We first study a system with one cavity mode and two mechanical oscillators which combines the concepts of levitated optomechanics and coherent scattering with standard dispersive optomechanics. Later, we study a more complicated…
