We show that under the effect of an external electric field and a gradient of chemical potential, a topological electric current can be induced in Weyl semimetals without inversion and mirror symmetries. We derive analytic expressions for the nonlinear conductivity tensor and show that it is nearly quantized for small tilting when the Fermi levels are close to the Weyl nodes. When the van Hove point is much larger than the largest Fermi level, the band structure is described by two linearly dispersing Weyl fermions with opposite chirality. In this case, the electrochemical response is fully quantized in terms of fundamental constants and the scattering time, and it can be used to measure directly the topological charge of Weyl points. We show that the electrochemical chiral current may be derived from an electromagnetic action similar to axion electrodynamics, where the position-dependent chiral Fermi level plays the role of the axion field. This posits our results as a direct consequence of the chiral anomaly.
We study longitudinal transport in Weyl semimetal nanowires, both in the absence and in the presence of a magnetic flux threading the nanowires. We identify two qualitatively different regimes of transport with respect to the chemical potential in the nanowires. In the "surface regime", for low doping, most of the conductance occurs through the Fermi-arc surface states, and it rises in steps of one quantum of conductance as a function of the chemical potential; furthermore, with varying flux the conductance changes in steps of one quantum of conductance with characteristic Fabry-Pérot interfer…
We study the time-development processes of spin and charge transport phenomena in a topological Dirac semimetal attached to a ferromagnetic insulator with a precessing magnetization. Compared to conventional normal metals, topological Dirac semimetals manifest a large inverse spin Hall effect when a spin current is pumped from the attached ferromagnetic insulator. It is shown that the induced charge current is semi-quantized, i.e., it depends only on the distance between the two Dirac points in momentum space and hardly depends on the disorder strength when the system remains in the topologica…
Real-time evolution and charge pumping in magnetic Weyl semimetals are studied by solving the time-dependent Schrödinger equations. In the adiabatic limit of the real-time evolution, we show that the total pumped charge is quantized in the magnetic Weyl semimetals as in the quantum Hall system although the Weyl semimetal has no bulk gap. We examine how the disorder affects the charge pumping. As a result, we show that the quantized pumped charge is robust against the small disorder and find that the pumped charge increases in the intermediate disorder region. We also examine the doping effects…
Floquet engineering, the concept of tailoring a system by a periodic drive, is increasingly exploited to design and manipulate topological phases of matter. In this work, we study periodically driven higher-order topological Dirac semimetals associated with a $k$-dependent quantized quadrupole moment by applying circularly polarized light. The undriven Dirac semimetals feature gapless higher-order hinge Fermi arc states which are the consequence of the higher-order topology of the Dirac nodes. Floquet Weyl semimetal phases with hybrid-order topology, characterized by both a $k$-dependent quant…
Thermoelectrics are promising by directly generating electricity from waste heat. However, (sub-)room-temperature thermoelectrics have been a long-standing challenge due to vanishing electronic entropy at low temperatures. Topological materials offer a new avenue for energy harvesting applications. Recent theories predicted that topological semimetals at the quantum limit can lead to a large, non-saturating thermopower and a quantized thermoelectric Hall conductivity approaching a universal value. Here, we experimentally demonstrate the non-saturating thermopower and quantized thermoelectric H…
Weyl semimetals expand research on topologically protected transport by adding bulk Berry monopoles with linearly dispersing electronic states and topologically robust, gapless surface Fermi arcs terminating on bulk node projections. Here, we show how the Nernst effect, combining entropy with charge transport, gives a unique signature for the presence of Dirac bands. The Nernst thermopower of NbP (maximum of 800 microV K-1 at 9 T, 109 K) exceeds its conventional thermopower by a hundredfold and is significantly larger than the thermopower of traditional thermoelectric materials. The Nernst eff…
Exploration of the novel relationship between magnetic order and topological semimetals has received enormous interest in a wide range of both fundamental and applied research. Here we predict that soft ferromagnetic (FM) material EuB6 can achieve multiple topological semimetal phases by simply tuning the direction of the magnetic moment. Explicitly, EuB6 is a topological nodal-line semimetal when the moment is aligned along the [001] direction, and it evolves into a Weyl semimetal with three pairs of Weyl nodes by rotating the moment to the [111] direction. Interestingly, we identify a novel …
The recently discovered topological Dirac semimetal represents a new exotic quantum state of matter. Topological Dirac semimetals can be viewed as three dimensional analogues of graphene, in which the Dirac nodes are protected by crystalline symmetry. It has been found that quantum confinement effect can gap out Dirac nodes and convert Dirac semimetal to a band insulator. The band insulator is either normal insulator or quantum spin Hall insulator depending on the thin film thickness. We present the study of disorder effects in thin film of Dirac semimetals. It is found that moderate Anderson …
So far, the circular photogalvanic effect (CPGE) is the only possible quantized signal in Weyl semimetals. With inversion and mirror symmetries broken, Weyl and multifold fermions in band structures with opposite chiralities can stay at different energies and generate a net topological charge. Such kind of net topological charge can present as a quantized signal in the circular polarized light induced injection current. According to current theoretical understanding, RhSi and its counterparts are believed to be the most promising candidate for the experimental observation of the quantized CPGE…
Nodal-Line Semimetals with Non-Quantized Berry Phase
Nanjing University（南京大学）；National Laboratory of Solid State Microstructures, School of Physics, and Collaborative Innovation Center of Advanced Microstructures, Nanjing University（南京大学固体微结构物理国家重点实验室、物理学院和先进微结构协同创新中心）；Jiangsu Physical Science Research Center and Jiangsu Key Laboratory of Quantum Information Science and Technology, Nanjing University（南京大学江苏物理科学研究中心和江苏省量子信息科学与技术重点实验室）
When two lasers are applied to a non-centrosymmetric material, light can be generated at the difference of the incoming frequencies $Δω$, a phenomenon known as difference frequency generation (DFG), well characterized in semiconductors. In this work, we derive a general expression for DFG in metals, which we use to show that the DFG in chiral topological semimetals under circular polarized light is quantized in units of $e^3/h^2$ and independent of material parameters, including the scattering time $τ$, when $Δω\gg τ^{-1}$. In this regime, DFG provides a simpler alternative to measure a quanti…
We propose the creation of a two-dimensional topological semimetal in a semiconductor artificial lattice with triangular symmetry. An in-plane magnetic field drives a quantum phase transition between the topological insulating and topological semimetal phases. The topological semimetal is characterized by robust band touching points which carry quantized Berry flux and edge states which terminate at the band touching points. The topological phase transition is predicted to occur at magnetic fields $\sim 4\text{T}$ in high mobility GaAs artificial lattices, and can be detected via the anomalous…
Considering a non-centrosymmetric, non-magnetic double Weyl semimetal (WSM) SrSi$_2$, we investigate the electron and hole pockets in bulk Fermi surface behavior that enables us to characterize the material as a type-I WSM. We study the structural handedness of the material and correlate it with the distinct surface Fermi surface at two opposite surfaces following an energy evolution. The Fermi arc singlet becomes doublet with the onset of spin orbit coupling that is in accordance with the topological charge of the Weyl Nodes (WNs). A finite energy separation between WNs of opposite chirality …
Simulating multi-node Weyl semimetals in a Mixed Floquet lattice
Indian Institute of Science Education and Research (IISER) Tirupati（印度科学教育研究所提鲁帕蒂分校）；Indian Institute of Science Education and Research Bhopal（印度科学教育研究所博帕尔分校）
Quantized Conductance through Surface States in High Quality Three-Dimensional Dirac Semimetal Cd$_3$As$_2$ Nanowire/Nanoribbon p-n Junctions
DGIST Research Institute, DGIST（大邱科学技术院研究学院）；Electrical and Computer Engineering, National University of Singapore（新加坡国立大学电气与计算机工程系）；Department of Physics, KTH Royal Institute of Technology（皇家理工学院物理系）；Industrial AX Innovation Research Institute and Sensor Technology Support Center, DGIST（大邱科学技术院工业AX创新研究所及传感器技术支持中心）；Department of Advanced Materials Chemistry, Korea University（韩国大学先进材料化学系）；Department of Physics and Chemistry, DGIST（大邱科学技术院物理化学系）；Department of Interdisciplinary Engineering, DGIST（大邱科学技术院交叉工程学系）；Institute of next generation semiconductor technology (INST), DGIST（大邱科学技术院下一代半导体技术研究所）
We develop a semiclassical theory of sound absorption in Weyl semimetals in magnetic fields. We focus on the contribution to the absorption that stems from the existence of Berry monopoles in the band structure of such materials, or, equivalently, due to the chiral anomaly and chiral magnetic effect. Sound absorption is shown to come primarily from the motion of Weyl nodes in energy space, associated with the propagation of a sound wave. We argue that acoustic magneto-chiral dichroism, which occurs when absorption of sound is different for opposite propagation directions, and for opposite dire…
Weyl semimetals are a new paradigmatic topological phase of matter featuring a gapless spectrum. One of its most distinctive features is the presence of Fermi arc surface states. Here, we report on atomistic simulations of the dc conductance and quantum Hall response of a minimal Weyl semimetal. By using scattering theory we show that a quantized Hall conductance with a non-vanishing longitudinal conductance emerges associated to the Fermi arc surface states with a remarkable robustness to high concentrations of defects in the system. Additionally, we predict that a slab of a Weyl semimetal wi…
Exotic topological states of matter such as Floquet topological insulator or Floquet Weyl semimetal can be induced by periodic driving. This work proposes a Floquet semimetal with Floquet-band holonomy. That is, the system is gapless, but as a periodic parameter viewed as quasimomentum of a synthetic dimension completes an adiabatic cycle, each Floquet band as a whole exchanges with other Floquet bands. The dynamical manifestations of such Floquet-band holonomy are studied. Under open boundary conditions, we discover anomalous chiral edge modes localized only at one edge, winding around the en…
We study the cyclotron resonance in the electron-hole joint Fermi surface of a type-II Weyl semimetal. In magnetic field, the electron and hole pockets touching at the Weyl node are hybridized to form quantized Landau levels corresponding to semiclassical 8-shaped orbits. We calculate the dynamical conductivities for the electric fields oscillating in $x$ and $y$-directions and find that the resonant frequencies in $x$ and $y$ differ by the factor of two, reflecting to the figure-of-eight electron motion in the real space. The peculiar anisotropy in the cyclotron resonance serves as a unique c…
We demonstrate that topological transport phenomena, characteristic of Weyl semimetals, namely the semi-quantized anomalous Hall effect and the chiral magnetic effect (equilibrium magnetic-field-driven current), may be thought of as two distinct manifestations of the same underlying phenomenon, the chiral anomaly. We show that the topological response in Weyl semimetals is fully described by a $θ$-term in the action for the electromagnetic field, where $θ$ is not a constant parameter, like e.g. in topological insulators, but is a field, which has a linear dependence on the space-time coordinat…
We propose a simple realization of the three-dimensional (3D) Weyl semimetal phase, utilizing a multilayer structure, composed of identical thin films of a magnetically-doped 3D topological insulator (TI), separated by ordinary-insulator spacer layers. We show that the phase diagram of this system contains a Weyl semimetal phase of the simplest possible kind, with only two Dirac nodes of opposite chirality, separated in momentum space, in its bandstructure. This particular type of Weyl semimetal has a finite anomalous Hall conductivity, chiral edge states, and occurs as an intermediate phase b…
We investigate the potential of the surface states of 3D nodal-line semimetals to produce surface and 3D quantized Hall effects in which the electronic currents flow unidirectionally along the surface of the material. This phenomenology is based on the fact that, irrespective of its orientation, a strong magnetic field gives rise to a zero Landau level with huge 2D degeneracy of states in the nodal-line semimetal. When the magnetic field is perpendicular to the plane of the nodal line, we show that the evanescent states within the nodal ring are transmuted into Landau surface states which corr…
The half-quantized Hall conductance is characteristic of quantum systems with parity anomaly. Here we investigate topological and transport properties of a class of parity anomalous semimetals, in which massive Dirac fermions coexist with massless Dirac fermions in momentum space or real space, and uncovered a distinct bulk-edge correspondence that the half-quantized Hall effect is realized via the bulk massless Dirac fermions while the nontrivial Berry curvature is provided by the massive Dirac fermions. The spatial distribution of the edge current decays away from the boundary in a power law…
In Weyl semimetals, there is an intriguing possibility of realizing a pseudo-magnetic field in presence of small strain due to certain special cases of static deformations. This pseudo-magnetic field can be large enough to form quantized Landau levels and thus become observable in Weyl semimetals. In this paper, we experimentally show the emergence of a pseudo-magnetic field (~ 3 Tesla) by Scanning Tunneling Spectroscopy (STS) on the doped Weyl semimetal Re-MoTe2, where distinct Landau level oscillations in the tunneling conductance are clearly resolved. The crystal lattice is intrinsically st…
Tunable two-dimensional Dirac-Weyl semimetal phase induced by altermagnetism
College of Physics, Hebei Normal University（河北师范大学物理学院）；International Center for Quantum Materials, School of Physics, Peking University（北京大学物理学院量子材料国际中心）；Hefei National Laboratory（合肥国家实验室）
We numerically study the three-dimensional (3D) quantum Hall effect (QHE) and magnetothermoelectric transport of Weyl semimetals in the presence of disorder. We obtain a bulk picture that the exotic 3D QHE emerges in a finite range of Fermi energy near the Weyl points determined by the gap between the $n=-1$ and $n=1$ Landau levels (LLs). The quantized Hall conductivity is attributable to the chiral zeroth LLs traversing the gap, and is robust against disorder scattering for an intermediate number of layers in the direction of the magnetic field. Moreover, we predict several interesting charac…
Motivated by recent transport experiments, we theoretically study the quantum Hall effect in topological semimetal films. Owing to the confinement effect, the bulk subbands originating from the chiral Landau levels establish energy gaps that have quantized Hall conductance and can be observed in relatively thick films. We find that the quantum Hall state is strongly anisotropic for different confinement directions not only due to the presence of the surface states but also because of the bulk chiral Landau levels. As a result, we re-examine the quantum Hall effect from the surface Fermi arcs a…
Typical Weyl semimetals host chiral surface states and hence show an anomalous Hall response. Although a Weyl semimetal phase is known to be robust against weak disorder, the influence of disorder on chiral states is not fully clarified so far. We study the behavior of such chiral states in the presence of disorder and its consequences on an anomalous Hall response, focusing on a thin slab of Weyl semimetal with chiral surface states along its edge. It is shown that weak disorder does not disrupt chiral edge states but crucially affects them owing to the renormalization of a mass parameter: th…
The 2D semimetal consisting of heavy holes and light electrons is studied. The consideration is based on assumption that electrons are quantized by magnetic field while holes remain classical. We assume also that the interaction between components is weak and the conversion between components is absent. The kinetic equation for holes colliding with quantized electrons is utilized. It has been stated that the inter-component friction and corresponding correction to the dissipative conductivity $σ_{xx}$ {\it do not vanish at zero temperature} due to degeneracy of the Landau levels. This correcti…
We investigate the 3D quantum Hall effect in Weyl semimetals and elucidate a global picture of the edge states. The edge states hosting 3D quantum Hall effect are combinations of Fermi arcs and chiral bulk Landau levels parallel to the magnetic field. The Hall conductance, $σ_{xz}^H$, shows quantized plateaus at Weyl nodes while tuning the magnetic field. However, the chiral Landau levels manipulate the quantization of Weyl orbits, especially under a tilted magnetic field, and the resulting edge states lead to distinctive Hall transport phenomena. A tilted magnetic field contributes an intrins…
The quantum Hall effect in three-dimensional Weyl semimetal (WSM) receives significant attention for the emergence of the Fermi loop where the underlying two-dimensional Hall conductivity, namely, sheet Hall conductivity, shows quantized plateaus. Considering the tilted lattice models for multi Weyl semimetals (mWSMs), we systematically study the Landau levels (LLs) and magneto-Hall conductivity in the presence of parallel and perpendicular (with respect to the Weyl node's separation) magnetic field, i.e., $\mathbf{ B}\parallel z$ and $\mathbf{B}\parallel x$, to explore the impact of tilting a…
We present results of a theoretical study of photocurrents in the Weyl semimetals belonging to the gyrotropic symmetry classes. We show that, in weakly gyrotropic symmetry classes C$_{nv}$ ($n = 3,4,6$), the circular photocurrent transverse to the incidence direction appears only with account, in the electron effective Hamiltonian, for both linear and quadratic or cubic in quasi-momentum spin-dependent terms as well as a spin-independent term resulting in the tilt of the cone dispersion. A polarization-independent magneto-induced photocurrent is predicted which is also allowed in gyrotropic sy…
The quantized conductance plateaus and zero conductance fluctuation are the general consequence of electron transport in chiral edge states of Hermitian Chern insulators. Here we show that the physics of electron transport through chiral or helical edge channels becomes much richer when the non-Hermicity is allowed. In the presence of an unbalanced non-Hermicity where the chiral edge states have finite-lifetime, the conductance of the edge channels is not quantized, but its conductance fluctuation is zero. For the balanced non-Hermicity, however, the chiral edge states have infinite-lifetime, …
We construct an exactly solvable lattice model of a fractional Weyl semimetal (FWS). The low energy theory of this strongly interacting state is that of a Weyl semimetal built out of fractionally charged fermions. We show the existence of a universally quantized and fractional circular photogalvanic effect (CPGE) and a violation of the Wiedemann-Franz law in the system. Together with a spectral gap in the single-particle electronic Green's function they provide strong experimental signatures for this exotic gapless state of matter.
The magnetoelectric coupling of electrons in a three-dimensional solid can be effectively described by axion electrodynamics. Here we report the discovery of the fractional magnetoelectric effect in chiral anomalous semimetals of the three-dimensional massless Wilson fermions, which have linear dispersions at the energy crossing point, and break the chiral symmetry at generic momenta. In the presence of electric and magnetic fields, the time-reversal and parity symmetry breaking give rise to the quarter-quantized topological magnetoelectric effect, which is directly related to the winding numb…
Chiral topological semimetals are materials that break both inversion and mirror symmetries. They host interesting phenomena such as the quantized circular photogalvanic effect (CPGE) and the chiral magnetic effect. In this work, we report a comprehensive theoretical and experimental analysis of the linear and non-linear optical responses of the chiral topological semimetal RhSi, which is known to host multifold fermions. We show that the characteristic features of the optical conductivity, which display two distinct quasi-linear regimes above and below 0.4 eV, can be linked to excitations of …
Parity Anomalous Semimetal with Minimal Conductivity Induced by an In-Plane Magnetic Field
Huawei Technologies Co., Ltd.（华为技术有限公司）；School of Sciences, Great Bay University（大湾区大学理学院）；Department of Physics and State Key Laboratory of Optical Quantum Materials, The University of Hong Kong（香港大学物理系及光学量子材料国家重点实验室）
We propose a simple scheme to construct a model whose Fermi surface is comprised of crossing-line nodes. The Hamiltonian consists of a normal hopping term and an additional term which is odd under the mirror reflection. The line nodes appear along the mirror-invariant planes, where each line node carries the quantized Berry magnetic flux. We explicitly construct a model with the $N$-fold rotational symmetry, where the $2N$ line nodes merge at the north and south poles. Photoirradiation induces a topological phase transition. When we apply photoirradiation along the $k_z$ axis, there emerge poi…
Topological semimetals in crystals with a chiral structure (which possess a handedness due to a lack of mirror and inversion symmetries) are expected to display numerous exotic physical phenomena, including fermionic excitations with large topological charge [1], long Fermi arc surface states [2,3], unusual magnetotransport [4] and lattice dynamics [5], as well as a quantized response to circularly polarized light [6]. To date, all experimentally confirmed topological semimetals exist in crystals that contain mirror operations, meaning that these properties do not appear. Here, we show that Al…
The high-magnetic-field thermoelectric effect in nodal-line semimetals with straight nodal lines was investigated. Three-dimensional (3D) Dirac/Weyl semimetals exhibit constant thermoelectric Hall conductivity at the high-magnetic-field quantum limit, resulting in a boundless linear increase of Seebeck coefficient. This is known as the quantized thermoelectric Hall effect (QTHE), and is expected to lead to high-performance thermoelectricity at low temperatures. Here, in addition to Dirac/Weyl semimetals, we demonstrated that 3D semimetals with straight nodal lines can also exhibit the QTHE und…
We develop a theory of the direct interband and indirect intraband photogalvanic effects in Weyl semimetals belonging to the gyrotropic classes with improper symmetry operations. At zero magnetic field, an excitation of such a material with circularly polarized light leads to a photocurrent whose direction depends on the light helicity. We show that in the semimetals of the C$_{2v}$ symmetry, an allowance for the tilt term in the effective Hamiltonian is enough to prevent cancellation of the photocurrent contributions from the Weyl cones of opposite chiralities. In the case of the C$_{4v}$ sym…
Lattice deformations act on the low-energy excitations of Dirac materials as effective axial vector fields. This allows to directly detect quantum anomalies of Dirac materials via the response to axial gauge fields. We investigate the parity anomaly in Dirac nodal line semimetals induced by lattice vibrations, and establish a topological piezoelectric effect; i.e., periodic lattice deformations generate topological Hall currents that are transverse to the deformation field. The currents induced by this piezoelectric effect are dissipationless and their magnitude is completely determined by the…
The magnetotransport properties of epitaxial films of Cd3As2, a paradigm three-dimensional Dirac semimetal, are investigated. We show that an energy gap opens in the bulk electronic states of sufficiently thin films and, at low temperatures, carriers residing in surface states dominate the electrical transport. The carriers in these states are sufficiently mobile to give rise to a quantized Hall effect. The sharp quantization demonstrates surface transport that is virtually free of parasitic bulk conduction and paves the way for novel quantum transport studies in this class of topological mate…
