We demonstrate and characterize the transfer of a levitating silica nanosphere between two optical tweezers, at low pressure. Both optical traps are mounted on the heads of optical fibers and placed on translation stages in vacuum chambers. Our setup allows to physically separate the particle loading environment from the experimental chamber, where the second tweezer can position the particle inside a high Finesse optical cavity. The separation prevents from spoiling the cavity mirrors and the chamber cleanliness during the particle loading phase. Our system provides a very reliable and simply reproducible protocol for preparing cavity optomechanics experiments with levitating nanoparticles, opening the way to systematic studies of quantum phenomena and easing the realization of sensing devices.
A double nanohole in a metal film was used to trap nanoparticles (20 nm diameter) and simultaneously record their Raman spectrum using the trapping laser as the excitation source. This allowed for the identification of characteristic Stokes lines for titania and polystyrene nanoparticles, showing the capability for material identification of nanoparticles once trapped. Increased Raman signal is observed for the trapping of multiple nanoparticles. This system combines the benefits of nanoparticle isolation and manipulation with unique identification.
A general quantum limit to the sensitivity of particle position measurements is derived following the simple principle of the Heisenberg microscope. The value of this limit is calculated for particles in the Rayleigh and Mie scattering regimes, and with parameters which are relevant to optical tweezers experiments. The minimum power required to observe the zero-point motion of a levitating bead is also calculated, with the optimal particle diameter always smaller than the wavelength. We show that recent optical tweezers experiments are within two orders of magnitude of quantum limited sensitiv…
Coherent scattering of an elliptically polarised tweezer into a cavity mode provides a promising platform for cooling levitated nanoparticles into their combined rotational and translational quantum regime [Phys. Rev. Lett. 126, 163603 (2021)]. This article presents the theory of how aspherical nanoparticles are affected by elliptically polarised laser beams, how two orthogonal cavity modes enable rotational and translational cooling, and how the resulting power spectra contain signatures of rotational non-linearities. We provide analytic expressions for the resulting trapping frequencies, opt…
Optical manipulation has attracted remarkable interest owing to its versatile and non-invasive nature. However, conventional optical trapping remains inefficient for the nanoscopic world. The emergence of plasmonics in recent years has brought a revolutionary change in overcoming limitations due to diffraction and the requirements for high trapping laser powers. Among the near-field optical trapping cavity-based systems, Fano resonant optical tweezers have a robust trapping capability. In this work, we experimentally demonstrate sequential trapping of 20 nm particles through the use of metamat…
We experimentally realize cavity cooling of all three translational degrees of motion of a levitated nanoparticle in vacuum. The particle is trapped by a cavity-independent optical tweezer and coherently scatters tweezer light into the blue detuned cavity mode. For vacuum pressures around $10^{-5}\,{\rm mbar}$, minimal temperatures along the cavity axis in the mK regime are observed. Simultaneously, the center-of-mass (COM) motion along the other two spatial directions is cooled to minimal temperatures of a few hundred $\rm mK$. Measuring temperatures and damping rates as the pressure is varie…
Surface enhanced Raman scattering (SERS) is optically sensitive and chemically specific to detect single molecule spectroscopic signatures. Facilitating this capability in optically-trapped nanoparticles at low laser power remains a significant challenge. In this letter, we show single molecule SERS signatures in reversible assemblies of trapped plasmonic nanoparticles using a single laser excitation (633 nm). Importantly, this trap is facilitated by the thermoplasmonic field of a single gold nanoparticle dropcasted on a glass surface. We employ bi-analyte SERS technique to ascertain the singl…
Coherent scattering of photons is a novel mechanism of optomechanical coupling for optically levitated nanoparticles promising strong, versatile interactions with light and between nanoparticles. We show that it allows efficient deterministic generation of Gaussian entanglement between two particles in separate tweezers. A combination of red- and blue-detuned tweezers brings a mechanical Bogoliubov mode to its ground state. An additional, dispersively coupled cavity mode can reduce noise in the orthogonal mode, resulting in strong entanglement as quantified by the logarithmic negativity and ve…
We put forward an enantioselective method for chiral nanoparticles using optical tweezers. We demonstrate that the optical trapping force in a typical, realistic optical tweezing setup with circularly-polarized trapping beams is sensitive to the chirality of core-shell nanoparticles, allowing for efficient enantioselection. It turns out that the handedness of the trapped particles can be selected by choosing the appropriate circular polarization of the trapping beam. The chirality of each individual trapped nanoparticle can be characterized by measuring the rotation of the equilibrium position…
Photovoltaic optoelectronic tweezers (PVOT) have been proven to be an efficient tool for the manipulation and massive assembly of micro/nano-objects. The technique relies on the strong electric fields produced by certain ferroelectric materials upon illumination due to the bulk photovoltaic effect (customarily LiNbO3:Fe). Despite the rapid development of PVOT and the achievement of high-quality 1D and 2D particle patterning, research efforts aimed at the fabrication of combinatorial structures made up of multiple types of particles have been scarce. Here, we have established the working princi…
Hopping of nanoparticles in optical tweezers governed by Mie resonances
Nonlinear Physics Center, Research School of Physics, Australian National University（澳大利亚国立大学物理研究学院非线性物理中心）；School of Optoelectronic Engineering and Instrumentation Science, Dalian University of Technology（大连理工大学光电工程与仪器科学学部）；Department of Electrical and Electronic Engineering, The University of Melbourne（墨尔本大学电气与电子工程系）；Photonics Laboratory, Physics Unit, Tampere University（坦佩雷大学物理学单元光子学实验室）
Plasmonic nanostructures can overcome Abbe's diffraction limit to generate strong gradient fields, enabling efficient optical trapping of nano-sized particles. However, it remains challenging to achieve stable trapping with low incident laser intensity. Here, we demonstrate a Fano resonance-assisted plasmonic optical tweezers (FAPOT), for single nanoparticle trapping in an array of asymmetrical split nano-apertures, milled on a 50 nm gold thin film. Stable trapping is achieved by tuning the trapping wavelength and varying the incident trapping laser intensity. A very large normalized trap stif…
The field of levitodynamics has made significant progress towards controlling and studying the motion of a levitated nanoparticle. Motional control relies on either autonomous feedback via a cavity or measurement-based feedback via external forces. Recent demonstrations of measurement-based ground-state cooling of a single nanoparticle employ linear velocity feedback, also called cold damping, and require the use of electrostatic forces on charged particles via external electrodes. Here we introduce a novel all-optical cold damping scheme based on spatial modulation of the trap position that i…
Conventional optical tweezers are generated by the intensity gradient of highly focused laser beams, but the requirement of strong intensity gradient limits the tunability of optical traps. Here we show a new type of optical tweezers with tunable potential wells by manipulating the phase gradient of light. Using a new method to calculate holograms, we can design desirable phase profiles and intensity distributions of optical patterns. Optical force arising from the phase gradient creates tunable potential wells for versatile optical manipulation, such as trapping nanoparticles in peanut-shaped…
Optical tweezers is a very well-established technique that has developed into a standard tool for trapping and manipulating micron and submicron particles with great success in the last decades. Although the nature of light enforces restrictions on the minimum particle size that can be efficiently trapped due to Abbe's diffraction limit, scientists have managed to overcome this problem by engineering new devices that exploit near-field effects. Nowadays, metallic nanostructures can be fabricated which, under laser illumination, produce a secondary plasmonic field that does not suffer from the …
A nanofiber-based optical tweezer is demonstrated. Trapping is achieved by combining attractive near-field optical gradient forces with repulsive electrostatic forces. Silica-coated Fe$_2$O$_3$ nanospheres of 300 diameter are trapped as close as 50 nm away from the surface with 810 $μ$W of optical power, with a maximum trap stiffness of 2.7 pN $μ$m$^{-1}$. Electrostatic trapping forces up to 0.5 pN are achieved, a factor of 50 larger than those achievable for the same optical power in conventional optical tweezers. Efficient collection of the optical field directly into the nanofiber enables u…
Optical tweezers, the three-dimensional confinement of a nanoparticle by a strongly focused beam of light, have been widely employed in investigating biomaterial nanomechanics, nanoscopic fluid properties, and ultrasensitive detections in various environments such as inside living cells, at gigapascal pressure, and under high vacuum. However, the cryogenic operation of solid-state-particle optical tweezers is poorly understood. In this study, we demonstrate the optical trapping of metallic and dielectric nanoparticles in superfluid helium below 2 K, which is two orders of magnitude lower than …
Optical tweezers, which are powerful tools for trapping and manipulating particles, have been widely used in many areas. However, their potential wells are typically symmetrical, which limit their capability of optical trapping and manipulation. Herein, we report an approach for dynamically creating asymmetrical potential wells, by employing variable phase gradient profiles generated by holograms. Its depth, stiffness and location of potential wells can be dynamically controlled. Moreover, the controllable transport of nanoparticle is experimentally demonstrated, which reveals that it exhibits…
Accurate delivery of small targets in high vacuum is a pivotal task in many branches of science and technology. Beyond the different strategies developed for atoms, proteins, macroscopic clusters and pellets, the manipulation of neutral particles over macroscopic distances still poses a formidable challenge. Here we report a novel approach based on a mobile optical trap operated under feedback control that enables long range 3D manipulation of a silica nanoparticle in high vacuum. We apply this technique to load a single nanoparticle into a high-finesse optical cavity through a load-lock vacuu…
The manipulation of microparticles using optical forces has led to many applications in the life and physical sciences. To extend optical trapping towards the nano-regime, in this work we demonstrate trapping of single nanoparticles in arrays of plasmonic coaxial nano-apertures with various inner disk configurations and theoretically estimate the associated forces. A high normalised experimental trap stiffness of 3.50fN/nm/mW for 20nm polystyrene particles is observed for an optimum design of 149nm for the nanodisk diameter at a trapping wavelength of 980nm. Theoretical simulations are used to…
Single-particle tracking and optical tweezers are powerful techniques for studying diverse processes at the microscopic scale. The stochastic behavior of a microscopically observable particle contains information about its interaction with surrounding molecules, and an optical tweezer can further facilitate this observation with its ability to constrain the particle to an area of interest. Although these techniques found their initial applications in biology, they can also shed new light on colloid and interface phenomena by unveiling nanoscale morphologies and molecular-level interactions in …
We demonstrate the measurement of nanoparticle shape by angularly resolved Rayleigh scattering of single optical levitated particles that are oriented in space via the trapping light in vacuum. This technique is applied to a range of particle geometries, from perfect spherical nanodroplets to octahedral nanocrystals. We show that this method can resolve shape differences down to a few nanometers and be applied in both low-damping environments, as demonstrated here, and in traditional overdamped fluids used in optical tweezers.
Particles that can be trapped in optical tweezers range from tens of microns down to tens of nanometres in size. Interestingly, this size range includes large macromolecules. We show experimentally, in agreement with theoretical expectations, that optical tweezers can be used to manipulate single molecules of polyethylene oxide suspended in water. The trapped molecules accumulate without aggregating, so this provides optical control of the concentration of macromolecules in solution. Apart from possible applications such as the micromanipulation of nanoparticles, nanoassembly, microchemistry, …
In this letter, we propose a new proof-of-concept of optical nano-tweezer on the basis of a pair of dielectric rectangular rods capable of generating a novel class of controlled finite-volume near field light capsules. The finite-difference time-domain simulations of light spatial structure and optical trapping forces of the gold nanoparticle immersed in water demonstrate the physical concept of an in-plane subwavelength optical capsule, integrated with the microfluidic mesoscale device. It is shown that refractive index and distance between dielectric rectangular rods can control the shape an…
We optically trap freestanding single metallic chiral nanoparticles using a standing-wave optical tweezer. We also incorporate within the trap a polarimetric setup that allows to perform in situ chiral recognition of single enantiomers. This is done by measuring the S_3 component of the Stokes vector of a light beam scattered off the trapped nanoparticle in the forward direction. This unique combination of optical trapping and chiral recognition, all implemented within a single setup, opens new perspectives towards the control, recognition, and manipulation of chiral objects at nanometer scale…
Plasmonic optical tweezers are a ubiquitous tool for the precise manipulation of nanoparticles and biomolecules at low photon flux, while femtosecond-laser optical tweezers can probe the nonlinear optical properties of the trapped species with applications in biological diagnostics. In order to adopt plasmonic optical tweezers in real-world applications, it is essential to develop large-scale fabrication processes without compromising the trapping efficiency. Here, we develop a novel platform for continuous wave (CW) and femtosecond plasmonic optical tweezers, based on gold-coated black silico…
Strong coupling and dark modes in the motion of a pair of levitated nanoparticles
CNR-INO（意大利国家研究委员会红外光学研究所）；Dipartimento di Fisica e Astronomia, Università degli Studi di Firenze（佛罗伦萨大学物理与天文系）；INFN, Sezione di Firenze（意大利国家核物理研究所佛罗伦萨分部）；European Laboratory for Non-Linear Spectroscopy (LENS)（欧洲非线性光谱学实验室）
Recent advances in nanotechnologies have prompted the need for tools to accurately and non invasively manipulate individual nanoobjects. Among the possible strategies, optical forces have been widely used to enable nano optical tweezers capable of trapping or moving a specimen with unprecedented accuracy. Here, we propose an architecture consisting of a nanotip excited with a plasmonic vortex enabling effective dynamical control of nanoparticles in three dimensions. The optical field generated by the structure can be used to manipulate single dielectric nanoparticles acting on the total angula…
Bio-compatible Au nanoparticles exhibit great advantages in the application of biomedical researches, such as bio-sensing, medical diagnosis, and cancer therapy. Bio-molecules can even be manipulated by laser tweezers with the optically trapped Au nanoparticles as handles. In this Letter, optical scattering torque arising from the coupled Au nanoparticles driven by circularly polarized light is theoretically presented. The coupled plasmon resonance modes boost the angular momentum transfer from photons to the Au nanoparticle dimers and trimers through light scattering, which does not bring any…
Internal Temperature and Center-of-Mass Dynamics of a Levitated Nanoparticle: A Simulator
Universidad de Buenos Aires, Facultad de Ciencias Exactas y Naturales（布宜诺斯艾利斯大学，理学院）；CONICET - Universidad de Buenos Aires, Instituto de Física de Buenos Aires (IFIBA)（阿根廷国家科学研究委员会-布宜诺斯艾利斯大学，布宜诺斯艾利斯物理研究所）
Advances in optical trapping design principles have led to tremendous progress in manipulating nanoparticles (NPs) with diverse functionalities in different environments using bulky systems. However, efficient control and manipulation of NPs in harsh environments require a careful design of contactless optical tweezers. Here, we propose a simple design of a fibered optical probe allowing the trapping of dielectric NPs in a contactless regime as well as a transfer of the angular momentum of light to the NP inducing its mechanical rotation. A polarization conversion from linear (guided fundament…
Optical levitation of dielectric particles in vacuum is a powerful technique for precision measurements, testing fundamental physics, and quantum information science. Conventional optical tweezers require bulky optical components for trapping and detection. Here we design and fabricate an ultrathin dielectric metalens with a high numerical aperture of 0.88 at 1064 nm in vacuum. It consists of 500 nm-thick silicon nano-antennas, which are compatible with ultrahigh vacuum. We demonstrate optical levitation of nanoparticles in vacuum with a single metalens. The trapping frequency can be tuned by …
The center-of-mass motion of optically trapped dielectric nanoparticles in vacuum is extremely well-decoupled from its environment, making a powerful tool for measurements of feeble sub-attonewton forces. We demonstrate a method to trap and manuever nanoparticles in an optical standing wave potential formed by retro-reflecting a laser beam from a metallic mirror surface. We can reliably position a $\sim 170$ nm diameter silica nanoparticle at distances of a few hundred nanometers to tens of microns from the surface of a gold-coated silicon mirror by transferring it from a single-beam tweezer t…
As a first approximation, the forces acting on optically trapped particles are commonly assumed to be conservative. The influence of the nonconservative force has been shown to be negligible in overdamped liquid environments. However, its impact in the underdamped regime remains unexplored. Here, we experimentally study the combined effects of gradient and scattering forces on the nonlinear dynamics of trapped particles at various air pressures, leading to significant low-frequency noise excess along the optical axis and the emergence of toroidal Brownian vortices. Our results supported, by nu…
Moving nanoparticles/atoms to study the nearfield interaction between them is one of the many approaches to explore the optical and electrical properties of these assemblies. Traditional approach included the self assembly by spinning or drying nanoparticles in aqua on the substrate is well practiced. Lithography technique is another popular approach to deposit limited nano/micro patterns on substrates. Later optical and mechanical manipulations were used to have more control over moving individual elements of nano and microstructures and even atoms. Optical tweezers, optical trapping and AFM …
We investigate lateral recoil forces exerted on nanoparticles located near plasmonic platforms with in-plane nonreciprocal response. To this purpose, we first develop a comprehensive theoretical framework based on the Lorentz force within the Rayleigh approximation combined with nonreciprocal Green's functions and then derive approximate analytical expressions to model lateral recoil forces, demonstrating their explicit dependence on the dispersion relation of the system and unveiling the mechanisms that govern them. In particular, a dominant lateral recoil force component appears due to the m…
