Besides the chemical constituents, it is the lattice geometry that controls the most important material properties. In many interesting compounds, the arrangement of elements leads to pronounced anisotropies, which reflect into a varying degree of quasi two-dimensionality of their low-energy excitations. Here, we start by classifying important families of correlated materials according to a simple measure for the tetragonal anisotropy of their ab initio electronic (band) structure. Second, we investigate the impact of a progressively large anisotropy in driving the non-locality of many-body effects. To this end, we tune the Hubbard model from isotropic cubic in three dimensions to the two-dimensional limit and analyze it using the dynamical vertex approximation. For sufficiently isotropic hoppings, we find the self-energy to be well separable into a static non-local and a dynamical local contribution. While the latter could potentially be obtained from dynamical mean-field approaches, we find the former to be non-negligible in all cases. Further, by increasing the model-anisotropy, we quantify the degree of quasi two-dimensionality which causes this "space-time separation" to break down. Our systematic analysis improves the general understanding of electronic correlations in anisotropic materials, heterostructures and ultra-thin films, and provides useful guidance for future realistic studies.
The decisive role of magnetic anisotropy even in systems with small anisotropy is illustrated for the honeycomb-layered antiferromagnets The decisive role of magnetic anisotropy in honeycomb layered Li$_3$Ni$_2$SbO$_6$ and Na$_3$Ni$_2$SbO$_6$ with $A$ = Li and Na. Both systems evolve long range magnetic order below $T_{\rm N}$ = 14 and 16.5~K, respectively. The magnetic phase diagrams obtained from static magnetisation studies up to 15~T imply competing antiferromagnetic phases and a tricritical point at $T_{\rm N}$. The phase boundaries are visible in the dynamic response of the antiferromagn…
The anisotropy of the electron scattering rate and lifetime $Γ_\mathbf{p}=1/τ_\mathbf{p}$ observed by Angle Resolved Photoemission Spectroscopy (ARPES) is evaluated using $s$-$d$ Kondo-Zener exchange Hamiltonian used previously to describe superconducting properties of high-$T_c$ cuprates; for correlation between critical temperature $T_c$ and BCS coupling constant, for example. The performed qualitative analysis reveals that "cold spots" correspond to nodal regions of the superconducting phase where the superconducting gap is zero, because the exchange interaction is annulled. Vice versa, "ho…
Spin Dynamics of Layered Triangular Antiferromagnets with Uniaxial Anisotropy
本文用MonteCarlo-分子动力学方法研究了具有反铁磁耦合的三角形层状晶格上具有单轴各向异性的半经典海森堡模型在有序相和顺磁相的自旋动力学.计算的重要量是全动力学结构函数$S(\bf q, ω)$、手征动力学结构函数$S_{chi}(ω)$、静态序参量和一些热力学量。结果表明，在有序相中存在对应于$S(\bf q, ω)$和$S_{chi}(ω)$的传播模，支持了最近的理论.我们的静态性质的结果表明，在每一层的磁有序是共面的3-亚晶格类型偏离120度结构。然而，在磁三聚化的存在下，我们发现3-亚晶格结构被削弱，并趋向于自旋的非共面性。
Perpendicular magnetic anisotropy of the new ferromagnetic semiconductor (Ba,K)(Zn,Mn)$_{2}$As$_{2}$ is studied by angle-dependent x-ray magnetic circular dichroism measurements. The large magnetic anisotropy with the anisotropy field of 0.85 T is deduced by fitting the Stoner-Wohlfarth model to the magnetic-field-angle dependence of the projected magnetic moment. Transverse XMCD spectra highlights the anisotropic distribution of Mn 3$d$ electrons, where the $d_{xz}$ and $d_{yz}$ orbitals are less populated than the $d_{xy}$ state because of the $D_{2d}$ splitting arising from the elongated Mn…
The quasi-two-dimensional antiferromagnet Ni$_2$P$_2$S$_6$ belongs to the family of magnetic van der Waals compounds that provides a rich material base for the realization of fundamental models of quantum magnetism in low dimensions. Here, we report high-frequency/high-magnetic field electron spin resonance measurements on single crystals of Ni$_2$P$_2$S$_6$. The results enable one to reliably determine the positive, "easy"-plane type of the single ion anisotropy of the Ni$^{2+}$ ions with the upper limit of its magnitude $\lesssim 0.7$ meV. The resonance response reveals strongly anisotropic …
The hallmark of superconductivity is the rigidity of the quantum-mechanical phase of electrons, responsible for superfluid behavior and Meissner effect. The strength of the phase stiffness is set by the Josephson coupling, which is strongly anisotropic in layered superconducting cuprates. So far, THz light pulses have been efficiently used to achieve non-linear control of the out-of-plane Josephson plasma mode, whose frequency scale lies in the THz range. However, the high-energy in-plane plasma mode has been assumed to be insensitive to THz pumping. Here, we show that THz driving of both low-…
The electronic and magnetic structure, including the Heisenberg model exchange interaction parameters, was explored for the recently proposed novel cuprate Cu$_2$F$_5$. Using the DFT+U calculation, it is shown that the compound is formed by two types of copper ions with $d^9$ and $d^8$ electronic configurations. We have found a very stable antiferromagnetic ordering with strong anisotropy of exchange interaction that results in the appearance of an unusual 2D-magnetism: within the (100)-plane the exchange between the S=1 and S=1/2 Cu ions has almost the same strength as between the two S=1 ion…
To get insight into the nature of the electronic fluid in the frustration-driven charge glasses, we investigate in-plane and out-of-plane charge transport for several quasi-triangular-lattice organic systems, $θ$-(BEDT-TTF)$_2$X [X=RbZn(SCN)$_4$, CsZn(SCN)$_4$ and I$_3$]. These compounds host a charge order, charge glass and Fermi liquid, depending on the strength of charge frustration. We find that the resistivity exhibits extremely two-dimensional (2D) anisotropy and contrasting temperature dependence between in the in-plane and out-of-plane directions in the charge glass phase, qualitativel…
MnBi2Te4(MBT) is a promising van der Waals layered antiferromagnetic (AF) topological insulator that combines a topologically non-trivial inverted Bi-Te band gap with ferromagnetic (FM) layers of Mn ions. We perform inelastic neutron scattering (INS) on co-aligned single crystals to study the magnetic interactions in MBT. Consistent with previous work, we find that the AF interlayer exchange coupling and uniaxial magnetic anisotropy have comparable strength, which supports metamagnetic transitions that allow access to different magnetic symmetries in applied fields. Modelling of the two-dimens…
Optical conductivity of layered topological semimetal TaNiTe$_5$
University of Zagreb（萨格勒布大学）；TU Wien（维也纳工业大学）；University of Fribourg（弗里堡大学）；University of West Bohemia in Pilsen（比尔森西波希米亚大学）；Brookhaven National Laboratory（布鲁克海文国家实验室）
