Edelstein effect is useful for electric control of magnetic moment. However, Joule heating created by a dissipative current is harmful for its practical applications. In this paper, we investigate two-dimensional noncentrosymmetric superconductors (NCSs) with either $s$-wave or $d$-wave symmetry, and demonstrate that a surface Edelstein effect is significantly enhanced in $d$-wave NCSs. The origin of the enhancement is attributed to surface Majorana states characteristic of gapless spin-singlet superconductors. In the view of superconducting spintronics, this result would give a route to magnetic domain switching by dissipationless supercurrent. We discuss a possible experimental observation in cuprate superconductor heterostructures and heavy fermion superlattices.
Unique properties of the optical activity in noncentrosymmetric superconductors: sum rule, missing area, and relation with the superconducting Edelstein effect
The magnetoelectric effect (or Edelstein effect) in noncentrosymmetric superconductors states that a supercurrent can induce spin magnetization. This is an intriguing phenomenon which has potential applications in superconducting spintronic devices. However, the original Edelstein effect only applies to superconductors with polar point group symmetry. In recent years, many new noncentrosymmetric superconductors have been discovered, such as superconductors with chiral lattice symmetry and superconducting transition metal dichalcogenides with various lattice structures. In this Rapid Communicat…
A comment is made on a letter (Phys. Rev. Lett. {\bf 102}, 067001) and a paper (Phys. Rev. B {\bf 83}, 020506) regarding the correct expression of the thermal current vertex for Cooper pairs.
Exciting new work on Bi2212 shows the presence of non-trivial spin-orbit coupling effects as seen in spin resolved ARPES data [Gotlieb et al., Science, 362, 1271-1275 (2018)]. Motivated by these observations we consider how the picture of spin-orbit coupling through local inversion symmetry breaking might be observed in cuprate superconductors. Furthermore, we examine two spin-orbit driven effects, the spin-Hall effect and the Edelstein effect, focusing on the details of their realizations within both the normal and superconducting states.
The quantization of magnetic flux in superconductors is usually seen as vortices penetrating the sample. While vortices are unstable in bulk type I superconductors, restricting the superconductor causes a variety of vortex structures to appear. We present a systematic study of giant vortex states in type I superconductors obtained by numerically solving the Ginzburg-Landau equations. The size of the vortices is seen to increase with decreasing film thickness. In type I superconductors, giant vortices appear at intermediate thicknesses but they do not form a well-defined vortex lattice. In the …
In this work, we show that a giant spin current can be injected into a nodal topological superconductor, using a normal paramagnetic lead, through a large number of zero energy Majorana fermions at the superconductor edge. The giant spin current is caused by the selective equal spin Andreev reflections (SESAR) induced by Majorana fermions. In each SESAR event, a pair of electrons with certain spin polarization are injected into the nodal topological superconductor, even though the pairing in the bulk of the nodal superconductor is spin-singlet s-wave. We further explain the origin of the spin …
Superconductivity in topological materials has attracted a great deal of interest in both electron physics and material sciences since the theoretical predictions that Majorana fermions can be realized in topological superconductors [1-4]. Topological superconductivity could be realized in a type II, band-inverted, InAs/GaSb quantum well if it is in proximity to a conventional superconductor. Here we report observations of the proximity effect induced giant supercurrent states in an InAs/GaSb bilayer system that is sandwiched between two superconducting tantalum electrodes to form a supercondu…
We considered a mesoscopic superconductor/normal metal (S/N) structure in which the N reservoirs are maintained at different temperatures. It is shown that in the absence of current between the N reservoirs a voltage difference $V_{T}$ arises between the superconducting and normal conductors. The voltage $V_{T}$ oscillates with increasing phase difference $ϕ$ between the superconductors, and its magnitude does not depend on the small parameter $(T/ε_{F}).$
The interplay of geometrical and Andreev quantization in mesoscopic superconductors leads to giant mesoscopic oscillations of energy levels as functions of the Fermi momentum and/or sample size. Quantization rules are formulated for closed quasiparticle trajectories in the presence of normal scattering at the sample boundaries. Two generic examples of mesoscopic systems are studied: (i) one dimensional Andreev states in a quantum box, (ii) a single vortex in a mesoscopic cylinder.
The vortex-vortex interaction potential in bulk superconductors is calculated within the Ginzburg-Landau (GL) theory and is obtained from a numerical solution of a set of two coupled non-linear GL differential equations for the vector potential and the superconducting order parameter, where the merger of vortices into a giant vortex is allowed. Further, the interaction potentials between a vortex and a giant vortex and between a vortex and an antivortex are obtained for both type-I and type-II superconductors. Our numerical results agree asymptotically with the analytical expressions for large…
Interfaces between materials with differently ordered phases present unique opportunities for exotic physical properties, especially the interplay between ferromagnetism and superconductivity in the ferromagnet/superconductor heterostructures. The investigation of zero- and pi-junctions has been of particular interest for both fundamental physical science and emerging technologies. Here, we report the experimental observation of giant oscillatory Gilbert damping in the superconducting Nb/NiFe/Nb junctions with respect to the NiFe thickness. This observation suggests an unconventional spin pump…
Superconductors, ideally diamagnetic when in the Meissner state, can also exhibit paramagnetic behavior due to trapped magnetic flux. In the absence of pinning such paramagnetic response is weak, and ceases with increasing sample thickness. Here we show that in multiband superconductors paramagnetic response can be observed even in slab geometries, and can be far larger than any previous estimate - even multiply larger than the diamagnetic Meissner response for the same applied magnetic field. We link the appearance of this giant paramagnetic response to the broad crossover between conventiona…
It has been noted previously that the sizable areal density of midgap states which must exist on any non-{n0m} surface of a d-wave superconductor can lead to a giant magnetic moment. Here we show that this effect is observable, and discuss two precise ways to observe it: (i) by directly measuring magnetic moment in a system with a large density of internal {110} surfaces, or (ii) by performing spin-polarized tunneling on a {110} surface. In both cases a sufficiently large magnetic field should be applied in the [1$\bar 1$0] direction.
Nonreciprocal or nonlinear responses in symmetry-broken systems are powerful probes of emergent properties in quantum materials, including superconductors, magnets, and topological materials. Recently, vortex matter has been recognized as a key ingredient of giant nonlinear responses in superconductors with broken inversion symmetry. However, nonlinear effects have been probed as excess voltage only under broken time-reversal symmetry. In this study, we report intrinsic rectification and nonlinear anomalous Hall effect under time-reversal symmetry in the noncentrosymmetric trigonal superconduc…
We discuss a new mechanism of microwave absorption in s- and d-wave superconductors, which arises in the presence of a dc supercurrent in the system. It produces a contribution to the ac conductivity that is proportional to the inelastic quasiparticle relaxation time. This contribution also determines the supercurrent dependence of the conductivity. It may significantly exceed the conventional contribution because in typical superconductors the inelastic relaxation time is several orders of magnitude longer than the elastic one. We show that the aforementioned contribution to the conductivity …
We discuss a novel physical mechanism which gives rise to a giant magnetoconductivity in non-centrosymmetric superconducting films. This mechanism is caused by a combination of spin-orbit interaction and inversion symmetry breaking in the system, and arises in the presence of an in-plane magnetic field ${\bf H}_\|$. It produces a contribution to the conductivity, which displays a strong dependence on the angle between the electric field ${\bf E}$ and ${\bf H}_\|$, and is proportional to the inelastic relaxation time of quasiparticles. Since in typical situations the latter is much larger than …
The temperature and electric field dependence of electronic contribution to the thermal conductivity (TC) of a granular superconductor is considered within a 3D model of inductive Josephson junction arrays. In addition to a low-temperature maximum of zero-field TC K(T,0) (controlled by mutual inductance L_0 and normal state resistivity R_n), the model predicts two major effects in applied electric field: (i) decrease of the linear TC, and (ii) giant enhancement of the nonlinear (i.e., grad T-dependent) TC with [K(T,E)-K(T,0)]/K(T,0) reaching 500% for parallel electric fields E=E_T (E_T=S_0|gra…
We present magnetoresistance measurements on all-amorphous ferromagnet (F) / superconductor (S) heterostructures. The F/S/F trilayers show large magnetoresistance peaks in a small field range around the coercive field of the F layers, at temperatures within and below the superconducting transition. This is interpreted as flux flow of weakly pinned vortices induced by the stray field of Bloch magnetic domains in the F layers. Bilayers show much smaller effects, implying that the Bloch walls of the F-layers in the trilayer line up and focus the stray fields. The data are used to discuss the expe…
In high-purity crystals of YBa_2Cu_3O_7, the quasiparticle (qp) lifetime τand the (weak-field) thermal Hall conductivity κ_{xy} undergo dramatic increases below 90K. We present a detailed picture of the behavior of κ_{xy} at low temperature, in particular its scaling properties, which are directly relevant to the issue of whether Landau quantization of the qp states occurs.
The fluctuating superconducting correlations emerging in dirty hybrid structures in conditions of the strong proximity effect are demonstrated to affect the validity range of the widely used formalism of Usadel equations at mesoscopic scales. In superconductor -- ferromagnet (SF) structures these giant mesoscopic fluctuations originating from the interference effects for the Cooper pair wave function in the presence of the exchange field can be responsible for an anomalously slow decay of superconducting correlations in a ferromagnet even when the non-collinear and spin-orbit effects are negli…
The pseudogap is a key property of the cuprate superconductors, whose understanding should illuminate the pairing mechanism. Recent experimental data support a close connection between the pseudogap and an oxygen-driven C4 symmetry breaking within the CuO2 plane unit cell. Using ab initio Molecular Dynamics, we demonstrate the existence of a strong nonlinear electron-oxygen vibrator coupling in two cuprates. In a mean field approach applied to this coupling within a model Hamiltonian, we derive a C4 splitting/pseudogap phase diagram in agreement with experiment - providing an explanation for t…
The spin-galvanic (inverse Edelstein) and inverse spin-Hall effects are calculated for a hybrid system that combines thin superconductor and Rashba-metal layers. These effects are produced by a nonequilibrium spin polarization which is injected into the normal metal layer. This polarization gives rise to an electric potential that relaxes within some characteristic length, which is determined by Andreev reflection. Within this length the dissipative electric current of quasiparticles in the normal layer converts into the supercurrent. This process involves only subgap states and at low tempera…
Enhanced microwave absorption, larger than that in the normal state, is observed in fine grains of type-II superconductors (MgB$_2$ and K$_3$C$_{60}$) for magnetic fields as small as a few $\%$ of the upper critical field. The effect is predicted by the theory of vortex motion in type-II superconductors, however its direct observation has been elusive due to skin-depth limitations; conventional microwave absorption studies employ larger samples where the microwave magnetic field exclusion significantly lowers the absorption. We show that the enhancement is observable in grains smaller than the…
Motivated by recent studies of odd-parity multipole order in condensed matter physics, we theoretically study magnetoelectric responses in an electric octupole state. Investigating the Edelstein effect and spin Hall effect in a locally noncentrosymmetric bilayer Rashba model, we clarify characteristic properties due to parity violation in the electric octupole state. Furthermore, a possible realization of electric octupole order in bilayer high-Tc cuprate superconductors is proposed. Our calculation of magnetic torque is consistent with recent experimental observation of a kink above the super…
We show that in superlattices with alternating superconducting (S) and ferromagnetic (F) layers the spontaneous magnetic field induced in the superconducting layers due to the electromagnetic proximity effect becomes dramatically enhanced compared to the previously studied S/F bilayers. The effect reveals itself for the in-plane orientation of the magnetic moments both for ferromagnetic and anti-ferromagnetic ordering of the moments in the F layers. In the finite size samples the magnetic field decays from the sample surface towards the bulk of the structure, and the decay length strongly depe…
The emergence of the electron-pocket only iron-based superconductor AxFe2-ySe2 (A = alkali metal) challenges the Fermi-surface nesting picture established in iron-pnictides. It was widely believed that magnetism is correlated with the superconductivity in AxFe2-ySe2. Unfortunately, the highly anisotropic exchange parameters and the disagreement between theoretical calculations and experimental results triggered a fierce debate on the nature of magnetism in AxFe2-ySe2. Here we find that the strong magnetic anisotropy is from the anisotropic biquadratic interaction. In order to accurately obtain…
We predict parametrically strong enhancement of the thermoelectric effect in metallic bilayers consisting of two superconductors separated by a spin-active interface. The physical mechanism for such an enhancement is directly related to electron-hole imbalance generated by spin-sensitive quasiparticle scattering at the interface between superconducting layers. We explicitly evaluate the thermoelectric currents flowing in the system and demonstrate that they can reach maximum values comparable to the critical ones for superconductors under consideration.
We study the ultrafast Kerr effect and high-harmonic generation in type-II superconductors by formulating a new model for a time-varying electromagnetic pulse normally incident on a thin-film superconductor. It is found that type-II superconductors exhibit exceptionally large $χ^{(3)}$ due to the progressive destruction of Cooper pairs, and display high-harmonic generation at low incident intensities, and the highest nonlinear susceptibility of all known materials in the THz regime. Our theory opens up new avenues for accessible analytical and numerical studies of the ultrafast dynamics of sup…
When a tunneling barrier between two superconductors is formed by a normal material that would be a superconductor in the absence of phase fluctuations, the resulting Josephson effect can undergo an enormous enhancement. We establish this novel proximity effect by a general argument as well as a numerical simulation and argue that it may underlie recent experimental observations of the giant proximity effect between two cuprate superconductors separated by a barrier made of the same material rendered normal by severe underdoping.
The theory of hole superconductivity proposes that superconductivity originates in the fundamental electron-hole asymmetry of condensed matter and that it is an 'undressing' transition. Here we propose that a natural consequence of this theory is that superconductors behave as giant atoms. The model predicts that the charge distribution in superconductors is inhomogeneous, with higher concentration of negative charge near the surface. Some of this negative charge will spill out, giving rise to a negative electron layer right outside the surface of the superconductor, which should be experiment…
The ground state with vorticity larger than one in mesoscopic superconductors in applied magnetic field may manifest as a `giant'-vortex, where all vortices coalesce into a single singularity of the order parameter. Such a multi-quanta vortex may split into individual vortices (and vice versa) as a function of e.g. applied current, magnetic field or temperature. Here we show that such transitions can be identified by heat-capacity measurements, as the formation or splitting of a giant-vortex results in a clear jump in measured heat capacity vs. external drive. We attribute this phenomenon to a…
We predict that in a bulk type-1.5 superconductor the competing magnetic responses of the two components of the order parameter can result in a vortex interaction that generates group-stabilized giant vortices and unusual vortex rings in the absence of any extrinsic pinning or confinement mechanism. We also find within the Ginzburg-Landau theory a rich phase diagram with successions of behaviors like type-1 -> type-1.5 -> type-2 -> type-1.5 as temperature decreases.
Giant vortices with higher phase-winding than $2π$ are usually energetically unfavorable, but geometric symmetry constraints on a superconductor in a magnetic field are known to stabilize such objects. Here, we show via microscopic calculations that giant vortices can appear in intrinsically non-superconducting materials, even without any applied magnetic field. The enabling mechanism is the proximity effect to a host superconductor where a current flows, and we also demonstrate that antivortices can appear in this setup. Our results open the possibility to study electrically controllable topo…
We consider the Nernst and Hall effects in fluctuation regime of chiral superconductors above transition temperatures, that are raised not by conventional Lorentz force, but by asymmetric scattering due to fluctuations of the Berry phase of the Bogoliubov-de Gennes Hamiltonian. It is found that these effects can be more significant than conventional ones for cleaner samples, exhibiting qualitatively distinct behaviors. The results provide systematic and comprehensive understanding for recent experimental observations of the Nernst effect in a clean URu$_2$Si$_2$ sample, which is suggested to b…
The influence of fractal clusters of a normal phase on the dynamics of a magnetic flux trapped in a percolative superconductor is considered. The critical current distribution and the current-voltage characteristics of fractal superconducting structures in the resistive state are obtained for an arbitrary fractal dimension of the cluster boundaries. The range of fractal dimensions, where the dispersion of critical currents becomes infinite, is found. It is revealed that the fractality of clusters depresses of the electric field caused by the magnetic flux motion thus increasing the critical cu…
Recent transport measurement finds giant negative thermal Hall signal in the pseudo-gap phase of the high temperature superconductors\cite{Taillefer}. Such a signal is found to increase in magnitude with decreasing doping and to reach its maximum in the half-filled antiferromagnetic ordered parent compounds. It is still elusive what is the implication of such a phenomena for the mechanism of the pseudo-gap phase. The observation of such a signal may also challenge our well established understanding of the parent compounds as perfect Heisenberg antiferromagnets. Here we show that such a giant t…
A strong mutual influence of superconductors (S) and ferromagnetic (F) conductors in hybrid F/S (Ni/Al) nanostructures is observed. The magnitude of a proximity-induced conductance on the F-side is more than two orders larger than that predicted by theory. Re-entrance of the superconductors to the normal state reciprocated by changes on the F-side has been found in low applied magnetic fields with new peaks in the differential resistance as an effect of the saturation magnetisation. An analysis has been developed providing a base for a numerical description of the system. PACS numbers: 74.50.+…
The Cooper-pair size (i.e., the BCS coherence length) in low-dimensional superconductors is dramatically modified by quantum-size effects. In particular, for nanowires made of conventional superconducting materials, we show that the coherence length exhibits size-dependent drops by two-three orders of magnitude and reaches values found in high-$T_c$ superconductors. This phenomenon is surprisingly similar to the well-known BCS-BEC crossover but with one important exception: it is driven by the transverse quantization of the electron spectrum rather than by the strength of the fermion-fermion i…
To examine the role of magnetism in superconductivity of iron-based superconductors, we first present first-principles optical calculations on three representative parent compounds: LaFeAsO, BaFe2As2 and LiFeAs. Both nonmagnetic (NM) and spin-density wave (SDW) with striped antiferromagnetic order are considered. Due to their layer structure, these compounds in NM states show anomalously large optical anisotropy with a conductivity ratio $σ_{zz}/σ{xx}$ as large as 313% in LaFeAsO and 530% in LiFeAs. Interestingly the giant optical anisotropy is significantly suppressed by SDW. On the other han…
While 203 K high temperature superconductivity in H3S has been interpreted by BCS theory in the dirty limit here we focus on the effects of hydrogen zero-point-motion and the multiband electronic structure relevant for multigap superconductivity near Lifshitz transitions. We describe how the topology of the Fermi surfaces evolves with pressure giving different Lifshitz-transitions. A neck-disrupting Lifshitz-transition (type 2) occurs where the van Hove singularity, vHs, crosses the chemical potential at 210 GPa and new small 2D Fermi surface portions appear with slow Fermi velocity where the …
When the Fermi level is near the top of a band the carriers (holes) are maximally dressed by electron-ion and electron-electron interactions. The theory of hole superconductivity predicts that only in that case can superconductivity occur, and that it is driven by $undressing$ of the carriers at the Fermi energy upon pairing. Indeed, experiments show that dressed hole carriers in the normal state become undressed electron carriers in the superconducting state. This leads to a description of superconductors as giant atoms, where undressed time-reversed electrons are paired and propagate freely …
In the present photoemission study of a cuprate superconductor Bi1.74Pb0.38Sr1.88CuO6+delta, we discovered a large scale dispersion of the lowest band, which unexpectedly follows the band structure calculation very well. The incoherent nature of the spectra suggests that the hopping-dominated dispersion occurs possibly with the assistance of local spin correlations. A giant kink in the dispersion is observed, and the complete self-energy containing all interaction information is extracted for a doped cuprate in the low energy region. These results recovered significant missing pieces in our cu…
Superconductivity and magnetism are generally incompatible because of the opposing requirement on electron spin alignment. When combined, they produce a multitude of fascinating phenomena, including unconventional superconductivity and topological superconductivity. The emergence of two-dimensional (2D)layered superconducting and magnetic materials that can form nanoscale junctions with atomically sharp interfaces presents an ideal laboratory to explore new phenomena from coexisting superconductivity and magnetic ordering. Here we report tunneling spectroscopy under an in-plane magnetic field …
We examine the isotope effect of superconductivity in systems with coexisting interactions of phonon and nonphonon mechanisms in addition to the direct Coulomb interaction. The interaction mediated by the spin fluctuations is discussed as an example of the nonphonon interaction. Extended formulas for the transition temperature Tc and the isotope-effect coefficient alpha are derived for cases (a) omega_np < omega_D and (b) omega_np > omega_D, where omega_np is an effective cutoff frequency of the nonphonon interaction that corresponds to the Debye frequency omega_D in the phonon interaction. In…
We discuss a mechanism of microwave absorption in conventional superconductors which is similar to the Debye absorption mechanism in molecular gases. The contribution of this mechanism to the \emph{ac} conductivity is proportional to the inelastic quasiparticle relaxation time $τ_\mathrm{\mathrm{in}}$ rather than the elastic one $τ_{\mathrm{el}}$ and therefore it can be much larger than the conventional one. The Debye contribution to the linear conductivity arises only in the presence of a \emph{dc} supercurrent in the system and its magnitude depends strongly on the orientation of the microwa…
