A long-lived multi-mode qubit register is an enabling technology for modular quantum computing architectures. For interfacing with superconducting qubits, such a quantum memory should be able to store incoming quantum microwave fields at the single-photon level for long periods of time, and retrieve them on-demand. Here, we demonstrate the partial absorption of a train of weak microwave fields in an ensemble of bismuth donor spins in silicon, their storage for 100 ms, and their retrieval, using a Hahn-echo-like protocol. The long storage time is obtained by biasing the bismuth donors at a clock transition. Phase coherence and quantum statistics are preserved in the storage.
The existence of vacuum fluctuations is one of the most important predictions of modern quantum field theory. In the vacuum state, fluctuations occurring at different frequencies are uncorrelated. However, if a parameter in the Lagrangian of the field is modulated by an external pump, vacuum fluctuations stimulate spontaneous downconversion processes, creating squeezing between modes symmetric with respect to half of the frequency of the pump. Here we show that by double parametric pumping of a superconducting microwave cavity, it is possible to generate another fundamental type of correlation…
A scheme for spatial multimode quantum memory is developed such that spatial-temporal structure of a weak signal pulse can be stored and recalled via cavity-assisted off-resonant Raman interaction with a strong angular-modulated control field in an extended $Λ$-type atomic ensemble. It is shown that effective multimode storage is possible when the Raman coherence spatial grating involves wave vectors with different longitudinal components relative to the paraxial signal field. The possibilities of implementing the scheme in the solid-state materials are discussed.
In this Letter, we demonstrate the generation of multimode entangled states of propagating microwaves. The entangled states are generated by parametrically pumping a multimode superconducting cavity. By combining different pump frequencies, applied simultaneously to the device, we can produce different entanglement structures in a programable fashion. The Gaussian output states are fully characterized by measuring the full covariance matrices of the modes. The covariance matrices are absolutely calibrated using an in situ microwave calibration source, a shot noise tunnel junction. Applying a v…
Interfacing photonic and solid-state qubits within a hybrid quantum architecture offers a promising route towards large scale distributed quantum computing. In that respect, hybrid quantum systems combining circuit QED with ions doped into solids are an attractive platform. There, the ions serve as coherent memory elements and reversible conversion elements of microwave to optical qubits. Among many possible spin-doped solids, erbium ions offer the unique opportunity of a coherent conversion of microwave photons into the telecom C-band at $1.54\,μ$m employed for long distance communication. In…
We report on coherent and multi-temporal mode storage of light using the full atomic frequency comb memory scheme. The scheme involves the transfer of optical atomic excitations in Pr3+:Y2SiO5 to spin-waves in the hyperfine levels using strong single-frequency transfer pulses. Using this scheme, a total of 5 temporal modes are stored and recalled on-demand from the memory. The coherence of the storage and retrieval is characterized using a time-bin interference measurement resulting in visibilities higher than 80%, independent of the storage time. This coherent and multimode spin-wave memory i…
Quantum memory is a fundamental building block for large-scale quantum networks. On-demand optical storage with a large bandwidth, a high multimode capacity and an integrated structure simultaneously is crucial for practical application. However, this has not been demonstrated yet. Here, we fabricate an on-chip waveguide in a $\mathrm {^{151}Eu^{3+}:Y_2SiO_5}$ crystal with insertion losses of 0.2 dB, and propose a novel pumping scheme to enable spin-wave atomic frequency comb (AFC) storage with a bandwidth of 11 MHz inside the waveguide. Based on this, we demonstrate the storage of 200 tempora…
We present a complete theoretical description of atomic storage states in the multimode framework by including spatial coherence in atomic collective operators and atomic storage states. We show that atomic storage states are Dicke states with the maximum cooperation number. In some limits, a set of multimode atomic storage states has been established in correspondence with multimode Fock states of the electromagnetic field. This gives better understanding of both the quantum and coherent information of optical field can be preserved and recovered in ultracold medium. In this treatment, we dis…
Here we demonstrate generating and storing entanglement in a solid state spin-wave quantum memory with on-demand read out using the process of rephased amplified spontaneous emission (RASE). Amplified spontaneous emission (ASE), resulting from an inverted ensemble of Pr$^{3+}$ ions doped into a Y$_2$SiO$_5$ crystal, generates entanglement between collective states of the praseodymium ensemble and the output light. The ensemble is then rephased using a four-level photon echo technique. Entanglement between the ASE and its echo is confirmed and the inseparability violation preserved when the RAS…
We present a nonlinear multimode superconducting electroacoustic system, where the interplay between superconducting kinetic inductance and piezoelectric strong coupling establishes an effective Kerr nonlinearity among multiple acoustic modes at 10 GHz that could hardly be achieved via intrinsic mechanical nonlinearity. By exciting this multimode Kerr system with a single microwave tone, we further demonstrate a coherent electroacoustic frequency comb and provide theoretical understanding of multimode nonlinear interaction in the superstrong coupling limit. This nonlinear superconducting elect…
Multiplexed quantum memories capable of storing and processing entangled photons are essential for the development of quantum networks. In this context, we demonstrate the simultaneous storage and retrieval of two entangled photons inside a solid-state quantum memory and measure a temporal multimode capacity of ten modes. This is achieved by producing two polarization entangled pairs from parametric down conversion and mapping one photon of each pair onto a rare-earth-ion doped (REID) crystal using the atomic frequency comb (AFC) protocol. We develop a concept of indirect entanglement witnesse…
Long-distance quantum communication through optical fibers is currently limited to a few hundreds of kilometres due to fiber losses. Quantum repeaters could extend this limit to continental distances. Most approaches to quantum repeaters require highly multimode quantum memories in order to reach high communication rates. The atomic frequency comb memory scheme can in principle achieve high temporal multimode storage, without sacrificing memory efficiency. However, previous demonstrations have been hampered by the difficulty of creating high-resolution atomic combs, which reduces the efficienc…
We propose to realize microwave quantum illumination in weak coupling regime based on multimode optomechanical systems. In our proposal the multimode together with a frequency-mismatch process could reduce mechanical thermal noise. Therefore, we achieve a significant reduction of error probability than conventional detector in weak coupling regime. Moreover, we optimize the signal-to-noise ratio for limited bandwidth by tuning the delay time of entangled wave-packets.
Coherent and reversible storage of multi-photon entanglement with a multimode quantum memory is essential for scalable all-optical quantum information processing. Although single photon has been successfully stored in different quantum systems, storage of multi-photon entanglement remains challenging because of the critical requirement for coherent control of photonic entanglement source, multimode quantum memory, and quantum interface between them. Here we demonstrate a coherent and reversible storage of biphoton Bell-type entanglement with a holographic multimode atomic-ensemble-based quantu…
Multimode cavity quantum electrodynamics ---where a two-level system interacts simultaneously with many cavity modes---provides a versatile framework for quantum information processing and quantum optics. Due to the combination of long coherence times and large interaction strengths, one of the leading experimental platforms for cavity QED involves coupling a superconducting circuit to a 3D microwave cavity. In this work, we realize a 3D multimode circuit QED system with single photon lifetimes of $2$ ms and cooperativities of $0.5-1.5\times10^9$ across 9 modes of a novel seamless cavity. We d…
We study spatial multimode quantum memories based on light storage in extended ensembles of Lambda-type atoms. We show that such quantum light-matter interfaces allow for highly efficient storage of many spatial modes. In particular, forward operating memories possess excellent scaling with the important physical parameters: quadratic scaling with the Fresnel number and even cubic with the optical depth of the atomic ensemble. Thus, the simultaneous use of both the longitudinal and transverse shape of the stored spin wave modes constitutes a valuable and so far overlooked resource for multimod…
Quantum transmission lines are a central to superconducting and hybrid quantum computing. Parallel to these developments are those of left-handed meta-materials. They have a wide variety of applications in photonics from the microwave to the visible range such as invisibility cloaks and perfect flat lenses. For classical guided microwaves, left-handed transmission lines have been proposed and studied on the macroscopic scale. We combine these ideas in presenting a left-handed/right-handed hybrid transmission line for applications in quantum optics on a chip. The resulting system allows circuit…
We show that a collection of lossy multi-chromatically modulated qubits can be used to dissipatively engineer arbitrary Gaussian states of a set of bosonic modes. Our ideas are especially suited to superconducting-circuit architectures, where all the required ingredients are experimentally available. The generation of such multimode Gaussian states is necessary for many applications, most notably measurement-based quantum computation. We build upon some of our previous proposals, where we showed how to generate single-mode and two-mode squeezed states through cooling and lasing. Special care m…
We experimentally demonstrate the storage of 1060 temporal modes onto a thulium-doped crystal using an atomic frequency comb (AFC). The comb covers 0.93 GHz defining the storage bandwidth. As compared to previous AFC preparation methods (pulse sequences i.e. amplitude modulation), we only use frequency modulation to produce the desired optical pumping spectrum. To ensure an accurate spectrally selective optical pumping, the frequency modulated laser is self-locked on the atomic comb. Our approach is general and should be applicable to a wide range of rare-earth doped material in the context of…
A method of reversible quantum optical data storage is presented using resonant Raman field excited spin coherence, where the spin coherence is stored in an inhomogeneously broadened spin ensemble. Unlike the photon echo method, present technique uses a 2 pi Raman optical rephasing pulse, and multimode (parallel) optical channels can be utilized, where the multimode access gives a great benefit to both all-optical and quantum information processing.
Microwave quantum memory promises advanced capabilities for noisy intermediate-scale superconducting quantum computers. Existing approaches to microwave quantum memory lack complete combination of high efficiency, long storage time, noiselessness and multi-qubit capacity. Here we report an efficient microwave broadband multimode quantum memory. The memory stores two spectral modes of single photon level microwave radiation in on-chip system of eight coplanar superconducting resonators. Single mode storage shows a power efficiency of up to $60\pm 3\%$ at single photon energy and more than $73\p…
Ensemble-based quantum memories are key to developing multiplexed quantum repeaters, able to overcome the intrinsic rate limitation imposed by finite communication times over long distances. Rare-earth ion doped crystals are main candidates for highly multimode quantum memories, where time, frequency and spatial multiplexing can be exploited to store multiple modes. In this context the atomic frequency comb (AFC) quantum memory provides large temporal multimode capacity, which can readily be combined with multiplexing in frequency and space. In this article, we derive theoretical formulas for …
We report the storage and retrieval of a small microwave field from a superconducting resonator into collective excitations of a spin ensemble. The spins are nitrogen-vacancy centers in a diamond crystal. The storage time of the order of 30 ns is limited by inhomogeneous broadening of the spin ensemble.
A long-lived and multimode quantum memory is a key component needed for the development of quantum communication. Here we present temporally multiplexed storage of 5 photonic polarization qubits encoded onto weak coherent states in a rare-earth-ion doped crystal. Using spin refocusing techniques we can preserve the qubits for more than half a millisecond. The temporal multiplexing allows us to increase the effective rate of the experiment by a factor of 5, which emphasizes the importance of multimode storage for quantum communication. The fidelity upon retrieval is higher than the maximum clas…
In this article the ability to record, store, and read out the quantum properties of light is studied. The discussion is based on high-speed and adiabatic models of quantum memory in lambda-configuration and in the limit of strong resonance. We show that in this case the equality between efficiency and squeezing ratio, predicted by the simple beamsplitter model, is broken. The requirement of the maximum squeezing in the output pulse should not be accompanied by the requirement of maximum efficiency of memory, as in the beamsplitter model. We have demonstrated a high output pulse squeezing, whe…
Multimode bulk acoustic systems show promise for use in superconducting quantum computation. They can serve as a medium term memory storage, with exceptional coherence times demonstrated, and they exhibit a mode density that is physically highly compact. Here we experimentally demonstrate accessing individual acoustic modes without being hindered by the uniform frequency spacing of the modes. We use sideband control where a low-frequency modulation is applied to the transmon qubit energy. The amplitude of the modulation defines the qubit-acoustic mode coupling, and its frequency detunes the ac…
Superconducting circuits and microwave signals are good candidates to realize quantum networks, which are the backbone of quantum computers. We have realized a quantum node based on a 3D microwave superconducting cavity parametrically coupled to a transmission line by a Josephson ring modulator. We first demonstrate the time-controlled capture, storage and retrieval of an optimally shaped propagating microwave field, with an efficiency as high as 80%. We then demonstrate a second essential ability, which is the timed-controlled generation of an entangled state distributed between the node and …
We present a general model for an atomic memory using ultra-short pulses of light, which allows both spatial and temporal multimode storage. The process involves the storage of a faint quantum light pulse into the spin coherence of the ground state of Lambda-type 3-level atoms, in the presence of a strong driving pulse. Our model gives a full description of the evolution of the field and of the atomic coherence in space and time throughout the writing and the read-out processes. It is valid for any frequency detuning, from the resonant case to the Raman case, and allows a detailed optimization…
An efficient multi-mode quantum memory is a crucial resource for long-distance quantum communication based on quantum repeaters. We propose a quantum memory based on spectral shaping of an inhomogeneously broadened optical transition into an atomic frequency comb (AFC). The spectral width of the AFC allows efficient storage of multiple temporal modes, without the need to increase the absorption depth of the storage material, in contrast to previously known quantum memories. Efficient readout is possible thanks to rephasing of the atomic dipoles due to the AFC structure. Long-time storage and o…
To advance the full potential of quantum networks one should be able to distribute quantum resources over long distances at appreciable rates. As a consequence, all components in the networks need to have large multimode capacity to manipulate photonic quantum states. Towards this end, a multimode photonic quantum memory, especially one operating at telecom wavelength, remains a key challenge. Here we demonstrate a spectro-temporally multiplexed quantum memory at 1532 nm. Multimode quantum storage of telecom-band heralded single photons is realized by employing the atomic frequency comb protoc…
Entanglement between photons at telecommunication wavelengths and long-lived quantum memories is one of the fundamental requirements of long-distance quantum communication. Quantum memories featuring on-demand read-out and multimode operation are additional precious assets that will benefit the communication rate. In this work we report the first demonstration of entanglement between a telecom photon and a collective spin excitation in a multimode solid-state quantum memory. Photon pairs are generated through widely non-degenerate parametric down-conversion, featuring energy-time entanglement …
We apply collective Raman scattering to create, store and retrieve spatially multimode light in warm rubidium-87 vapors. The light is created in a spontaneous Stokes scattering process. This is accompanied by the creation of counterpart collective excitations in the atomic ensemble -- the spin waves. After a certain storage time we coherently convert the spin waves into the light in deterministic anti-Stokes scattering. The whole process can be regarded as a delayed four-wave mixing which produces pairs of correlated, delayed random images. Storage of higher order spatial modes up to microseco…
We investigate an acoustical analog of circuit quantum electrodynamics that facilitates compact high-Q (${>}20,000$) microwave-frequency cavities with dense spectra. We fabricate and characterize a device that comprises a flux tunable transmon coupled to a $300\,\mathrm{μm}$ long surface acoustic wave resonator. For some modes, the qubit-cavity coupling reaches $6.5\,\mathrm{MHz}$, exceeding the cavity loss rate ($200\,\mathrm{kHz}$), qubit linewidth ($1.1\,\mathrm{MHz}$), and the cavity free spectral range ($4.8\,\mathrm{MHz}$), placing the device in both the strong coupling and strong multim…
The ability to store multiple optical modes in a quantum memory allows for increased efficiency of quantum communication and computation. Here we compute the multimode capacity of a variety of quantum memory protocols based on light storage in ensembles of atoms. We find that adding a controlled inhomogeneous broadening improves this capacity significantly.
We propose a method that enables efficient storage and retrieval of a photonic excitation stored in an ensemble quantum memory consisting of Lambda-type absorbers with non-zero Stokes shift. We show that this can be used to implement a multimode quantum memory storing multiple frequency-encoded qubits in a single ensemble, and allowing their selective retrieval. The read-out scheme applies to memory setups based on both electromagnetically-induced transparency and stimulated Raman scattering, and spatially separates the output signal field from the control fields.
A quantum memory at microwave frequencies, able to store the state of multiple superconducting qubits for long times, is a key element for quantum information processing. Electronic and nuclear spins are natural candidates for the storage medium as their coherence time can be well above one second. Benefiting from these long coherence times requires to apply the refocusing techniques used in magnetic resonance, a major challenge in the context of hybrid quantum circuits. Here we report the first implementation of such a scheme, using ensembles of nitrogen-vacancy (NV) centres in diamond couple…
We experimentally investigate the optical storage of perfect optical vortex (POV) and spatially multimode perfect optical vortex (MPOV) beams via electromagnetically induced transparency (EIT) in a hot vapor cell. In particular, we study the role that phase gradients and phase singularities play in reducing the blurring of the retrieved images due to atomic diffusion. Three kinds of manifestations are enumerated to demonstrate such effect. Firstly, the suppression of the ring width broadening is more prominent for POVs with larger orbital angular momentum (OAM). Secondly, the retrieved double-…
We analyze the performance of a quantum computer architecture combining a small processor and a storage unit. By focusing on integer factorization, we show a reduction by several orders of magnitude of the number of processing qubits compared with a standard architecture using a planar grid of qubits with nearest-neighbor connectivity. This is achieved by taking advantage of a temporally and spatially multiplexed memory to store the qubit states between processing steps. Concretely, for a characteristic physical gate error rate of $10^{-3}$, a processor cycle time of 1 microsecond, factoring a…
We theoretically study electro-optic light modulation based on the quantum model where the linear electro-optic effect and the externally applied microwave field result in the interaction between optical cavity modes. The model assumes that the number of interacting modes is finite and effects of the mode overlapping coefficient on the strength of the intermode interaction can be taken into account through dependence of the coupling coefficient on the mode characteristics. We show that, under certain conditions, the model is exactly solvable and, in the semiclassical approximation where the mi…
Solid-state impurity spins with optical control are currently investigated for quantum networks and repeaters. Among these, rare-earth-ion doped crystals are promising as quantum memories for light, with potentially long storage time, high multimode capacity, and high bandwidth. However, with spins there is often a tradeoff between bandwidth, which favors electronic spin, and memory time, which favors nuclear spins. Here, we present optical storage experiments using highly hybridized electron-nuclear hyperfine states in $^{171}$Yb$^{3+}$:Y$_2$SiO$_5$, where the hybridization can potentially of…
We present a system which allows to tune the coupling between a superconducting resonator and a transmission line. This storage resonator is addressed through a second, coupling resonator, which is frequency-tunable and controlled by a magnetic flux applied to a superconducting quantum interference device (SQUID). We experimentally demonstrate that the lifetime of the storage resonator can be tuned by more than three orders of magnitude. A field can be stored for 18 μs when the coupling resonator is tuned off resonance and it can be released in 14 ns when the coupling resonator is tuned on res…
Coherent pulse control for quantum memory is viable in the optical domain but nascent in microwave quantum circuits. We show how to realize coherent storage and on-demand pulse retrieval entirely within a superconducting circuit by exploiting and extending existing electromagnetically induced transparency technology in superconducting quantum circuits. Our scheme employs a linear array of superconducting artificial atoms coupled to a microwave transmission line.
Quantum interfaces (QIs) that generate entanglement between a multimode atomic memory and a photon forms a multiplexed repeater node and hold promise to greatly improve quantum repeater rates. Recently, the temporal multimode spin-wave memory that is entangled with a photon has been demonstrated with cold atoms. However, due to additional noise generated in multimode operation, the fidelity of spin-wave-photon entanglement significantly decreases with the mode number. So far, the improvement on temporal-multimode entanglement fidelity via suppressing the additional noise remains unexplored. He…
The addition of nonlinearity to an harmonic resonator provides a route to complex dynamical behaviour of resonant modes, including coupling between them. We present a superconducting device that makes use of the nonlinearity of Josephson junctions to introduce a controlled, tunable, nonlinear inductance to a thin film coplanar waveguide resonator. Considering the device as a potential quantum optical component in the microwave regime, we create a sensitive bifurcation amplifier and then demonstrate spectroscopy of other resonant modes via the intermode coupling. We find that the sensitivity of…
Broadband and Large-Multimode Quantum Optical Storage with Rare-Earth Ions in Solids
Chimie ParisTech, PSL University, CNRS, Institut de Recherche de Chimie Paris（巴黎高等化学学院，PSL大学，法国国家科学研究中心，巴黎化学研究所）；Institute for Quantum Materials and Technologies (IQMT), Karlsruhe Institute of Technology（卡尔斯鲁厄理工学院量子材料与技术研究所）；Institut de Chimie Moléculaire et des Matériaux d’Orsay CNRS, Université Paris-Saclay UMR 8182（奥赛分子与材料化学研究所，法国国家科学研究中心，巴黎-萨克雷大学）；Institute of Nanotechnology (INT), Karlsruhe Institute of Technology（卡尔斯鲁厄理工学院纳米技术研究所）；Karlsruhe Nano Micro Facility (KNMFi), Karlruhe Institute of Technology (KIT)（卡尔斯鲁厄纳米微设施，卡尔斯鲁厄理工学院）；Centre Européen de Sciences Quantiques (CESQ), Institut de Science et d’Ingénierie Supramoléculaires (ISIS), Strasbourg（欧洲量子科学中心，超分子科学与工程研究所，斯特拉斯堡）
Entanglement distribution and quantum storage of more than 8000 modes over a metropolitan network
University of Geneva（日内瓦大学）；Aalto University（阿尔托大学）；Chimie ParisTech, PSL University, CNRS, Institut de Recherche de Chimie Paris（巴黎高等化学学院，PSL大学，法国国家科学研究中心，巴黎化学研究 institute）
We report the generation of a type-I multimode two-photon state on a rubidium D$_2$ line (780 nm) using periodically poled KTiOPO$_4$ crystals. With a degenerate optical parametric oscillator far below threshold, we observe an oscillatory correlation function, the cross-correlation between two photons shows a cavity bandwidth of about 7.8 MHz. We also use a Fabry-P$\acute{\rm{e}}$rot etalon to filter its most longitudinal modes and observe its time correlation function. The experimental data are well fitted to theoretical curves. This system could be utilized for demonstrating storage and retr…
We experimentally investigate electromagnetically-induced transparency (EIT) created on an inhomogeneously broadened 5S_1/2-5P_1/2 transition in rubidium vapor using a control field of a complex temporal shape. A comb-shaped transparency spectrum enhances the delay-bandwidth product and the light storage capacity for a matched probe pulse by a factor of about 50 compared to a single EIT line [D. D. Yavuz, Phys. Rev. A 75, 031801 (2007)]. If the temporal mode of the control field is slowly changed while the probe is propagating through the EIT medium, the probe will adiabatically follow, provid…
We study the entanglement of the superconducting charge qubit with the quantized electromagnetic field in a microwave cavity. It can be controlled dynamically by a classical external field threading the SQUID within the charge qubit. Utilizing the controllable quantum entanglement, we can demonstrate the dynamic process of the quantum storage of information carried by charge qubit. On the other hand, based on this engineered quantum entanglement, we can also demonstrate a progressive decoherence of charge qubit with quantum jump due to the coupling with the cavity field in quasi-classical stat…
