This paper reports on a detailed performance characterization of a recently developed optical single-sideband (OSSB) laser system based on an IQ modulator and second-harmonic generation for rubidium atom interferometry experiments. The measured performance is used to evaluate the noise contributions of this OSSB laser system when it is applied to drive stimulated Raman transitions in $^{87}$Rb for precision measurements of gravitational acceleration. The laser system suppresses unwanted sideband components, but additional phase shift compensation needs to be applied when performing frequency chirps with such an OSSB laser system. The total phase noise contribution of the OSSB laser system in the current experiment is 72 mrad for a single atom-interferometry sequence with interrogation times of $T=120$ ms, which corresponds to a relative precision of 32 n$g$ per shot. The dominant noise sources are found in the relative intensity fluctuations between sideband and carrier components and the phase noise of the microwave source.
A frequency doubled I/Q modulator based optical single-sideband (OSSB) laser system is demonstrated for atomic physics research, specifically for atom interferometry where the presence of additional sidebands causes parasitic transitions. The performance of the OSSB technique and the spectrum after second harmonic generation are measured and analyzed. The additional sidebands are removed with better than 20 dB suppression, and the influence of parasitic transitions upon stimulated Raman transitions at varying spatial positions is shown to be removed beneath experimental noise. This technique w…
Low-phase-noise and pure-spectrum Raman light is vital for high-precision atom interferometry by two-photon Raman transition. A preferred and prevalent solution for Raman light generation is electro-optic phase modulation. However, phase modulation inherently brings in double sidebands, resulting in residual sideband effects of multiple laser pairs beside Raman light in atom interferometry. Based on a well-designed rectangular fiber Bragg grating and an electro-optic modulator, optical single-sideband modulation has been realized at 1560 nm with a stable suppression ratio better than -25 dB de…
We present a new electro-optic modulation technique that enables a single laser diode to realize a cold-atom source and a quantum inertial sensor based on matter-wave interferometry. Using carrier-suppressed dual single-sideband modulation, an IQ modulator generates two optical sidebands from separate radio-frequency (rf) signals. These sidebands are controlled independently in frequency, phase, and power using standard rf components. Our laser source exhibits improved rejection of parasitic sidebands compared to those based on phase modulators, which generate large systematic shifts in atom i…
We present a theoretical study of atomic laser-assisted photoionization emission (LAPE). We consider an atom driven by a linearly polarized XUV laser in two different scenarios: i) a single attosecond pulse (in both the streaking and sideband regimes) and ii) an attosecond pulse train. The process takes place assisted by a linearly polarized infrared (IR) laser field. In all these cases the energy and angle-resolved photoelectron spectrum (PES) is determined by a leading contribution, related to the intracycle factor [Gramajo et al., J. Phys. B 51, 055603 (2018)], complemented by other ones, d…
We show that nonlinear dynamics in diode lasers with optical injection leads to frequency tunable microwave sidebands which are suitable for atomic physics experiments. We demonstrate the applicability of the sidebands in an experiment where rubidium atoms are magneto-optically trapped with both the trap and the re-pump optical frequencies derived from one optically injected laser. We find linewidth narrowing in the optical spectrum of the injected laser at both the injection frequency and the sideband frequency. With strong optical injection which leads to frequency locking we find a complete…
We demonstrate phase locking of two ultraviolet laser sources by modulating a fundamental infrared laser with 4th-order sidebands using an electro-optic modulator and phase locking of one sideband to a second fundamental infrared laser. Subsequent sum frequency generation and second harmonic generation successfully translates the frequency offset to the ultraviolet domain. The phase lock at 139 GHz is confirmed through stimulated Raman transitions for thermometry of $^9$Be$^+$ ions confined in a cryogenic Penning trap. This technique might be used for sideband cooling of single $^9$Be$^+$ ions…
A compact and robust laser system for atom interferometry based on a frequency-doubled telecom laser is presented. Thanks to an original stabilization architecture on a saturated absorption setup, we obtain a frequency-agile laser system allowing fast tuning of the laser frequency over 1 GHz in few ms using a single laser source. The different laser frequencies used for atom interferometry are generated by changing dynamically the frequency of the laser and by creating sidebands using a phase modulator. A laser system for Rubidium 87 atom interferometry using only one laser source based on a f…
We present here a simple laser system for a laser cooled atom interferometer, where all functions (laser cooling, interferometry and detection) are realized using only two extended cavity laser diodes, amplified by a common tapered amplifier. One laser is locked by frequency modulation transfer spectroscopy, the other being phase locked with an offset frequency determined by an Field-Programmable Gate Array (FPGA) controlled Direct Digital Synthesizer (DDS), which allows for efficient and versatile tuning of the laser frequency. Raman lasers are obtained with a double pass acousto-optic modula…
We introduce high-harmonic sideband spectroscopy (HHSS) and show that it can be a robust probe of attosecond charge migration (CM) in a halogenated carbon-chain molecule. We simulate both the CM and harmonic-generation (HHG) dynamics using ab initio time-dependent density-functional theory. We find that CM dynamics initiated along the molecular backbone induces sidebands in the HHG spectrum driven by a delayed laser pulse that is polarized perpendicular to the molecular axis. Monitoring the spectrum as either the HHG laser frequency or the relative delay is scanned allows for the extraction of…
We describe an optical bench in which we lock the relative frequencies or phases of a set of three lasers in order to use them in a cold atoms interferometry experiment. As a new feature, the same two lasers serve alternately to cool atoms and to realize the atomic interferometer. This requires a fast change of the optical frequencies over a few GHz. The number of required independent laser sources is then only 3, which enables the construction of the whole laser system on a single transportable optical bench. Recent results obtained with this optical setup are also presented.
We present a diode laser system optimized for laser cooling and atom interferometry with ultra-cold rubidium atoms aboard sounding rockets as an important milestone towards space-borne quantum sensors. Design, assembly and qualification of the system, combing micro-integrated distributed feedback (DFB) diode laser modules and free space optical bench technology is presented in the context of the MAIUS (Matter-wave Interferometry in Microgravity) mission. This laser system, with a volume of 21 liters and total mass of 27 kg, passed all qualification tests for operation on sounding rockets and i…
We have demonstrated a frequency-stabilized tunable 318.6 nm ultraviolet (UV) laser system for the single-photon 6S1/2 - nP (n = 70 ~ 100) Rydberg excitation of cesium atoms. The 637.2 nm laser produced by single-pass sum frequency generation from two infrared fiber lasers is offset locked to a high-finesse ultra-low expansion (ULE) optical cavity placed in ultra-high vacuum using the electronic sideband locking technique. The generated 318.6 nm UV laser via cavity-enhanced second-harmonic generation can be continuously tuned over 4 GHz by indirectly changing modulation frequency on the electr…
Laser cooling of atoms usually necessitates several laser frequencies. Alkaline atoms, for example, are cooled by two lasers with a frequency difference in the Gigahertz range. This gap cannot be closed with simple shifting techniques. Here, we present a method of generating sidebands at 6.6 GHz by modulating the current of a tapered amplifier which is seeded by an unmodulated master laser. The sidebands enable trapping of 1.1*10^9 Rubidium 87 atoms in a chip-based magneto-optical trap. Compared to the direct modulation of the master laser, this method allows for an easy implementation, a fast…
Atom interferometry using stimulated Raman transitions in a retroreflected configuration is the first choice in high precision measurements because it provides low phase noise, high quality Raman wavefront and simple experimental setup. However, it cannot be used for atoms at zero velocity because two pairs of Raman lasers are simultaneously resonant. Here we report a method which allows to lift this degeneracy by using a frequency chirp on the Raman lasers. Using this technique, we realize a Mach-Zehnder atom interferometer hybridized with a force balanced accelerometer which provides horizon…
We report the laser cooling of a single $^{40}\text{Ca}^+$ ion in a Penning trap to the motional ground state in one dimension. Cooling is performed in the strong binding limit on the 729-nm electric quadrupole $S_{1/2}\leftrightarrow D_{5/2}$ transition, broadened by a quench laser coupling the $D_{5/2}$ and $P_{3/2}$ levels. We find the final ground state occupation to be $98\pm1\%$. We measure the heating rate of the trap to be very low with $\dot{\bar{n}}\approx 0.3\pm0.2\textrm{s}^{-1}$ for trap frequencies from $150-400\textrm{kHz}$, consistent with the large ion-electrode distance.
We present an innovative fiber laser system for both cesium and rubidium manipulation. The architecture is based on frequency conversion of two lasers at 1560 nm and 1878 nm. By taking advantage of existing fiber components at these wavelengths, we demonstrate an all fiber laser system delivering 350 mW at 780 nm for rubidium and 210 mW at 852 nm for cesium. This result highlights the promising nature of such laser system especially for Cs manipulation for which no fiber laser system has been reported. It offers new perspectives for the development of atomic instruments dedicated to onboard ap…
We present a modular rack-mounted laser system for the cooling and manipulation of neutral rubidium atoms which has been developed for a portable gravimeter based on atom interferometry that will be capable of performing high precision gravity measurements directly at sites of geophysical interest. This laser system is constructed in a compact and mobile design so that it can be transported to different locations, yet it still offers improvements over many conventional laboratory-based laser systems. Our system is contained in a standard 19" rack and emits light at five different frequencies s…
We present results on a free-space atom interferometer operating on the first order magnetically insensitive |F=1,mF=0> -> |F=2,mF=0> transition of Bose-condensed 87Rb atoms. A pulsed atom laser is output-coupled from a Bose-Einstein condensate and propagates through a sequence of two internal state beam splitters, realized via coherent Raman transitions between the two interfering states. We observe Ramsey fringes with a visibility close to 100% and determine the current and the potentially achievable interferometric phase sensitivity. This system is well suited to testing recent proposals fo…
We demonstrate the enhancement and optimization of a cold strontium atomic beam from a two-dimensional magneto-optical trap (2D-MOT) transversely loaded from a collimated atomic beam by adding a sideband frequency to the cooling laser. The parameters of the cooling and sideband beams were scanned to achieve the maximum atomic beam flux and compared with Monte Carlo simulations. We obtained a 2.3 times larger, and 4 times brighter, atomic flux than a conventional, single-frequency 2D-MOT, for a given total power of 200 mW. We show that the sideband-enhanced 2D-MOT can reach the loading rate per…
We present a single solid-state laser system to cool, coherently manipulate and detect $^{25}$Mg$^+$ ions. Coherent manipulation is accomplished by coupling two hyperfine ground state levels using a pair of far-detuned Raman laser beams. Resonant light for Doppler cooling and detection is derived from the same laser source by means of an electro-optic modulator, generating a sideband which is resonant with the atomic transition. We demonstrate ground-state cooling of one of the vibrational modes of the ion in the trap using resolved-sideband cooling. The cooling performance is studied and disc…
We present a novel technique to phase-lock two lasers with controllable frequency difference. In our setup, one sideband of a current modulated Vertical-Cavity Surface-Emitting Laser (VCSEL) is phase locked to the master laser by injection seeding, while another sideband of the VCSEL is used to phase lock the slave laser. The slave laser is therefore locked in phase with the master laser, with a frequency difference tunable up to about 35 GHz. The sideband suppression rate of the slave laser is more than 30dB at 30 uW seed power. The heterodyne spectrum between master and slave has a linewidth…
We measure the photoelectron energy spectra from strong-field ionization of Kr in a two-color laser pulse consisting of a strong 400-nm field and a weak 800-nm field. The intensities of the main above-threshold ionization (ATI) and sideband peaks in the photoelectron energy spectra oscillate roughly oppositely with respect to the relative phase between the two-color components. We study the photoelectron interferometry in strong-field ATI regime from the view of interference of different electron trajectories in order to extend RABBITT type analysis to the strong-field regime. Based on the str…
We present a local measurement of gravity combining Bloch oscillations and atom interferometry. With a falling distance of 0.8 mm, we achieve a sensitivity of 2x10-7 g with an integration time of 300 s. No bias associated with the Bloch oscillations has been measured. A contrast decay with Bloch oscillations has been observed and attributed to the spatial quality of the laser beams. A simple experimental configuration has been adopted where a single retro-reflected laser beam is performing atoms launch, stimulated Raman transitions and Bloch oscillations. The combination of Bloch oscillations …
A low noise laser system for atom interferometry is realized with phase-locked fiber lasers, where the performance of the OPLL is greatly enhanced by the FEOM feedback loop and the narrow linewidths. The laser system demonstrated contribute 2.2 mrad per shot to the interferometer noise and permit continuous long-term operation for more than 115 hours without relocking in the field test. Also, the mobile gravimeter equipped with this phase-locked laser system reaches a sensitivity as good as 29 uGal/\sqrt{Hz} and a resolution of 1.1 uGal within 1500 s, demonstrating performances comparable to t…
In this paper, we report a new scheme to amplify a microwave signal carried on a laser light at $λ$=852nm. The amplification is done via a semiconductor tapered amplifier and this scheme is used to drive stimulated Raman transitions in an atom interferometer. Sideband generation in the amplifier, due to self-phase and amplitude modulation, is investigated and characterized. We also demonstrate that the amplifier does not induce any significant phase-noise on the beating signal. Finally, the degradation of the performances of the interferometer due to the amplification process is shown to be ne…
Motional ground state cooling and internal state preparation are important elements for quantum logic spectroscopy (QLS), a class of quantum information processing. Since QLS does not require the high gate fidelities usually associated with quantum computation and quantum simulation, it is possible to make simplifying choices in ion species and quantum protocols at the expense of some fidelity. Here, we report sideband cooling and motional state detection protocols for $^{138}$Ba$^+$ of sufficient fidelity for QLS without an extremely narrowband laser or the use of a species with hyperfine str…
We present a compact and stable dual-wavelength laser source for onboard atom interferometry with two different atomic species. It is based on frequency-doubled telecom lasers locked on a femtosecond optical frequency comb. We take advantage of the maturity of fiber telecom technology to reduce the number of free-space optical components which are intrinsically less stable, and to make the setup immune to vibrations and thermal fluctuations. The source provides the frequency agility and phase stability required for atom interferometry and can easily be adapted to other cold atom experiments. W…
We demonstrate a narrow-linewidth 780 nm laser system with up to 40 W power and a frequency modulation bandwidth of 230 MHz. Efficient overlap on nonlinear optical elements combines two pairs of phase-locked frequency components into a single beam. Serrodyne modulation with a high-quality sawtooth waveform is used to perform frequency shifts with > 96.5 % efficiency over tens of MHz. This system enables next-generation atom interferometry by delivering simultaneous, Stark-shift-compensated dual beam splitters while minimizing spontaneous emission.
We demonstrate Ramsey-Bordé (RB) atom interferometry for high performance laser stabilization with fractional frequency instability $<2 \times 10^{-16}$ for timescales between 10 and 1000s. The RB spectroscopy laser interrogates two counterpropagating $^{40}$Ca beams on the $^1$S$_0$ -- $^3$P$_1$ transition at 657 nm, yielding 1.6 kHz linewidth interference fringes. Fluorescence detection of the excited state population is performed on the (4s4p) $^3$P$_1$ -- (4p$^2$) $^3$P$_0$ transition at 431 nm. Minimal thermal shielding and no vibration isolation are used. These stability results surpass …
Single neutral atoms trapped in optical tweezers and laser-coupled to Rydberg states provide a fast and flexible platform to generate configurable atomic arrays for quantum simulation. The platform is especially suited to study quantum spin systems in various geometries. However, for experiments requiring continuous trapping, inhomogeneous light shifts induced by the trapping potential and temperature broadening impose severe limitations. Here we show how Raman sideband cooling allows one to overcome those limitations, thus, preparing the stage for Rydberg dressing in tweezer arrays.
We propose a scheme for ultrafast real-time imaging of laser-induced collective electron oscillations (Mie plasmons) in gas phase metal clusters by interferometrically stable scanning of two intense few-cycle optical laser pulses. The feasibility of our nonlinear spectral interferometry method with experimentally accessible observables is tested in a theoretical case study on simple-metal clusters (Na$_{147}$). The results show that the plasmon period and lifetime as well as the phase and relative amplitude of the collective electron motion can be extracted with sub-fs resolution. The access t…
We present a theoretical study of atomic ionization due to an XUV pulse in the presence of an infrared laser. Within the strong field approximation and considering the periodicity and symmetry of the transition matrix we show that the photoelectron spectrum can be described from the contribution during only one (or half) infrared cycle. These symmetry and periodicity properties impress selection rules which destructively cancel certain sideband orders favoring others. In particular, we analyze the photoionization of Argon in four geometrical arrangements of the polarization vector and the phot…
We present an analytic and numerical study for realizing single photon sideband cooling in an ultracold sample of fermionic Lithium trapped in a periodic optical potential. We develop an analytical model and obtain a master equation for the bound level populations. The cooling sequence is simulated both with a laser at a fixed frequency and with a frequency sweep. Finally, a Monte Carlo simulation is performed taking into account the full hyperfine spectrum of $^6\!$Li. We find that a gas of $^6\!$Li atoms loaded from a Magneto-Optical trap into a deep optical lattice can be cooled down to a $…
We report on the first realization of sub-Doppler laser cooling of 39K atoms using degenerate 3D Raman sideband cooling. We take advantage of the well-resolved excited hyperfine states on the D1 optical transition to produce spin polarized samples with $1.4 \times 10^8$ atoms at temperatures of 1.8 $μ$K. The phase-space densities are $\geq 10^{-4}$, which significantly improves the initial conditions for a subsequent evaporative cooling step. The presented cooling technique using the D1 line can be adapted to other atomic species and is applicable to high-resolution imaging schemes in far off-…
We report a simple technique for stabilization of a laser frequency at the wings of an atomic resonance. The reference signal used for stabilization issues from interference effects obtained in a low-quality cavity filled with a resonant atomic vapour. For a frequency detuned at 2.6 GHz from the $^{133}$Cs D$_2$ 6S$_{1/2}$ F=4 to 6P$_{3/2}$ F'= 5 transition, the fractional frequency Allan deviation is $10^{-8}$ for averaging times of 300 s, corresponding to a frequency deviation of 4 MHz. Adequate choice of the atomic density and of the cell thickness allows locking the laser at detunings larg…
Atom interferometry has become one of the most powerful technologies for precision measurements. To develop simple, precise, and versatile atom interferometers for inertial sensing, we demonstrate an atom interferometer measuring acceleration, rotation, and inclination by pointing Raman beams toward individual faces of a pyramidal mirror. Only a single diode laser is used for all functions, including atom trapping, interferometry, and detection. Efficient Doppler-sensitive Raman transitions are achieved without the velocity selecting the atom sample, and with zero differential AC Stark shift b…
A method of sideband Raman cooling to the vibrational ground state of the $m=0$ Zeeman sublevel in a far-detuned two-dimensional optical lattice is proposed. In our scheme, the Raman coupling between vibrational manifolds of the adjacent Zeeman sublevels is shifted to the red sideband due to the ac Stark effect induced by a weak pump field. Thus, cooling and optical pumping to $m=0$ is achieved by purely optical means with coplanar cw laser beams. The optical lattice and cooling parameters are estimated in the framework of simple theoretical models. An application of the transverse sideband co…
The uniformity of the intensity and phase of laser beams is crucial to high-performance atom interferometers. Inhomogeneities in the laser intensity profile cause contrast reductions and systematic effects in interferometers operated with atom sources at micro-Kelvin temperatures, and detrimental diffraction phase shifts in interferometers using large momentum transfer beam splitters. We report on the implementation of a so-called top-hat laser beam in a long-interrogation-time cold-atom interferometer to overcome the issue of the inhomogeneous laser intensity encountered when using Gaussian l…
Any slight variations in the fundamental constants of Nature, which may be induced by dark matter or some yet-to-be-discovered cosmic field, would characteristically alter the phase of a light beam inside an interferometer, which can be measured extremely precisely. Laser and maser interferometry may be applied to searches for the linear-in-time drift of the fundamental constants, detection of topological defect dark matter through transient-in-time effects and for a relic, coherently oscillating condensate, which consists of scalar dark matter fields, through oscillating effects. Our proposed…
The laser-like coherent emission at 391nm from N$_2$ gas irradiated by strong 800nm pump laser and weak 400nm seed laser is theoretically investigated. Recent experimental observations are well simulated, including temporal profile, optical gain and periodic modulation of the 391nm signal from N$_2^+$. Our calculation sheds light on the long standing controversy on whether population inversion is indispensable for the optical gain. We demonstrate the Ramsey interference fringes of the emission intensity at 391nm formed by additionally injecting another 800nm pump or 400nm seed, which are well …
We demonstrate single-photon time-domain interference in a new realm. We observe interferences in the photon counting statistics with two separate mode-locked femtosecond lasers of slightly different repetition frequencies, each emitting a comb of evenly spaced spectral lines over a wide spectral span. We exploit the interference pattern for spectroscopic diagnostics over a broad spectral range. An experimental proof-of-concept shows that the emerging technique of high-resolution dual-comb Fourier transform spectroscopy can be performed at light powers that are a billion-fold weaker than those…
We analyze the optomechanics of an atomic Bose-Einstein condensate interacting with the optical lattice inside a laser-pumped optical cavity and subject to a uniform bias force such as gravity. An atomic wave packet in a tilted lattice undergoes Bloch oscillations; in a cavity the backaction of the atoms on the light leads to a time-dependent modulation of the intracavity lattice at the Bloch frequency. When the Bloch frequency is on the order of the cavity damping rate we find transport of the atoms either up or down the lattice. The transport dynamics can be interpreted as a manifestation of…
Stimulated emission is the process fundamental to laser operation, thereby producing coherent photon output. Despite negatively-charged nitrogen-vacancy (NV$^-$) centres being discussed as a potential laser medium since the 1980's, there have been no definitive observations of stimulated emission from ensembles of NV$^-$ to date. Reasons for this lack of demonstration include the short excited state lifetime and the occurrence of photo-ionisation to the neutral charge state by light around the zero-phonon line. Here we show both theoretical and experimental evidence for stimulated emission fro…
