Comparative scintillation performance of EJ-309, EJ-276, and a novel organic glass
T. A. Laplace, B. L. Goldblum, J. E. Bevins, D. L. Bleuel, E. Bourret, J. A. Brown, E. J. Callaghan, J. S. Carlson, P. L. Feng, G. Gabella, K. P. Harrig, J. J. … 展开作者
T. A. Laplace, B. L. Goldblum, J. E. Bevins, D. L. Bleuel, E. Bourret, J. A. Brown, E. J. Callaghan, J. S. Carlson, P. L. Feng, G. Gabella, K. P. Harrig, J. J. Manfredi, C. Moore, F. Moretti, M. Shinner, A. Sweet, Z. W. Sweger
An organic glass scintillator developed by Sandia National Laboratories was characterized in terms of its light output and pulse shape discrimination (PSD) properties and compared to commercial liquid (EJ-309) and plastic (EJ-276) organic scintillators. The electron light output was determined through relative comparison of the $^{137}$Cs Compton edge location. The proton light yield was measured using a double time-of-flight technique at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a tunable broad-spectrum neutron source and an array of pulse-shape-discriminating observation scintillators, a continuous measurement of the proton light yield was performed for EJ-309 (200 keV$-$3.2 MeV), EJ-276 (170 keV$-$4.9 MeV), and the organic glass (50 keV$-$20 MeV). Finally, the PSD properties of the organic glass, EJ-309, and EJ-276 were evaluated using an AmBe source and compared via a figure-of-merit metric. The organic glass exhibited a higher electron light output than both EJ-309 and EJ-276. Its proton light yield and PSD performance were comparable to EJ-309 and superior to that of EJ-276. With these performance characteristics, the organic glass scintillator is well poised to replace current state-of-the-art PSD-capable scintillators in a range of fast neutron detection applications.
The scintillation anisotropy effect for proton recoil events has been investigated in five pure organic crystalline materials: anthracene, trans-stilbene, p-terphenyl, bibenzyl, and diphenylacetylene. These measurements include characterization of the scintillation response for one hemisphere of proton recoil directions in each crystal. In addition to standard measurements of the total light output and pulse shape at each angle, the prompt and delayed light anisotropies are analyzed, allowing for investigation of the singlet and triplet molecular excitation behaviors independently. This work p…
A novel algorithm for the discrimination of neutron and γ-ray with wavelet transform modulus maximum (WTMM) in an organic scintillation has been investigated. Voltage pulses arising from a BC501A organic liquid scintillation detector in a mixed radiation field have been recorded with a fast digital sampling oscilloscope. The performances of most pulse shape discrimination methods in scintillation detection systems using time-domain features of the pulses are affected intensively by noise. However, the WTMM method using frequency-domain features exhibits a strong insensitivity to noise and can …
The CHErenkov / Scintillation Separation experiment (CHESS) has been used to demonstrate the separation of Cherenkov and scintillation light in both linear alkylbenzene (LAB) and LAB with 2g/L of PPO as a fluor (LAB/PPO). This is the first such demonstration for the more challenging LAB/PPO cocktail and improves on previous results for LAB. A time resolution of 338 +/- 12 ps FWHM results in an efficiency for identifying Cherenkov photons in LAB/PPO of 70 +/- 3% and 63 +/- 8% for time- and charge-based separation, respectively, with scintillation contamination of 36 +/- 5% and 38 +/- 4%. LAB/PP…
The proton light yield of organic scintillators has been measured extensively in recent years using fast waveform digitizers and large discrepancies exist in the values reported by different authors. In this letter, we address principles of digital signal processing that must be considered when conducting scintillator light yield measurements. Digitized waveform pulse height values are only proportional to the amount of scintillation light if the temporal shape of the scintillation pulse is independent of the amount of energy deposited. This is not the case for scintillation pulses resulting f…
We report on a comparison study of the $^{3}$He gas proportional tube and the $^{6}$Li incorporated scintillation glasses on thermal neutron detection efficiency. Both $^{3}$He and $^{6}$Li are used commonly for thermal neutron detection because of their high neutron capture absorption coefficient. By using a neutron source $^{252}$Cf and a paraffin moderator in an alignment system, we can get a small beam of thermal neutrons. A flash ADC is used to measure the thermal neutron spectrum of each detector, and the detected number of events is determined from the spectrum, then we can calculate th…
A light-yield calibration of an NE 213A organic liquid scintillator detector has been performed using both monoenergetic and polyenergetic gamma-ray sources. Scintillation light was detected in a photomultiplier tube, and the corresponding pulses were subjected to waveform digitization on an event-by-event basis. The resulting Compton edges have been analyzed using a Geant4 simulation of the detector which models both the interactions of the ionizing radiation as well as the transport of scintillation photons. The simulation is calibrated and also compared to well-established prescriptions use…
This paper reports a series of measurements that characterize the directional dependence of the scintillation response of crystalline melt-grown and solution-grown stilbene to incident DT and DD neutrons. These measurements give the amplitude and pulse shape dependence on the proton recoil direction over one hemisphere of the crystal, confirming and extending previous results in the literature for melt-grown stilbene and providing the first measurements for solution-grown stilbene. In similar measurements of liquid and plastic detectors, no directional dependence was observed, confirming the h…
In this manuscript we report on the scintillation properties and pulse shape discrimination (PSD) performance of new organic glass scintillator. Two cylindrical samples with dimensions of 2x2 inches were tested. Additionally, this two samples were used in stack configuration in order to measure the PSD characteristics of a sample with a size of 2x4 inches. The study covers the measurements of neutron/gamma discrimination capability, emission spectra, photoelectron yield and analysis of the light pulse shapes originating from events related to gamma-rays and fast neutrons. The results were comp…
The NUCLEUS experiment aims at measuring the coherent elastic scattering of nuclear reactor antineutrinos off nuclei using cryogenic calorimeters. Operating at an overburden of 3m.w.e., muon-induced backgrounds are expected to be dominant. It is therefore essential to develop an efficient muon veto, with a detection efficiency of more than 99%. This will be realized in NUCLEUS through a compact cube assembly of plastic scintillator panels. In order to prevent a large unshielded area where the cryostat intersects the shielding arrangement without unnecessarily increasing the induced detector de…
The detection of primary scintillation light in combination with the charge or secondary scintillation signals is an efficient technique to determine the events t=0 as well as particle / photon separation in large mass TPC detectors filled with noble gases and/or condensed noble gases. The aim of this work is to demonstrate that costly photo-multipliers could be replaced by cheap novel photosensitive gaseous detectors: wire counters, GEMs or glass capillary tubes coupled with CsI photocathodes. We have performed systematic measurements with Ar, Kr and Xe gas at pressures in the range of 1-50 a…
Scintillators are employed for particle detection and identification using light-pulse shapes and light quenching factors. We developed a comprehensive model describing the light generation and quenching in CaWO$_4$ single crystals used for direct dark matter search. All observed particle-dependent light-emission characteristics can be explained quantitatively, light-quenching factors and light-pulse shapes are calculated on a microscopic basis. This model can be extended to other scintillators such as inorganic crystal scintillators, liquid noble gases or organic liquid scintillators.
In order to develop a high spatial resolution (micron level) thermal neutron detector, a detector assembly composed of cerium doped lithium glass microfibers, each with a diameter of 1\,$μ$m, is proposed, where the neutron absorption location is reconstructed from the observed charged particle products that result from neutron absorption. To suppress the cross talk of the scintillation light, each scintillating fiber is surrounded by air-filled glass capillaries with the same diameter as the fiber. This pattern is repeated to form a bulk microfiber detector. On one end, the surface of the dete…
A successfull application of Geiger-mode multipixel avalanche diodes (GMAPDs) for pulse-shape discrimination in alpha-beta spectrometry using organic liquid scintillator is described in this paper. Efficient discrimination of alpha and beta components in the emission of radioactive isotopes is achieved for alpha energies above 0.3 MeV. The ultra-compact design of the scintillating detector helps to efficiently suppress cosmic-ray and ambient radiation background. This approach allows construction of hand-held robust devices for monitoring of radioactive contamination in various environmental c…
Organic liquid scintillators are used in a wide variety of applications in experimental nuclear and particle physics. Boron-loaded scintillators are particularly useful for detecting neutron captures, due to the high thermal neutron capture cross section of $^{10}$B. These scintillators are commonly used in neutron detectors, including the DarkSide-50 neutron veto, where the neutron may produce a signal when it scatters off protons in the scintillator or when it captures on $^{10}$B. Reconstructing the energy of these recoils is complicated by scintillation quenching. Understanding how nuclear…
Liquid noble based particle detectors often use the organic wavelength shifter 1,1,4,4- tetraphenyl-1,3-butadiene (TPB) which shifts UV scintillation light to the visible regime, facilitating its detection, but which also can scintillate on its own. Dark matter searches based on this type of detector commonly rely on pulse-shape discrimination (PSD) for background mitigation. Alpha-induced scintillation therefore represents a possible background source in dark matter searches. The timing characteristics of this scintillation determine whether this background can be mitigated through PSD. We ha…
This paper presents the model-based design and evaluation of an instrument that estimates incident neutron direction using the kinematics of neutron scattering by hydrogen-1 nuclei in an organic scintillator. The instrument design uses a single, nearly contiguous volume of organic scintillator that is internally subdivided only as necessary to create optically isolated pillars. Scintillation light emitted in a given pillar is confined to that pillar by a combination of total internal reflection and a specular reflector applied to the four sides of the pillar transverse to its long axis. The sc…
The response of a position-sensitive Li-glass based scintillation detector to focused beams of 2.5 MeV protons and deuterons has been investigated. The beams were scanned across the detector in 0.5 mm horizontal and vertical steps perpendicular to the beams. Scintillation light was registered using an 8 by 8 pixel multi-anode photomultiplier tube. The signal amplitudes were recorded for each pixel on an event-by-event basis. Several pixels generally registered considerable signals at each beam location. The number of pixels above set thresholds were investigated, with the optimization of the s…
TetraPhenyl Butadiene is the wavelength shifter most widely used in combination with liquid Argon. The latter emits scintillation photons with a wavelength of 127 nm that need to be downshifted to be detected by photomultipliers with glass or quartz windows. TetraPhenyl Butadiene has been demonstrated to have an extremely high conversion efficiency, possibly higher than 100 % for 127 nm photons, while there is no precise information about the time dependence of its emission. It is usually assumed to be exponentially decaying with a characteristic time of the order of one ns, as an extrapolatio…
In recent years, demand for scintillation detectors with high time resolution (better than 100 ps) has emerged in high-energy physics and medical imaging applications. In particular, time of flight positron emission tomography (TOF-PET) can greatly benefit from increasing time resolution of scintillators, which leads to the increase of signal-to-noise ratio, decrease of patient dose, and achievement of the superior spatial resolution of PET images. Currently, extensive research of various types of materials is carried out to achieve the best time resolution. In this review, the recent progress…
Fast-neutron/gamma-ray pulse-shape discrimination has been performed for the organic liquid scintillators NE 213A and EJ 305 using a time-of-flight based neutron-tagging technique and waveform digitization on an event-by-event basis. Gamma-ray sources and a Geant4-based simulation were used to calibrate the scintillation-light yield. The difference in pulse shape for the neutron and gamma-ray events was analysed by integrating selected portions of the digitized waveform to produce a figure-of-merit for neutron/gamma-ray separation. This figure-of-merit has been mapped as a function of detector…
Scintillators with pulse-shape discrimination (PSD) capability are of great interest to many fields in the scientific community. The ability to discern a gamma ray from a neutron using PSD varies between different types of scintillator materials and dopants. A new generation of organic scintillator materials with PSD capability were studied to determine their radiation hardness to ionizing and non-ionizing radiation. The PSD capability, average pulse shapes, and light output of four types of organic scintillator were characterized before and after neutron and gamma-ray irradiation. The main go…
Plastic scintillators that can discriminate between gamma rays, fast neutrons, and thermal neutrons were synthesized and characterized while considering the balance between processing and performance at the kilogram scale. These trade-offs were necessitated by the inclusion of 0.1 wt. % lithium-6 to enable detection of thermal neutrons. The synthesis and processing of these plastic scintillators on the kilogram scale required consideration of many factors. First, a comonomer (methacrylic acid) was used to solubilize salts of lithium-6, which allow for a thermal-neutron capture reaction that pr…
The characteristics of the Solid-state Neutron Detector, under development for neutron-scattering measurements at the European Spallation Source, have been simulated with a Geant4-based computer code. The code models the interations of thermal neutrons and ionising radiation in the 6Li-doped scintillating glass of the detector, the production of scintillation light and the transport of optical, scintillation photons through the the scintillator, en route to the photo-cathode of the attached multi-anode photomultiplier. Factors which affect the optical-photon transport, such as surface finish, …
A new type of neutron detector, named Stack Structure Solid organic Scintillator (S$^4$), consisting of multi-layer plastic scintillators with capability to suppress low-energy $γ$ rays under high-counting rate has been constructed and tested. To achieve $\it{n}$-$γ$ discrimination, we exploit the difference in the ranges of the secondary charged particles produced by the interactions of neutrons and $γ$ rays in the scintillator material. The thickness of a plastic scintillator layer was determined based on the results of Monte Carlo simulations using the Geant4 toolkit. With layer thicknesses…
We report on the study of a new liquid scintillator target for neutrino interactions in the framework of the research and development program of the BOREXINO solar neutrino experiment. The scintillator consists of 1,2-dimethyl-4-(1-phenylethyl)-benzene (phenyl-o-xylylethane, PXE) as solvent and 1,4-diphenylbenzene (para-Terphenyl, p-Tp) as primary and 1,4-bis(2-methylstyryl)benzene (bis-MSB) as secondary solute. The density close to that of water and the high flash point makes it an attractive option for large scintillation detectors in general. The study focused on optical properties, radioac…
Electron anti-neutrinos are commonly detected in liquid scintillator experiments via inverse beta decay, by looking at the coincidence between the reaction products, neutron and positron. Prior to positron annihilation, an electron-positron pair may form an orthopositronium (o-Ps) state, with a mean life of a few ns. Even if the o-Ps decay is speeded up by spin flip or pick off effects, it may introduce distortions in the photon emission time distribution, crucial for position reconstruction and pulse shape discrimination algorithms in anti-neutrino experiments. Reversing the problem, the o-Ps…
The scintillation detection systems of liquid argon time projection chambers (LArTPCs) require wavelength shifters to detect the 128 nm scintillation light produced in liquid argon. Tetraphenyl butadiene (TPB) is a fluorescent material that can shift this light to a wavelength of 425 nm, lending itself well to use in these detectors. We can coat the glass of photomultiplier tubes (PMTs) with TPB or place TPB-coated plates in front of the PMTs. In this paper, we investigate the degradation of a chemical TPB coating in a laboratory or factory environment to assess the viability of long-term TPB …
Performance and pulse shape discrimination of glass scintillator SG101 for neutron detection
School of Physics, Sun Yat-sen University（中山大学物理学院）；Institut Franco-Chinois de l’Énergie Nucléaire , Sun Yat-sen University（中法核能源学院，中山大学）；School of Science, Sun Yat-sen University（中山大学理学院）；Beijing Hoton Technology Co.Ltd.（北京霍顿科技有限公司）
We has set up a light scattering spectrometer to study the depolarization of light scattering in linear alkylbenzene. From the scattering spectra it can be unambiguously shown that the depolarized part of light scattering belongs to Rayleigh scattering. The additional depolarized Rayleigh scattering can make the effective transparency of linear alkylbenzene much better than it was expected. Therefore sufficient scintillation photons can transmit through the large liquid scintillator detector of JUNO. Our study is crucial to achieving the unprecedented energy resolution 3\%/$\sqrt{E\mathrm{(MeV…
