The instability of a Fermi surface against Ising nematic order destroys the quasiparticle character of the low-energy degrees of freedom. Therefore, observables exhibit deviations from Fermi liquid behavior which gives rise to the term Ising nematic quantum critical metal. To obtain a theoretical description we use a finite-temperature version of Eliashberg theory which allows to treat the strong coupling between quantum and thermal fluctuations in the absence of well-defined quasiparticles. Here, we use this self-consistent, diagrammatic approach to compute, in particular, the nematic susceptibility and the non-Fermi liquid correlations. Upon decreasing the temperature, the susceptibility crosses over from a $(T \log T)^{-1}$ to $T^{-2/3}$ behavior, which is induced by the absence of quasiparticles and restores the Ising nematic critical scaling. Correspondingly, the fermions obey a simple $ω/T$ scaling law at low enough temperatures. However, this regime is characterized by strong IR-UV mixing since the proportionality factors exhibit a dependence on the spectral width of the non-quasiparticle excitations and on the underlying lattice. Tuning the parameters of the model, therefore, gives rise to several scenarios for the breakdown of the scaling theory. We discuss them within the Eliashberg approach and estimate the related crossover scales. We also show that the leading order vertex corrections do not change the scaling with temperature or coupling constants.
Recent Raman scattering experiments have revealed a "quasi-elastic peak" in $\mathrm{FeSe_{1-x}S_x}$ near an Ising-nematic quantum critical point (QCP) \cite{zhang17}. Notably, the peak occurs at sub-temperature frequencies, and softens as $T^α$ when temperature is decreased toward the QCP, with $α>1$. In this work, we present a theoretical analysis of the low-frequency Raman response using a memory matrix approach. We show that such a quasi-elastic peak is associated with the relaxation of an Ising-nematic deformation of the Fermi surface. Specifically, we find that the peak frequency is prop…
At low temperatures in ultraclean GaAs-AlGaAs heterojunctions, high fractional Landau levels break rotational symmetry, leading to increasingly anisotropic transport properties as temperature is lowered below $\sim$150mK. While the onset of transport anisotropy is well described by an XY model of an electron nematic in the presence of a weak uniform symmetry-breaking term, the low temperature behavior deviates significantly from this model. We find that inclusion of interactions between the electron nematic and the underlying crystalline lattice in the form of a 4-fold symmetry breaking term i…
We study finite temperature properties of metals close to an Ising-nematic quantum critical point in two spatial dimensions. In particular we show that at any finite temperature there is a regime where order parameter fluctuations are characterized by a dynamical critical exponent $z=2$, in contrast to $z=3$ found at zero temperature. Our results are based on a simple Eliashberg-type approach, which gives rise to a boson self-energy proportional to $Ω/γ(T)$ at small momenta, where $γ(T)$ is the temperature dependent fermion scattering rate. These findings might shed some light on recent Monte-…
The paradigmatic example of a continuous quantum phase transition is the transverse field Ising ferromagnet. In contrast to classical critical systems, whose properties depend only on symmetry and the dimension of space, the nature of a quantum phase transition also depends on the dynamics. In the transverse field Ising model, the order parameter is not conserved and increasing the transverse field enhances quantum fluctuations until they become strong enough to restore the symmetry of the ground state. Ising pseudo-spins can represent the order parameter of any system with a two-fold degenera…
Motivated by the recent inelastic neutron scattering (INS) measurements in the iron pnictides which show a strong anisotropy of spin excitations in directions perpendicular and parallel to the ordering wave-vector even above the magnetic transition temperature $T_N$, we study the frustrated Heisenberg model with a biquadratic spin-spin exchange interaction. Using the Dyson-Maleev (DM) representation, which proves appropriate for all temperature regimes, we find that the spin-spin dynamical structure factors are in excellent agreement with experiment, exhibiting breaking of the $C_4$ symmetry e…
The NMR spectrum of FeSe shows a dramatic broadening on cooling towards the bulk nematic phase at $T_s=90$ K, due to the formation of a quasi-static, short-range-ordered nematic domain structure. However, a quantitative understanding of the NMR broadening and its relationship to the nematic susceptibility is still lacking. Here, we show that the temperature and pressure dependence of the broadening is in quantitative agreement with the mean-field Edwards-Anderson parameter of an Ising-nematic model in the presence of random-field disorder introduced by non-magnetic impurities. Furthermore, the…
The Ising nematic quantum critical point (QCP) associated with the zero temperature transition from a symmetric to a nematic {\it metal} is an exemplar of metallic quantum criticality. We have carried out a minus sign-free quantum Monte Carlo study of this QCP for a two dimensional lattice model with sizes up to $24\times 24$ sites. The system remains non-superconducting down to the lowest accessible temperatures. The results exhibit critical scaling behavior over the accessible ranges of temperature, (imaginary) time, and distance. This scaling behavior has remarkable similarities with recent…
Motivated by the properties of the iron chalcogenides, we study the phase diagram of a generalized Heisenberg model with frustrated bilinear-biquadratic interactions on a square lattice. We identify zero-temperature phases with antiferroquadrupolar and Ising-nematic orders. The effects of quantum fluctuations and interlayer couplings are analyzed. We propose the Ising-nematic order as underlying the structural phase transition observed in the normal state of FeSe, and discuss the role of the Goldstone modes of the antiferroquadrupolar order for the dipolar magnetic fluctuations in this system.…
We consider two-dimensional metals near a Pomeranchuk instability which breaks 90$^\circ$ lattice rotation symmetry. Such metals realize strongly-coupled non-Fermi liquids with critical fluctuations of an Ising-nematic order. At low temperatures, impurity scattering provides the dominant source of momentum relaxation, and hence a non-zero electrical resistivity. We use the memory matrix method to compute the resistivity of this non-Fermi liquid to second order in the impurity potential, without assuming the existence of quasiparticles. Impurity scattering in the $d$-wave channel acts as a rand…
The Schwinger-boson theory of the frustrated square lattice antiferromagnet yields a stable, gapped $\mathbb{Z}_2$ spin liquid ground state with time-reversal symmetry, incommensurate spin correlations and long-range Ising-nematic order. We obtain an equivalent description of this state using fermionic spinons (the fermionic spinons can be considered to be bound states of the bosonic spinons and the visons). Upon doping, the $\mathbb{Z}_2$ spin liquid can lead to a fractionalized Fermi liquid (FL*) with small Fermi pockets of electron-like quasiparticles, while preserving the $\mathbb{Z}_2$ to…
We present a model of classical hard-core dimers on the square lattice that contains an Ising nematic phase in its phase diagram. We consider a model with an attractive interaction for parallel dimers on a given plaquette of the square lattice and an attractive interaction for neighboring parallel dimers on the same row ({\it viz} column) of the lattice. By extensive Monte carlo simulations we find that with a finite density of holes the phase diagram has, with rising temperatures, a columnar crystalline phase, an Ising nematic liquid phase and a disordered fluid phase, separated by Ising cont…
Many-body systems subject to a high-frequency drive can show intriguing thermalization behavior. Prior to heating to a featureless infinite-temperature state, these systems can spend an exponentially long time in prethermal phases characterized by various kinds of order. Here, we uncover the rich non-equilibrium phase diagram of a driven frustrated two-dimensional Ising magnet with competing short-range ferromagnetic and long-range dipolar interactions. We show that the ordered stripe and nematic phases, which appear in equilibrium as a function of temperature, underpin subsequent prethermal p…
In an isotropic strongly interacting quantum liquid without quasiparticles, general scaling arguments imply that the dimensionless ratio $(k_B /\hbar)\, η/s$, where $η$ is the shear viscosity and $s$ is the entropy density, is a universal number. We compute the shear viscosity of the Ising-nematic critical point of metals in spatial dimension $d=2$ by an expansion below $d=5/2$. The anisotropy associated with directions parallel and normal to the Fermi surface leads to a violation of the scaling expectations: $η$ scales in the same manner as a chiral conductivity, and the ratio $η/s$ diverges …
We study the the interplay between spontaneously broken valley symmetry and spatial disorder in multivalley semiconductors in the quantum Hall regime. In cases where valleys have anisotropic electron dispersion a previous long-wavelength analysis [Phys. Rev. B 82, 035428 (2010)] identified two new phases exhibiting the QHE. The first is the quantum Hall Ising nematic (QHIN), a phase with long-range orientational order manifested in macroscopic transport anisotropies. The second is the quantum Hall random-field paramagnet (QHRFPM) that emerges when the Ising ordering is disrupted by quenched di…
We report results of low-temperature heat capacity, magnetocaloric effect and neutron diffraction measurements of TmVO$_{4}$, an insulator that undergoes a continuous ferroquadrupolar phase transition associated with local partially-filled $4f$ orbitals of the thulium (Tm$^{3+}$) ions. The ferroquadrupolar transition, a realization of Ising nematicity, can be tuned to a quantum critical point using a magnetic field oriented along the $c$-axis of the tetragonal crystal lattice, which acts as an effective transverse field for the Ising-nematic order. In small magnetic fields, the thermal phase t…
We present a renormalization group theory for the onset of Ising-nematic order in a Fermi liquid in two spatial dimensions. This is a quantum phase transition, driven by electron interactions, which spontaneously reduces the point-group symmetry from square to rectangular. The critical point is described by an infinite set of 2+1 dimensional local field theories, labeled by points on the Fermi surface. Each field theory contains a real scalar field representing the Ising order parameter, and fermionic fields representing a time-reversed pair of patches on the Fermi surface. We demonstrate that…
Understanding optical conductivity data in the optimally doped cuprates in the framework of quantum criticality requires a strongly-coupled quantum critical metal which violates hyperscaling. In the simplest scaling framework, hyperscaling violation can be characterized by a single non-zero exponent $θ$, so that in a spatially isotropic state in $d$ spatial dimensions, the specific heat scales with temperature as $T^{(d-θ)/z}$, and the optical conductivity scales with frequency as $ω^{(d-θ-2)/z}$ for $ω\gg T$, where $z$ is the dynamic critical exponent. We study the Ising-nematic critical poin…
Using functional renormalization group methods, we study an effective low-energy model describing the Ising-nematic quantum critical point in two-dimensional metals. We treat both gapless fermionic and bosonic degrees of freedom on equal footing and explicitly calculate the momentum and frequency dependent effective interaction between the fermions mediated by the bosonic fluctuations. Following earlier work by S.-S. Lee for a one-patch model, Metlitski and Sachdev [Phys. Rev. B {\bf{82}}, 075127] recently found within a field-theoretical approach that certain three-loop diagrams strongly modi…
An electron nematic is a translationally invariant state which spontaneously breaks the discrete rotational symmetry of a host crystal. In a clean square lattice, the electron nematic has two preferred orientations, while dopant disorder favors one or the other orientations locally. In this way, the electron nematic in a host crystal maps to the random field Ising model (RFIM). Since the electron nematic has anisotropic conductivity, we associate each Ising configuration with a resistor network, and use what is known about the RFIM to predict new ways to test for electron nematicity using nois…
Using determinantal quantum Monte Carlo, we compute the properties of a lattice model with spin $\frac 1 2$ itinerant electrons tuned through a quantum phase transition to an Ising nematic phase. The nematic fluctuations induce superconductivity with a broad dome in the superconducting $T_c$ enclosing the nematic quantum critical point. For temperatures above $T_c$, we see strikingly non-Fermi liquid behavior, including a "nodal - anti nodal dichotomy" reminiscent of that seen in several transition metal oxides. In addition, the critical fluctuations have a strong effect on the low frequency o…
We revisit the problem of electrons on a square lattice below half filling close to an Ising-nematic quantum critical point. For Fermi surfaces with sufficiently strong antinodal nesting, the static nematic susceptibility is maximal at the antinodal nesting wave vector within a simple RPA calculation. We present a detailed analysis of the nematic susceptibility within Eliashberg theory and show that the strong interaction between Fermions in the antinodal regions shifts the maximum of the nematic susceptibility to slightly larger wave vectors. The corresponding order is akin to the incommensur…
The quantum phase transition in iron-based superconductors with 'half-Dirac' node at the electron Fermi surface as a $T=0$ structural phase transition described in terms of nematic order is discussed. An effective low energy theory that describes half-Dirac nodal Fermions and their coupling to Ising nematic order that describes the phase transition is derived and analyzed using renormalization group (RG) study of the large-$N_f$ version of the theory. The inherent absence of Lorentz invariance of the theory leads to RG flow structure where the velocities $v_F$ and $v_Δ$ at the paired half-Dira…
Electronic nematicity, a correlated state that spontaneously breaks rotational symmetry, is observed in several layered quantum materials. In contrast to their liquid-crystal counterparts, the nematic director cannot usually point in an arbitrary direction (XY nematics), but is locked by the crystal to discrete directions (Ising nematics),resulting in strongly anisotropic fluctuations above the transition. Here, we report on the observation of nearly isotropic XY-nematic fluctuations, via elastoresistance measurements, in hole-doped Ba$_{1-x}$Rb$_{x}$Fe$_{2}$As$_{2}$ iron-based superconductors…
Spin-driven nematic order that has been proposed for iron-based superconductors is generated by pronounced fluctuations of a striped density wave state. On the other hand it is a well known fact that nematic order parameter couples bilinearly to the strain, which supresses the fluctuations of the nematic order parameter itself and lowers the upper critical dimension, yielding mean-field behaviour of the nematic degrees of freedom for $d>2$. This is consistent with the measured Currie-Weiss behaviour of the nematic susceptibility. Here we reconcile this apparent contradiction between pronounced…
Electrical transport properties near an electronic Ising-nematic quantum critical point in two dimensions are of both theoretical and experimental interest. In this work, we derive a kinetic equation valid in a broad regime near the quantum critical point using the memory matrix approach. The formalism is applied to study the effect of the critical fluctuations on the dc resistivity through different scattering mechanisms, including umklapp, impurity scattering, and electron-hole scattering in a compensated metal. We show that electrical transport in the quantum critical regime exhibits a rich…
Using a specially designed Monte Carlo algorithm with directed loops, we investigate the triangular lattice Ising antiferromagnet with coupling beyond nearest neighbour. We show that the first-order transition from the stripe state to the paramagnet can be split, giving rise to an intermediate nematic phase in which algebraic correlations coexist with a broken symmetry. Furthermore, we demonstrate the emergence of several properties of a more topological nature such as fractional edge excitations in the stripe state, the proliferation of double domain walls in the nematic phase, and the Kastel…
We analyze the scaling theory of two-dimensional metallic electron systems in the presence of critical bosonic fluctuations with small wave vectors, which are either due to a U(1) gauge field, or generated by an Ising nematic quantum critical point. The one-loop dynamical exponent z=3 of these critical systems was shown previously to be robust up to three-loop order. We show that the cancellations preventing anomalous contributions to z at three-loop order have special reasons, such that anomalous dynamical scaling emerges at four-loop order.
Quantum spin ice materials, pyrochlore magnets with competing Ising and transverse exchange interactions, have been widely discussed as candidates for a quantum spin-liquid ground state. Here, motivated by quantum chemical calculations for Pr pyrochlores, we present the results of a study for frustrated transverse exchange. Using a combination of variational calculations, exact diagonalisation, numerical linked-cluster and series expansions, we find that the previously-studied U(1) quantum spin liquid, in its pi-flux phase, transforms into a nematic quantum spin liquid at a high-symmetry, SU(2…
TmVO$_4$ exhibits ferroquadrupolar order below 2.15 K with a well-isolated non-Kramers ground state doublet, and is a model system to understand Ising nematic order. We present $^{51}$V nuclear magnetic resonance data as a function of field orientation in a single crystal. Although the spectra are well understood in terms of direct dipolar hyperfine couplings, the spin lattice relaxation rate exhibits strong anisotropy that cannot be understood in terms of magnetic fluctuations. We find that the spin lattice relaxation rate scales with the shear elastic constant associated with the ferroquadru…
We report high-resolution measurements of the in-plane thermal expansion anisotropy in the vicinity of the electronic nematic phase in Sr$_3$Ru$_2$O$_7$ down to very low temperatures and in varying magnetic field orientation. For fields applied along the c-direction, a clear second-order phase transition is found at the nematic phase, with critical behavior compatible with the two-dimensional Ising universality class (although this is not fully conclusive). Measurements in a slightly tilted magnetic field reveal a broken four-fold in-plane rotational symmetry, not only within the nematic phase…
Nematic Ising superconductivity with hidden magnetism in few-layer 6R-TaS2
Peking University(北京大学);Beijing Academy of Quantum Information Sciences(北京量子信息科学研究院);Shanghai Jiao Tong University(上海交通大学);Southern University of Science and Technology(南方科技大学);ShanghaiTech University(上海科技大学);Fudan University(复旦大学);University of Chinese Academy of Sciences(中国科学院大学);Hefei National Laboratory(合肥国家实验室);Hong Kong University of Science and Technology(香港科技大学)
As in between liquid and crystal phases lies a nematic liquid crystal, which breaks rotation with preservation of translation symmetry, there is a nematic superfluid phase bridging a superfluid and a supersolid. The nematic order also emerges in interacting electrons and has been found to largely intertwine with multi-orbital correlation in high-temperature superconductivity, where Ising nematicity arises from a four-fold rotation symmetry $C_4$ broken down to $C_2$. Here we report an observation of a three-state ($\mathbb{Z}_3$) quantum nematic order, dubbed "Potts-nematicity", in a system of…
Recent neutron scattering observations by Plumb et al. [1] reveal that the ground state of $FeSc_2S_4$ is magnetic with two distinct Fe environments, instead of a quantum spin liquid as had been previously thought. Starting with the relevant O(N)-symmetric vector model of $FeSc_2S_4$, we study how the discrete ($Z_2$) and continuous rotational symmetries are successively broken, yielding nematic and ordered phases. At high temperatures, we find that the nematic order parameter falls as $T^{-γ}$ ($γ>0$), and therefore, $FeSc_2S_4$ lacks any distinct nematic ordering temperature. This feature in…
We use inelastic neutron scattering to study the temperature and energy dependence of the spin excitation anisotropy in uniaxial-strained electron-doped iron pnictide BaFe$_{1.9}$Ni$_{0.1}$As$_2$ near optimal superconductivity ($T_c=20$ K). Our work has been motivated by the observation of in-plane resistivity anisotropy in the paramagnetic tetragonal phase of electron-underdoped iron pnictides under uniaxial pressure, which has been attributed to a spin-driven Ising-nematic state or orbital ordering. Here we show that the spin excitation anisotropy, a signature of the spin-driven Ising-nemati…
We explore the propagation of a single hole in the quantum compass model, whose nematic ground state is given by mutually decoupled antiferromagnetic chains. The compass model can be seen as the strong-coupling limit of a spinless two-band Hubbard model, which we study here using mean field theory and the variational cluster approach. Due to the symmetries of the compass model, the inherent disorder along one lattice direction turns out not to affect hole motion and doping a hole consequently does not lift the subextensive degeneracy of the nematic phase. In order to broaden and deepen underst…
We examine the quantum theory of the spontaneous breaking of lattice rotation symmetry in d-wave superconductors on the square lattice. This is described by a field theory of an Ising nematic order parameter coupled to the gapless fermionic quasiparticles. We determine the structure of the renormalization group to all orders in a 1/N_f expansion, where N_f is the number of fermion spin components. Asymptotically exact results are obtained for the quantum critical theory in which, as in the large N_f theory, the nematic order has a large anomalous dimension, and the fermion spectral functions a…
We address the quantum-critical behavior of a two-dimensional itinerant ferromagnetic systems described by a spin-fermion model in which fermions interact with close to critical bosonic modes. We consider Heisenberg ferromagnets, Ising ferromagnets, and the Ising nematic transition. Mean-field theory close to the quantum critical point predicts a superconducting gap with spin-triplet symmetry for the ferromagnetic systems and a singlet gap for the nematic scenario. Studying fluctuations in this ordered phase using a nonlinear sigma model, we find that these fluctuations are not suppressed by a…
We show that the interference between scattering by impurities and by critical spin fluctuations gives rise to anisotropic transport in the Ising-nematic state of the iron pnictides. The effect is closely related to the non-Fermi liquid behavior of the resistivity near an antiferromagnetic quantum critical point. Our theory not only explains the observed sign of the resistivity anisotropy $Δρ$ in electron doped systems, but also predicts a sign change of $Δρ$ upon sufficient hole doping. Furthermore, our model naturally addresses the changes in $Δρ$ upon sample annealing and alkaline-earth sub…
Considerations of the bad-metal behavior led to an early proposal for a quantum critical point under a P for As doping in the iron pnictides, which has since been experimentally observed. We study here an effective model for the isoelectronically tuned pnictides using a large-$N$ approach. The model contains antiferromagnetic and Ising-nematic order parameters appropriate for $J_1$-$J_2$ exchange-coupled local moments on an Fe square lattice, and a damping caused by coherent itinerant electrons. The zero-temperature magnetic and Ising transitions are concurrent and essentially continuous. The …
The origin of the 90 K nematic transition in the chalcogenide FeSe, which displays no magnetic order down to T=0, remains a major puzzle for a unifying theory for the iron-based superconductors. We analyze this problem in light of recent experimental data which reveal very small Fermi pockets in this material. We show that the smallness of the Fermi energy leads to a near-degeneracy between magnetic fluctuations and fluctuations in the charge-current density-wave channel. While the two fluctuation modes cooperate to promote the same preemptive Ising-nematic order, they compete for primary orde…
We report a Raman scattering study of nematic degrees of freedom in the iron-based superconductor parent compound BaFe$_2$As$_2$ under tunable uniaxial strain. We demonstrate that the polarization resolved arsenic (As) phonon intensity can be used to monitor the nematic order parameter as a function of both temperature and strain. At low temperature in the nematic ordered phase we use it to track the continuous and reversible orientation of nematic domains under variable strain. At higher temperature, the evolution of the As phonon intensity under strain reflects an enhanced nematic susceptibi…
Nematic order is the breaking of rotational symmetry in the presence of translational invariance. While originally defined in the context of liquid crystals, the concept of nematic order has arisen in crystalline matter with discrete rotational symmetry, most prominently in the tetragonal Fe-based superconductors where the parent state is four-fold symmetric. In this case the nematic director takes on only two directions, and the order parameter in such "Ising-nematic" systems is a simple scalar. Here, using a novel spatially-resolved optical polarimetry technique, we show that a qualitatively…
Motivated by recent reports of nematic order in twisted bilayer graphene (TBG), we investigate the impact of the triangular moiré superlattice degrees of freedom on nematicity. In TBG, the nematic order parameter is not Ising-like, as it is the case in tetragonal crystals, but has a 3-state Potts character related to the threefold rotational symmetry ($C_{3z}$) of the moiré superlattice. We find that even in the presence of static strain that explicitly breaks the $C_{3z}$ symmetry, the system can still undergo a nematic-flop phase transition that spontaneously breaks in-plane twofold rotation…
The development of collective long-range order via phase transitions occurs by the spontaneous breaking of fundamental symmetries. Magnetism is a consequence of broken time-reversal symmetry while superfluidity results from broken gauge invariance. The broken symmetry that develops below 17.5K in the heavy fermion compound URu2Si2 has long eluded such identification. Here we show that the recent observation of Ising quasiparticles in URu2Si2 results from a spinor order parameter that breaks double time-reversal symmetry, mixing states of integer and half-integer spin. Such "hastatic order" hyb…
The broken symmetry that develops below 17.5K in the heavy fermion compound URu2Si2 has long eluded identification. Here we argue that the recent observation of Ising quasiparticles in URu2Si2 results from a spinor hybridization order parameter that breaks double time-reversal symmetry by mixing states of integer and half-integer spin. Such "hastatic order" (hasta:[Latin]spear) hybridizes Kramers conduction electrons with Ising, non-Kramers 5f2 states of the uranium atoms to produce Ising quasiparticles. The development of a spinorial hybridization at 17.5K accounts for both the large entropy …
We study the character of an Ising nematic quantum phase transition (QPT) deep inside a d-wave superconducting state with nodal quasiparticles in a two-dimensional tetragonal crystal. We find that, within a 1/N expansion, the transition is continuous. To leading order in 1/N, quantum fluctuations enhance the dispersion anisotropy of the nodal excitations, and cause strong scattering which critically broadens the quasiparticle (qp) peaks in the spectral function, except in a narrow wedge in momentum space near the Fermi surface where the qp's remain sharp. We also consider the possible existenc…