The interplay between disorder and transport is a problem central to the understanding of a broad range of physical processes, most notably the ability of a system to reach thermal equilibrium. Disorder and many body interactions are known to compete, with the dominance of one or the other giving rise to fundamentally different dynamical phases. Here we investigate the spin diffusion dynamics of 13C in diamond, which we dynamically polarize at room temperature via optical spin pumping of engineered color centers. We focus on low-abundance, strongly hyperfine-coupled nuclei, whose role in the polarization transport we expose through the integrated impact of variable radio-frequency excitation on the observable bulk 13C magnetic resonance signal. Unexpectedly, we find good thermal contact throughout the nuclear spin bath, virtually independent of the hyperfine coupling strength, which we attribute to effective carbon-carbon interactions mediated by the electronic spin ensemble. In particular, observations across the full range of hyperfine couplings indicate the nuclear spin diffusion constant takes values up to two orders of magnitude greater than that expected from homo-nuclear spin couplings. Our results open intriguing opportunities to study the onset of thermalization in a system by controlling the internal interactions within the bath.
Strongly polarizing weakly coupled $^{13}$C nuclear spins with optically pumped nitrogen-vacancy center
金刚石中氮空位（NV）中心周围核自旋极化的增强由于其广泛的应用而引起了人们的广泛关注。本文对如何利用基态能级反交叉的光泵NV中心优化动态核极化进行了理论分析和综合理解。我们的结果不仅为最近观测到的强耦合$^{13}$ C核的极化对磁场的依赖性提供了无参数的解释和清晰的物理图象[H. J. Wang \textit{et al} .，国家通信4，1（2013）]，而且还证明了在弱光泵浦和适当选择的磁场下强耦合弱耦合$^{13}$ C核的可能性。这允许用于NMR应用的$^{13}$ C核自旋极化的灵敏磁性控制和$^{13}$ C核自旋噪声的显著抑制以延长NV自旋相干时间。
We present theoretical description of Voigt and Faraday effect based optically pumped magnetometers using the Floquet expansion. Our analysis describes the spin-operator dynamics of the first, $\hat{F}(t)$, and second, $\hat{F}^2(t)$, order moments and takes into account of different pumping profiles and decoherence effects. We find that the theoretical results are in good agreement with the experimental demonstrations over a wide range of fields and pumping conditions. Finally, the theoretical analysis presented here is generalized and can be extended to different magnetometry schemes with ar…
The nitrogen-vacancy (N-V) center in diamond is a widely-used platform for quantum information processing and metrology. The electron-spin state of N-V center could be initialized and readout optically, and manipulated by resonate microwave fields. In this work, we analyze the dependence of electron-spin initialization on widths of laser pulses. We build a numerical model to simulate this process and verify the simulation results in experiment. Both simulations and experiments reveal a fact that shorter laser pulses are helpful to the electron-spin polarization. We therefore propose to use ext…
We experimentally demonstrate the temporary removal of thermal photons from a microwave mode at 1.45 GHz through its interaction with the spin-polarized triplet states of photo-excited pentacene molecules doped within a p-terphenyl crystal at room temperature. The crystal functions electromagnetically as a narrow-band cryogenic load, removing photons from the otherwise room-temperature mode via stimulated absorption. The noise temperature of the microwave mode dropped to $50^{+18}_{-32}$ K (as directly inferred by noise-power measurements) while the metal walls of the cavity enclosing the mode…
The ability to optically initialize the electronic spin of the nitrogen-vacancy (NV) center in diamond has long been considered a valuable resource to enhance the polarization of neighboring nuclei, but efficient polarization transfer to spin species outside the diamond crystal has proven challenging. Here we demonstrate variable-magnetic-field, microwave-enabled cross-polarization from the NV electronic spin to protons in a model viscous fluid in contact with the diamond surface. Slight changes in the cross-relaxation rate as a function of the wait time between successive repetitions of the t…
Optically pumped magnetometers are becoming a promising alternative to cryogenically-cooled superconducting magnetometers for detecting and imaging biomagnetic fields. Magnetic field detection is a completely non-invasive method, which allows one to study the function of excitable human organs with a sensor placed outside the human body. For instance, magnetometers can be used to detect brain activity or to study the activity of the heart. We have developed a highly sensitive miniature optically pumped magnetometer based on cesium atomic vapor kept in a paraffin-coated glass container. The mag…
We study the effect of optical polarization squeezing on the performance of a sensitive, quantum-noise-limited optically pumped magnetometer. We use Bell-Bloom (BB) optical pumping to excite a $^{87}$Rb vapor containing $8.2 \cdot 10^{12} \mathrm{atoms/cm^3}$ and Faraday rotation to detect spin precession. The sub-$\mathrm{pT}/\sqrt{\mathrm{Hz}}$ sensitivity is limited by spin projection noise (photon shot noise) at low (high) frequencies. Probe polarization squeezing both improves high-frequency sensitivity and increases measurement bandwidth, with no loss of sensitivity at any frequency, a d…
Laser cooling of atomic motion enables a wide variety of technological and scientific explorations using cold atoms. Here we focus on the effect of laser cooling on the photons instead of on the atoms. Specifically, we show that non-interacting photons can thermalize with the atoms to a grand canonical ensemble with a non-zero chemical potential. This thermalization is accomplished via scattering of light between different optical modes, mediated by the laser cooling process. While optically thin modes lead to traditional laser cooling of the atoms, the dynamics of multiple scattering in optic…
Sensitivity Scaling and Limits of Cavity Enhancement in Miniaturized Optically Pumped Magnetometers
ICFO - Institut de Ciències Fotòniques, The Barcelona Institute of Science and Technology（光子科学研究所，巴塞罗那科技研究院）；ICREA - Institució Catalana de Recerca i Estudis Avançats（加泰罗尼亚高级研究学院）
Spin-polarised atomic ensembles probed by light based on the Faraday interaction are a versatile platform for numerous applications in quantum metrology and quantum information processing. Here we consider an ensemble of Alkali atoms that are continuously optically pumped and probed. Due to the collective scattering of photons at large optical depth, the steady state of atoms does not correspond to an uncorrelated tensor-product state, as is usually assumed. We introduce a self-consistent method to approximate the steady state including the pair correlations, taking into account the multilevel…
Optically induced nuclear spin polarization in a single GaAs/AlGaAs quantum well probed by a resistance detection method in the fractional quantum Hall regime
Using holography, we model experiments in which a 2+1D strange metal is pumped by a laser pulse into a highly excited state, after which the time evolution of the optical conductivity is probed. We consider a finite-density state with mildly broken translation invariance and excite it by oscillating electric field pulses. At zero density, the optical conductivity would assume its thermalized value immediately after the pumping has ended. At finite density, pulses with significant DC components give rise to slow exponential relaxation, governed by a vector quasinormal mode. In contrast, for hig…
