Optical tweezers is a very well-established technique that has developed into a standard tool for trapping and manipulating micron and submicron particles with great success in the last decades. Although the nature of light enforces restrictions on the minimum particle size that can be efficiently trapped due to Abbe's diffraction limit, scientists have managed to overcome this problem by engineering new devices that exploit near-field effects. Nowadays, metallic nanostructures can be fabricated which, under laser illumination, produce a secondary plasmonic field that does not suffer from the diffraction limit. This advance offers a great improvement in nanoparticle trapping, as it relaxes the trapping requirements compared to conventional optical tweezers. In this work, we review the fundamentals of conventional optical tweezers, the so-called plasmonic tweezers, and related phenomena. Starting from the conception of the idea by Arthur Ashkin until recent improvements and applications, we present some of the challenges faced by these techniques as well as their future perspectives. Emphasis in this review is on the successive improvements of the techniques and the innovative aspects that have been devised to overcome some of the main challenges.
Plasmonic nanostructures can overcome Abbe's diffraction limit to generate strong gradient fields, enabling efficient optical trapping of nano-sized particles. However, it remains challenging to achieve stable trapping with low incident laser intensity. Here, we demonstrate a Fano resonance-assisted plasmonic optical tweezers (FAPOT), for single nanoparticle trapping in an array of asymmetrical split nano-apertures, milled on a 50 nm gold thin film. Stable trapping is achieved by tuning the trapping wavelength and varying the incident trapping laser intensity. A very large normalized trap stif…
We have used a gold nanohole array to trap single polystyrene nanoparticles, with a mean diameter of 30 nm, into separated hot spots located at connecting nanoslot regions. A high trap stiffness of approximately 0.85 fN/(nmmW) at a low incident laser intensity of ~0.51 mW/um2 at 980 nm was obtained. The experimental results were compared to the simulated trapping force and a reasonable match was achieved. This plasmonic array is useful for lab-on-a-chip applications and has particular appeal for trapping multiple nanoparticles with predefined separations or arranged in patterns in order to stu…
Optical manipulation has attracted remarkable interest owing to its versatile and non-invasive nature. However, conventional optical trapping remains inefficient for the nanoscopic world. The emergence of plasmonics in recent years has brought a revolutionary change in overcoming limitations due to diffraction and the requirements for high trapping laser powers. Among the near-field optical trapping cavity-based systems, Fano resonant optical tweezers have a robust trapping capability. In this work, we experimentally demonstrate sequential trapping of 20 nm particles through the use of metamat…
Controlling the transport, trapping, and filtering of nanoparticles is important for many applications. By virtue of their weak response to gravity and their thermal motion, various physical mechanisms can be exploited for such operations on nanoparticles. However, the manipulation based on optical forces is potentially most appealing since it constitutes a highly deterministic approach. Plasmonic nanostructures have been suggested for this purpose, but they possess the disadvantages of locally generating heat and trapping the nanoparticles directly on surface. Here, we propose the use of diel…
A nanofiber-based optical tweezer is demonstrated. Trapping is achieved by combining attractive near-field optical gradient forces with repulsive electrostatic forces. Silica-coated Fe$_2$O$_3$ nanospheres of 300 diameter are trapped as close as 50 nm away from the surface with 810 $μ$W of optical power, with a maximum trap stiffness of 2.7 pN $μ$m$^{-1}$. Electrostatic trapping forces up to 0.5 pN are achieved, a factor of 50 larger than those achievable for the same optical power in conventional optical tweezers. Efficient collection of the optical field directly into the nanofiber enables u…
Optical dipole-traps are used in various scientific fields, including classical optics, quantum optics and biophysics. Here, we propose and implement a dipole-trap for nanoparticles that is based on focusing from the full solid angle with a deep parabolic mirror. The key aspect is the generation of a linear-dipole mode which is predicted to provide a tight trapping potential. We demonstrate the trapping of rod-shaped nanoparticles and validate the trapping frequencies to be on the order of the expected ones. The described realization of an optical trap is applicable for various other kinds of …
The manipulation of microparticles using optical forces has led to many applications in the life and physical sciences. To extend optical trapping towards the nano-regime, in this work we demonstrate trapping of single nanoparticles in arrays of plasmonic coaxial nano-apertures with various inner disk configurations and theoretically estimate the associated forces. A high normalised experimental trap stiffness of 3.50fN/nm/mW for 20nm polystyrene particles is observed for an optimum design of 149nm for the nanodisk diameter at a trapping wavelength of 980nm. Theoretical simulations are used to…
While conventional optical trapping techniques can trap objects with submicron dimensions, the underlying limits imposed by the diffraction of light generally restrict their use to larger or higher refractive index particles. As the index and diameter decrease, the trapping difficulty rapidly increases; hence, the power requirements for stable trapping become so large as to quickly denature the trapped objects in such diffraction-limited systems. Here, we present an evanescent field based device capable of confining low index nanoscale particles using modest optical powers as low as 1.2 mW, wi…
Optical tweezers, the three-dimensional confinement of a nanoparticle by a strongly focused beam of light, have been widely employed in investigating biomaterial nanomechanics, nanoscopic fluid properties, and ultrasensitive detections in various environments such as inside living cells, at gigapascal pressure, and under high vacuum. However, the cryogenic operation of solid-state-particle optical tweezers is poorly understood. In this study, we demonstrate the optical trapping of metallic and dielectric nanoparticles in superfluid helium below 2 K, which is two orders of magnitude lower than …
Optical tweezers, which are powerful tools for trapping and manipulating particles, have been widely used in many areas. However, their potential wells are typically symmetrical, which limit their capability of optical trapping and manipulation. Herein, we report an approach for dynamically creating asymmetrical potential wells, by employing variable phase gradient profiles generated by holograms. Its depth, stiffness and location of potential wells can be dynamically controlled. Moreover, the controllable transport of nanoparticle is experimentally demonstrated, which reveals that it exhibits…
We propose a dielectric structure which focuses the laser light well beyond the diffraction limit and thus considerably enhances the exerted optical trapping force upon dielectric nanoparticles. Although the structure supports a Fabry-Perot resonance, it actually acts as a nanoantenna in that the role of the resonance is to funnel the laser light into the structure. In comparison with the lens illuminating the structure, the proposed structure offers roughly a 10000-fold enhancement in the trapping force - part of this enhancement comes from an 80-fold enhancement in the field intensity, and t…
A double nanohole in a metal film was used to trap nanoparticles (20 nm diameter) and simultaneously record their Raman spectrum using the trapping laser as the excitation source. This allowed for the identification of characteristic Stokes lines for titania and polystyrene nanoparticles, showing the capability for material identification of nanoparticles once trapped. Increased Raman signal is observed for the trapping of multiple nanoparticles. This system combines the benefits of nanoparticle isolation and manipulation with unique identification.
We demonstrate scaffolding of plasmonic nanoparticles by topological defects induced by colloidal microspheres to match their surface boundary conditions with a uniform far-field alignment in a liquid crystal host. Displacing energetically costly liquid crystal regions of reduced order, anisotropic nanoparticles with concave or convex shapes not only stably localize in defects but also self-orient with respect to the microsphere surface. Using laser tweezers, we manipulate the ensuing nanoparticle-microsphere colloidal dimers, probing the strength of elastic binding and demonstrating self-asse…
We demonstrate a silicon nitride trench waveguide deposited with bowtie antennas for plasmonic enhanced optical trapping. The sub-micron silicon nitride trench waveguides were fabricated with conventional optical lithography in a low cost manner. The waveguides embrace not only low propagation loss and high nonlinearity, but also the inborn merits of combining micro-fluidic channel and waveguide together. Analyte contained in the trapezoidal trench channel can interact with the evanescent field from the waveguide beneath. The evanescent field can be further enhanced by plasmonic nanostructures…
Plasmonic nanopores are extensively investigated as single molecules detectors. The main limitations in plasmonic nanopore technology are the too fast translocation velocity of the molecule through the pore and the consequent very short analysis times, as well as the possible instabilities due to local heating. The most interesting approach to control the translocation of molecules and enable longer acquisition times is represented by the ability to efficiently trap and tune the motion of nanoparticles that can be used to tag molecules. Here, we theoretically investigate the performance of a m…
Surface-enhanced Raman spectroscopy (SERS) sensing of DNA sequences by plasmonic nanopores could pave a way to new generation single-molecule sequencing platforms. The SERS discrimination of single DNA bases depends critically on the time that a DNA strand resides within the plasmonic hot spot. However, DNA molecules flow through the nanopores so rapidly that the SERS signals collected are not sufficient for single-molecule analysis. In this work, we report an approach to control the time that molecules reside in the hot spot by physically adsorbing them onto a gold nanoparticle and then trapp…
Reconfigurable Magnetic Nanopore Platform for Selective Trapping
CIC nanoGUNE；University of the Basque Country (UPV/EHU)（巴斯克大学）；Aix Marseille Univ, CNRS, Centrale Med, Institut Fresnel（艾克斯马赛大学、法国国家科学研究中心、中央马赛学院、菲涅尔研究所）；Istituto Italiano di Tecnologia（意大利理工学院）；Umeå University（于默奥大学）；Università degli Studi di Modena e Reggio Emilia（摩德纳和雷焦艾米利亚大学）
We demonstrate an optical conveyor belt for levitated nano-particles over several centimeters inside both air-filled and evacuated hollow-core photonic crystal fibers (HCPCF). Detection of the transmitted light field allows three-dimensional read-out of the particle center-of-mass motion. An additional laser enables axial radiation pressure based feedback cooling over the full fiber length. We show that the particle dynamics is a sensitive local probe for characterizing the optical intensity profile inside the fiber as well as the pressure distribution along the fiber axis. In contrast to prev…
We put forward an enantioselective method for chiral nanoparticles using optical tweezers. We demonstrate that the optical trapping force in a typical, realistic optical tweezing setup with circularly-polarized trapping beams is sensitive to the chirality of core-shell nanoparticles, allowing for efficient enantioselection. It turns out that the handedness of the trapped particles can be selected by choosing the appropriate circular polarization of the trapping beam. The chirality of each individual trapped nanoparticle can be characterized by measuring the rotation of the equilibrium position…
We report on rotating an optically trapped silica nanoparticle in vacuum by transferring spin angular momentum of light to the particle's mechanical angular momentum. At sufficiently low damping, realized at pressures below $10^{-5}$ mbar, we observe rotation frequencies of single 100 nm particles exceeding 1 GHz. We find that the steady-state rotation frequency scales linearly with the optical trapping power and inversely with pressure, consistent with theoretical considerations based on conservation of angular momentum. Rapidly changing the polarization of the trapping light allows us to ext…
Recent advances in nanotechnologies have prompted the need for tools to accurately and non invasively manipulate individual nanoobjects. Among the possible strategies, optical forces have been widely used to enable nano optical tweezers capable of trapping or moving a specimen with unprecedented accuracy. Here, we propose an architecture consisting of a nanotip excited with a plasmonic vortex enabling effective dynamical control of nanoparticles in three dimensions. The optical field generated by the structure can be used to manipulate single dielectric nanoparticles acting on the total angula…
Optical levitation of dielectric particles in vacuum is a powerful technique for precision measurements, testing fundamental physics, and quantum information science. Conventional optical tweezers require bulky optical components for trapping and detection. Here we design and fabricate an ultrathin dielectric metalens with a high numerical aperture of 0.88 at 1064 nm in vacuum. It consists of 500 nm-thick silicon nano-antennas, which are compatible with ultrahigh vacuum. We demonstrate optical levitation of nanoparticles in vacuum with a single metalens. The trapping frequency can be tuned by …
In this paper, we study a stable optomechanical system based on a nanoparticle chain coupled to a waveguide mode. Under the plane wave excitation the nanoparticles form a stable self-organized periodic chain array along the direction of the waveguide through the transverse binding effect. We show that owing to the long-range interaction between the nanoparticles the trapping potential for each nanoparticle in the chain increases linearly with the system size making the formation of long chains more favourable. We propose that this effect can be observed with an optical nanofiber which is a ver…
A simple yet effective achiral platform using elliptical nanoholes for chiroptical analysis is demonstrated. Under linearly polarized excitation, an elliptical nanohole in a thin gold film can generate a localized chiral optical field for chiroptical analysis and simultaneously serve as a near-field optical trap to capture dielectric and plasmonic nanospheres. In particular, the trapping potential is enantioselective for dielectric nanospheres, i.e., the hole traps or repels the dielectric nanoparticles depending on the sample chirality. For plasmonic nanospheres, the trapping potential well i…
We demonstrate the measurement of nanoparticle shape by angularly resolved Rayleigh scattering of single optical levitated particles that are oriented in space via the trapping light in vacuum. This technique is applied to a range of particle geometries, from perfect spherical nanodroplets to octahedral nanocrystals. We show that this method can resolve shape differences down to a few nanometers and be applied in both low-damping environments, as demonstrated here, and in traditional overdamped fluids used in optical tweezers.
Optical trapping of metallic microparticles remains a big challenge because of the strong scattering and absorption of light by the particles. In the paper, we report a new mechanism for stable trapping of metallic microparticles by using a tightly focused linearly polarized Gaussian spot. We theoretically and experimentally demonstrated that metallic microparticles were confined off the optical axis by such a trap. In the meanwhile, transverse spinning motion occurred as a consequence of the asymmetric force field acting on the particle by the trap. The off-axis trapping and transverse spinni…
We present a sensor capable of detecting solution-based nanoparticles using an optical fiber tip functionalized with a photonic crystal cavity. When sensor tips are retracted from a nanoparticle solution after being submerged, we find that a combination of convective fluid forces and optically-induced trapping cause an aggregation of nanoparticles to form directly on cavity surfaces. A simple readout of quantum dot photoluminescence coupled to the optical fiber shows that nanoparticle presence and concentration can be detected through modified cavity properties. Our sensor can detect both gold…
Forces on a nanoparticle in an optical trap are analysed. Brownian motion is found to be one of the major challenges to trap a nanoparticle. Accordingly, suitable spatial electric field distribution of laser beam is suggested to enhance the trapping force on a nanoparticle. Theoretical analysis is carried out to obtain conditions for stable optical trap by incorporating the temperature variation at large laser intensities. Numerical analysis is made for single quantum dot of CdS in buffer solution irradiated by an Nd:YAG laser.
We propose and evaluate a new type of optical force microscope based on a standing wave optical trap. Our microscope, calibrated in-situ and operating in a dynamic mode, is able to trap, without heating, a single metallic nanoparticle of 150 nm that acts as a highly sensitive probe for external radiation pressure. An Allan deviation-based stability analysis of the setup yields an optimal 0.1 Hz measurement bandwidth over which the microscope is thermally limited. Over this bandwidth, and with a genuine sine-wave external drive, we demonstrate an optical force resolution down to 3 fN in water a…
Non-invasive and ultra-accurate optical manipulation of nanometer objects has recently gained a growing interest as a powerful enabling tool in nanotechnology and biophysics. In this context, Self-Induced Back-Action (SIBA) trapping in nano-optical cavities has shown a unique potential for trapping and manipulating nanometer-sized objects under low optical intensities. Yet, the existence of the SIBA effect has that far only been evidenced indirectly through its enhanced trapping performances. In this article we present for the first time a direct experimental evidence of the self-reconfigurati…
Coherent scattering of an elliptically polarised tweezer into a cavity mode provides a promising platform for cooling levitated nanoparticles into their combined rotational and translational quantum regime [Phys. Rev. Lett. 126, 163603 (2021)]. This article presents the theory of how aspherical nanoparticles are affected by elliptically polarised laser beams, how two orthogonal cavity modes enable rotational and translational cooling, and how the resulting power spectra contain signatures of rotational non-linearities. We provide analytic expressions for the resulting trapping frequencies, opt…
Microcavity and whispering gallery mode (WGM) biosensors derive their sensitivity from monitoring frequency shifts induced by protein binding at sites of highly confined field intensities, where field strengths can be further amplified by excitation of plasmon resonances in nanoparticle layers. Here, we propose a mechanism based on optical trapping of a protein at the site of plasmonic field enhancements for achieving ultra sensitive detection in only microliter-scale sample volumes, and in real-time. We demonstrate femto-Molar sensitivity corresponding to a few 1000s of macromolecules. Simula…
We optically trap freestanding single metallic chiral nanoparticles using a standing-wave optical tweezer. We also incorporate within the trap a polarimetric setup that allows to perform in situ chiral recognition of single enantiomers. This is done by measuring the S_3 component of the Stokes vector of a light beam scattered off the trapped nanoparticle in the forward direction. This unique combination of optical trapping and chiral recognition, all implemented within a single setup, opens new perspectives towards the control, recognition, and manipulation of chiral objects at nanometer scale…
The controllable positioning of a vacuum-levitated object near a material surface is of importance for studying short-range forces, such as Casimir forces, interfacial friction forces, or gravity in yet unexplored parameter regimes. Here we optically levitate a nanoparticle in a laser beam strongly focused on a dielectric membrane. By investigating the motion of the trapped particle in vacuum, we map the position-dependent optical potential of the particle. We interferometrically measure the distance between the particle and the surface and demonstrate stable trapping in sub-wavelength proximi…
We introduce a method for analyzing the physical properties of nanoparticles in fluids via the competition between viscous drag and optical forces. By flowing particles through a microfluidic device containing an optical microcavity which acts as a combined optical trap and sensor, the variation of the rate of trapping events with the different forces can be established. A clear threshold behaviour is observed which provides a measure of a parameter combining the dielectric polarizability and the hydrodynamic radius. This technique could be applied in combination with other analytic techniques…
Nanoparticles levitated by optical fields under vacuum conditions have applications in quantum science, the study of nanothermodynamics and precision sensing. Existing techniques for loading optical traps require ambient conditions, and often involve dispersion in liquids, which can contaminate delicate optics and lead to enhanced optical absorption and heating. Here we present a clean, dry and generic mechanism for directly loading optical traps at pressures down to 1\,mbar, exploiting Laser Induced Acoustic Desorption. Our method allows rapid and efficient trapping, and is also suitable for …
Enantioselective optical trapping and characterization of all dielectric disorder-enabled chiral particles
Instituto de Física, Universidade Federal do Rio de Janeiro（里约热内卢联邦大学物理研究所）；Laboratoire Kastler Brossel, Sorbonne Université, CNRS, ENS-PSL, Collège de France（巴黎高等师范学院-PSL研究大学、法兰西公学院、法国国家科学研究中心和索邦大学卡斯特勒·布罗塞尔实验室）
Optical trapping of magnetic Fe-oxide particles is notoriously difficult due to their high refractive indices, not to mention high absorptivity at the trapping infra-red wavelengths. We synthesize Fe co-doped NaYF4:Yb,Er ferromagnetic upconversion particles that not only have refractive indices conducive for optical trapping, but also heat less than Haematite particles at off-resonant wavelengths. These particles are hexagonal shaped with dimensions of the order of 3 micrometer and also bear high coercivity of 20 mT and saturation magnetisation of 1 Am^2/kg. This enables simultaneous use of op…
We propose and demonstrate purely optical feedback cooling of neutral nanoparticles in an optical lattice to an occupation number of $0.85\pm0.20$. The cooling force is derived from the optical gradients of displaced optical lattices produced with two sidebands on the trapping laser. To achieve highly accurate position observations required for cooling near the ground state, we reduce the laser intensity noise to a relative power noise of $\unit[6\times10^{-8}]{/Hz}$ in a frequency band of $\unit[30]{kHz}$ to $\unit[600]{kHz}$. We establish a reproducible method for neutralizing nanoparticles …
