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arXiv 2007.06234cond-mat.str-el
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阻挫层状体系PdCrO $_2$的非常规磁性和电子态

Unconventional magnetism and electronic state in frustrated layered system PdCrO$_2$

Evgenia V. Komleva, Valentin Yu. Irkhin, Igor V. Solovyev, Mikhail I. Katsnelson, Sergey V. Streltsov

摘要:

对磁阻挫层状材料PdCrO $_2$进行了第一性原理计算和模型考虑。交换参数的计算结果与居里-外斯温度($θ$)的实验数据一致。我们表明,实验观察到的强烈抑制的内尔温度($T_N$)相比,居里-外斯温度是由于三个主要因素。首先,正如所预期的,这与层状结构和沿$c$轴的相对较小的交换相互作用有关。第二,理想的面内120 $^{\circ}$磁结构的变形对于提供有限的$T_N$值是至关重要的。然而,这两个因素仍然不足以解释低$T_N$和大挫折因素$|θ|/T_N$。因此,我们提出了一个方案的异国情调的非费米液态PdCrO $_2$以上$T_N$的安德森晶格模型的框架内,这似乎定性地解释其所有的主要特点。

英文摘要:

First-principles calculations and a model consideration of magnetically frustrated layered material PdCrO$_2$ are performed. The results on the exchange parameters are in agreement with the experimental data on the Curie-Weiss temperature ($θ$). We show that experimentally observed strong suppression of the Néel temperature ($T_N$) in comparison with the Curie-Weiss temperature is due to three main factors. First, as expected, this is connected with the layered structure and relatively small exchange interaction along the $c$ axis. Second, deformation of the ideal in-plane 120$^{\circ}$ magnetic structure is crucial to provide finite $T_N$ value. However, these two factors are still insufficient to explain low $T_N$ and the large frustration factor $|θ|/T_N$. Thus, we suggest a scenario of an exotic non-Fermi-liquid state in PdCrO$_2$ above $T_N$ within the frameworks of the Anderson lattice model, which seems to explain qualitatively all its main peculiarities.

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