Electrons in moiré flat band systems can spontaneously break time reversal symmetry, giving rise to a quantized anomalous Hall effect. Here we use a superconducting quantum interference device to image stray magnetic fields in one such system composed of twisted bilayer graphene aligned to hexagonal boron nitride. We find a magnetization of several Bohr magnetons per charge carrier, demonstrating that the magnetism is primarily orbital in nature. Our measurements reveal a large change in the magnetization as the chemical potential is swept across the quantum anomalous Hall gap consistent with the expected contribution of chiral edge states to the magnetization of an orbital Chern insulator. Mapping the spatial evolution of field-driven magnetic reversal, we find a series of reproducible micron scale domains whose boundaries host chiral edge states.
Several moiré systems created by various twisted bilayers have manifested magnetism under flatband conditions leading to enhanced interaction effects. We theoretically study stability of moiré flatband ferromagnetism against collective excitations, with a focus on the effects of Bloch band quantum geometry. The spin magnon spectrum is calculated using different approaches, including Bethe-Salpeter equation, single mode approximation, and an analytical theory. One of our main results is an analytical expression for the spin stiffness in terms of the Coulomb interaction potential, the Berry curv…
The flat bands resulting from moiré superlattices in magic-angle twisted bilayer graphene (MATBG) and ABC-trilayer graphene aligned with hexagonal boron nitride (ABC-TLG/hBN) have been shown to give rise to fascinating correlated electron phenomena such as correlated insulators and superconductivity. More recently, orbital magnetism associated with correlated Chern insulators was found in this class of layered structures centered at integer multiples of n0, the density corresponding to one electron per moiré superlattice unit cell. Here we report the experimental observation of ferromagnetism …
Moir{é} superlattice realized in two-dimensional heterostructures offers an exciting platform to access strongly-correlated electronic states. In this work, we study transition metal dichalcogenides (TMD) Moir{é} superlattices with time-reversal-symmetry and nontrivial spin{/valley}-Chern numbers. Utilizing realistic material parameters and the method of exact diagonalization, we find that at a certain twisting angle and fractional filling, gapped fractional topological states, i.e., fractional Chern insulators, are naturally {stabilized} by simply introducing the Coulomb repulsion. In contras…
Moiré Fractional Chern Insulators III: Hartree-Fock Phase Diagram, Magic Angle Regime for Chern Insulator States, the Role of the Moiré Potential and Goldstone Gaps in Rhombohedral Graphene Superlattices
Many-body interactions between carriers lie at the heart of correlated physics. The ability to tune such interactions would open the possibility to access and control complex electronic phase diagrams on demand. Recently, moiré superlattices formed by two-dimensional materials have emerged as a promising platform for quantum engineering such phenomena. The power of the moiré system lies in the high tunability of its physical parameters by tweaking layer twist angle, electrical field, moiré carrier filling, and interlayer coupling. Here, we report that optical excitation can drastically tune th…
Emergence of a symmetry-broken Chern insulator near a moiré Kondo breakdown
Shanghai Jiao Tong University（上海交通大学）；Cornell University（康奈尔大学）；Kavli Institute at Cornell for Nanoscale Science（康奈尔纳米科学卡弗里研究所）；Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所凝聚态物理国家实验室）；Tsung-Dao Lee Institute, Shanghai Jiao Tong University（上海交通大学李政道研究所）；National Institute for Materials Science（国立材料研究所）；Hefei National Laboratory（合肥国家实验室）；Max Planck Institute for the Structure and Dynamics of Matter（马克斯·普朗克物质结构动力学研究所）
Chern-Textured Exciton Insulators with Valley Spiral Order in Moiré Materials
Rudolf Peierls Centre for Theoretical Physics（鲁道夫·皮尔斯理论物理中心）；Princeton Center for Theoretical Science, Princeton University（普林斯顿大学理论科学中心）；Department of Physics, University of Zurich（苏黎世大学物理系）；Department of Physics, Ghent University（根特大学物理系）
Exciton-roton mode in moiré fractional Chern insulators
Tsinghua University（清华大学）；Institute for Advanced Study, Tsinghua University（清华大学高等研究院）；Frontier Science Center for Quantum Information, Beijing（北京量子前沿科学中心）
Studies on two-dimensional electron systems in a strong magnetic field first revealed the quantum Hall (QH) effect, a topological state of matter featuring a finite Chern number (C) and chiral edge states. Haldane later theorized that Chern insulators with integer QH effects could appear in lattice models with complex hopping parameters even at zero magnetic field. The ABC-trilayer graphene/hexagonal boron nitride (TLG/hBN) moiré superlattice provides an attractive platform to explore Chern insulators because it features nearly flat moiré minibands with a valley-dependent electrically tunable …
Tunable high-Chern-number Chern insulators in rhombohedral tetralayer graphene/hBN moiré superlattices
State Key Laboratory of Micro-nano Engineering Science, Tsung-Dao Lee lnstitute & School of Physics and Astronomy, Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Shanghai Jiao Tong University（上海交通大学微纳电子工程科学国家重点实验室、李政道研究所及物理与天文学院人工结构与量子控制教育部重点实验室）；Department of Physics, City University of Hong Kong（香港城市大学物理系）；Research Center for Electronic and Optical Materials, National Institute for Materials Science（国家材料研究所电子与光学材料研究中心）；Research Center for Materials Nanoarchitectonics, National Institute for Materials Science（国家材料研究所材料纳米结构研究中心）；Hefei National Laboratory（合肥国家实验室）；Shanghai Research Center for Quantum Sciences（上海量子科学研究中心）；Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area (Guangdong)（粤港澳大湾区量子科学中心（广东））；Department of Physics, Southern University of Science and Technology（南方科技大学物理系）；Department of Physics, Hong Kong University of Science and Technology（香港科技大学物理系）
The "Moiré Capacitor Effect" and Stabilization of Fractional Chern Insulators in Rhombohedral Graphene Superlattices
Center for Computational Quantum Physics, Flatiron Institute（Flatiron研究所计算量子物理中心）；Laboratoire de Physique de l’Ecole normale supérieure, ENS, Université PSL, CNRS, Sorbonne Université, Université Paris-Diderot, Sorbonne Paris Cité（巴黎高等师范学院物理实验室，ENS，PSL大学，CNRS，索邦大学，巴黎第七大学，索邦巴黎城）；Department of Physics, Princeton University（普林斯顿大学物理系）；Donostia International Physics Center（圣塞巴斯蒂安国际物理中心）；Princeton Center for Theoretical Science, Princeton University（普林斯顿大学理论科学中心）；Department of Physics, University of Texas at Dallas（德克萨斯大学达拉斯分校物理系）；IKERBASQUE, Basque Foundation for Science（伊卡巴斯基克，巴斯克科学基金会）；Department of Physics, Massachusetts Institute of Technology（麻省理工学院物理系）
Twisted double- and mono-bilayer graphene are graphene-based moiré materials hosting strongly correlated fermions in a gate-tunable conduction band with a topologically non-trivial character. Using unbiased exact diagonalization complemented by unrestricted Hartree-Fock calculations, we find that the strong electron-electron interactions lead to a non-coplanar magnetic state, which has the same symmetries as the tetrahedral antiferromagnet on the triangular lattice and can be thought of as a skyrmion lattice commensurate with the moiré scale, competing with a set of ferromagnetic, topological …
Moiré systems have emerged in recent years as a rich platform to study strong correlations. Here, we will discuss a simple, experimentally feasible setup based on periodically strained graphene that reproduces several key aspects of twisted moiré heterostructures -- but without introducing a twist. We consider a monolayer graphene sheet subject to a $C_2$-breaking periodic strain-induced psuedomagnetic field (PMF) with period $L_M \gg a$, along with a scalar potential of the same period. This system has {\it almost ideal} flat bands with valley-resolved Chern number $\pm 1$, where the deviatio…
The Chern insulator displays a quantized Hall effect without Landau levels. In a landmark paper in 1988, Haldane showed that a Chern insulator could be realized through complex next-nearest-neighbor hopping in a honeycomb lattice. Despite its profound impact on the field of topological physics and recent implementation in cold-atom experiments, the Haldane model has remained elusive in solid-state materials. Here, we report the experimental realization of a Haldane Chern insulator in AB-stacked MoTe2/WSe2 moiré bilayers, which form a honeycomb moiré lattice with two sublattices residing in dif…
We theoretically study the effect of magnetic moiré superlattice on the topological surface states by introducing a continuum model of Dirac electrons with a single Dirac cone moving in the time-reversal symmetry breaking periodic pontential. The Zeeman-type moiré potentials generically gap out the moiré surface Dirac cones and give rise to isolated flat Chern minibands with Chern number $\pm1$. This result provides a promising platform for realizing the time-reversal breaking correlated topological phases. In a $C_6$ periodic potential, when the scalar $U_0$ and Zeeman $Δ_1$ moiré potential s…
Interaction-driven spontaneous symmetry breaking lies at the heart of many quantum phases of matter. In moiré systems, broken spin/valley 'flavour' symmetry in flat bands underlies the parent state out of which ultimately correlated and topological ground states emerge. However, the microscopic mechanism of such flavour symmetry breaking and its connection to the low-temperature many-body phases remain to be understood. Here, we investigate the symmetry-broken many-body ground state of magic angle twisted bilayer graphene (MATBG) and its nontrivial topology using simultaneous thermodynamic and…
Competing Chern states revealed by quasiparticle charging in moiré rhombohedral graphene
Cornell University（康奈尔大学）；Max Planck Institute for the Structure and Dynamics of Matter（马克斯·普朗克物质结构与动力学研究所）；Massachusetts Institute of Technology（麻省理工学院）；Florida State University（佛罗里达州立大学）；National Institute for Materials Science（国立材料研究所）
We study the edge spectrum of twisted sheets of single layer and bilayer graphene in cases where the continuum model predicts a valley Chern insulator -- an insulating state in which the occupied moiré mini-bands from each valley have a net Chern number, but both valleys together have no net Chern number, as required by time reversal symmetry. In a simple picture, such a state might be expected to have chiral valley polarized counter-propagating edge states. We present results from exact diagonalization of the tight-binding model of commensurate structures in the ribbon geometry. We find that …
We predict that in a twisted homobilayer of transition-metal dichalcogenide MoS$_2$, spin-orbit coupling in the conduction band states from $\pm K$ valleys can give rise to moiré flat bands with nonzero Chern numbers in each valley. The nontrivial band topology originates from a unique combination of angular twist and local mirror symmetry breaking in each individual layer, which results in unusual skyrmionic spin textures in momentum space with skyrmion number $\mathcal{S} = \pm 2$. Our Hartree-Fock analysis further suggests that density-density interactions generically drive the system at $1…
Moiré flatbands, occurring, e.g., in twisted bilayer graphene at magic angles, have attracted ample interest due to their high degree of experimental tunability and the intriguing possibility of generating novel strongly interacting phases. Here we consider the core problem of Coulomb interactions within fractionally filled spin and valley polarized Moiré flatbands and demonstrate that the dual description in terms of holes, which acquire a nontrivial hole dispersion, provides key physical intuition and enables the use of standard perturbative techniques for this strongly correlated problem. I…
The interplay of topological characteristics in real space and reciprocal space can lead to the emergence of unconventional topological phases. In this Letter, we implement a novel mechanism for generating higher-Chern flat bands on the basis of twisted bilayer graphene (TBG) coupled to topological magnetic structures in the form of the skyrmion lattice. In particular, we discover a scenario for generating $|C|=2$ dispersionless electronic bands when the skyrmion periodicity and the moiré periodicity are matched. Following the Wilczek argument, the statistics of the charge-carrying excitations…
The entanglement Chern number, the Chern number for the entanglement Hamiltonian, is used to charac- terize the Kane-Mele model, which is a typical model of the quantum spin Hall phase with the time reversal symmetry. We first obtain the global phase diagram of the Kane-Mele model in terms of the entanglement spin Chern number, which is defined by using a spin subspace as a subspace to be traced out in preparing the entanglement Hamiltonian. We further demonstrate the effectiveness of the entanglement Chern number without the time reversal symmetry and spin conservation by extending the Kane-M…
Nanyang Technological University（南洋理工大学）；Nanjing Tech University（南京工业大学）；National Institute for Materials Science（国立材料研究所）；CNRS（法国国家科学研究中心）；Université Côte d’Azûr（蔚蓝海岸大学）；Sorbonne Université（索邦大学）；National University of Singapore（新加坡国立大学）；Center for Quantum Technologies（量子技术中心）；Quantum Science and Engineering Center (QSec)（量子科学与工程中心）
Chern insulator ferromagnets are characterized by a quantized anomalous Hall effect, and have so far been identified experimentally in magnetically-doped topological insulator (MTI) thin films and in bilayer graphene moir{é} superlattices. We classify Chern insulator ferromagnets as either spin or orbital, depending on whether the orbital magnetization results from spontaneous spin-polarization combined with spin-orbit interactions, as in the MTI case, or directly from spontaneous orbital currents, as in the moir{é} superlattice case. We argue that in a given magnetic state, characterized for …
We propose a new mechanism to explain the quantum anomalous Hall (QAH) effect and the electric-field-induced topological phase transition in AB-stacked MoTe${}_2$/WSe${}_2$ moiré heterobilayers at $ν=1$ hole filling. We suggest that the Chern band of the QAH state is generated from an intrinsic band inversion composed of the highest two moiré hole bands with opposite valley numbers and a gap opening induced by two Coulomb-interaction-driven magnetic orders. These magnetic orders, including an in-plane $120^{\circ}$-Néel order and an in-plane ferromagnetic order, interact with moiré bands via c…
Laboratoire de Physique des Solides, Université Paris-Saclay, CNRS（巴黎萨克雷大学固体物理实验室，法国国家科学研究中心）；O. Ya. Usikov Institute for Radiophysics and Electronics, National Academy of Sciences of Ukraine（乌克兰国家科学院O.Ya.尤西科夫无线电物理与电子研究所）；Research Center for Electronic and Optical Materials, National Institute for Materials Science（国立材料研究所电子与光学材料研究中心）；International Center for Materials Nanoarchitectonics, National Institute for Materials Science（国立材料研究所国际材料纳米架构中心）；Centre de nanosciences et de nanotechnologies, Université Paris-Saclay, CNRS（巴黎萨克雷大学纳米科学与纳米技术中心，法国国家科学研究中心）
