Due to their strong and tunable interactions, Rydberg atoms can be used to realize fast two-qubit entangling gates. We propose a generalization of a generic two-qubit Rydberg-blockade gate to multi-qubit Rydberg-blockade gates which involve both many control qubits and many target qubits simultaneously. This is achieved by using strong microwave fields to dress nearby Rydberg states, leading to asymmetric blockade in which control-target interactions are much stronger than control-control and target-target interactions. The implementation of these multi-qubit gates can drastically simplify both quantum algorithms and state preparation. To illustrate this, we show that a 25-atom GHZ state can be created using only three gates with an error of 7.8%.
We review here the studies performed about interactions in an assembly of cold Rydberg atoms. We focus more specially the review on the dipole-dipole interactions and on the effect of the dipole blockade in the laser Rydberg excitation, which offers attractive possibilities for quantum engineering. We present first the various interactions between Rydberg atoms. The laser Rydberg excitation of such an assembly is then described with the introduction of the dipole blockade phenomenon. We report recent experiments performed in this subject by starting with the case of a pair of atoms allowing th…
By coupling a probe transition to a Rydberg state using electro-magnetically induced transparency (EIT) we map the strong dipole-dipole interactions onto an optical field. We characterize the resulting cooperative optical non-linearity as a function of probe strength and density. We show that the effect of dipole blockade cannot be described using a mean-field but requires an $N$-atom cooperative model. Good quantitative agreement is obtained for three atoms per blockade with the $n=60$ Rydberg state. We place an upper-limit on the dephasing rate of the blockade spheres of $<110$ kHz.
We theoretically study a quantum destructive interference (QDI) induced photon blockade in a two-qubit driven cavity QED system with dipole-dipole interaction (DDI). In the absence of dipole-dipole interaction, we show that a QDI-induced photon blockade can be achieved only when the qubit resonance frequency is different from the cavity mode frequency. When DDI is introduced the condition for this photon blockade is strongly dependent upon the pump field frequency, and yet is insensitive to the qubit-cavity coupling strength. Using this tunability feature we show that the conventional energy-l…
The dipole blockade phenomenon is a direct consequence of strong dipole-dipole interaction, where only single atom can be excited because the doubly excited state is shifted out of resonance. The corresponding two-body entanglement with non-zero concurrence induced by the dipole blockade effect is an important resource for quantum information processing. Here, we propose a novel physical mechanism for realizing dipole blockade without the dipole-dipole interaction, where two qubits coupled to a cavity, are driven by a coherent field. By suitably chosen placements of the qubits in the cavity an…
We report a model that makes it possible to analyze quantitatively the dipole blockade effect on the dynamical evolution of a two two-level atom system driven by an external laser field. The multiple excitations of the atomic sample are taken into account. We find very large concurrence in the dipole blockade regime. We further find that entanglement can be tuned by changing the intensity of the exciting laser. We also report a way to lift the dipole blockade paving the way to manipulate in a controllable way the blockade effects. We finally report how a continuous monitoring of the dipole blo…
We show that microwave spectroscopy of a dense Rydberg gas trapped on a superconducting atom chip in the dipole blockade regime reveals directly the dipole-dipole many-body interaction energy spectrum. We use this method to investigate the expansion of the Rydberg cloud under the effect of repulsive van der Waals forces and the breakdown of the frozen gas approximation. This study opens a promising route for quantum simulation of many-body systems and quantum information transport in chains of strongly interacting Rydberg atoms.
Results of numerical Monte Carlo simulations for the Stark-tuned Förster resonance and dipole blockade between two to five cold rubidium Rydberg atoms in various spatial configurations are presented. The effects of the atoms' spatial uncertainties on the resonance amplitude and spectra are investigated. The feasibility of observing coherent Rabi-like population oscillations at a Förster resonance between two cold Rydberg atoms is analyzed. Spectra and the fidelity of the Rydberg dipole blockade are calculated for various experimental conditions, including nonzero detuning from the Förster reso…
We describe a technique for manipulating quantum information stored in collective states of mesoscopic ensembles. Quantum processing is accomplished by optical excitation into states with strong dipole-dipole interactions. The resulting ``dipole blockade'' can be used to inhibit transitions into all but singly excited collective states. This can be employed for a controlled generation of collective atomic spin states as well as non-classical photonic states and for scalable quantum logic gates. An example involving a cold Rydberg gas is analyzed.
We study theoretically and experimentally the competing blockade and anti-blockade effects induced by spontaneously generated contaminant Rydberg atoms in driven Rydberg systems. These contaminant atoms provide a source of strong dipole-dipole interactions and play a crucial role in the system's behavior. We study this problem theoretically using two different approaches. The first is a cumulant expansion approximation, in which we ignore third-order and higher connected correlations. Using this approach for the case of resonant drive, a many-body blockade radius picture arises, and we find qu…
We demonstrate experimentally that a single Rb atom excited to the $79d_{5/2}$ level blocks the subsequent excitation of a second atom located more than $10 μ\rm m$ away. The observed probability of double excitation of $\sim 30%$ is consistent with a theoretical model based on calculations of the long range dipole-dipole interaction between atoms.
We analyze the effects of Zeeman degeneracies on the long-range interactions between like Rydberg atoms, with particular emphasis on applications to quantum information processing using van der Waals blockade. We present a general analysis of how degeneracies affect the primary error sources in blockade experiments, emphasizing that blockade errors are sensitive primarily to the weakest possible atom-atom interactions between the degenerate states, not the mean interaction strength. We present explicit calculations of the van der Waals potentials in the limit where the fine-structure interacti…
We study a novel regime of the Rydberg excitation blockade using highly Stark-shifted, yet long-living, states of Rb atoms subject to electric fields above the classical ionization limit. Such states allow tuning the dipole-dipole interaction strength while their ionization rate can be changed over two orders of magnitude by small variations of the electric field. We demonstrate laser excitation of the interacting Rydberg states followed by their detection using controlled ionization and magnified imaging with high spatial and temporal resolution. Our work reveals the hitherto unexplored possi…
We propose a scheme for controlling interactions between Rydberg-excited neutral atoms in order to perform a fast high-fidelity quantum gate. Unlike dipole-blockade mechanisms already found in the literature, we drive resonantly the atoms with a state-dependent excitation to Rydberg levels, and we exploit the resulting dipole-dipole interaction to induce a controlled atomic motion in the trap, in a similar way as discussed in recent ion-trap quantum computing proposals. This leads atoms to gain the required gate phase, which turns out to be a combination of a dynamic and a geometrical contribu…
We show that two-time, second-order correlations of scattered photons from planar arrays and chains of atoms display nonclassical features that can be described by a superatom picture of the canonical single-atom $g_2(τ)$ resonance fluorescence result. For the superatom, the single-atom linewidth is replaced by the linewidth of the underlying collective low light-intensity eigenmode. Strong light-induced dipole-dipole interactions lead to a correlated response, suppressed joint photon detection events, and dipole blockade that inhibits multiple excitations of the collective atomic state. For t…
We present an efficient method for producing $N$ particle entangled states using Rydberg blockade interactions. Optical excitation of Rydberg states that interact weakly, yet have a strong coupling to a second control state is used to achieve state dependent qubit rotations in small ensembles. On the basis of quantitative calculations we predict that an N=8 Schrödinger cat state can be produced with a fidelity of 84% in cold Rb atoms.
We present a new scheme for cluster states generation based on atomic ensembles and the dipole blockade mechanism. The protocol requires identical single photon sources, one ensemble per physical qubit, and regular photodetectors. The general entangling procedure is presented, as well as a procedure that generates Q-qubit GHZ states with probability p ~ eta^{Q/2}, where eta is the combined detection and source efficiency. This is significantly more efficient than any known robust probabilistic entangling operation. The GHZ states form the basic building block for universal cluster states - a r…
We study the quantum melting of quasi-one-dimensional lattice models in which the dominant energy scale is given by a repulsive dipolar interaction. By constructing an effective low-energy theory, we show that the melting of crystalline phases can occur into two distinct liquid phases, having the same algebraic decay of density-density correlations, but showing a different non-local correlation function expressing string order. We present possible experimental realizations using ultracold atoms and molecules, introducing an implementation based on resonantly driven Rydberg atoms that offers ad…
The dipole blockade effect at laser excitation of mesoscopic ensembles of Rydberg atoms lies in the fact that the excitation of one atom to a Rydberg state blocks the excitation of other atoms due to the shift in the collective energy levels of interacting Rydberg atoms. It is used to obtain the entangled qubit states based on single neutral atoms in optical traps. In this paper, we present our experimental results on the observation of the dipole blockade for mesoscopic ensembles of 1-5 atoms when they are detected by the selective field ionization method. We investigated the spectra of the t…
In the famous quantum communication scheme developed by Duan {\it et al.}[L.M. Duan, M.D. Lukin, J.I. Cirac, and P. Zoller, Nature (London) {\bf 414} 413 (2001)], the probability of successful generating a symmetric collective atomic state with a single-photon emitted have to be far smaller than 1 to obtain an acceptable entangled state. Because of strong dipole-dipole interaction between two Rydberg atoms, more than one simultaneous excitations in an atomic ensembles are greatly suppressed, which makes it possible to excite a mesoscopic cold atomic ensemble into a singly-excited symmetric col…
We demonstrate theoretically a scheme for cluster state generation, based on atomic ensembles and the dipole blockade mechanism. In the protocol, atomic ensembles serve as single qubit systems. Therefore, we review single-qubit operations on qubit defined as collective states of atomic ensemble. Our entangling protocol requires nearly identical single-photon sources, one ultra-cold ensemble per physical qubit, and regular photodetectors. The general entangling procedure is presented, as well as a procedure that generates in a single step Q-qubit GHZ states with success probability p_success ~ …
The resonant dipole-dipole interaction between highly excited Rydberg levels dominates the interaction of neutral atoms at short distances scaling as $1/r^3$. Here we take advantage of the combined effects of strong dipole-dipole interaction and multifrequency driving fields to propose one type of selective Rydberg pumping mechanism. In the computational basis of two atoms $\{|00\rangle, |01\rangle,|10\rangle,|11\rangle\}$, this mechanism allows $|11\rangle$ to be resonantly pumped upwards to the single-excited Rydberg states while the transitions of the other three states are suppressed. From…
One of the important nonclassical effects in quantum optics is the anti-bunching, which has been observed in a large class of physical systems - including light-harvesting antennas with cyclic structures. The units of the ring couple with adjacent ones through dipole-dipole interactions. We show how this strong dipole-dipole interaction leads to photon-blockade resulting in the suppression of double excitation pathway and anti-bunching in photosynthesis systems. The robustness of the photon blockade is demonstrated against the disorder in the ring structures. We hypothesis that the effect may …
We propose to use adiabatic rapid passage with a chirped laser pulse in the strong dipole blockade regime to deterministically excite only one Rydberg atom from randomly loaded optical dipole traps or optical lattices. The chirped laser excitation is shown to be insensitive to the random number \textit{N} of the atoms in the traps. Our method overcomes the problem of the $\sqrt {N} $ dependence of the collective Rabi frequency, which was the main obstacle for deterministic single-atom excitation in the ensembles with unknown \textit{N}, and can be applied for single-atom loading of dipole trap…
The dipole blockade between Rydberg atoms has been proposed as a basic tool in quantum information processing with neutral atoms. Here we demonstrate experimentally the Rydberg blockade of two individual atoms separated by 4 $μ$m. Moreover, we show that, in this regime, the single atom excitation is enhanced by a collective two-atom behavior associated with the excitation of an entangled state. This observation is a crucial step towards the deterministic manipulation of entanglement of two or more atoms using the Rydberg dipole interaction.
The interaction blockade phenomenon isolates the motion of a single quantum particle within a multi-particle system, in particular for coherent oscillations in and out of a region affected by the blockade mechanism. For identical quantum particles with Bose statistics, the presence of the other particles is still felt by a bosonic stimulation factor $\sqrt{N}$ that speeds up the coherent oscillations, where $N$ is the number of bosons. Here we propose an experiment to observe this enhancement factor with a small number of bosonic atoms. The proposed protocol realises an asymmetric double well …
We describe a mechanism for a controlled generation of a pure Bell state with correlated atoms that involve two or zero excitations. The mechanism inhibits transitions into singly excited collective states of a two-atom system by shifting them from their unperturbed energies. The shift is accomplished by the dipole-dipole interaction between the atoms. The creation of the Bell state is found to be dependent on the relaxation of the atomic excitation. When the relaxation is not present or can be ignored, the state of the system evolves harmonically between a separable to the maximally entangled…
We propose an exotic multi-qubit Toffoli gate protocol via asymmetric Rydberg blockade, benefiting from the use of a spheroidal configuration to optimize the gate performance. The merit of a spheroidal structure lies in a well preservation of strong blocked energies between all control-target atom pairs within the sphere, which can persistently keep the blockade error at a low level. On the basis of optimization for three different types of $(2+1)$-$qubit$ gate units to minimize the antiblockade error, the gate fidelity of an optimal $(6+1)$-$qubit$ configuration can attain as high as $0.9841$…
Nonreciprocal Photon Blockade in an Asymmetric Cavity
North University of China（中北大学）；Shanxi Key Laboratory of Graphene Sensing Materials and Devices, North University of China（中北大学石墨烯传感材料与器件山西省重点实验室）；School of Semiconductor and Physics, North University of China（中北大学半导体与物理学院）；School of Instrument and Intelligent Future Technology, North University of China（中北大学仪器与智能未来技术学院）；Academy for Advanced Interdisciplinary Research, North University of China（中北大学交叉科学研究院）
We propose to apply stimulated adiabatic passage to transfer atoms from their ground state into Rydberg excited states. Atoms a few micrometers apart experience a dipole-dipole interaction among Rydberg states that is strong enough to shift the atomic resonance and inhibit excitation of more than a single atom. We show that the adiabatic passage in the presence of this interaction between two atoms leads to robust creation of maximally entangled states and to two-bit quantum gates. For many atoms, the excitation blockade leads to an effective implementation of collective-spin and Jaynes-Cummin…
Due to its potential for implementing a scalable quantum computer, multiqubit Toffoli gate lies in the heart of quantum information processing. In this article, we demonstrate a multiqubit blockade gate with atoms arranged in a three-dimension spheroidal array. The gate performance is greatly improved by the method of optimizing control-qubit distributions on the spherical surface via evolutionary algorithm, which leads to an enhanced asymmetric Rydberg blockade. This spheroidal configuration, not only arises a well preservation for the dipole blockade energy between arbitrary control-target p…
We calculate pair potential curves for interacting Rydberg atoms in a constant electric field and use them to determine the effective $C_3$ dipole-dipole and $C_6$ van der Waals coefficients. We compare the $C_3$ and $C_6$ with experiments where the angle of a polarizing electric field is varied with respect to the axis of a quasi-1-dimensional trap at ultracold temperatures. The dipoles produced via polarization of the atoms have an angular dependent dipole-dipole interaction. We focus on the interaction potential of two rubidium Rydberg atoms in $50S_{1/2}$ states in the blockade regime. For…
Electromagnetically induced transparency (EIT) in a ladder system involving a Rydberg level is known to yield giant optical nonlinearities for the probe field, even in the few-photon regime. This enhancement is due to the strong dipole-dipole interactions between Rydberg atoms and the resulting excitation blockade phenomenon. In order to study such highly correlated media, ad hoc models or low-excitation assumptions are generally used to tackle their dynamical response to optical fields. Here, we study the behaviour of a cavity Rydberg-EIT setup in the non-equilibrium quantum field formalism, …
The Rydberg excitation blockade has been at the heart of an impressive array of recent achievements; however, state-mixing interactions can compromise its efficiency. When ultracold atoms are excited to Rydberg states near Förster resonance, up to $\sim 50\%$ of atoms can be found in dipole coupled product states within tens of ns after excitation. There has been disagreement in the literature regarding the mechanism by which this mixing occurs. We use state-selective field ionization spectroscopy to measure, on a shot-by-shot basis, the distribution of Rydberg states populated during narrowba…
We propose and analyze the implementation of a two qubit quantum gate using circular Rydberg states with maximum orbital angular momentum. The intrinsic quantum gate error is limited by the finite Rydberg lifetime and finite Rydberg blockade shift. Circular states have much longer radiative lifetimes than low orbital angular momentum states and are therefore candidates for high fidelity gate operations. We analyze the dipole-dipole interaction of two circular state Rydberg atoms and present numerical simulations of quantum process tomography to find the intrinsic fidelity of a Rydberg blockade…
We study many-body quantum coherence and interaction blockade in two Josephson-linked Bose-Einstein condensates. We introduce universal operators for characterizing many-body coherence without limitations on the system symmetry and total particle number $N$. We reproduce the results for both coherence fluctuations and number squeezing in {\em symmetric} systems of large $N$, and reveal several peculiar phenomena that may occur in {\em asymmetric} systems and systems of small $N$. For asymmetric systems, we show that, due to an interplay between asymmetry and inter-particle interaction, the coh…
Resonant laser excitation of multiple Rydberg atoms are prohibited, leading to Rydberg blockade, when the long-range van der Waals interactions are stronger than the laser-atom coupling. Rydberg blockade can be violated, i.e. simultaneous excitation of more than one Rydberg atoms, by off-resonant laser excitation, causing an excitation antiblockade. Rydberg antiblockade gives rise to strongly correlated many-body dynamics and spin-orbit coupling, and also finds quantum computation applications. Instead of commonly used van der Waals interactions, we investigate antiblockade dynamics of two Ryd…
We investigate the single-photon blockade (1PB) in the quasichiral regime of atom-photon interaction that mediates via dissipative environment, where the effective atom-photon interaction is asymmetrical but achiral. The synthetic magnetic current in the closed-loop coupling breaks down the reciprocity of atom-photon interaction, resulting in an asymmetrical and even completely unidirectional effective coupling between two selected quantum states. As an example, we couple the single-atom cavity-QED (cQED) system to a strongly dissipative auxiliary cavity. We find that in the quasichiral regime…
Rydberg blockaded gate is a fundamental ingredient for scalable quantum computation with neutral Rydberg atoms. However the fidelity of such a gate is intrinsically limited by a blockade error coming from a Rydberg level shift that forbids its extensive use. Based on a dark-state adiabatic passage, we develop a novel protocol for realizing a two-atom blockade-error-free quantum gate in a hybrid system with simultaneous van der Waals (vdWsI) and resonant dipole-dipole interactions (DDI). The basic idea relies on converting the roles of two interactions, which is, the DDI serves as one time-depe…
Current proposals focusing on neutral atoms for quantum computing are mostly based on using single atoms as quantum bits (qubits), while using cavity induced coupling or dipole-dipole interaction for two-qubit operations. An alternative approach is to use atomic ensembles as qubits. However, when an atomic ensemble is excited, by a laser beam matched to a two-level transition (or a Raman transition) for example, it leads to a cascade of many states as more and more photons are absorbed^1. In order to make use of an ensemble as a qubit, it is necessary to disrupt this cascade, and restrict the …
We analyze the influence of dipole-dipole interactions between Rydberg atoms on the generation of Abelian artificial gauge potentials and fields. When two Rydberg atoms are driven by a uniform laser field, we show that the combined atom-atom and atom-field interactions give rise to new, nonuniform, artificial gauge potentials. We identify the mechanism responsible for the emergence of these gauge potentials. Analytical expressions for the latter indicate that the strongest artificial magnetic fields are reached in the regime intermediate between the dipole blockade regime and the regime in whi…
We investigate the implementation of a controlled-Z gate on a pair of Rydberg atoms in spatially separated dipole traps where the joint excitation of both atoms into the Rydberg level is strongly suppressed (the Rydberg blockade). We follow the adiabatic gate scheme of Jaksch et al. [1], where the pair of atoms are coherently excited using lasers, and apply it to the experimental setup outlined in Gaëtan et al. [2]. We apply optimisation to the experimental parameters to improve gate fidelity, and consider the impact of several experimental constraints on the gate success.
We describe a novel method for producing Greenberger-Horne-Zeilinger states in cold atoms coupled to a superconducting coplanar cavity. In the proposed scheme, atoms interact between each other by virtual photon exchange via a cavity mode. These interactions cause an asymmetric Rydberg blockade mechanism that suppresses simultaneous excitations into different atomic Rydberg levels, thus forcing all atoms to occupy the same Rydberg state. This mechanism has effect even if the atoms are separated by distances of the order of millimeters. The atomic populations are transferred adiabatically from …
Creation of quantum computer is outstanding fundamental and practical problem. The quantum computer could be used for execution of very complicated tasks which are not solvable with the classical computers. The first prototype of solid state quantum computer was created in 2009 with superconducting qubits. However, it suffers from the decoherent processes and it is desirable to find more practical encoding of qubits with long-lived coherence. It could be single impurity or vacancy centers in solids, but their interaction with electromagnetic radiation is rather weak. So, here, ensembles of ato…
Single atoms in dipole microtraps or optical tweezers have recently become a promising platform for quantum computing and simulation. Here we report a detailed theoretical analysis of the physics underlying an implementation of a Rydberg two-qubit gate in such a system -- a cornerstone protocol in quantum computing with single atoms. We focus on a blockade-type entangling gate and consider various decoherence processes limiting its performance in a real system. We provide numerical estimates for the limits on fidelity of the maximally entangled states and predict the full process matrix corres…
The dipole blockade of Rydberg excitations is a hallmark of the strong interactions between atoms in these high-lying quantum states. One of the consequences of the dipole blockade is the suppression of fluctuations in the counting statistics of Rydberg excitations, of which some evidence has been found in previous experiments. Here we present experimental results on the dynamics and the counting statistics of Rydberg excitations of ultra-cold Rubidium atoms both on and off resonance, which exhibit sub- and super-Poissonian counting statistics, respectively. We compare our results with numeric…
Fast Quantum Gates for Neutral Atoms Separated by a Few Tens of Micrometers
University of Strasbourg and CNRS, CESQ and ISIS (UMR 7006)（斯特拉斯堡大学与法国国家科学研究中心，CESQ与ISIS联合研究实验室）；Department of Chemistry, Norwegian University of Science and Technology（挪威科技大学化学系）
Arrays of qubits encoded in the ground-state manifold of neutral atoms trapped in optical (or magnetic) lattices appear to be a promising platform for the realization of a scalable quantum computer. Two-qubit conditional gates between nearest-neighbor qubits in the array can be implemented by exploiting the Rydberg blockade mechanism, as was shown by D. Jaksch et al. [Phys. Rev. Lett. 85, 2208 (2000)]. However, the energy shift due to dipole-dipole interactions causing the blockade falls off rapidly with the interatomic distance and protocols based on direct Rydberg blockade typically fail to …
We present an entanglement scheme for Rydberg atoms using the van der Waals interaction phase induced by Ramsey-type pulsed interactions. This scheme realizes not only controlled phase operations between atoms at a distance larger than Rydberg blockade distance, but also various counter-intuitive entanglement examples, including two-atom entanglement in the presence of a closer third atom and $W$-state generation for partially-blockaded three atoms. Experimental realization is conducted with single rubidium atoms loaded in an array of optical tweezer dipole traps, to demonstrate the proposed e…
We experimentally study the optical- and terahertz- induced rotational dynamics of asymmetric molecules in the gas phase. Terahertz and optical fields are identified as two distinct control handles over asymmetric molecules, as they couple to the rotational degrees of freedom via the molecular- dipole and polarizability selectively. The distinction between those two rotational handles is highlighted by different types of quantum revivals observed in long duration (>100ps) field-free rotational evolution. The experimental results are in excellent agreement with Random Phase Wave Function simula…
