We present a theoretical study of atomic ionization due to an XUV pulse in the presence of an infrared laser. Within the strong field approximation and considering the periodicity and symmetry of the transition matrix we show that the photoelectron spectrum can be described from the contribution during only one (or half) infrared cycle. These symmetry and periodicity properties impress selection rules which destructively cancel certain sideband orders favoring others. In particular, we analyze the photoionization of Argon in four geometrical arrangements of the polarization vector and the photoelectron momentum direction.
We report the observation of multiple ionization of Argon through multi-XUV-photon absorption induced by an unprecedentedly powerful laser driven high-harmonic-generation source. Comparing the measured intensity dependence of the yield of the different Argon charge states with numerical calculations we can infer the different channels -direct and sequential- underlying the interaction. While such studies were feasible so far only with FEL sources, this work connects highly-non-linear-XUV-processes with the ultra-short time scales, inherent to the harmonic pulses, and highlights the advanced pe…
In this work, sidebands suppression brought by buffer gas argon (Ar) in cesium Faraday anomalous dispersion optical filter (FADOF) at 852 nm is investigated. FADOF performances at different Ar pressures (0 torr, 1 torr, 5 torr and 10 torr) are compared, and a single-peak transmittance spectrum with peak transmittance up to 80% is achieved at the high Ar pressure. A detailed analysis shows that, this sidebands suppression comes from the depopulation enhancement by the buffer gas. This result can be generalized to other FADOFs with similar level structures such as the D2 lines of other alkali me…
We study the ionization of atomic hydrogen in the direction of polarization due to a linearly polarized XUV pulse in the presence a strong field IR. We describe the photoelectron spectra as an interference problem in the time domain. Electron trajectories steming from different optical laser cycles give rise to intercycle interference energy peaks known as sidebands. These sidebands are modulated by a grosser structure coming from the intracycle interference of the two electron trajectories born during the same optical cycle. We make use of a simple semiclassical model which offers the possibi…
We present a theoretical study of atomic laser-assisted photoionization emission (LAPE). We consider an atom driven by a linearly polarized XUV laser in two different scenarios: i) a single attosecond pulse (in both the streaking and sideband regimes) and ii) an attosecond pulse train. The process takes place assisted by a linearly polarized infrared (IR) laser field. In all these cases the energy and angle-resolved photoelectron spectrum (PES) is determined by a leading contribution, related to the intracycle factor [Gramajo et al., J. Phys. B 51, 055603 (2018)], complemented by other ones, d…
We present a theoretical study of ionization of the hydrogen atom due to an XUV pulse in the presence of an IR laser with both fields linearly polarized in the same direction. In particular, we study the energy distribution of photoelectrons emitted perpendicularly to the polarization direction. By means of a very simple semiclassical model which considers electron trajectories born at different ionization times, the electron energy spectrum can be interpreted as the interplay of Intra and Intercycle interferences. The intracycle interference pattern stems from the coherent superposition of fo…
We report a joint experimental and theoretical study of a three-sideband (3-SB) modification of the "reconstruction of attosecond beating by interference of two-photon transitions" (RABBIT) setup. The 3-SB RABBIT scheme makes it possible to investigate phases resulting from interference between transitions of different orders in the continuum. Furthermore, the strength of this method is its ability to focus on the atomic phases only, independent of a chirp in the harmonics, by comparing the RABBIT phases extracted from specific SB groups formed by two adjacent harmonics. We verify earlier pred…
We consider the ionization of neon induced by a femtosecond laser pulse composed of overlapping, linearly polarized bichromatic extreme ultraviolet and infrared fields. In particular, we study the effects of the infrared light on a two-pathway ionization scheme for which Ne 2s22p53s1P is used as intermediate state. Using time-dependent calculations, supported by a theoretical approach based on the strong-field approximation, we analyze the ionization probability and the photoelectron angular distributions associated with the different sidebands of the ionization spectrum. Complex oscillations …
A theoretical study of ionization of the hydrogen atom due to an XUV pulse in the presence of an IR laser is presented. Well-established theories are usually used to describe the problem of laser assisted photoelectron effect. However, the well-known soft-photon approximation firstly posed by Maquet et al in Journal of Modern Optics 54, 1847 (2007) and Kazansky's theory in Phys. Rev. A 82, 033420 (2010) completely fails to predict the electron emission prependicularly to the polarization direction. Making use of a simple semiclassical model, we study the angle-resolved energy distribution of p…
Two XUV-photon double ionization of Ne, induced by an intense few-pulse attosecond train with a ~ 4 fs envelope duration is investigated experimentally and theoretically. The experiment is performed at ELI-ALPS utilizing the recently constructed 10 Hz gas phase high-order harmonic generation SYLOS GHHG-COMPACT beamline. A total pulse energy up to ~1 μJ generated in Argon in conjunction with high reflectivity optics in the XUV region, allowed the observation of the doubly charged state of Ne induced by 40 eV central XUV photon energies. The interaction of the intense attosecond pulse train with…
Multi-electron dynamics in atoms and molecules very often occur on sub- to few-femtosecond timescales. The available intensities of extreme-ultraviolet (XUV) attosecond pulses have previously only allowed the time-resolved investigation of two-photon, two-electron interactions. Here we demonstrate attosecond control over double and triple ionization of argon atoms involving the absorption of up to five XUV photons. In an XUV-pump XUV-probe measurement using a pair of attosecond pulse trains (APTs), the Ar$^{2+}$ ion yield exhibits a weak delay dependence, showing that its generation predominan…
In the present work we report on the current progress of the recently constructed GW attosecond extreme ultraviolet (XUV) source developed at the Institute of Electronic Structure and Laser of the Foundation for Research and Technology-Hellas (I.E.S.L-FO.R.T.H.). By the implementation of a compact-collinear polarization gating arrangement, the generation of a broadband, coherent XUV quasi-continuum produced by the interaction of a many-cycle infrared field with a gas phase medium is achieved. The spectral width of the XUV emission generated in Xenon, is spanning in the range of 17-32 eV and ca…
Time- and Angle-resolved photoelectron spectroscopy from surfaces can be used to record the dynamics of electrons and holes in condensed matter on ultrafast time scales. However, ultrafast photoemission experiments using extreme-ultraviolet (XUV) light have previously been limited by either space-charge effects, low photon flux, or limited tuning range. In this article, we describe space-charge-free XUV photoelectron spectroscopy experiments with up to 5 nA of average sample current using a tunable cavity-enhanced high-harmonic source operating at 88 MHz repetition rate. The source delivers $ …
The two-color above-threshold ionization (ATI) of atoms and ions is investigated for a vortex Bessel beam in the presence of a strong near-infrared (NIR) light field. While the photoionization is caused by the photons from the weak but extreme ultra-violet (XUV) vortex Bessel beam, the energy and angular distribution of the photoelectrons and their sideband structure are affected by the plane-wave NIR field. We here explore the energy spectra and angular emission of the photoelectrons in such two-color fields as a function of the size and location of the target (atoms) with regard to the beam …
We perform numerical simulations for photoionization of the argon atom when exposed to a combined field of an infrared laser (abbreviated IR) and its 13th harmonic (H13) by solving the Time-Dependent Schrödinger Equation (TDSE)], noting that the associated energy spectrum displays a harmonic peak dressed by the IR and other peaks called side-bands SB+-n corresponds to the absorption (+n) and the emission (-n) of the n-infrared photons above the ionization threshold. In two-color H13+IR photoionization of argon, the analysis of the angular distribution of the ejected electron in the continuum, …
We present the first demonstration of two-photon double ionization of neon using an intense extreme ultraviolet (XUV) attosecond pulse train (APT) in a photon energy regime where both direct and sequential mechanisms are allowed. For an APT generated through high-order harmonic generation (HHG) in argon we achieve a total pulse energy close to 1 $μ$J, a central energy of 35 eV and a total bandwidth of $\sim30$ eV. The APT is focused by broadband optics in a neon gas target to an intensity of $3\cdot10^{12} $W$\cdot$cm$^{-2}$. By tuning the photon energy across the threshold for the sequential …
Photoelectron spectra and photoelectron angular distributions obtained in photoionization reveal important information on e.g. charge transfer or hole coherence in the parent ion. Here we show that optimal control of the underlying quantum dynamics can be used to enhance desired features in the photoelectron spectra and angular distributions. To this end, we combine Krotov's method for optimal control theory with the time-dependent configuration interaction singles formalism and a splitting approach to calculate photoelectron spectra and angular distributions. The optimization target can accou…
Technical design report of a complete and compact broadband high-harmonics femtosecond beamline based on a modular hollow waveguide for photons generation centered on the upper region of the extreme ultraviolet spectral range
Institut de Physique et Chimie des Materiaux, CNRS, IPCMS, UMR 7504（材料物理与化学研究所）；Université de Caen Normandie, ENSICAEN, CNRS/IN2P3, LPC Caen UMR6534（卡昂诺曼底大学）
We investigate the role of excited states in High-order Harmonic Generation by studying the spectral, spatial and temporal characteristics of the radiation produced near the ionization threshold of argon by few-cycle laser pulses. We show that the population of excited states can lead either to direct XUV emission through Free Induction Decay or to the generation of high-order harmonics through ionization from these states and recombination to the ground state. By using the attosecond lighthouse technique, we demonstrate that the high-harmonic emission from excited states is temporally delayed…
Photoelectron spectroscopy of 3s3p doubly excited helium dressed with strong near-infrared laser fields
Nagoya University（名古屋大学）；RIKEN, SPring-8 Center（理化学研究所 SPring-8 中心）；Fu-Jen Catholic University（辅仁大学）；Japan Synchrotron Radiation Research Institute（日本同步辐射研究机构）；University of Toyama（富山大学）
We analyze interference processes in atomic ionization induced by a two-color laser with fundamental frequency $ω$ and its second harmonic $2ω$. The interplay between inter- and intracycle interference processes give rise to multiphoton peaks which can be named as main or ATI peaks and sidebands, in analogy to the well-known RABBIT (reconstruction of attosecond harmonic beating by interference of two-photon transitions). We use the saddle point approximation (SPA) to extract the complex ionization times of the interfering electron trajectories. Changing the relative phase between the two color…
