J. Nunn, K. Reim, K. C. Lee, V. O. Lorenz, B. Sussman, I. A. Walmsley, D. Jaksch
备注:
Published version. Many thanks are due to Christoph Simon for his help and suggestions. (This acknowledgement is missing from the final draft: apologies!)
The ability to store multiple optical modes in a quantum memory allows for increased efficiency of quantum communication and computation. Here we compute the multimode capacity of a variety of quantum memory protocols based on light storage in ensembles of atoms. We find that adding a controlled inhomogeneous broadening improves this capacity significantly.
We study spatial multimode quantum memories based on light storage in extended ensembles of Lambda-type atoms. We show that such quantum light-matter interfaces allow for highly efficient storage of many spatial modes. In particular, forward operating memories possess excellent scaling with the important physical parameters: quadratic scaling with the Fresnel number and even cubic with the optical depth of the atomic ensemble. Thus, the simultaneous use of both the longitudinal and transverse shape of the stored spin wave modes constitutes a valuable and so far overlooked resource for multimod…
Ensemble-based quantum memories are key to developing multiplexed quantum repeaters, able to overcome the intrinsic rate limitation imposed by finite communication times over long distances. Rare-earth ion doped crystals are main candidates for highly multimode quantum memories, where time, frequency and spatial multiplexing can be exploited to store multiple modes. In this context the atomic frequency comb (AFC) quantum memory provides large temporal multimode capacity, which can readily be combined with multiplexing in frequency and space. In this article, we derive theoretical formulas for …
The sources, which generate atom-photon quantum correlations or entanglement based on quantum memory, are basic blocks for building quantum repeaters (QRs). For achieving highly entanglement-generation rates in ensemble-based QRs, spatial-, temporal- and spectral-multimode memories are needed. The previous temporal-multimode memories are based on rephrasing mechanisms in inhomogeneous-broadened media. Here, by applying a train of multi-direction write pulses into a homogeneous-broadened atomic ensemble to induce Duan-Lukin-Cirac-Zoller-like Raman processes, we prepare up to 19 pairs of modes, …
Future quantum networks will enable the distribution of entanglement between distant locations and allow applications in quantum communication, quantum sensing and distributed quantum computation. At the core of this network lies the ability of generating and storing entanglement at remote, interconnected quantum nodes. While remote physical systems of various nature have been successfully entangled, none of these realisations encompassed all of the requirements for network operation, such as telecom-compatibility and multimode operation. Here we report the demonstration of heralded entangleme…
In this article the ability to record, store, and read out the quantum properties of light is studied. The discussion is based on high-speed and adiabatic models of quantum memory in lambda-configuration and in the limit of strong resonance. We show that in this case the equality between efficiency and squeezing ratio, predicted by the simple beamsplitter model, is broken. The requirement of the maximum squeezing in the output pulse should not be accompanied by the requirement of maximum efficiency of memory, as in the beamsplitter model. We have demonstrated a high output pulse squeezing, whe…
Multiplexed quantum memories capable of storing and processing entangled photons are essential for the development of quantum networks. In this context, we demonstrate the simultaneous storage and retrieval of two entangled photons inside a solid-state quantum memory and measure a temporal multimode capacity of ten modes. This is achieved by producing two polarization entangled pairs from parametric down conversion and mapping one photon of each pair onto a rare-earth-ion doped (REID) crystal using the atomic frequency comb (AFC) protocol. We develop a concept of indirect entanglement witnesse…
Diffusion is the main limitation of storage time in spatially multimode applications of warm atomic vapors. Precise knowledge of diffusional decoherence in the system is desired for designing most of vapor memory setups. Here we present a novel, efficient and direct method of measuring unbiased diffusional decoherence, clearly distinguished from all other decoherence sources. We found the normalized diffusion coefficients of rubidium atoms in noble gases to be as follows: neon 0.20 cm$^{2}$/s, krypton 0.068 cm$^{2}$/s and we are the first to give an experimental result for rubidium in xenon: 0…
Quantum memory is one of key ingredients consisting of quantum networks, therefore storing light at single photon level is an important step for realizing quantum networks. A photon, encoded in a high-dimensional state, can significantly increase the information capacity that a photon can carry. Furthermore, quantum memories with the ability to store multiple optical modes offer advantages in speed and robustness over single mode memories in quantum communication and computation. So far, there is no any report about the storage and retrieval of multiple mode images at single photon level. Here…
Entanglement between photons at telecommunication wavelengths and long-lived quantum memories is one of the fundamental requirements of long-distance quantum communication. Quantum memories featuring on-demand read-out and multimode operation are additional precious assets that will benefit the communication rate. In this work we report the first demonstration of entanglement between a telecom photon and a collective spin excitation in a multimode solid-state quantum memory. Photon pairs are generated through widely non-degenerate parametric down-conversion, featuring energy-time entanglement …
We study the feasibility of meaningful proof-of-principle demonstrations of several quantum repeater protocols with photon (single-photon and photon-pair) sources and atomic-ensemble based quantum memories. We take into account non-unit memory efficiencies that decay exponentially with time, which complicates the calculation of repeater rates. We discuss implementations based on quantum dots, parametric down-conversion, rare-earth-ion doped crystals, and Rydberg atoms. Our results provide guidance for the near-term implementation of long-distance quantum repeater demonstrations, suggesting tha…
Atomic ensembles are effective memory nodes for quantum communication network due to the long coherence time and the collective enhancement effect for the nonlinear interaction between an ensemble and a photon. Here we investigate the possibility of achieving the entanglement distillation for nonlocal atomic ensembles by the input-output process of a single photon as a result of cavity quantum electrodynamics. We give an optimal entanglement concentration protocol (ECP) for two-atomic-ensemble systems in a partially entangled pure state with known parameters and an efficient ECP for the system…
We develop a three-dimensional theory for quantum memories based on light storage in ensembles of Lambda-type atoms, where two long-lived atomic ground states are employed. We consider light storage in an ensemble of finite spatial extent and we show that within the paraxial approximation the Fresnel number of the atomic ensemble and the optical depth are the only important physical parameters determining the quality of the quantum memory. We analyze the influence of these parameters on the storage of light followed by either forward or backward read-out from the quantum memory. We show that f…
We propose a method that enables efficient storage and retrieval of a photonic excitation stored in an ensemble quantum memory consisting of Lambda-type absorbers with non-zero Stokes shift. We show that this can be used to implement a multimode quantum memory storing multiple frequency-encoded qubits in a single ensemble, and allowing their selective retrieval. The read-out scheme applies to memory setups based on both electromagnetically-induced transparency and stimulated Raman scattering, and spatially separates the output signal field from the control fields.
Here we demonstrate generating and storing entanglement in a solid state spin-wave quantum memory with on-demand read out using the process of rephased amplified spontaneous emission (RASE). Amplified spontaneous emission (ASE), resulting from an inverted ensemble of Pr$^{3+}$ ions doped into a Y$_2$SiO$_5$ crystal, generates entanglement between collective states of the praseodymium ensemble and the output light. The ensemble is then rephased using a four-level photon echo technique. Entanglement between the ASE and its echo is confirmed and the inseparability violation preserved when the RAS…
Quantum memories are enabling devices for extending the reach of quantum key distribution (QKD) systems. The required specifications for memories are, however, often considered too demanding for available technologies. One can change this mindset by introducing memory-assisted measurement-device-independent QKD (MDI-QKD), which imposes less stringent conditions on the memory modules. It has been shown that, in the case of {\em fast} single-qubit memories, we can reach rates and distances not attainable by single no-memory QKD links. Single-qubit memories, such as single atoms or ions, have, cu…
Inspired by recent developments in the control and manipulation of quantum dot nuclear spins, which allow for the transfer of an electron spin state to the surrounding nuclear-spin ensemble for storage, we propose a quantum repeater scheme that combines individual quantum dot electron spins and nuclear-spin ensembles, which serve as spin-photon interfaces and quantum memories respectively. We consider the use of low-strain quantum dots embedded in high-cooperativity optical microcavities. Quantum dot nuclear-spin ensembles allow for the long-term storage of entangled states, and heralded entan…
Inhomogeneously broadened spin ensembles play an important role in present-day implementation of hybrid quantum processing architectures. When coupled to a resonator such an ensemble may serve as a multi-mode quantum memory for the resonator field, and by employing spin-refocusing techniques the quantum memory time can be extended to the coherence time of individual spins in the ensemble. In the present paper we investigate such a memory protocol capable of storing an unknown resonator-field state, and we examine separately the various constituents of the protocol: the storage and read-out par…
We show that an ensemble of identical d-level atoms can be efficiently described by d-1 collective oscillator degrees of freedom in the vicinity of a product state with all atoms in the same, but otherwise arbitrary single-particle state. We apply our description to two different kinds of spin squeezing: (i) when each spin-F atom is individually squeezed without creating interatomic entanglement and (ii) when a particular collective atomic oscillator mode is squeezed via quantum non-demolition (QND) measurement and feedback. When combined in sequence, the order of the two methods is relevant i…
Entangled quantum states in high-dimensional space show many advantages compared with entangled states in two-dimensional space. The former enable quantum communication with higher channel capacity, enable more efficient quantum-information processing, and are more feasible for closing the detection loophole in Bell test experiments. Establishing high-dimensional entangled memories is essential for long-distance communication, but its experimental realization is lacking. We experimentally established high-dimensional entanglement in orbital angular momentum space between two atomic ensembles s…
Quantum theoretical treatment of coherent forward scattering of light in a polarized atomic ensemble with an arbitrary angular momentum is developed. We consider coherent forward scattering of a weak radiation field interacting with a realistic multi-level atomic transition. Based on the concept of an effective Hamiltonian and on the Heisenberg formalism, we discuss the coupled dynamics of the quantum fluctuations of the polarization Stokes components of propagating light and of the collective spin fluctuations of the scattering atoms. We show that in the process of coherent forward scattering…
Quantum correlations between long lived quantum memories and telecom photons that can propagate with low loss in optical fibers are an essential resource for the realization of large scale quantum information networks. Significant progress has been realized in this direction with atomic and solid state systems. Here, we demonstrate quantum correlations between a telecom photon and a multimode on-demand solid state quantum memory. This is achieved by mapping a correlated single photon onto a spin collective excitation in a Pr$^{3+}$:Y$_2$SiO$_5$ crystal for a controllable time. The stored singl…
An efficient multi-mode quantum memory is a crucial resource for long-distance quantum communication based on quantum repeaters. We propose a quantum memory based on spectral shaping of an inhomogeneously broadened optical transition into an atomic frequency comb (AFC). The spectral width of the AFC allows efficient storage of multiple temporal modes, without the need to increase the absorption depth of the storage material, in contrast to previously known quantum memories. Efficient readout is possible thanks to rephasing of the atomic dipoles due to the AFC structure. Long-time storage and o…
Multiparameter estimation, which aims to simultaneously determine multiple parameters in the same measurement procedure, attracts extensive interests in measurement science and technologies. Here, we propose a multimode many-body quantum interferometry for simultaneously estimating linear and quadratic Zeeman coefficients via an ensemble of spinor atoms. Different from the scheme with individual atoms, by using an $N$-atom multimode GHZ state, the measurement precisions of the two parameters can simultaneously attain the Heisenberg limit, and they respectively depend on the hyperfine spin numb…
We propose a Raman quantum memory scheme that uses several atomic ensembles to store and retrieve the multimode highly entangled state of an optical quantum frequency comb, such as the one produced by parametric down-conversion of a pump frequency comb. We analyse the efficiency and the fidelity of such a quantum memory. Results show that our proposal may be helpful to multimode information processing using the different frequency bands of an optical frequency comb.
Superradiance, the enhanced collective emission of light from a coherent ensemble of quantum systems, has been typically studied in atomic ensembles. In this work we study the enhanced emission of energy from coherent ensembles of harmonic oscillators. We show that it should be possible to observe harmonic oscillator superradiance in a variety of physical platforms such as waveguide arrays in integrated photonics and resonator arrays in circuit QED. We find general conditions specifying when emission is superradiant and subradiant and find that superradiant, subradiant and dark states take the…
In recent years, remarkable progress has been made towards encoding and processing quantum information in the large Hilbert space of bosonic modes. Mechanical resonators are of great interest for this purpose, since they confine many high quality factor modes into a small volume and can be easily integrated with many different quantum systems. An important yet challenging task is to create direct interactions between different mechanical modes. Here we demonstrate an in-situ tunable beam-splitter-type interaction between several mechanical modes of a high-overtone bulk acoustic wave resonator.…
$W$-type entangled states can be used as quantum channels for, e.g., quantum teleportation, quantum dense coding, and quantum key distribution. In this work, we propose a way to generate a macroscopic $W$-type entangled coherent state using quantum memories in circuit QED. The memories considered here are nitrogen-vacancy center ensembles (NVEs), each located in a different cavity. This proposal does not require initially preparing each NVE in a coherent state instead of a ground state, which should significantly reduce its experimental difficulty. For most of the operation time, each cavity r…
Quantum repeaters, which are indispensable for long-distance quantum communication, are necessary for extending the entanglement from short distance to long distance; however, high-rate entanglement distribution, even between adjacent repeater nodes, has not been realized. In a recent work by C. Jones, et al., New J. Phys. 18, 083015 (2016), the entanglement distribution rate between adjacent repeater nodes was calculated for a plurality of quantum dots, nitrogen-vacancy centers in diamond, and trapped ions adopted as quantum memories inside the repeater nodes. Considering practical use, arran…
A scheme for spatial multimode quantum memory is developed such that spatial-temporal structure of a weak signal pulse can be stored and recalled via cavity-assisted off-resonant Raman interaction with a strong angular-modulated control field in an extended $Λ$-type atomic ensemble. It is shown that effective multimode storage is possible when the Raman coherence spatial grating involves wave vectors with different longitudinal components relative to the paraxial signal field. The possibilities of implementing the scheme in the solid-state materials are discussed.
We present a protocol for the teleportation of the quantum state of a pulse of light onto the collective spin state of an atomic ensemble. The entangled state of light and atoms employed as a resource in this protocol is created by probing the collective atomic spin, Larmor precessing in an external magnetic field, off resonantly with a coherent pulse of light. We take here for the first time full account of the effects of Larmor precession and show that it gives rise to a qualitatively new type of multimode entangled state of light and atoms. The protocol is shown to be robust against the dom…
High-visibility interference of photon echoes generated in spatially separated solid-state atomic ensembles is demonstrated. The solid state ensembles were LiNbO$_3$ waveguides doped with Erbium ions absorbing at 1.53 $μ$m. Bright coherent states of light in several temporal modes (up to 3) are stored and retrieved from the optical memories using two-pulse photon echoes. The stored and retrieved optical pulses, when combined at a beam splitter, show almost perfect interference, which demonstrates both phase preserving storage and indistinguishability of photon echoes from separate optical memo…
For the last decade quantum memories have been intensively studied for potential applications to quantum information and communications using atomic and ionic ensembles. With the importance of a multimode storage capability in quantum memories, on-demand control of reversible inhomogeneous broadening of an optical medium has been broadly investigated recently. However, the photon storage time in these researches is still too short to apply for long-distance quantum communications. In this paper, we demonstrate new physics of spin population decay dependent ultralong photon storage method, wher…
A three-dimensional multimode lumped-element resonator for collective spin manipulation and dispersive readout
Hefei National Research Center for Physical Sciences at the Microscale and School of Physical Sciences, University of Science and Technology of China(中国科学技术大学物理科学学院、合肥微尺度物质科学国家研究中心);Shanghai Research Center for Quantum Science and CAS Center for Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China(中国科学技术大学、上海量子科学研究与探索中心、中国科学院量子信息与量子物理学前沿卓越创新中心)
A long-lived and multimode quantum memory is a key component needed for the development of quantum communication. Here we present temporally multiplexed storage of 5 photonic polarization qubits encoded onto weak coherent states in a rare-earth-ion doped crystal. Using spin refocusing techniques we can preserve the qubits for more than half a millisecond. The temporal multiplexing allows us to increase the effective rate of the experiment by a factor of 5, which emphasizes the importance of multimode storage for quantum communication. The fidelity upon retrieval is higher than the maximum clas…
Long-lived optical quantum memories are of great importance for scalable distribution of entanglement over remote networks (e.g. quantum repeaters). Long-lived storage generally relies on storing the optical states as spin excitations since these often exhibit long coherence times. To extend the storage time beyond the intrinsic spin dephasing time one can use dynamical decoupling techniques. However, it has been shown that dynamical decoupling introduces noise in optical quantum memories based on ensembles of atoms. In this article a simple model is proposed to calculate the resulting signal-…
Solid-state impurity spins with optical control are currently investigated for quantum networks and repeaters. Among these, rare-earth-ion doped crystals are promising as quantum memories for light, with potentially long storage time, high multimode capacity, and high bandwidth. However, with spins there is often a tradeoff between bandwidth, which favors electronic spin, and memory time, which favors nuclear spins. Here, we present optical storage experiments using highly hybridized electron-nuclear hyperfine states in $^{171}$Yb$^{3+}$:Y$_2$SiO$_5$, where the hybridization can potentially of…
Photon-echo based quantum memories use inhomogeneously broadened, optically thick ensembles of absorbers to store a weak optical signal and employ various protocols to rephase the atomic coherences for information retrieval. We study the application of two consecutive, frequency-chirped control pulses for coherence rephasing in an ensemble with a 'natural' inhomogeneous broadening. Although propagation effects distort the two control pulses differently, chirped pulses that drive adiabatic passage can rephase atomic coherences in an optically thick storage medium. Combined with spatial phase mi…
We present the possibility of steering the direction of correlations between the off-resonant Raman scattered photons from the angularly multimode atomic memory based on warm rubidium vapors. Using acousto-optic deflectors (AOD) driven by different modulation frequencies we experimentally change the angle of incidence of the laser beams on the atomic ensemble. Performing correlations measurements for various deflection angles we verify that we can choose the anti-Stokes light propagation direction independently of the correlated Stokes scattered light in the continuous way. As a result we can …
Long-distance quantum communication through optical fibers is currently limited to a few hundreds of kilometres due to fiber losses. Quantum repeaters could extend this limit to continental distances. Most approaches to quantum repeaters require highly multimode quantum memories in order to reach high communication rates. The atomic frequency comb memory scheme can in principle achieve high temporal multimode storage, without sacrificing memory efficiency. However, previous demonstrations have been hampered by the difficulty of creating high-resolution atomic combs, which reduces the efficienc…
Interfacing photonic and solid-state qubits within a hybrid quantum architecture offers a promising route towards large scale distributed quantum computing. In that respect, hybrid quantum systems combining circuit QED with ions doped into solids are an attractive platform. There, the ions serve as coherent memory elements and reversible conversion elements of microwave to optical qubits. Among many possible spin-doped solids, erbium ions offer the unique opportunity of a coherent conversion of microwave photons into the telecom C-band at $1.54\,μ$m employed for long distance communication. In…
We analyze the properties of a Raman quantum light-atom interface in long atomic ensemble and its applications as a quantum memory or two-mode squeezed state generator. We consider the weak-coupling regime and include both Stokes and anti-Stokes scattering and the effects of Doppler broadening in buffer gas assuming frequent velocity-averaging collisions. We find the Green functions describing multimode transformation from input to output fields of photons and atomic excitations. Proper mode basis is found via singular value decomposition for short interaction times. It reveals that triples of…
We investigate the problem of optimally reversing the action of an arbitrary quantum channel C which acts independently on each component of an ensemble of n identically prepared d-dimensional quantum systems. In the limit of large ensembles, we construct the optimal reversing channel R* which has to be applied at the output ensemble state, to retrieve a smaller ensemble of m systems prepared in the input state, with the highest possible rate m/n. The solution is found by mapping the problem into the optimal reversal of Gaussian channels on quantum-classical continuous variable systems, which …
We report on the observation of multimode strong coupling of a small ensemble of atoms interacting with the field of a 30-m long fiber resonator containing a nanofiber section. The collective light--matter coupling strength exceeds the free spectral range and the atoms couple to consecutive longitudinal resonator modes. The measured transmission spectra of the coupled atom-resonator system provide evidence of this regime, realized with a few hundred atoms with an intrinsic single-atom cooperativity of 0.26. These results are the starting point for studies in a new setting of light-matter inter…
Quantum repeaters promise to deliver long-distance entanglement overcoming noise and loss in realistic quantum channels. A promising class of repeaters, based on atomic ensemble quantum memories and linear optics, follow the proposal by Duan et al [Nature 414, 413, 2001]. Here we analyse this protocol in terms of a very general model for the quantum memories employed. We derive analytical expressions for scaling of entanglement with memory imperfections, dark counts, loss and distance, and apply our results to two specific quantum memory protocols. Our methods apply to any quantum memory with …
We investigate theoretically the coupling of a cavity mode to a continuous distribution of emitters. We discuss the influence of the emitters inhomogeneous broadening on the existence and on the coherence properties of the polaritonic peaks. We find that their coherence depends crucially on the shape of the distribution and not only on its width. Under certain conditions the coupling to the cavity protects the polaritonic states from inhomogeneous broadening, resulting in a longer storage time for a quantum memory based on emitters ensembles. When two different ensembles of emitters are couple…
Inhomogeneous Light-Matter Coupling as a Resource for Noiseless Quantum Memories
Centre for Quantum Technologies, Singapore(新加坡量子技术中心);National University of Singapore, Department of Materials Science and Engineering, Singapore(新加坡国立大学材料科学与工程系);National University of Singapore, Faculty of Science, Singapore(新加坡国立大学理学院);MajuLab, CNRS-UCA-SU-NUS-NTU International Joint Research Laboratory(MajuLab,CNRS-南法大学-索邦大学-新加坡国立大学-南洋理工大学国际联合实验室)
Memory-assisted quantum key distribution (MA-QKD) has recently been proposed as a technique to improve the rate-versus-distance behavior of QKD systems by using existing, or nearly-achievable, quantum technologies. The promise is that MA-QKD would require less demanding quantum memories than the ones needed for probabilistic quantum repeaters. Nevertheless, early investigations suggest that, in order to beat the conventional no-memory QKD schemes, the quantum memories used in the MA-QKD protocols must have high bandwidth-storage products and short interaction times. Among different types of qu…
Tripartite Entanglement in Multimode Cavity Quantum Electrodynamics
Department of Computer Science, Purdue University(普渡大学计算机科学系);Department of Physics and Astronomy, Rice University(莱斯大学物理与天文学系);Department Materials Science and Engineering, Ohio State University(俄亥俄州立大学材料科学与工程系)
Encoding logical quantum information in harmonic oscillator modes is a promising and hardware-efficient approach to the realization of a quantum computer. In this work, we propose to encode logical qubits in grid states of an ensemble of harmonic oscillator modes. We first discuss general results about these multimode bosonic codes; how to design them, how to practically implement them in different experimental platforms and how lattice symmetries can be leveraged to perform logical non-Clifford operations. We then introduce in detail two two-mode grid codes based on the hypercubic and D4 latt…