Organic scintillators exhibit fast timing, high detection efficiency for fast neutrons and pulse shape discrimination (PSD) capability. PSD is essential in mixed radiation fields, where different types of radiation need to be detected and discriminated. In neutron measurements for nuclear security and non proliferation effective PSD is crucial, because a weak neutron signature needs to be detected in the presence of a strong gamma-ray background. The most commonly used deterministic PSD technique is charge integration (CI). This method requires the optimization of specific parameters to obtain the best gamma-neutron separation. These parameters depend on the scintillating material and light readout device and typically require a lengthy optimization process and a calibration reference measurement with a mixed source. In this paper, we propose a new method based on the scintillation fluorescence physics that enables to find the optimum PSD integration gates using only a gamma-ray emitter. We demonstrate our method using three organic scintillation detectors: deuterated trans-stilbene, small-molecule organic glass, and EJ-309. In all the investigated cases, our method allowed finding the optimum PSD CI parameters without the need of iterative optimization.
A pulse-shape discrimination method based on artificial neural networks was applied to pulses simulated for different background, signal and signal-like interactions inside a germanium detector. The simulated pulses were used to investigate variations of efficiencies as a function of used training set. It is verified that neural networks are well-suited to identify background pulses in true-coaxial high-purity germanium detectors. The systematic uncertainty on the signal recognition efficiency derived using signal-like evaluation samples from calibration measurements is estimated to be 5\%. Th…
The basic principles of detection of fast neutrons with liquid scintillator detectors are reviewed, together with a real example in the form of the Neutron Wall array. Two of the challenges in neutron detection, discrimination of neutrons and gamma rays and identification of cross talk between detectors due to neutron scattering, are briefly discussed, as well as possible solutions to these problems. The possibilities of using digital techniques for pulse-shape discrimination are examined. Results from a digital and analog versions of the zero cross-over algorithm are presented. The digital pu…
Fast-neutron/gamma-ray pulse-shape discrimination has been performed for the organic liquid scintillators NE 213A and EJ 305 using a time-of-flight based neutron-tagging technique and waveform digitization on an event-by-event basis. Gamma-ray sources and a Geant4-based simulation were used to calibrate the scintillation-light yield. The difference in pulse shape for the neutron and gamma-ray events was analysed by integrating selected portions of the digitized waveform to produce a figure-of-merit for neutron/gamma-ray separation. This figure-of-merit has been mapped as a function of detector…
A comparative study of the neutron-$γ$ Pulse Shape Discrimination (PSD) with seven organic scintillators is performed using an identical setup and digital electronics. The scintillators include plastics (EJ-299-33 and a plastic prototype), single crystals (stilbene and the recent doped $p$-terphenyl) and liquids (BC501A, NE213 and the deuterated liquid BC537). First, the overall PSD performance of the different scintillators is compared and threshold neutron energies for a given discrimination quality are determined. Then, using statistical arguments, two intrinsic contributions to the PSD cap…
Various pulse shape discrimination methods have been used to solve the neutron-gamma discrimination problem. But most of them are limited to off-line calculation due to the computation amount and FPGA performance. In order to realize real time discriminating neutron and gamma, a new algorithm based on the traditional pulse shape discrimination methods was proposed in this paper. The new algorithm takes into account the physical properties of the pulse signal, which greatly reduces the computation and dead time without losing the precision, and can work on FPGA directly. It has a good performan…
The continued advancements of Silicon Photomultipliers (SiPMs) have made them viable photosensors for low recoil energy Pulse Shape Discrimination (PSD) between fast neutron and gamma interactions when coupled to an appropriate scintillator. At the same time, the large number of channels in a typical array calls for the development of low-cost and low-power electronics. A custom integrated circuit (ASIC) is an ideal solution for this purpose. To assess the requirements for such an ASIC, studies were performed using two scintillators, Stilbene and EJ-276, coupled to a 6 x 6 mm SiPM from Onsemi.…
Discrimination of the detection of fast neutrons and gamma rays in a liquid scintillator detector has been investigated using digital pulse-processing techniques. An experimental setup with a 252Cf source, a BC-501 liquid scintillator detector, and a BaF2 detector was used to collect waveforms with a 100 Ms/s, 14 bit sampling ADC. Three identical ADC's were combined to increase the sampling frequency to 300 Ms/s. Four different digital pulse-shape analysis algorithms were developed and compared to each other and to data obtained with an analogue neutron-gamma discrimination unit. Two of the di…
A successfull application of Geiger-mode multipixel avalanche diodes (GMAPDs) for pulse-shape discrimination in alpha-beta spectrometry using organic liquid scintillator is described in this paper. Efficient discrimination of alpha and beta components in the emission of radioactive isotopes is achieved for alpha energies above 0.3 MeV. The ultra-compact design of the scintillating detector helps to efficiently suppress cosmic-ray and ambient radiation background. This approach allows construction of hand-held robust devices for monitoring of radioactive contamination in various environmental c…
A digital pulse shape discrimination system based on a programmable module NI-5772 has been established and tested with EJ-301 liquid scintillation detector. The module was operated by means of running programs developed in LabVIEW with the sampling frequency up to 1.6GS/s. Standard gamma sources 22Na, 137Cs and 60Co were used to calibrate the EJ-301 liquid scintillation detector, and the gamma response function has been obtained. Digital algorithms for charge comparison method and zero-crossing method have been developed. The experimental results showed that both digital signal processing (DS…
First studies of event discrimination with a Broad-Energy Germanium (BEGe) detector are presented. A novel pulse shape method, exploiting the characteristic electrical field distribution inside BEGe detectors, allows to identify efficiently single-site events and to reject multi-site events. The first are typical for neutrinoless double beta decays (0-nu-2-beta) and the latter for backgrounds from gamma-ray interactions. The obtained survival probabilities of backgrounds at energies close to Q(76Ge) = 2039 keV are 0.93% for events from 60Co, 21% from 226Ra and 40% from 228Th. This background s…
The SNO+ liquid scintillator experiment is under construction in the SNOLAB facility in Canada. The success of this experiment relies upon accurate characterization of the liquid scintillator, linear alkylbenzene (LAB). In this paper, scintillation decay times for alpha and electron excitations in LAB with 2 g/L PPO are presented for both oxygenated and deoxygenated solutions. While deoxygenation is expected to improve pulse shape discrimination in liquid scintillators, it is not commonly demonstrated in the literature. This paper shows that for linear alkylbenzene, deoxygenation improves disc…
Digital pulse shape discrimination has become readily available to distinguish nuclear recoil and electronic recoil events in scintillation detectors. We evaluate digital implementations of pulse shape discrimination algorithms discussed in the literature, namely the Charge Comparison Method, Pulse-Gradient Analysis, Fourier Series and Standard Event fitting. In addition, we present a novel algorithm based on a Laplace Transform. Instead of reducing the performance of these algorithms to a single Figure of Merit, we evaluate them as function of recoil energy. Specifically, using commercial EJ-…
This work describes a class of liquid scintillators that contain mostly water (>50 wt. % of the entire composition) and can discriminate between interactions induced by neutrons and gamma rays. By balancing the interface interactions between the components of the formulation, these scintillators form emulsions that can be thermodynamically stable. This approach, which considers a quantity known as the hydrophilic-lipophilic difference, requires consideration of the salinity and temperature as well as characterization of the surfactants and oil phase. Emulsions comprised of water and various oi…
In beam test experiments have been carried out for particle identification using digital pulse shape analysis in a 500~$μ$m thick Neutron Transmutation Doped (nTD) silicon detector with an indigenously developed FPGA based 12 bit resolution, 1 GHz sampling digitizer. The nTD Si detector was used in a low-field injection setup to detect light heavy-ions produced in reactions of $\sim$ 5 MeV/A $^{7}$Li and $^{12}$C beams on different targets. Pulse height, rise time and current maximum have been obtained from the digitized charge output of a high bandwidth charge and current sensitive pre-amplif…
A novel algorithm for the discrimination of neutron and γ-ray with wavelet transform modulus maximum (WTMM) in an organic scintillation has been investigated. Voltage pulses arising from a BC501A organic liquid scintillation detector in a mixed radiation field have been recorded with a fast digital sampling oscilloscope. The performances of most pulse shape discrimination methods in scintillation detection systems using time-domain features of the pulses are affected intensively by noise. However, the WTMM method using frequency-domain features exhibits a strong insensitivity to noise and can …
We characterized the light output response of a new 140 cm3 stilbene-d12 crystal up to 14.1 MeV neutron energies using a coincidence neutron scattering system. We also characterized its light output response to alpha particles in the 5 to 6~MeV energy range. The excellent PSD capability of the stilbene-d$_{12}$ detector allowed us to select light pulses produced by particles of increasing ionization density, namely electrons, protons, deuterium-ions, and alpha particles. The measured fast decay component of the light pulses is increasingly quenched as the ionization density of the particle in …
Fast digitisers and digital pulse processing have been widely used for spectral application and pulse shape discrimination (PSD) owing to their advantages in terms of compactness, higher trigger rates, offline analysis, etc. Meanwhile, the noise of readout electronics is usually trivial for organic, plastic, or liquid scintillator with PSD ability because of their poor intrinsic energy resolution. However, LaBr3(Ce) has been widely used for its excellent energy resolution and has been proven to have PSD ability for alpha/gamma particles. Therefore, designing a digital acquisition system for su…
(Gd,La)$_2$Si$_2$O$_7$:Ce (La-GPS:Ce) is a new scintillator material with high light output, high energy resolution, and fast decay time. Moreover, the scintillator has a good light output even at high temperature (up to 150$^\circ$C) and is non-hygroscopic in nature; thus, it is especially suitable for underground resource exploration. Particle identification greatly expands the possible applications of scintillator. For resource exploration, the particle identification should be completed in a single pulse only. The pulse-shape discrimination of the scintillator was confirmed. We compared tw…
Frequency gradient analysis (FGA) effectively discriminates neutrons and gamma rays by examining the frequency-domain features of the photomultiplier tube anode signal. This approach is insensitive to noise but is inevitably affected by the baseline drift, similar to other pulse shape discrimination methods. The baseline drift effect is attributed to the factors such as power line fluctuation, dark current, noise disturbances, hum, and pulse tail in front-end electronics. This effect needs to be elucidated and quantified before the baseline shift can be estimated and removed from the captured …
The CDEX (China Dark matter Experiment) now deploys ~10 kg pPCGe (p-type Point Contact Germanium) detectors in CJPL (China Jinping Underground Laboratory). It aims to detect rare events such as dark matter and 0vbb (neutrinoless double beta decay). The discrimination of bulk and very bulk events are essential for improvements of the analysis threshold of dark matter. Very bulk events are generated near the p+ point surface of pPCGe, which are usually from radioactive materials of electronic devices. Due to different locations of charge collection, bulk and very bulk events have different pulse…
In this study, we evaluate and compare the pulse shape discrimination (PSD) performance of multipixel photon counters (MPPCs, also known as silicon photomultiphers - SiPMs) with that of a typical photomultiplier tube (PMT) when testing using CsI(Tl) scintillators. We use the charge comparison method, whereby we discriminate different types of particles by the ratio of charges integrated within two time-gates (the delayed part and the entire digitized waveform). For a satisfactory PSD performance, a setup should generate many photoelectrons (p.e.) and collect their charges efficiently. The PMT …
A brief outline of Dark Matter detection experiments using liquid argon technology is presented. The Pulse Shape background discrimination method (PSD) is described and the example of its use in 2.3 l R&D detector is given. Methods of calculating sensitivity of a Dark Matter detector are discussed and used to estimate the possible improvement of sensitivity after introduction of isotopically depleted liquid argon.
In the framework of the ``ULTIMA'' project, we use ultra cold superfluid 3He bolometers for the direct detection of single particle events, aimed for a future use as a dark matter detector. One parameter of the pulse shape observed after such an event is the thermalization time constant. Until now it was believed that this parameter only depends on geometrical factors and superfluid 3He properties, and that it is independent of the nature of the incident particles. In this report we show new results which demonstrate that a difference for muon- and neutron events, as well as events simulated b…
This paper describes the implementation and performance of CsI(Tl) pulse shape discrimination for the Belle II electromagnetic calorimeter, representing the first application of CsI(Tl) pulse shape discrimination for particle identification at an electron-positron collider. The pulse shape characterization algorithms applied by the Belle II calorimeter are described. Control samples of $γ$, $μ^+$, $π^\pm$, $K^\pm$ and $p/\bar{p}$ are used to demonstrate the significant insight into the secondary particle composition of calorimeter clusters that is provided by CsI(Tl) pulse shape discrimination…
In particle physics experiments, pulse shape discrimination (PSD) is a powerful tool for eliminating the major background from signals. However, the analysis methods have been a bottleneck to improving PSD performance. In this study, two machine learning methods -- multilayer perceptron and convolutional neural network -- were applied to PSD, and their PSD performance was compared with that of conventional analysis methods. Three calcium-based halide scintillators were grown using the vertical Bridgman--Stockbarger method and used for the evaluation of PSD. Compared with conventional analysis …
We measured the decay time of the scintillation pulses produced by electron and nuclear recoils in CaF2(Eu) by a new fitting method. In the recoil energy region 5-30 keVee, we found differences of the decay time between electron and nuclear recoil events. In the recoil energy region above 20 keVee, we found that the decay time is independent of the recoil energy.
There are recent interests with CsI(Tl) scintillating crystals for Dark Matter experiments. The key merit is the capability to differentiate nuclear recoil (nr) signatures from the background $β/ γ$-events due to ambient radioactivity on the basis of their different pulse shapes. One of the major experimental challenges is to perform such pulse shape analysis in the statistics-limited domain where the light output is close to the detection threshold. Using data derived from measurements with low energy $γ$'s and nuclear recoils due to neutron elastic scatterings, it was verified that the pulse…
The use of Time-over-Threshold (TOT) for the discrimination between fast neutrons and gamma-rays is advantageous when large number of detection channels are required due to the simplicity of its implementation. However, the results obtained using the standard, Constant Threshold TOT (CT-TOT) are usually inferior to those obtained using other pulse shape discrimination (PSD) methods, such as Charge Comparison or Zero-Crossing approaches, especially for low amplitude neutron/gamma-ray pulses. We evaluate another TOT approach for fast neutron/gamma-ray PSD using Constant-Fraction Time-over-Thresh…
We report on the characterization of two inverted coaxial Ge detectors in the context of being employed in future $^{76}$Ge neutrinoless double beta ($0νββ$) decay experiments. It is an advantage that such detectors can be produced with bigger Ge mass as compared to the planar Broad Energy Ge detectors (BEGe) that are currently used in the GERDA $0νββ$ decay experiment. This will result in lower background for the search of $0νββ$ decay due to a reduction of cables, electronics and holders. The measured resolution near the $^{76}$Ge Q-value at 2039 keV is 2.5 keV and their pulse-shape characte…
Pulse shape discrimination with pure CsI scintillators is investigated as a method for separating energy deposits by energetic neutrons and photons at particle physics experiments. Using neutron data collected near the European XFEL XS1 beam window the pulse shape discrimination capabilities of pure CsI are studied and compared to CsI(Tl) using near-identical detector setups, which were operated in parallel. The inelastic interactions of 100MeV neutrons are observed to produce a slower scintillation emission in pure CsI relative to energy deposits from cosmic muons. By employing a charge-ratio…
Superheated drop detector (SDD) consisting of drops of superheated liquid of halocarbon is irradiated to neutrons and gamma-rays from 252Cf fission neutron source and 137Cs gamma source separately. The analysis of pulse height of the signals in the neutron and gamma-ray sensitive temperature provides strong information on the identification of neutron and gamma-ray induced events.
There is a key research issue to accurately select out neutron signals and discriminate gamma signals from a mixed radiation field in the neutron detection. This paper proposes a fractal spectrum discrimination approach by means of different spectrum characteristics of neutron and gamma. Figure of merit and average discriminant error ratio are adopted together to evaluate the discriminant effects. Different neutron and gamma signals with various noises and pulse pile-ups are simulated according to real data in the literature. The proposed approach is compared with the digital charge integratio…
Pulse shape discrimination plays a key role in improving the signal-to-background ratio in NEOS analysis by removing fast neutrons. Identifying particles by looking at the tail of the waveform has been an effective and plausible approach for pulse shape discrimination, but has the limitation in sorting low energy particles. As a good alternative, the convolutional neural network can scan the entire waveform as they are to recognize the characteristics of the pulse and perform shape classification of NEOS data. This network provides a powerful identification tool for all energy ranges and helps…
SuperCDMS is the next phase of the Cryogenic Dark Matter Search experiment, which measures both phonon and charge signals generated by particle recoils within a germanium target mass. Charge signals are employed both in the definition of a fiducial volume and in the rejection of electron recoil background events. Alternatively, phonons generated by the charge carriers can also be used for the same two goals. This paper describes preliminary efforts to observe and quantify these contributions to the phonon signal and then use them to reject background events. A simple analysis using only one pu…
Cs$_2$LiLaBr$_6$:Ce$^{3+}$ (CLLB) is an elpasolite scintillator that offers excellent linearity and gamma-ray energy resolution and sensitivity to thermal neutrons with the ability to perform pulse-shape discrimination (PSD) to distinguish gammas and neutrons. Our investigation of CLLB has indicated the presence of intrinsic radioactive alpha background that we have determined to be from actinium contamination of the lanthanum component. We measured the pulse shapes for gamma, thermal neutron, and alpha events and determined that PSD can be performed to separate the alpha background with a mod…
In the last decade, Direct Dark Matter searches has become a very active research program, spawning dozens of projects world wide and leading to contradictory results. It is on this stage that the Dark matter Experiment with liquid Argon and Pulse shape discrimination (DEAP) is about to enter. With a 3600~kg liquid argon target and a 1000~kg fiducial mass, it is designed to run background free during 3 years, reaching an unprecedented sensitivity of 10$^{-46}$~cm$^2$ for a WIMP mass of 100 GeV. In order to achieve this impressive feat, the collaboration followed a two-pronged approach: a caref…
The scintillation mechanism in NaI:Tl crystals produces different pulse shapes that are dependent on the incoming particle type. The time distribution of scintillation light from nuclear recoil events decays faster than for electron recoil events and this difference can be categorised using various Pulse Shape Discrimination (PSD) techniques. In this study, we measured nuclear and electron recoils in a NaI:Tl crystal, with electron equivalent energies between 2 and 40 keV. We report on a new PSD approach, based on an event-type likelihood; this outperforms the charge-weighted mean-time, which …
We report on the results of the positional-dependent pulse shape discrimination (PSD) parameter observed within a monolithic CLLB scintillation crystal. CLLB, a relatively novel inorganic scintillation crystal, is capable of PSD between gamma rays, neutrons, and alpha particles. In this work, we observed distinguishable differences in the pulse shapes for gamma-ray-induced events. The CLLB crystals used for this experiment are 5 cm (diameter) by 10 cm (length). By using monoenergetic 2.614 MeV photons from a set of thoriated welding rods and performing collimated scans along the length of the …
The GERDA experiment searches for neutrinoless double beta ($0νββ$) decay in $^{76}$Ge using an array of high purity germanium (HPGe) detectors immersed in liquid argon (LAr). Phase II of the experiment uses 30 new broad energy germanium (BEGe) detectors with superior pulse shape discrimination capabilities compared to the previously used semi-coaxial detector design. By far the largest background component for BEGe detectors in GERDA are n$^+$-surface events from $^{42}$K $β$ decays which are intrinsic in LAr. The $β$ particles with up to 3.5 MeV can traverse the 0.5 to 0.9 mm thick electrode…
Scintillators with pulse-shape discrimination (PSD) capability are of great interest to many fields in the scientific community. The ability to discern a gamma ray from a neutron using PSD varies between different types of scintillator materials and dopants. A new generation of organic scintillator materials with PSD capability were studied to determine their radiation hardness to ionizing and non-ionizing radiation. The PSD capability, average pulse shapes, and light output of four types of organic scintillator were characterized before and after neutron and gamma-ray irradiation. The main go…
The GRIT (Granularity, Resolution, Identification, Transparency) Silicon array is intended to measure direct reactions. Its design is based on several layers (three layers in the forward direction, two backward) of custom-made trapezoidal and square detectors. The first stage is 500 μm thick and features 128x128 orthogonal strips. Pulse shape analysis for particle identification is implemented for this first layer. Given the compacity of this array and the large number of channels involved (>7,500), an integrated preamplifier, iPACI, that gives charge and current information has been developed…
Pulse shape discrimination using CsI(Tl) scintillators to perform neutral hadron particle identification is explored with emphasis towards application at high energy electron-positron collider experiments. Through the analysis of the pulse shape differences between scintillation pulses from photon and hadronic energy deposits using neutron and proton data collected at TRIUMF, it is shown that the pulse shape variations observed for hadrons can be modelled using a third scintillation component for CsI(Tl), in addition to the standard fast and slow components. Techniques for computing the hadron…
We demonstrate the use of a convolutional neural network to perform neutron-gamma pulse shape discrimination, where the only inputs to the network are the raw digitised SiPM signals from a dual scintillator detector element made of 6LiF:ZnS(Ag) scintillator and PVT plastic. A realistic labelled dataset was created to train the network by exposing the detector to an AmBe source, and a data-driven method utilsing a separate PMT was used to assign labels to the recorded signals. This approach is compared to the charge integration and continuous wavelet transform methods and is found to provide su…
Max Planck Institute for Physics（马克斯·普朗克物理研究所）；Technical University of Munich（慕尼黑工业大学）
Experiments searching for rare processes like neutrinoless double beta decay heavily rely on the identification of background events to reduce their background level and increase their sensitivity. We present a novel machine learning based method to recognize one of the most abundant classes of background events in these experiments. By combining a neural network for feature extraction with a smaller classification network, our method can be trained with only a small number of labeled events. To validate our method, we use signals from a broad-energy germanium detector irradiated with a $^{228…
Pulse shape discrimination (PSD) is one of the most distinctive features of liquid scintillators. Since the introduction of the scintillation techniques in the field of particle detection, many studies have been carried out to characterize intrinsic properties of the most common liquid scintillator mixtures in this respect. Several application methods and algorithms able to achieve optimum discrimination performances have been developed. However, the vast majority of these studies have been performed on samples of small dimensions. The Counting Test Facility, prototype of the solar neutrino ex…
Liquid-argon scintillation detectors are used in fundamental physics experiments and are being considered for security applications. Previous studies have suggested that the addition of small amounts of xenon dopant improves performance in light or signal yield, energy resolution, and particle discrimination. In this study, we investigate the detector response for xenon dopant concentrations from 9 +/- 5 ppm to 1100 +/- 500 ppm xenon (by weight) in 6 steps. The 3.14-liter detector uses tetraphenyl butadiene (TPB) wavelength shifter with dual photomultiplier tubes and is operated in single-phas…
Scintillators capable of detecting both neutrons and gamma-rays have generated considerable interest. In particular, the use of such scintillators with silicon photomultipliers (SiPMs) enables low-power and compact-geometry applications. Three types of Li-loaded scintillators, CLYC, CLLB, and NaIL, have been tested with a custom-designed SiPM array for temperatures between --20 and 50$^{\circ}$C. The array consists of four 6x6~mm$^2$ SiPMs arranged in a 2x2 configuration. Pulse shape discrimination is used for neutron and gamma identification. Because the pulse shape changes with temperature, …
We present a straightforward method for particle identification and background rejection in $^3$He proportional counters for use in neutron detection. By measuring the risetime and pulse height of the preamplifier signals, one may define a region in the risetime versus pulse height space where the events are predominately from neutron interactions. For six proportional counters surveyed in a low-background environment, we demonstrate the ability to reject alpha-particle events with an efficiency of 99%. By applying the same method, we also show an effective rejection of microdischarge noise ev…
A Discrete Fourier Transform Method (DFTM) for discrimination between the signal of neutrons and gamma rays in organic scintillation detectors is presented. The method is based on the transformation of signals into the frequency domain using the sine and cosine Fourier transforms in combination with the discrete Fourier transform. The method is largely benefited from considerable differences that usually is available between the zero-frequency components of sine and cosine and the norm of the amplitude of the DFT for neutrons and gamma-ray signals. Moreover, working in frequency domain natural…
We present measurements of the scintillation pulse shape in liquid xenon for nuclear recoils (NR) and electronic recoils (ER) at electric fields of 0 to 0.5 kV/cm for energies $<$ 15 keV and $<$ 70 keV electron-equivalent, respectively. The average pulse shapes are well-described by an effective model with two exponential decay components, where both decay times are fit parameters. We find significant broadening of the pulse for ER due to delayed luminescence from the recombination process. In addition to the effective model, we fit a model describing the recombination luminescence for ER at z…
