Topological insulators (TIs) in three space dimensions can be characterized by a quantized magnetoelectric coefficient. However, this coupling does not have experimentally observable consequences in the presence of time-reversal symmetry, because the contributions of both bulk and surface states cancel each other. Instead, the characteristic response of a TI is a nonlinear magnetoelectric effect. Field theoretic aspects of the nonlinear magnetoelectric response and numerical calculations for experimentally relevant geometries are discussed. Distinct from this effect, the magnetoelectric coupling would bind a charge $\pm e/2$ in response to a monopole, which is referred to as Witten effect. If time reversal is broken explicitly, for instance, by a Zeeman field acting on the surface layer, the electromagnetic response of a TI can be described by a half-integer quantum Hall effect of surface electrons.
One of the hallmarks of time-reversal-symmetric topological insulators in three dimensions is the topological magnetoelectric effect (TME). So far, a time-reversal breaking variant of this effect has attracted much attention, in the sense that the induced electric charge changes sign when the direction of an externally applied magnetic field is reversed. Theoretically, this effect is described by the so-called axion term. Here, we discuss a time-reversal-symmetric TME, where the electric charge depends only on the magnitude of the magnetic field but is independent of its sign. We obtain this n…
Chromium(III) oxide is a classical collinear antiferromagnet with a linear magnetoelectric effect. We are presenting the measurements of the magnetoelectric susceptibility $α$ of a sputter-deposited 500-nm film and a bulk single-crystal of Cr$_\mathrm{2}$O$_\mathrm{3}$. We investigated the magnetic phase-transition and the critical exponent $β$ of the sublattice magnetization near Néel temperature. For the films, an exponent of 0.49(1) was found below 293 K, and changed to 1.06(4) near the Néel temperature of 298 K. For the single-crystal, the exponent was constant at 0.324(4). We investigated…
Magnetoelectric responses are a fundamental characteristic of materials that break time-reversal and inversion symmetries (notably multiferroics) and, remarkably, of "topological insulators" in which those symmetries are unbroken. Previous work has shown how to compute spin and lattice contributions to the magnetoelectric tensor. Here we solve the problem of orbital contributions by computing the frozen-lattice electronic polarization induced by a magnetic field. One part of this response (the "Chern-Simons term") can appear even in time-reversal-symmetric materials and has been previously sho…
We present a theory of magnetoelectric magnon-photon coupling in cavities hosting noncentrosymmetric magnets. Analogously to nonreciprocal phenomena in multiferroics, the magnetoelectric coupling is time-reversal and inversion asymmetric. This asymmetry establishes a means for exceptional tunability of magnon-photon coupling, which can be switched on and off by reversing the magnetization direction. Taking the multiferroic skyrmion-host Cu$_2$OSeO$_3$ with ultralow magnetic damping as an example, we reveal the electrical activity of skyrmion eigenmodes and propose it for magnon-photon splittin…
Controlling magnetism using voltage is highly desired for applications, but remains challenging due to fundamental contradiction between polarity and magnetism. Here we propose a mechanism to manipulate magnetic domain walls in ferrimagnetic or ferromagnetic multiferroics using electric field. Different from those studies based on static domain-level couplings, here the magnetoelectric coupling relies on the collaborative spin dynamics around domain walls. Accompanying the reversal of spin chirality driven by polarization switching, a "rolling-downhill"-like motion of domain wall is achieved a…
Topological fragility and bilinear magnetoelectric resistance in gapless edge states
Université Paris-Saclay, CEA, CNRS, SPEC（巴黎萨克雷大学、法国原子能和替代能源委员会、法国国家科学研究中心、SPEC）；Université Paris-Saclay, CNRS, Laboratoire de Physique des Solides（巴黎萨克雷大学、法国国家科学研究中心、固体物理实验室）；The Institute for Functional Intelligent Materials (I-FIM), National University of Singapore（新加坡国立大学功能智能材料研究所）
Topological insulators with a time reversal symmetry breaking perturbation near the surface present a magnetoelectric response that is quantized when the frequency of the probing fields is much smaller than the surface gap induced by the perturbation. In this work we describe the intrinsic finite frequency magnetoelectric response of topological insulators for frequencies of the order and larger than the surface gap, including the experimentally relevant case where the system is metallic. This response affects physical observable quantities and will give rise to new finite frequency phenomena …
We show that bilayer graphene exhibits magneto-electric effects that are formally similar to those commonly seen in band insulators with broken inversion and time-reversal symmetries. Three unusual features characterize the magneto-electric responses exhibited by bilayer graphene: (i) unlike most other magneto-electric media, bilayer graphene is a conductor, (ii) bilayer graphene has a non-quantized magneto-electric coupling even though its electronic structure does not break parity and time-reversal symmetry, and (iii) the magnitude of the magneto-electric coupling in bilayer graphene is dete…
The valleys in hexagonal two-dimensional systems with broken inversion symmetry carry an intrinsic orbital magnetic moment. Despite this, such systems possess zero net magnetization unless additional symmetries are broken, since the contributions from both valleys cancel. A nonzero net magnetization can be induced through applying both uniaxial strain to break the rotational symmetry of the lattice and an in-plane electric field to break time-reversal symmetry owing to the resulting current. This creates a magnetoelectric effect whose strength is characterized by a magnetoelectric susceptibili…
Magnetization can be induced by an electric field in systems without inversion symmetry $\mathcal{P}$ and time-reversal symmetry $\mathcal{T}$. This phenomenon is called the magnetoelectric (ME) effect. The spin ME effect has been actively studied in multiferroics. The orbital ME effect also exists and has been mainly discussed in topological insulators at zero temperature. In this paper, we study the intrinsic orbital ME response in metals at finite temperature using the Kubo formula. The intrinsic response originates from the Fermi sea and does not depend on the dissipation. Especially in sy…
The interface between a topological insulator and a ferromagnetic insulator exhibits an interesting interplay of topological Dirac electrons and magnetism. As has been shown recently, the breaking of time-reversal invariance by magnetic order generates a Chern-Simons term in the action, that in turn leads to a Berry phase and a magnetoelectric effect of topological origin. Here, we consider the system in the presence of long-range Coulomb interaction between the Dirac electrons, and find that the magnetoelectric effect of the fluctuating electric field becomes non-local. We derive a Landau-Lif…
In noncentrosymmetric superconductors (NCSs), the conversion of a charge current into spin magnetization - the so called magnetoelectric effect - is the direct indicator of the unconventional, mixed-parity order parameter. This paper proposes a scheme to detect the magnetoelectric effect by anomalous, equal-spin Andreev tunneling in NCS/ferromagnet contacts. The proposal relies on the ability to generate spin-polarized triplet pairing by passing an electric current through an NCS. Such an induced triplet pairing bears a similarity to the paradigmatic nonunitary pairing in triplet superfluids w…
We present spin transport studies on a low-field, room-temperature magnetoelectric multiferroic polycrystalline $\text{Sr}_{3}\text{Co}_{2}\text{Fe}_{24}\text{O}_{41}$ (SCFO)|Pt heterostructure wherein a highly tunable transverse conical magnetic phase is responsible for static and dynamic magnetoelectric coupling. We measured angular dependence of spin Hall magnetoresistance (SMR) at constant magnetic fields ($H$) in the range of 50 to 100 kOe. Application of field below the critical value (2.5 kOe), yielded negative SMR and the $H$-evolution of normalized SMR exhibited a negative gradient. F…
Topological insulators (TIs) exhibit a quantized magnetoelectric response when time-reversal symmetry is broken on its surface. This unusual electromagnetic (EM) response is a unique macroscopic manifestation of the quantum Hall effect on the TI surface and it is described by a quantized Chern-Simons theory. In this paper, we construct the Green's function (GF) describing the EM response of two topological media separated by a cylindrical interface. This GF, in the appropriate limits, describes the magnetoelectric effect of both i) a cylindrical TI surrounded by a dielectric fluid, and ii) a T…
A general formula for the average vector potential of bulk periodic systems is proposed and shown to set the boundary conditions at magnetic interfaces. For antiferromagnetic materials, the study reveals a unique relation between the macroscopic potential and the orientation-dependent magnetic quadrupole, as a result of the different crystalline and magnetic symmetries. In particular, at surfaces and interfaces of a truncated bulk without inversion and time-reversal symmetries, the average vector potential exhibits a discontinuity, which results in an interfacial magnetic field. In general, ho…
The magnitude of the inverse Faraday effect (IFE), a static magnetization due to an ac electric field, can be strongly increased in a mesoscopic sample, sensitive to time-reversal symmetry (TRS) breaking. Random rectification of ac voltages leads to a magnetization flux, which can be detected by an asymmetry of Hall resistances in a multi-terminal setup. In the absence of applied magnetic field through a chaotic quantum dot the IFE scale, quadratic in voltage, is found as an analytic function of the ac frequency, screening, and coupling to the contacts and floating probes, and numerically it d…
We propose a new method for calculating the Chern-Simons orbital magnetoelectric coupling, conventionally parametrized in terms of a phase angle $θ$. According to previous theories, $θ$ can be expressed as a 3D Brillouin-zone integral of the Chern-Simons 3-form defined in terms of the occupied Bloch functions. Such an expression is valid only if a smooth and periodic gauge has been chosen in the entire Brillouin zone, and even then, convergence with respect to the $\mathbf{k}$-space mesh density can be difficult to obtain. In order to solve this problem, we propose to relax the periodicity con…
University of Science and Technology of China（中国科学技术大学）；Shenzhen University（深圳大学）；Hefei National Laboratory, University of Science and Technology of China（中国科学技术大学合肥国家实验室）；Quantum Science Center of Guangdong-Hongkong-Macao Greater Bay Area (Guangdong)（粤港澳大湾区量子科学中心（广东））；The University of Hong Kong（香港大学）
We consider antiferromagnets breaking both time-reversal (Theta) and a primitive lattice translational symmetry (T) of a crystal but preserving the combination S = Theta T. The S symmetry leads to a Z_2 topological classification of insulators, separating the ordinary insulator phase from the "antiferromagnetic topological insulator" (AFTI) phase. This state is similar to the "strong" topological insulator with time-reversal symmetry, and shares with it such properties as a quantized magnetoelectric effect. However, for certain surfaces the surface states are intrinsically gapped with a half-q…
When time-reversal symmetry is broken on its surface, topological insulators exhibit a magnetoelectric response which is described by axion electrodynamics. A direct consequence of this theory is the appearance of a magnetic field that resembles the one produced by a magnetic image monopole when a point-like electric charge is located near the surface of the material. In this paper we investigate the more realistic problem when the point-like charge is replaced by a finite size sphere at constant potential. We calculate the electromagnetic fields using the potential formulation in a particular…
A quantized version of the magnetoelectric effect, known as the topological magnetoelectric effect, can exist in a time-reversal invariant topological insulator with all its surface states gapped out by magnetism. This topological phase, called the axion insulator phase, has been theoretically proposed but is still lack of conclusive experimental evidence due to the small signal of topological magnetoelectric effect. In this work, we propose that the dynamical in-plane magnetization in an axion insulator can generate a "pseudo-electric field", which acts on the surface state of topological ins…
The magnetoelectric coupling of electrons in a three-dimensional solid can be effectively described by axion electrodynamics. Here we report the discovery of the fractional magnetoelectric effect in chiral anomalous semimetals of the three-dimensional massless Wilson fermions, which have linear dispersions at the energy crossing point, and break the chiral symmetry at generic momenta. In the presence of electric and magnetic fields, the time-reversal and parity symmetry breaking give rise to the quarter-quantized topological magnetoelectric effect, which is directly related to the winding numb…
Twisted graphene systems have draw significant attention due to the discoveries of various correlated and topological phases. In particular, recently the alternating twisted trilayer graphene is discovered to exhibit unconventional superconductivity, which motivates us to study the electronic structures and possible interesting correlation effects of this class of alternating twisted graphene systems. In this work we consider generic alternating twisted multilayer graphene (ATMG) systems with $M$-$L$-$N$ stacking configurations, in which the $M$ ($L$) graphene layers and the $L$ ($N$) layers a…
A wide class of materials that were discovered to carry a topologically protected phase order has led to a highly active area of research called topological insulators. This phenomenon has radically changed our thinking because of their robust quantum coherent behavior showing two-dimensional Dirac-type metallic surface states and simultaneously insulating bulk states. The Dirac SSs are induced by the strong spin-orbit coupling as well as protected by the time reversal symmetry. Breaking TRS in a TI with ferromagnetic perturbation can lead to many exotic quantum phenomena, such as the quantum …
We construct exactly soluble lattice models for fractionalized, time reversal invariant electronic insulators in 2 and 3 dimensions. The low energy physics of these models is exactly equivalent to a non-interacting topological insulator built out of fractionally charged fermionic quasiparticles. We show that some of our models have protected edge modes (in 2D) and surface modes (in 3D), and are thus fractionalized analogues of topological insulators. We also find that some of the 2D models do not have protected edge modes -- that is, the edge modes can be gapped out by appropriate time reversa…
Topological states of quantum matter have attracted great attention in condensed matter physics and materials science. The study of time-reversal-invariant (TRI) topological states in quantum materials has made tremendous progress in both theories and experiments. As a great success, thousands of TRI topological materials are predicted through sweeping search. Richer exotic phenomena are expected to appear in magnetic topological materials because of varied magnetic configurations, but this study falls much behind due to the complex magnetic structures and transitions. Here, we predict the tet…
One of the intriguing properties characteristic to three-dimensional topological materials is the topological magnetoelectric phenomena arising from a topological term called the $θ$ term. Such magnetoelectric phenomena are often termed the axion electrodynamics, since the $θ$ term has exactly the same form as the action describing the coupling between a hypothetical elementary particle, axion, and a photon. The axion was proposed about forty years ago to solve the so-called strong CP problem in quantum chromodynamics, and is now considered as a candidate for dark matter. In this tutorial, we …
The relation between bulk topological invariants and experimentally observable physical quantities is a fundamental property of topological insulators and superconductors. In the case of chiral symmetric systems in odd spatial dimensions such as time-reversal invariant topological superconductors and topological insulators with sublattice symmetry, this relation has not been well understood. We clarify that the winding number which characterizes the bulk Z non-triviality of these systems can appear in electromagnetic and thermal responses in a certain class of heterostructure systems. It is al…
The 'magnetoelectric effect' arises from the coupling between magnetic and electric properties in materials. The Z2 invariant of topological insulators (TIs) leads to a quantized version of this phenomenon, known as the topological magnetoelectric (TME) effect. This effect can be realized in a new topological phase called an 'axion insulator' whose surface states are all gapped but the interior still obeys time reversal symmetry. We demonstrate such a phase using electrical transport measurements in a quantum anomalous Hall (QAH) sandwich heterostructure, in which two compositionally different…
Breaking the time-reversal symmetry of a topological insulator (TI) by ferromagnetism can induce exotic magnetoelectric phenomena such as quantized anomalous Hall (QAH) effect. Experimental observation of QAH effect in a magnetically doped TI requires ferromagnetism not relying on the charge carriers. We have realized the ferromagnetism independent of both polarity and density of carriers in Cr-doped BixSb2-xTe3 thin films grown by molecular beam epitaxy. Meanwhile, the anomalous Hall effect is found significantly enhanced with decreasing carrier density, with the anomalous Hall angle reaching…
Topological insulators are new states of matter with a bulk gap and robust gapless surface states protected by time-reversal symmetry. When time-reversal symmetry is broken, the surface states are gapped, which induces a topological response of the system to electromagnetic field--the topological magnetoelectric effect. In this paper we study the behavior of topological surface states in heterostructures formed by a topological insulator and a magnetic insulator. Several magnetic insulators with compatible magnetic structure and relatively good lattice matching with topological insulators ${\r…
Topological insulators can exhibit strong magnetoelectric effects when their time-reversal symmetry is broken. In this Letter we consider the magneto-optical Kerr and Faraday effects of a topological insulator thin film weakly exchange-coupled to a ferromagnet. We find that its Faraday rotation has a universal value at low-frequencies, $θ_{\mathrm{F}} = \mathrm{tan}^{-1}\,α$ where $α$ is the vacuum fine structure constant, and that it has a giant Kerr rotation $θ_{\mathrm{K}} = π/2$. These properties follow from a delicate interplay between thin-film cavity confinement and the surface Hall con…
Topological insulators with the time reversal symmetry broken exhibit strong magnetoelectric and magneto-optic effects. While these effects are well-understood in or near equilibrium, nonequilibrium physics is richer yet less explored. We consider a topological insulator thin film, weakly coupled to a ferromagnet, out of thermal equilibrium with a cold environment (quantum electrodynamics vacuum). We show that the heat flow to the environment is strongly circularly polarized, thus carrying away angular momentum and exerting a purely fluctuation-driven torque on the topological insulator film. …
We study the homotopy classification of symmetry representations to describe the bulk topological invariants protected by the combined operation of a two-fold rotation $C_{2z}$ and time-reversal $T$ symmetries. We define topological invariants as obstructions to having smooth Bloch wave functions compatible with a momentum-independent symmetry representation. When the Bloch wave functions are required to be smooth, the information on the band topology is contained in the symmetry representation. This implies that the $d$-dimensional homotopy class of the unitary matrix representation of the sy…
Axion Insulator State in Hundred-Nanometer-Thick Magnetic Topological Insulator Sandwich Heterostructures
Department of Physics, The Pennsylvania State University（宾夕法尼亚州立大学物理系）；Department of Physics, Hong Kong University of Science and Technology（香港科技大学物理系）；Materials Research Institute, The Pennsylvania State University（宾夕法尼亚州立大学材料研究所）
Two-dimensional electron systems with spin-orbit coupling in the proximity of a superconductor and a magnetic insulator have recently been considered as promising candidates to realize topological superconducting phases. Here we discuss electromagnetic response properties of these systems. Breaking of time-reversal symmetry leads to an anomalous Hall effect with a characteristic non-monotonic gate voltage dependence and a Hall conductivity that can change a sign as temperature is varied. The imaginary part of the Hall conductivity at finite frequency, which shows up for example in the Kerr rot…
Coupling of the spin and orbital degrees of freedom on the surface of a strong three-dimensional insulator, on the one hand, and textured magnetic configuration in an adjacent ferromagnetic film, on the other, is studied using a combination of transport and thermodynamic considerations. Expressing exchange coupling between the localized magnetic moments and Dirac electrons in terms of the electrons' out-of-plane orbital and spin magnetizations, we relate the thermodynamic properties of a general ferromagnetic spin texture to the physics in the zeroth Landau level. Persistent currents carried b…
Topological insulators (TI) are a new class of quantum materials with insulating bulk enclosed by topologically protected metallic boundaries. The surface states of three-dimensional TIs have spin helical Dirac structure, and are robust against time reversal invariant perturbations. This extraordinary property is notably exemplified by the absence of backscattering by nonmagnetic impurities and the weak antilocalization (WAL) of Dirac fermions. Breaking the time reversal symmetry (TRS) by magnetic element doping is predicted to create a variety of exotic topological magnetoelectric effects. He…
Weyl semimetals exhibit exotic Fermi-arc surface states, which strongly affect their electromagnetic properties. We derive analytical expressions for all components of the composite density-spin response tensor for the surfaces states of a Weyl-semimetal model obtained by closing the band gap in a topological insulating state and introducing a time-reversal-symmetry-breaking term. Based on the results, we discuss the electromagnetic susceptibilities, the current response, and other physical effects arising from the density-spin response. We find a magnetoelectric effect caused solely by the Fe…
