Free electrons provide a powerful tool to probe material properties at atomic-scale spatial resolution. Recent advances in ultrafast electron microscopy enable the manipulation of free electron wavefunctions using laser pulses. It would be of great importance if one could combine the spatial resolution of electron probes with the ability of laser pulses to probe coherent phenomena in quantum systems. To this end, we propose a novel technique that leverages free electrons that are coherently-shaped by laser pulses to measure quantum coherence in materials. Developing a quantum theory of electron-qubit interactions in materials, we show how the energy spectrum of laser-shaped electrons enables measuring the qubit Block-sphere state and decoherence time (T2). Finally, we present how such shaped electrons can detect and quantify superradiance from multiple qubits. Our scheme could be implemented in an ultrafast transmission electron microscope (UTEM), opening the way towards the full characterization of the state of quantum systems at atomic-scale resolution.
A detailed derivation of the master equation of the cavity radiation of a coherently prepared $Y$-shaped four-level correlated emission laser is presented. The outline of the procedures that can be employed in analytically solving the stochastic differential equations and the rate equations of various correlations are also provided. It is shown that coherently preparing the atoms in the upper two energy levels and the lower, initially, can lead to a genuine continuous variable tripartite entanglement. Moreover, preparing the atoms in the coherent superposition, other than the possible maximum …
We report on the simultaneous observation, by delayed Bragg diffraction, of four- and six-wave mixing processes in a coherently prepared atomic ensemble consisting of cold cesium atoms. For each diffracted order, we observe different temporal pulse shapes and dependencies with the intensities of the exciting fields, evidencing the different mechanisms involved in each process. The various observations are well described by a simplified analytical theory, which considers the atomic system as an ensemble of three-level atoms in Λ configuration.
We describe parametric down conversion process in a two-level atomic gas, where the atoms are in a superposition state of relevant energy levels. This superposition results in splitting of the phase matching condition into three different conditions. Another, more important, peculiarity of the system under discussion is the nonsaturability of amplification coefficients with increasing pump wave intensity, under "sideband" generation conditions.
We present a scheme to obtain the coherently enhanced Raman scattering in atomic vapor which is induced by a spin wave initially written by a weak write laser. The enhancement of Raman scattering is dependent on the number and the spatial distribution of the flipped atoms generated by the weak write laser. Such an enhanced Raman scattering may have practical applications in quantum information, nonlinear optics and laser spectroscopy because of its simplicity.
We experimentally demonstrate an optical pumping technique to pump a dilute rubidium vapor into the mF = 0 ground states. The technique utilizes selection rules that forbid the excitation of the mF = 0 state by linearly-polarized light. A substantial increase in the transparency contrast of coherent population trapping in the clock transition is demonstrated.
Scalable and efficient quantum computation with photonic qubits requires (i) deterministic sources of single-photons, (ii) giant nonlinearities capable of entangling pairs of photons, and (iii) reliable single-photon detectors. In addition, an optical quantum computer would need a robust reversible photon storage devise. Here we discuss several related techniques, based on the coherent manipulation of atomic ensembles in the regime of electromagnetically induced transparency, that are capable of implementing all of the above prerequisites for deterministic optical quantum computation with sing…
Motivated by the recent experiment [V.A. Sautenkov, Yu.V. Rostovtsev, and M.O. Scully, Phys. Rev. A 72, 065801 (2005)], we develop a theoretical model in which the field intensity fluctuations resulted from resonant interaction of a dense atomic medium with laser field having finite bandwidth. The intensity-intensity cross correlation between two circular polarized beams can be controlled by the applied external magnetic field. A smooth transition from perfect correlations to anti-correlations (at zero delay time) of the outgoing beams as a function of the magnetic field strength is observed. …
We report the observation of small group velocities of order 90 meters per second, and large group delays of greater than 0.26 ms, in an optically dense hot rubidium gas (~360 K). Media of this kind yield strong nonlinear interactions between very weak optical fields, and very sharp spectral features. The result is in agreement with previous studies on nonlinear spectroscopy of dense coherent media.
Simultaneous strong coherent pumping of the two transitions of a V-level atom with very differentdecay rates has been predicted to create almost perfect inversion on the narrower transition. Usingthe example of the blue and red transitions in Strontium we show that for suitable operatingconditions the corresponding resonant gain can be used to continuously operate a laser on thenarrow transition. In particular, for a strong detuning of the pump field with respect to the narrowtransition, coherent laser emission occurs close to the bare atomic transition frequency exhibitingonly a negligible co…
We propose a procedure to achieve a complete energy conversion between laser pulses carrying orbital angular momentum (OAM) in a cloud of cold atoms characterized by a double-Λatom-light coupling scheme. A pair of resonant spatially dependent control fields prepare atoms in a position-dependent coherent population trapping state, while a pair of much weaker vortex probe beams propagate in the coherently driven atomic medium. Using the adiabatic approximation we derive the propagation equations for the probe beams. We consider a situation where the second control field is absent at the entrance…
We demonstrate the use of an optical frequency comb to coherently control and entangle atomic qubits. A train of off-resonant ultrafast laser pulses is used to efficiently and coherently transfer population between electronic and vibrational states of trapped atomic ions and implement an entangling quantum logic gate with high fidelity. This technique can be extended to the high field regime where operations can be performed faster than the trap frequency. This general approach can be applied to more complex quantum systems, such as large collections of interacting atoms or molecules.
We report a detailed investigation on the generation of pulse pairs during the readout of a coherence grating stored in a cold atomic ensemble. The pulse shapes and the split of the retrieved energy between the two pulses are studied as a function of the relative intensities of the two reading fields, and a minimum is observed for the total retrieved energy. We introduce a simplified analytical theory for the process, considering a three-level atomic system, which explains all the most striking experimental features.
We predict the possibility of sharp, high-contrast resonances in the optical response of a broad class of systems, wherein interference effects are generated by coherent perturbation or interaction of dark states. The properties of these resonances can be manipulated to design a desired atomic response.
Spin-orbit coupling of optical vector vortices in coherently prepared media
Institute of Theoretical Physics and Astronomy, Vilnius University（维尔纽斯大学理论物理与天文研究所）；Laser Research Center, Vilnius University（维尔纽斯大学激光研究中心）；Département Physique, Faculté des Sciences, Aix-Marseille Université（艾克斯-马赛大学理学院物理系）；Baltic Institute of Advanced Technology（波罗的海高级技术研究所）
A broadband squeezed vacuum photon field is characterized by a complex squeezing function. We show that by controlling the wavelength dependence of its phase it is possible to change the dynamics of the atomic polarization interacting with the squeezed vacuum. Such a phase modulation effectively produces a finite range temporal interaction kernel between the two quadratures of the atomic polarization yielding the change in the decay rates as well as the appearance of additional oscillation frequencies. We show that decay rates slower than the spontaneous decay rate can be achieved even for a s…
Stochastic perturbation of two-level atoms strongly driven by a coherent light field is analyzed by the quantum trajectory method. A new method is developed for calculating the resonance fluorescence spectra from numerical simulations. It is shown that in the case of dominant incoherent perturbation, the stochastic noise can unexpectedly create phase correlation between the neighboring atomic dressed states. This phase correlation is responsible for quantum interference between the related transitions resulting in anomalous modifications of the resonance fluorescence spectra.
Several sequential operations are usually needed for implementing controlled quantum gates and generating entanglement between a pair of quantum bits. Based on the conditional quantum dynamics for a two-ion system beyond the Lamb-Dicke limit, here we propose a theoretical scheme for manipulating two-qubit quantum information, i.e., implementing a universal two-qubit quantum gate and generating a two-qubit entangled state, by using a pair of simultaneous laser pulses. Neither the Lamb-Dicke approximation nor the auxiliary atomic level are required. The experimental realizability of this simple …
We describe a general technique that allows for an ideal transfer of quantum correlations between light fields and metastable states of matter. The technique is based on trapping quantum states of photons in coherently driven atomic media, in which the group velocity is adiabatically reduced to zero. We discuss possible applications such as quantum state memories, generation of squeezed atomic states, preparation of entangled atomic ensembles and quantum information processing.
Two light pulses propagating with ultra-slow group velocities in a coherently prepared atomic gas exhibit dissipation-free nonlinear coupling of an unprecedented strength. This enables a single-photon pulse to coherently control or manipulate the quantum state of the other. Processes of this kind result in generation of entangled states of radiation field and open up new prospectives for quantum information processing.
In this tutorial we provide a short review of attosecond pulse characterization techniques and a pedagogical account of a recently proposed method called Pulse Analysis by Delayed Absorption (PANDA) [Pabst and Dahlström, Phys. Rev. A, 94, 13411 (2016)]. We discuss possible implementations of PANDA in alkali atoms using either principal quantum number wave packets or spin-orbit wave packets. The main merit of the PANDA method is that it can be used as a pulse characterization method that is free from atomic latency effects, such as scattering phase shifts and long-lived atomic resonances. Final…
Trapped atomic ensembles are convenient systems for quantum information storage in the long-lived sublevels of the electronic ground state and its conversion to propagating optical photons via stimulated Raman processes. Here we investigate a phase-matched emission of photons from a coherently prepared atomic ensemble. We consider an ensemble of cold atoms in an elongated harmonic trap with normal density distribution, and determine the parameters of paraxial optics to match the mode geometry of the emitted radiation and optimally collect it into an optical waveguide.
We discuss methods for coherently controlling mesoscopic atomic ensembles where the number of atoms varies randomly from one experimental run to the next. The proposed schemes are based on adiabatic passage and Rydberg blockade and can be used for implementation of a scalable quantum register formed by an array of randomly loaded optical dipole traps.
Spontaneous photon scattering by an atomic qubit is a notable example of environment-induced error and is a fundamental limit to the fidelity of quantum operations. In the scattering process the qubit loses its distinctive and coherent character owing to its entanglement with the photon. Using a single trapped ion we show that by utilizing the information carried by the photon we are able to coherently reverse this process and correct for the scattering error. We further used quantum process tomography to characterize the photon-scattering error and its correction scheme and demonstrate a corr…
We study multipartite entanglement in non-equilibrium quantum phase transition (NEQPT) attainable in a coherently driven atomic ensemble undergoing collective decay. The NEQPT arises in the steady state of the system as the drive field strength is varied in comparison with the decay parameter. A close connection is observed between the critical behavior and the multi-partite entanglement in the system determined via the von Neumann entropy. The derivative of the von Neumann entropy shows Lambda-type behavior typical of the second order phase transitions. We further show that the calculated bi-…
We report and propose a simple scheme to achieve efficient and fast coherent population transfer (CPT) by utilizing either a nonlinearly chirped Gaussian shaped few-cycle laser pulse or an unchirped sinc-shaped few-cycle laser pulse. The proposed scheme is shown to be fairly robust against the variation of the laser parameters such as temporal pulse width, chirp rates, carrier envelope phases and Rabi frequencies. We find that compared to the so-called stimulated Raman adiabatic passage (STIRAP) technique, our scheme for complete population transfer with few-cycle Gaussian shaped laser pulses …
We study entanglement harvesting for matter systems such as atoms, ions or molecules, whose center of mass degrees of freedom are quantum delocalized and which couple to a relativistic quantum field. We employ a generalized Unruh-deWitt detector model for the light-matter interaction, and we investigate how the coherent spreading of the quantum center of mass wave function of two delocalized detector systems impacts their ability to become entangled with one another, via their respective interaction with a quantum field. For very massive detectors with initially highly localized centers of mas…
We investigate the effect of degenerate atomic states on the exciton delocalization of dipole-dipole interacting Rydberg assemblies. Using a frozen gas and regular one-, two-, and three-dimensional lattice arrangements as examples, we see that degeneracies can enhance the delocalization compared to the situation when there is no degeneracy. Using the Zeeman splitting provided by a magnetic field, we controllably lift the degeneracy to study in detail the transition between degenerate and non-degenerate regimes.
We show how two circular polarization components of a linearly polarized pulse, propagating through a coherently driven dilute atomic vapor, can be well resolved in time domain by weak measurement. Slower group velocity of one of the components due to electromagnetically induced transparency leads to a differential group delay between the two components. For low number density, this delay may not be large enough to temporally resolve the two components. We show how this can be enhanced in terms of mean time of arrival of the output pulse through a post-selected polarizer. We demonstrate the id…
We show that it is possible to ``store'' quantum states of single-photon fields by mapping them onto {\it collective} meta-stable states of an optically dense, coherently driven medium inside an optical resonator. An adiabatic technique is suggested which allows to transfer non-classical correlations from traveling-wave single-photon wave-packets into atomic states and vise versa with nearly 100% efficiency. In contrast to previous approaches involving single atoms, the present technique does not require the strong coupling regime corresponding to high-Q micro-cavities. Instead, intracavity El…
For a transition $F_e=0\leftrightarrow F_g=1$ driven by a linearly polarized light and probed by a circularly light, quantum coherence effects are investigated. Due to the coherence between the drive Rabi frequency and Zeeman splitting, electromagnetically induced transparency, electromagnetically induced absorption, and the transition from positive to negative dispersion are obtained, as well as the populations coherently oscillating in a wide spectral region. At the zero pump-probe detuning, the subluminal and superluminal light propagation is predicted. Finally, coherent population trapping…
The quadrupole S$_{1/2}$ -- D$_{5/2}$ optical transition of a single trapped Ca$^+$ ion, well suited for encoding a quantum bit of information, is coherently coupled to the standing wave field of a high finesse cavity. The coupling is verified by observing the ion's response to both spatial and temporal variations of the intracavity field. We also achieve deterministic coupling of the cavity mode to the ion's vibrational state by selectively exciting vibrational state-changing transitions and by controlling the position of the ion in the standing wave field with nanometer-precision.
We report a combined theoretical and experimental study of the spectral and polarization dependence of near resonant radiation coherently backscattered from an ultracold gas of 85Rb atoms. Measurements in an approximately 6 MHz range about the 5s^{2}S_{1/2}- 5p^{2}P_{3/2}, F=3 - F'=4 hyperfine transition are compared with simulations based on a realistic model of the experimental atomic density distribution. In the simulations, the influence of heating of the atoms in the vapor, magnetization of the vapor, finite spectral bandwidth, and other nonresonant hyperfine transitions are considered. G…
Coherent transport of atoms trapped in an optical lattice can be controlled by microwave-induced spin flips that correlate with site-to-site hopping. We study the controllability of homogeneous one-dimensional systems of noninteracting atoms in the absence of site addressability. Given these restrictions, we construct a deterministic protocol to map an initially localized Wannier state to a wave packet that that is coherently distributed over n sites. This is extended to analytic solutions for arbitrary unitary maps given homogenous systems and in the presence of time-dependent uniform forces.…
Spontaneous Raman emission in atomic gases provides an attractive source of photon pairs with a controllable delay. We show how this technique can be implemented in solid state systems by appropriately shaping the inhomogeneous broadening. Our proposal is eminently feasible with current technology and provides a realistic solution to entangle remote rare-earth doped solids in a heralded way.
We consider three- and four-level atomic lasers that are either incoherently (unidirectionally) or coherently (bidirectionally) pumped, the single-mode cavity being resonant with the laser transition. The intra-cavity Fano factor and the photo-current spectral density are evaluated on the basis of rate equations. According to that approach, fluctuations are caused by jumps in active and detecting atoms. The algebra is considerably simpler than the one required by Quantum-Optics treatments. Whenever a comparison can be made, the expressions obtained coincide. The conditions under which the outp…
The manipulation of matterwave represents a milestone in the history of quantum mechanics. It was at the basis of its experimental validation through the observation of diffraction of matter on crystals, as well as grating and Young's double-slit interference with electrons, neutron, atoms and molecules. More recently matterwave manipulation has become a building block in the implementation of quantum devices such as quantum sensors and it plays an essential role in many proposals for implementing quantum computers. In this letter we coherently control the spatial extent of the wavefunction by…
We present here an all--optical scheme for the experimental realization of a quantum phase gate. It is based on the polarization degree of freedom of two travelling single photon wave-packets and exploits giant Kerr nonlinearities that can be attained in coherently driven ultracold atomic media.
For the coherently driven Λ-type three-level systems the general ready-to-calculate expression for the susceptibility tensor at the frequency of the weak probe field is obtained for the arbitrary polarization of the strong coupling laser field and arbitrary values of the angular momenta of resonant atomic levels. The dependence of the relative difference in the group velocities of the two polarization components of the probe field on the polarization of the coupling field is studied.
We demonstrate the efficient generation of Raman sidebands in a medium coherently prepared in a dark state by continuous-wave low-intensity laser radiation. Our experiment is performed in sodium vapor excited in $Λ$ configuration on the D$_{1}$ line by two laser fields of resonant frequencies $ω_{1}$ and $ω_{2}$, and probed by a third field $% ω_{3}$. First-order sidebands for frequencies $ω_{1}$, $ω_{2}$ and up to the third-order sidebands for frequency $ω_{3}$ are observed. The generation starts at a power as low as 10 microwatt for each input field. Dependencies of the intensities of both i…
We analyse the experiment by Hultgren et al. [Phys. Rev. A {\bf 87}, 031404 (2013)] on orbital alignment and quantum beats in coherently excited atomic fine-structure manifolds produced by short-pulse laser photodetachment of C$^-$, Si$^-$ and Ge$^-$ negative ions, and derive a formula that describes the beats. Analysis of the experimental data enables us to extract the non-coherent background contribution for each species, and indicates the need for a full density matrix treatment of the problem.
The efficiency of an ensemble-based optical quantum memory depends critically on the strength of the atom-light coupling. An optical cavity is an effective method to enhance atom-light coupling strength, with the drawback that cavities can be difficult to integrate into a memory setup. In this work we show coherent enhancement of atom-light coupling via an interference effect. The light to be absorbed into the atomic ensemble is split and used to drive the atoms from opposite ends of the ensemble. We compare this method theoretically to a cavity enhanced scheme and present experimental results…
Cold atomic ensembles and spinor Bose-Einstein condensates (BECs) are potential candidates for quantum memories as they have long coherence times and can be coherently controlled. Unlike most candidates for quantum memories which are genuine or effective single particle systems, in atomic ensembles the quantum information is stored as a spin coherent state involving a very large number of atoms. A typical task with such ensembles is to drive the state towards a particular quantum state. While such quantum control methods are well-developed for qubit systems, it is a non-trivial task to extend …
Large optical nonlinearities occurring in a coherently prepared atomic system are shown to produce phase shifts of order $π$. Such an effect may be observed in ultracold rubidium atoms where it could be feasibly exploited toward the realization of a polarization phase gate.
Quantum networks are composed of quantum nodes that interact coherently by way of quantum channels and open a broad frontier of scientific opportunities. For example, a quantum network can serve as a `web' for connecting quantum processors for computation and communication, as well as a `simulator' for enabling investigations of quantum critical phenomena arising from interactions among the nodes mediated by the channels. The physical realization of quantum networks generically requires dynamical systems capable of generating and storing entangled states among multiple quantum memories, and of…
We study the population dynamics of a ring-shaped optical lattice with a high number of particles per site and a low, below ten, number of wells. Using a localized on-site basis defined in terms of stationary states, we were able to construct a multiple-mode model depending on relevant hopping and on-site energy parameters. We show that in case of two wells, our model corresponds exactly to the latest improvement of the two-mode model. We derive a formula for the self-trapping period, which turns out to be chiefly ruled by the on-site interaction energy parameter. By comparing to time dependen…
We analyze the operation of a novel sensor based on atom interferometry, which can achieve supra-classical sensitivity by exploiting quantum correlations in mixed states of many qubits. The interferometer is based on quantum gates which use coherently-controlled Rydberg interactions between a single atom (which acts as a control qubit) and an atomic ensemble (which provides register qubits). In principle, our scheme can achieve precision scaling with the size of the ensemble - which can extend to large numbers of atoms - while using only single-qubit operations on the control and bulk operatio…
A cavity-modified master equation is derived for a coherently driven, V-type three-level atom coupled to a single-mode cavity in the bad cavity limit. We show that population inversion in both the bare and dressed-state bases may be achieved, originating from the enhancement of the atom-cavity interaction when the cavity is resonant with an atomic dressed-state transition. The atomic populations in the dressed state representation are analysed in terms of the cavity-modified transition rates. The atomic fluorescence spectrum and probe absorption spectrum also investigated, and it is found that…
Adiabatic preparation of a fractional quantum Hall fluid by coherently pumping atoms from a Bose-Einstein condensate
Pitaevskii BEC Center, INO-CNR and Dipartimento di Fisica, Università di Trento（皮塔耶夫斯基玻色-爱因斯坦凝聚中心，意大利国家研究委员会物质研究所和特伦托大学物理系）；Department of Physics, TU Dortmund University（多特蒙德大学物理系）；Technische Universität Berlin, Institut für Physik und Astronomie（柏林工业大学物理与天文学研究所）
Optimally-shaped electromagnetic fields have the capacity to coherently control the dynamics of quantum systems and thus offer a promising means for controlling molecular transformations relevant to chemical, biological, and materials applications. Currently, advances in this area are hindered by the prohibitive cost of the quantum dynamics simulations needed to explore the principles and possibilities of molecular control. However, the emergence of nascent quantum-computing devices suggests that efficient simulations of quantum dynamics may be on the horizon. In this article, we study how qua…
We report on deterministic generation of 18-qubit genuinely entangled Greenberger-Horne-Zeilinger (GHZ) state and multi-component atomic Schrödinger cat states of up to 20 qubits on a quantum processor, which features 20 superconducting qubits interconnected by a bus resonator. By engineering a one-axis twisting Hamiltonian enabled by the resonator-mediated interactions, the system of qubits initialized coherently evolves to an over-squeezed, non-Gaussian regime, where atomic Schrödinger cat states, i.e., superpositions of atomic coherent states including GHZ state, appear at specific time int…
Atomic interferometers have been studied as a promising device for precise sensing of external fields. Among various configurations, a particular configuration with a butterfly-shaped geometry has been designed to sensitively probe field gradients. We introduce a Stern-Gerlach (SG) butterfly interferometer by incorporating magnetic field in the conventional butterfly-shaped configuration. Atomic trajectories of the interferometer can be flexibly adjusted by controlling magnetic fields to increase the sensitivity of the interferometer, while the conventional butterfly interferometer using Raman…
Calibrating the strength of the light-matter interaction is an important experimental task in quantum information and quantum state engineering protocols. The strength of the off-resonant light-matter interaction in multi-atom spin oscillators can be characterized by the coupling rate $Γ_\text{S}$. Here we utilize the Coherently Induced Faraday Rotation (CIFAR) signal for determining the coupling rate. The method is suited for both continuous and pulsed readout of the spin oscillator, relying only on applying a known polarization modulation to the probe laser beam and detecting a known optical…
We review methods for coherently controlling Rydberg quantum states of atomic ensembles using Adiabatic Rapid Passage and Stimulated Raman Adiabatic Passage. These methods are commonly used for population inversion in simple two-level and three-level systems. We show that adiabatic techniques allow us to control population and phase dynamics of complex entangled states of mesoscopic atomic ensembles for quantum information processing with Rydberg atoms. We also propose several schemes of single-qubit and two-qubit gates based on adiabatic passage, Rydberg blockade and Förster resonances in Ryd…
We consider the stability and dynamics of multiple dark solitons in cigar-shaped Bose-Einstein condensates (BECs). Our study is motivated by the fact that multiple matter-wave dark solitons may naturally form in such settings as per our recent work [Phys. Rev. Lett. 101, 130401 (2008)]. First, we study the dark soliton interactions and show that the dynamics of well-separated solitons (i.e., ones that undergo a collision with relatively low velocities) can be analyzed by means of particle-like equations of motion. The latter take into regard the repulsion between solitons (via an effective rep…
We investigate dynamics of atomic and molecular systems exposed to intense, shaped chaotic fields and a weak femtosecond laser pulse theoretically. As a prototype example, the photoionization of a hydrogen atom is considered in detail. The net photoionization undergoes an optimal enhancement when a broadband chaotic field is added to the weak laser pulse. The enhanced ionization is analyzed using time-resolved wavepacket evolution and the population dynamics of the atomic levels. We elucidate the enhancement produced by spectrally-shaped chaotic fields of two different classes, one with a tuna…
