The quantum-limit Hall effect at $ν= nh/eB\sim O(1)$ that hosts a variety of exotic quantum phenomena requires demanding strong magnetic field $B$ and low carrier density $n$. We propose to realize quantum-limit Hall effect even in the presence of large carrier density residues $n_e$ and $n_h$ relative to the magnetic field $B$ in topological semimetals, where a single Fermi surface contour allow both electron-type and hole-type carriers and approaches charge neutrality as $n_e\sim n_h$. The underlying filling factor $ν= |n_e-n_h|h/eB$ explicitly violates the Onsager's relation for quantum oscillations.
We propose an unconventional type of Hall effect in a topological Dirac semimetal with ferromagnetic electrodes. The topological Dirac semimetal itself has time-reversal symmetry, whereas attached ferromagnetic electrodes break it, causing the large Hall response. This induced Hall effect is a characteristic of the helical surface/edge states that arise in topological materials, such as topological Dirac semimetals or quantum spin Hall insulators. We compute the Hall conductance/resistance and the Hall angle by using a lattice model with four-terminal geometry. For topological Dirac semimetals…
The tunable carrier density plays a key role in the investigation of novel transport properties in three-dimensional topological semimetals. Here we demonstrate that the carrier density as well as the mobility of Dirac semimetal Cd3As2 nanoplates can be effectively tuned by the in-situ thermal treatment at 350 K for one hour, both showing a non-monotonic evolution with the thermal cycling treatments. The upward shift of Fermi level relative to the Dirac nodes blurs the surface Fermi-arc states, accompanying with an anomalous phase shift of oscillations of bulk states due to the change of topol…
In addition to the well known chiral anomaly, Dirac semimetals have been argued to exhibit mirror anomaly, close analogue to the parity anomaly of ($2+1$)-dimensional massive Dirac fermions. The observable response of such anomaly is manifested in a singular step-like anomalous Hall response across the mirror-symmetric plane in the presence of a magnetic field. Although this result seems to be valid in type-II Dirac semimetals (strictly speaking, in the linearized theory), we find that type-I Dirac semimetals do not possess such an anomaly in anomalous Hall response even at the level of the li…
Recently, a new type of Weyl semimetal called type-II Weyl semimetal has been proposed. Unlike the usual (type-I) Weyl semimetal, which has a point-like Fermi surface, this new type of Weyl semimetal has a tilted conical spectrum around the Weyl point. Here we calculate the anomalous Hall conductivity of a Weyl semimetal with a tilted conical spectrum for a pair of Weyl points, using the Kubo formula. We find that the Hall conductivity is not universal and can change sign as a function of the parameters quantifying the tilts. Our results suggest that even for the case where the separation betw…
Motivated by recent transport experiments, we theoretically study the quantum Hall effect in topological semimetal films. Owing to the confinement effect, the bulk subbands originating from the chiral Landau levels establish energy gaps that have quantized Hall conductance and can be observed in relatively thick films. We find that the quantum Hall state is strongly anisotropic for different confinement directions not only due to the presence of the surface states but also because of the bulk chiral Landau levels. As a result, we re-examine the quantum Hall effect from the surface Fermi arcs a…
Typical Weyl semimetals host chiral surface states and hence show an anomalous Hall response. Although a Weyl semimetal phase is known to be robust against weak disorder, the influence of disorder on chiral states is not fully clarified so far. We study the behavior of such chiral states in the presence of disorder and its consequences on an anomalous Hall response, focusing on a thin slab of Weyl semimetal with chiral surface states along its edge. It is shown that weak disorder does not disrupt chiral edge states but crucially affects them owing to the renormalization of a mass parameter: th…
We investigate the topological phase derived by time-reversal breaking fields in a nonsymmorphic symmetry-protected two-dimensional Dirac semimetal. When the nonsymmorphic symmetry is preserved even in the presence of the field, the two-dimensional electronic states change into two distinct topological phases with the insulating gap. One phase is well-known as quantum Hall states with chiral edge modes accompanying the Hall current, but the other one is an unconventional topological phase with helical edge modes in the absence of time-reversal symmetry.
We theoretically study the circularly polarized light-induced Floquet state in line-node semimetals with time-reversal symmetry and inversion symmetry. It is found that the Floquet state can show the photovoltaic anomalous Hall effect when an applied circularly polarized light gaps out the line node in the bulk and leave Weyl point nodes. The Hall conductivity is sensitive to the location of Fermi level: When the Fermi level locates at the node, the Hall conductivity depends on the radius of line node and is nearly independent of the intensity of light. Away from the line node, the Hall conduc…
In this work, we propose a ferromagnetic Bi$_2$Se$_3$ as a candidate to hold the coexistence of Weyl- and nodal-line semimetal phases, which breaks the time reversal symmetry. We demonstrate that the type-I Weyl semimetal phase, type-I-, type-II- and their hybrid nodal-line semimetal phases can arise by tuning the Zeeman exchange field strength and the Fermi velocity. Their topological responses under U(1) gauge field are also discussed. Our results raise a new way for realizing Weyl and nodal-line semimetals and will be helpful in understanding the topological transport phenomena in three-dim…
We experimentally investigate a non-linear Hall effect for three-dimensional WTe$_2$ and Cd$_3$As$_2$ single crystals, representing Weyl and Dirac semimetals, respectively. We observe finite second-harmonic Hall voltage, which depends quadratically on the longitudinal current in zero magnetic field. Despite this observation well corresponds to the theoretical predictions, only magnetic field dependence allows to distinguish the non-linear Hall effect from a thermoelectric response. We demonstrate that second-harmonic Hall voltage shows odd-type dependence on the direction of the magnetic field…
We investigate the 3D quantum Hall effect in Weyl semimetals and elucidate a global picture of the edge states. The edge states hosting 3D quantum Hall effect are combinations of Fermi arcs and chiral bulk Landau levels parallel to the magnetic field. The Hall conductance, $σ_{xz}^H$, shows quantized plateaus at Weyl nodes while tuning the magnetic field. However, the chiral Landau levels manipulate the quantization of Weyl orbits, especially under a tilted magnetic field, and the resulting edge states lead to distinctive Hall transport phenomena. A tilted magnetic field contributes an intrins…
We show that an electric field applied to a strained topological Dirac semimetal, such as Na3Bi and Cd3As2, induces a spin Hall current that is quadratic in the electric field. By regarding the strain as an effective "axial magnetic field" for the Dirac electrons, we investigate the electron and spin transport semiclassically in terms of the chiral kinetic theory. The nonlinear spin Hall effect arises as the cross effect between the regular Hall effect driven by the axial magnetic field and the anomalous Hall effect coming from the momentum-space topology. It provides an efficient way to gener…
We generalize a semiclassical theory and use the argument of angular momentum conservation to examine the ballistic transport in lightly-doped Weyl semimetals, taking into account various phase-space Berry curvatures. We predict universal transverse shifts of the wave-packet center in transmission and reflection, perpendicular to the direction in which the Fermi energy or velocities change adiabatically. The anomalous shifts are opposite for electrons with different chirality, and can be made imbalanced by breaking inversion symmetry. We discuss how to utilize local gates, strain effects, and …
After the experimental realization, the Berry curvature dipole (BCD) induced nonlinear Hall effect (NLHE) has attracted tremendous interest to the condensed matter community. Here, we investigate another family of Hall effect, namely, chiral anomaly induced nonlinear Hall effect (CNHE) in multi-Weyl semimetal (mWSM). In contrast to the BCD induced NLHE, CNHE appears because of the combination of both chiral anomaly and anomalous velocity due to non-trivial Berry curvature. Using the semiclassical Boltzmann theory within the relaxation time approximation, we show that, in contrast to the chiral…
The Weyl semimetal is characterized by three-dimensional linear band touching points called Weyl nodes. These nodes come in pairs with opposite chiralities. We show that the coupling of circularly polarized photons with these chiral electrons generates a Hall conductivity without any applied magnetic field in the plane orthogonal to the light propagation. This phenomenon comes about because with all three Pauli matrices exhausted to form the three-dimensional linear dispersion, the Weyl nodes cannot be gapped. Rather, the net influence of chiral photons is to shift the positions of the Weyl no…
Intrinsic spin Hall conductivities are calculated for strong spin-orbit Bi$_{1-x}$Sb$_x$ semimetals, from the Kubo formula and using Berry curvatures evaluated throughout the Brillouin zone from a tight-binding Hamiltonian. Nearly-crossing bands with strong spin-orbit interaction generate giant spin Hall conductivities in these materials, ranging from 474 ($\hbar$/e)($Ω$cm)$^{-1}$ for bismuth to 96 ($\hbar$/e)($Ω$cm)$^{-1}$ for antimony; the value for bismuth is more than twice that of platinum. The large spin Hall conductivities persist for alloy compositions corresponding to a three-dimensio…
We propose the linear and nonlinear planar Hall effect (PHE) in tilted Weyl semimetals in the presence of an in-plane magnetic and electric field, where the field-induced Berry connection (FBC) plays a key role. We show that the PHE is ascribed to the quantum metric, distinct from the well-known chiral anomaly-induced PHE arising from the Berry curvature. Using a tilting vector to describe the model, we demonstrate the constrains on the linear and nonlinear PHE by the tilting directions. The linear PHE is intrinsic that is determined by the topological properties of energy bands, whereas the n…
Magnus Hall effect (MHE) is a non-linear Hall effect requiring no external magnetic field, which can be observed when an in-built electric field couples to the Berry curvature of the bandstructure, producing a current in the transverse direction. In this paper, we explore MHE in the context of various three-dimensional semimetals, incorporating various features like tilt, anisotropy, and multi-fold degeneracy. We numerically calculate the Magnus Hall conductivity tensors and transport coefficients, within the framework of the Boltzmann transport theory. Although MHE was originally predicted fo…
Anisotropic magnetoresistance is the change tendency of resistance of a material on the mutual orientation of the electric current and the external magnetic field. Here, we report experimental observations in the Dirac semimetal Cd3As2 of giant anisotropic magnetoresistance and its transverse version, called the planar Hall effect. The relative anisotropic magnetoresistance is negative and up to -68% at 2 K and 10 T. The high anisotropy and the minus sign in this isotropic and nonmagnetic material are attributed to a field-dependent current along the magnetic field, which may be induced by the…
From the Kubo formula for transport in a tilted Weyl semimetal we calculate the absorptive part of the dynamic conductivity for both right and left handed circular polarized light. These depend on the real part of the longitudinal conductivity and the imaginary part of the transverse (Hall) conductivity. We include the effect of the chiral anomaly which pumps charge from negative to positive chirality node when the usual ${\bs E}\cdot{\bs B}$ term is included in the electrodynamics and obtain analytic expressions. To calculate the Hall angle we further provide expressions for the imaginary par…
We theoretically investigate the transport and magnetotransport properties of three-dimensional Weyl semimetals. Using the RPA-Boltzmann transport scattering theory for electrons scattering off randomly distributed charged impurities, together with an effective medium theory to average over the resulting spatially inhomogeneous carrier density, we smoothly connect our results for the minimum conductivity near the Weyl point with known results for the conductivity at high carrier density. In the presence of a non-quantizing magnetic field, we predict that for both high and low carrier densities…
We investigate an unconventional topological phase transition that occurs in quantum spin Hall (QSH) systems when applying an external in-plane magnetic field. We show that this transition between QSH and trivial insulator phases is separated by a stable topological gapless phase, which is protected by the combination of particle-hole and reflection symmetries, and thus, we dub it as crystalline Weyl semimetal. We explore the stability of this new phase when particle-hole symmetry breaking terms are present. Especially, we predict a robust unconventional topological phase transition to be visi…
We numerically study the three-dimensional (3D) quantum Hall effect (QHE) and magnetothermoelectric transport of Weyl semimetals in the presence of disorder. We obtain a bulk picture that the exotic 3D QHE emerges in a finite range of Fermi energy near the Weyl points determined by the gap between the $n=-1$ and $n=1$ Landau levels (LLs). The quantized Hall conductivity is attributable to the chiral zeroth LLs traversing the gap, and is robust against disorder scattering for an intermediate number of layers in the direction of the magnetic field. Moreover, we predict several interesting charac…
The electronic structure of multilayer graphenes depends strongly on the number of layers as well as the stacking order. Here we explore the electronic transport of purely ABA-stacked trilayer graphenes in a dual-gated field-effect device configuration. We find that both the zero-magnetic-field transport and the quantum Hall effect at high magnetic fields are distinctly different from the monolayer and bilayer graphenes, and that they show electron-hole asymmetries that are strongly suggestive of a semimetallic band overlap. When the ABA trilayers are subjected to an electric field perpendicul…
We propose a simple realization of the three-dimensional (3D) Weyl semimetal phase, utilizing a multilayer structure, composed of identical thin films of a magnetically-doped 3D topological insulator (TI), separated by ordinary-insulator spacer layers. We show that the phase diagram of this system contains a Weyl semimetal phase of the simplest possible kind, with only two Dirac nodes of opposite chirality, separated in momentum space, in its bandstructure. This particular type of Weyl semimetal has a finite anomalous Hall conductivity, chiral edge states, and occurs as an intermediate phase b…
We investigate the influence of surface states on the nonlinear Hall response of non-centrosymmetric time-reversal invariant Weyl semimetals. To do so, we perform a tomography of the Berry curvature dipole in a slab system using a minimal two-band model. We find that in the type-I phase, the nonlinear Hall response is not particularly sensitive to the presence of Fermi arcs or other trivial surface states. However, in the type-II phase, we find that these surface states contribute substantially to the Berry curvature dipole, leading to a strong thickness dependence of the nonlinear Hall respon…
The recent discovery of the quantum nonlinear Hall effect has revived the field of nonlinear transport. Here, we predict magnetic field-induced nonlinear Hall effect in time-reversal symmetric Weyl semimetal. We show that the interplay of the band geometric quantities, such as the Berry curvature, and the magnetic part of the Lorentz force can give rise to finite nonlinear Hall conductivity that is linear in the magnetic field. Such nonlinear Hall conductivity can manifest through nonlinear transport measurement as well as nonlinear optical phenomena like photocurrent and the second harmonic g…
We theoretically investigate the spin Hall conductivity (SHC) in topological Dirac semimetals (TDSMs) whose Dirac points are protected by rotational symmetry. On the basis of a general phase diagram of the system with time-reversal, inversion and four-fold rotational symmetries, we reveal that the SHC is sensitive to the phase to which the system belong. The phase and the SHC are characterized by the mirror Chern numbers and the presence or absence of gapless bulk Dirac points. It is also found that the representative TDSM Cd$_3$As$_2$ supports a large and negative SHC $σ_{xy}^z\sim -10^4 (\hb…
Magnetic Weyl semimetals exhibit intriguing transport phenomena due to their non-trivial band structure. Recent experiments in bulk crystals of the shandite-type Co$_3$Sn$_2$S$_2$ have shown that this material system is a magnetic Weyl semimetal. To access the length scales relevant for chiral transport, it is mandatory to fabricate microstructures of this fascinating compound. We therefore have cut micro-ribbons (typical size $0.3~\times~3~\times~50$μ$m^3$) from Co$_3$Sn$_2$S$_2$ single crystals using a focused beam of Ga$^{2+}$-ions and investigated the impact of the sample dimensions and po…
We report on electronic transport measurements of electrostatically gated nano-devices of the semimetal WTe\textsubscript{2}. High mobility metallic behavior is achieved in the 2D limit by encapsulating thin flakes in an inert atmosphere. At low temperatures, we find that a large magnetoresistance can be turned on and off by electrostatically doping the system between a semimetallic state and an electron-only metallic state, respectively. We confirm the nature of the two regimes by analyzing the magnetoresistance and Hall effect with a two-carrier model, as well as by analysis of Shubnikov-de …
Recently, higher-order topological matter and 3D quantum Hall effects have attracted great attention. The Fermi-arc mechanism of the 3D quantum Hall effect proposed in Weyl semimetals is characterized by the one-sided hinge states, which do not exist in all the previous quantum Hall systems and more importantly pose a realistic example of the higher-order topological matter. The experimental effort so far is in the Dirac semimetal Cd$_3$As$_2$, where however time-reversal symmetry leads to hinge states on both sides of the top/bottom surfaces, instead of the aspired one-sided hinge states. We …
We study the positive longitudinal magnetoconductivity (LMC) and planar Hall effect as emergent effects of the chiral anomaly in Weyl semimetals, following a recent-developed theory by integrating the Landau quantization with Boltzmann equation. It is found that, in the weak magnetic field regime, the LMC and planar Hall conductivity (PHC) obey $\cos^{6}θ$ and $\cos^{5}θ\sin θ$ dependences on the angle $θ$ between the magnetic and electric fields. For higher magnetic fields, the LMC and PHC cross over to $\cos^{2}θ$ and $\cosθ\sinθ$ dependences, respectively. Interestingly, the PHC could exhib…
Cd3As2 is a model material of Dirac semimetal with a linear dispersion relation along all three directions in the momentum space. The unique band structure of Cd3As2 makes it with both Dirac and topological properties. It can be driven into a Weyl semimetal by the symmetry breaking or a topological insulator by enhancing the spin-orbit coupling. Here we report the temperature and gate voltage dependent magnetotransport properties of Cd3As2 nanoplates with Fermi level near the Dirac point. The Hall anomaly demonstrates the two-carrier transport accompanied by a transition from n-type to p-type …
We study the chiral electric separation effect (CESE) in Weyl semimetals (WSM). Within the model based on the kinetic equation we show that there is a non-zero chirality current in external electric and magnetic fields. We distinguish longitudinal, in-plane transverse, Hall, and anomalous Hall components of the CESE. It is shown that the first two components are quadratic in electric field and linear in magnetic field, while the Hall component is quadratic in both the electric and magnetic fields. All three are due to the chiral anomaly. In WSMs the chirality current can be associated with the…
Starting from a minimal model for a 2D nodal loop semimetal, we study the effect of chiral mass gap terms. The resulting Dirac loop anomalous Hall insulator's Chern number is the phase winding number of the mass gap terms on the loop. We provide simple lattice models, analyze the topological phases and generalize a previous index characterizing topological transitions. The responses of the Dirac loop anomalous Hall and quantum spin Hall insulators to a magnetic field's vector potential are also studied both in weak and strong field regimes, as well as the edge states in a ribbon geometry.
Skyrmion lattices as a novel type of chiral spin states are attracting increasing attention, owing to their peculiar properties stemming from real-space topological properties. At the same time, the properties of magnetic Weyl semimetals with complex $k$-space topology are moving into the focus of research in spintronics. We consider the Hall transport properties and orbital magnetism of skyrmion lattices imprinted in topological semimetals, by employing a minimal model of a 2D mixed Weyl semimetal which, as a function of the magnetization direction, exhibits two Chern insulator phases separat…
We investigate the potential of the surface states of 3D nodal-line semimetals to produce surface and 3D quantized Hall effects in which the electronic currents flow unidirectionally along the surface of the material. This phenomenology is based on the fact that, irrespective of its orientation, a strong magnetic field gives rise to a zero Landau level with huge 2D degeneracy of states in the nodal-line semimetal. When the magnetic field is perpendicular to the plane of the nodal line, we show that the evanescent states within the nodal ring are transmuted into Landau surface states which corr…
The peculiar shape of the Fermi surface of topological nodal line semimetals at low carrier concentrations results in their unusual optical and transport properties. We analytically investigate the linear optical responses of three and two-dimensional nodal line semimetals using the Kubo formula. The optical conductivity of a three-dimensional nodal line semimetal is anisotropic. Along the axial direction (\textit{i.e.}, the direction perpendicular to the nodal-ring plane), the Drude weight has a linear dependence on the chemical potential at both low and high carrier dopings. For the radial d…
Here we study the single-particle, electronic transport and optical properties of a gapped system described by a simple two-band Hamiltonian with inverted valence bands. We analyze its properties in the three-dimensional (3D) and the two-dimensional (2D) case. The insulating phase changes into a metallic phase when the band gap is set to zero. The metallic phase in the 3D case is characterized by a nodal surface. This nodal surface is equivalent to a nodal ring in two dimensions. Within a simple theoretical framework, we calculate the density of state, the total and effective charge carrier co…
We predict a nonlinear Hall effect in certain Weyl semimetals with broken inversion symmetry. When the energy dispersions about pairs of Weyl nodes are skewed -- the Weyl cones are "tilted" -- the concerted actions of the anomalous velocity and the chiral anomaly give rise to the nonlinear Hall effect. This Hall conductivity is linear in both electric and magnetic fields, and depends critically on the tilting of the Weyl cones. We also show that this effect does not rely on a finite Berry curvature dipole, in contrast to the intrinsic quantum nonlinear Hall effect that was recently observed in…
We present a time- and angular-resolved photoemission (TR-ARPES) study of the transition- metal dichalcogenide WTe2, a candidate type II Weyl semimetal exhibiting extremely large magne- toresistence. Using femtosecond light pulses, we characterize the unoccupied states of the electron pockets above the Fermi level. We track the relaxation dynamics of photoexcited electrons along the unoccupied band structure and into a bulk hole pocket. Following the ultrafast carrier relaxation, we report remarkably similar decay dynamics for electrons and holes. Our results corroborate the hypothesis that ca…
Large intrinsic anomalous Hall effect (AHE) due to the Berry curvature in magnetic topological semimetals is attracting enormous interest due to its fundamental importance and technological relevance. Mechanisms resulting in large intrinsic AHE include diverging Berry curvature in Weyl semimetals, anticrossing nodal rings or points of non-trivial bands, and noncollinear spin structures. Here we show that a half-topological semimetal (HTS) state near a topological critical point can provide a new mechanism for driving an exceptionally large AHE. We reveal this through a systematic experimental …
Antiferromagnetic Weyl semimetal Mn$_3$Sn has shown to generate strong intrinsic anomalous Hall effect (AHE) at room temperature, due to large momentum-space Berry curvature from the time-reversal symmetry breaking electronic bands of the Kagome planes. This prompts us to investigate intrinsic spin Hall effect, a transverse phenomenon with identical origin as the intrinsic AHE. We report inverse spin Hall effect experiments in nanocrystalline Mn$_3$Sn nanowires at room temperature using spin absorption method which enables us to quantitatively derive both the spin diffusion length and the spin…
We study the intrinsic and extrinsic Hall effects in disordered magnetic Weyl semimetals numerically. We show that in Weyl metals, where the Fermi energy deviates from the Weyl point, the Hall and longitudinal conductances exhibit a specific relation, which is distinguished from the well-known relation in integer quantum Hall systems. Around the Weyl point, the Hall conductance increases with increasing longitudinal conductance. This increasing behavior indicates the existence of additional contributions to the Hall conductance from the subbands of Weyl cones besides that from the bulk Berry c…
The high-magnetic-field thermoelectric effect in nodal-line semimetals with straight nodal lines was investigated. Three-dimensional (3D) Dirac/Weyl semimetals exhibit constant thermoelectric Hall conductivity at the high-magnetic-field quantum limit, resulting in a boundless linear increase of Seebeck coefficient. This is known as the quantized thermoelectric Hall effect (QTHE), and is expected to lead to high-performance thermoelectricity at low temperatures. Here, in addition to Dirac/Weyl semimetals, we demonstrated that 3D semimetals with straight nodal lines can also exhibit the QTHE und…
Observation of Weyl and Dirac Fermions in condensed matter systems is one of the most important discoveries. Among the very few available tools to characterize Weyl semimetals through electrical transport, negative magnetoresistance is most commonly used. Considering shortcomings of this method, new tools to characterize chiral anomaly in Weyl semimetals are desirable. We employ planar Hall effect as an effective technique in half Heusler Weyl semimetal GdPtBi to study chiral anomaly. This compound exhibits a large value of 1.5 mohm cm planar Hall resistivity at 2 K and in 9 T. Our analysis re…
