Magnetic excitations in van der Waals (vdW) materials, especially in the two-dimensional (2D) limit, are an exciting research topic from both the fundamental and applied perspectives. Using temperature-dependent, magneto-Raman spectroscopy, we identify the hybridization of two-magnon excitations with two separate E$_\mathrm{g}$ phonons in MnPSe$_3$, a magnetic vdW material that could potentially host 2D antiferromagnetism. Results from first principles calculations of the phonon and magnon spectra further support our identification. The Raman spectra's rich temperature dependence through the magnetic transition displays an avoided-crossing behavior in the phonons' frequency and a concurrent decrease in their lifetimes. We construct a model based on the interaction between a discrete level and a continuum that reproduces these observations. The strong magnon-phonon hybridization reported here highlights the need to understand its effects on spin transport experiments in magnetic vdW materials.
Theory of phonon-magnon hybridization and angular momentum in CrI$_3$ and CrBr$_3$
Université de Liège（列日大学）；Fonds de la Recherche Scientifique（科学科研基金）；European Theoretical Spectroscopy Facility（欧洲理论光谱设施）；Institut de Ciència de Materials de Barcelona (ICMAB-CSIC)（巴塞罗那材料科学研究所）；ICREA-Institució Catalana de Recerca i Estudis Avançats（加泰罗尼亚高级研究与教育研究院）；University of Utrecht（乌得勒支大学）
Van der Waals magnets are uniquely positioned at the intersection between two-dimensional materials, antiferromagnetic spintronics, and magnonics. The interlayer exchange interaction in these materials enables antiferromagnetic resonances to be accessed at GHz frequencies. Consequently, these layered antiferromagnets are intriguing materials out of which quantum hybrid magnonic devices can be fashioned. Here, we use both a modified macrospin model and micromagnetic simulations to demonstrate a comprehensive antiferromagnetic resonance spectra in van der Waals magnets near the ultrathin (monola…
We theoretically study magnon-phonon hybrid excitations (magnon-polarons) in two-dimensional antiferromagnets on a honeycomb lattice. With an in-plane Dzyaloshinskii-Moriya interaction (DMI) allowed from mirror symmetry breaking from phonons, we find non-trivial Berry curvature around the anti-crossing rings among magnon and both optical and acoustic phonon bands, which gives rise to finite Chern numbers. We show that the Chern numbers of the magnon-polaron bands can be manipulated by changing the magnetic field direction or strength. We evaluate the thermal Hall conductivity reflecting the no…
We report the observation of anomalous peak structures induced by hybridized magnon-phonon excitation (magnon polarons) in the magnetic field dependence of the spin Peltier effect (SPE) in a Lu$_{2}$Bi$_{1}$Fe$_{4}$Ga$_{1}$O$_{12}$ (BiGa:LuIG) with Pt contact. The SPE peaks coincide with magnetic fields tuned to the threshold of magnon-polaron formation, consistent with the previous observation in the spin Seebeck effect. The enhancement of SPE is attributed to the lifetime increase in spin current caused by magnon-phonon hybridization in BiGa:LuIG.
Emergent cooperative motions of individual degrees of freedom, i.e. collective excitations, govern the low-energy response of system ground states under external stimulations and play essential roles for understanding many-body phenomena in low-dimensional materials. The hybridization of distinct collective modes provides a route towards coherent manipulation of coupled degrees of freedom and quantum phases. In magnets, strong coupling between collective spin and lattice excitations, i.e., magnons and phonons, can lead to coherent quasi-particle magnon polarons. Here, we report the direct obse…
Multimode magnon-phonon cavity driven by symmetry-locked strain fields
Auburn University（奥本大学）；University of Wisconsin-Madison（威斯康星大学麦迪逊分校）；University of California, Davis（加州大学戴维斯分校）；University of North Carolina at Chapel Hill（北卡罗来纳大学教堂山分校）；Columbia University（哥伦比亚大学）；Pacific Northwest National Laboratory（太平洋西北国家实验室）
We report the experimental observation in thin films of the hybridization of the uniform ferromagnetic resonance mode with nonuniform magnons as a result of the two-magnon scattering mechanism, leading to a frequency-pulling effect on the ferromagnetic resonance. This effect, when not properly accounted for, leads to a discrepancy in the dependence of the ferromagnetic resonance field on frequency for different field orientations. The frequency-pulling effect is the complement of the broadening of the ferromagnetic resonance lineshape by two-magnon scattering and can be calculated using the sa…
We report thermal control of mode hybridization between the ferromagnetic resonance (FMR) and a planar resonator (notch filter) working at 4.74 GHz. The chosen magnetic material is a ferrimagnetic insulator (Yttrium Iron Garnet: YIG) covered by 6 nm of platinum (Pt). A current induced heating method has been used in order to enhance the temperature of the YIG/Pt system. The device permits us to control the transmission spectra and the magnon-photon coupling strength at room temperature. These experimental findings reveal potentially applicable tunable microwave filtering function.
Karlsruhe Institute of Technology（卡尔斯鲁厄理工学院）；Jiangsu University（江苏大学）；Forschungszentrum Jülich GmbH（于利希研究中心有限公司）；Johannes Gutenberg-University Mainz（美因茨约翰内斯·古腾堡大学）
Hybrid magnonic systems host a variety of characteristic quantum phenomena such as the magnetically-induced transparency (MIT) and Purcell effect, which are considered useful for future coherent quantum information processing. In this work, we experimentally demonstrate a tunable MIT effect in the Y3Fe5O12(YIG)/Permalloy(Py) magnon-magnon coupled system via changing the magnetic field orientations. By probing the magneto-optic effects of Py and YIG, we identify clear features of MIT spectra induced by the mode hybridization between the uniform mode of Py and the perpendicular standing spin-wav…
Spin Inertia as a Source of Topological Magnons: Chiral Edge States from Coupled Precession and Nutation
Indian Institute of Technology (Indian School of Mines)（印度理工学院（印度矿业学院））；RWTH Aachen University（亚琛工业大学）；University of Münster（明斯特大学）；HUN-REN Wigner Research Centre for Physics（匈牙利研究网络维格纳物理研究中心）；Budapest University of Technology and Economics（布达佩斯技术与经济大学）
Topological electronics has extended its richness to non-electronic systems where phonons and magnons can play the role of electrons. In particular, topological phases of magnons can be enabled by the Dzyaloshinskii-Moriya interaction (DMI) which acts as an effective spin-orbit coupling. We show that besides DMI, an alternating arrangement of Heisenberg exchange interactions critically determines the magnon band topology, realizing a magnonic analog of the Su-Schrieffer-Heeger model. On a honeycomb ferromagnet with perpendicular anisotropy, we calculate the topological phase diagram, the chira…
The hybridization of magnons (spin waves) with phonons, if sufficiently strong and comprising long wavelength excitations, may offer a new playground when manipulating the magnetically ordered systems with light. Applying a magnetic field to a quasi-2D antiferromagnet, FePS3, we tune the magnon-gap excitation towards coincidence with the initially lower-in-energy phonon modes. Hybrid magnon-phonon modes, the magnon polarons are unveiled with demonstration of a pronounced avoided crossing between the otherwise bare magnon and phonon excitations. The magnon polarons in FePS3 are primary traced w…
We theoretically investigate the magnetoelastic coupling (MEC) and its effect on magnon transport in two-dimensional antiferromagnets with a honeycomb lattice. MEC coeffcient along with magnetic exchange parameters and spring constants are computed for monolayers of transition metal trichalcogenides with Néel order ($\text{MnPS}_3$ and $\text{VPS}_3$) and zigzag order ($\text{CrSiTe}_3$, $\text{NiPS}_3$ and $\text{NiPSe}_3$) by $ab$ $initio$ calculations. Using these parameters, we predict that the spin-Nernst coefficient is significantly enhanced due to magnetoelastic coupling. Our study show…
We perform thermodynamic and inelastic neutron scattering (INS) measurements to study the lattice dynamics (phonons) of a cubic collinear antiferromagnet Cu$_3$TeO$_6$ which hosts topological spin excitations (magnons). While the specific heat and thermal conductivity results show that the thermal transport is dominated by phonons, the deviation of the thermal conductivity from a pure phononic model indicates that there is a strong coupling between magnons and phonons. In the INS measurements, we find a mode in the excitation spectra at 4.5 K, which exhibits a slight downward dispersion around…
Emergence of multiple quasi-ferromagnetic magnon modes induced by strong magnetoelastic coupling in $TmFeO_3$ single crystal
Johannes Gutenberg University Mainz（约翰内斯·古腾堡美因茨大学）；Shanghai University（上海大学）；Shanghai Jiao Tong University（上海交通大学）；Norwegian University of Science and Technology（挪威科技大学）
We study the collective dynamics of two distant magnets coherently coupled by acoustic phonons that are transmitted through an intercalated crystal. By tuning the ferromagnetic resonances of the two magnets to an acoustic resonance of the crystal, we control a coherent three levels system. We show that the parity of the phonon mode governs the nature of the indirect coupling between the magnets: the resonances with odd / even phonon modes correspond to out-of-phase / in-phase lattice displacements at the magnets, leading to bright / dark states in response to uniform microwave magnetic fields,…
Cavity-magnon polaritons (CMPs) are the associated quasiparticles of the hybridization between cavity photons and magnons in a magnetic sample placed in a microwave resonator. In the strong coupling regime, where the macroscopic coupling strength exceeds the individual dissipation, there is a coherent exchange of information. This renders CMPs as promising candidates for future applications such as in information processing. Recent advances on the study of the CMP now allow not only for creation of CMPs on demand, but also for tuning of the coupling strength - this can be thought of as enhanci…
Spintronics and quantum information science are two promising candidates for innovating information processing technologies. The combination of these two fields enables us to build solid-state platforms for studying quantum phenomena and for realizing multi-functional quantum tasks. For a long time, however, the intersection of these two fields was limited. This situation has changed significantly over the last few years because of the remarkable progress in coding and processing information using magnons. On the other hand, significant advances in understanding the entanglement of quasi-parti…
Tunable Ultrastrong Magnon-Magnon Coupling and Squeezed States in a Triaxial Van der Waals Antiferromagnet
National Key Laboratory of Spintronics and School of Physics, Nanjing University（南京大学自旋电子学国家重点实验室和物理学院）；School of Science, Nanjing University of Posts and Telecommunications（南京邮电大学理学院）；Laboratory of Solid State Microstructures, Nanjing University（南京大学固体微结构实验室）；State Key Laboratory of Spintronics, Nanjing University（南京大学自旋电子学国家重点实验室）
Magnetochiral effect (MChE) of phonons, a nonreciprocal acoustic property arising due to the symmetry principles, is demonstrated in a chiral-lattice ferrimagnet Cu$_2$OSeO$_3$. Our high-resolution ultrasound experiments reveal that the sound velocity differs for parallel and antiparallel propagation with respect to the external magnetic field.The sign of the nonreciprocity depends on the chirality of the crystal in accordance with the selection rule of the MChE. The nonreciprocity is enhanced below the magnetic ordering temperature and at higher ultrasound frequencies, which is quantitatively…
Key Role of Charge Disproportionation in Monoclinic Semiconducting Fe$_2$PO$_5$, a Room-Temperature d-Wave Altermagnet Candidate
Iowa State University（爱荷华州立大学）；South Dakota State University（南达科他州立大学）；University of Nebraska-Lincoln（内布拉斯加大学林肯分校）；Nebraska Center for Materials and Nanoscience（内布拉斯加材料与纳米科学中心）；Ames National Laboratory, U.S. Department of Energy（美国能源 Ames 国家实验室）
Spin waves in ferrimagnetic yttrium iron garnet (YIG) films with ultralow magnetic damping are relevant for magnon-based spintronics and low-power wave-like computing. The excitation frequency of spin waves in YIG is rather low in weak external magnetic fields because of its small saturation magnetization, which limits the potential of YIG films for high-frequency applications. Here, we demonstrate how exchange-coupling to a CoFeB film enables efficient excitation of high-frequency perpendicular standing spin waves (PSSWs) in nanometer-thick (80 nm and 295 nm) YIG films using uniform microwave…
The interactions between elementary excitations such as phonons, plasmons, magnons, or particle-hole pairs, drive emergent functionalities and electronic instabilities such as multiferroic behaviour, anomalous thermoelectric properties, polar order, or superconductivity. Whereas various hybrid excitations have been studied extensively, the feed-back of prototypical elementary excitations on the crystal electric fields (CEF), defining the environment in which the elementary excitations arise, has been explored for very strong coupling only. We report high-resolution neutron spectroscopy and ab-…
