The uniformity of the intensity and phase of laser beams is crucial to high-performance atom interferometers. Inhomogeneities in the laser intensity profile cause contrast reductions and systematic effects in interferometers operated with atom sources at micro-Kelvin temperatures, and detrimental diffraction phase shifts in interferometers using large momentum transfer beam splitters. We report on the implementation of a so-called top-hat laser beam in a long-interrogation-time cold-atom interferometer to overcome the issue of the inhomogeneous laser intensity encountered when using Gaussian laser beams. We characterize the intensity and relative phase profiles of the top-hat beam and demonstrate its gain in atom-optics efficiency over a Gaussian beam, in agreement with numerical simulations. We discuss the application of top-hat beams to improve the performance of different architectures of atom interferometers.
A low noise laser system for atom interferometry is realized with phase-locked fiber lasers, where the performance of the OPLL is greatly enhanced by the FEOM feedback loop and the narrow linewidths. The laser system demonstrated contribute 2.2 mrad per shot to the interferometer noise and permit continuous long-term operation for more than 115 hours without relocking in the field test. Also, the mobile gravimeter equipped with this phase-locked laser system reaches a sensitivity as good as 29 uGal/\sqrt{Hz} and a resolution of 1.1 uGal within 1500 s, demonstrating performances comparable to t…
We present a compact and stable dual-wavelength laser source for onboard atom interferometry with two different atomic species. It is based on frequency-doubled telecom lasers locked on a femtosecond optical frequency comb. We take advantage of the maturity of fiber telecom technology to reduce the number of free-space optical components which are intrinsically less stable, and to make the setup immune to vibrations and thermal fluctuations. The source provides the frequency agility and phase stability required for atom interferometry and can easily be adapted to other cold atom experiments. W…
Atom interferometry has become one of the most powerful technologies for precision measurements. To develop simple, precise, and versatile atom interferometers for inertial sensing, we demonstrate an atom interferometer measuring acceleration, rotation, and inclination by pointing Raman beams toward individual faces of a pyramidal mirror. Only a single diode laser is used for all functions, including atom trapping, interferometry, and detection. Efficient Doppler-sensitive Raman transitions are achieved without the velocity selecting the atom sample, and with zero differential AC Stark shift b…
A compact and robust laser system for atom interferometry based on a frequency-doubled telecom laser is presented. Thanks to an original stabilization architecture on a saturated absorption setup, we obtain a frequency-agile laser system allowing fast tuning of the laser frequency over 1 GHz in few ms using a single laser source. The different laser frequencies used for atom interferometry are generated by changing dynamically the frequency of the laser and by creating sidebands using a phase modulator. A laser system for Rubidium 87 atom interferometry using only one laser source based on a f…
We demonstrate a narrow-linewidth 780 nm laser system with up to 40 W power and a frequency modulation bandwidth of 230 MHz. Efficient overlap on nonlinear optical elements combines two pairs of phase-locked frequency components into a single beam. Serrodyne modulation with a high-quality sawtooth waveform is used to perform frequency shifts with > 96.5 % efficiency over tens of MHz. This system enables next-generation atom interferometry by delivering simultaneous, Stark-shift-compensated dual beam splitters while minimizing spontaneous emission.
We present here a simple laser system for a laser cooled atom interferometer, where all functions (laser cooling, interferometry and detection) are realized using only two extended cavity laser diodes, amplified by a common tapered amplifier. One laser is locked by frequency modulation transfer spectroscopy, the other being phase locked with an offset frequency determined by an Field-Programmable Gate Array (FPGA) controlled Direct Digital Synthesizer (DDS), which allows for efficient and versatile tuning of the laser frequency. Raman lasers are obtained with a double pass acousto-optic modula…
We demonstrate Ramsey-Bordé (RB) atom interferometry for high performance laser stabilization with fractional frequency instability $<2 \times 10^{-16}$ for timescales between 10 and 1000s. The RB spectroscopy laser interrogates two counterpropagating $^{40}$Ca beams on the $^1$S$_0$ -- $^3$P$_1$ transition at 657 nm, yielding 1.6 kHz linewidth interference fringes. Fluorescence detection of the excited state population is performed on the (4s4p) $^3$P$_1$ -- (4p$^2$) $^3$P$_0$ transition at 431 nm. Minimal thermal shielding and no vibration isolation are used. These stability results surpass …
We describe an optical bench in which we lock the relative frequencies or phases of a set of three lasers in order to use them in a cold atoms interferometry experiment. As a new feature, the same two lasers serve alternately to cool atoms and to realize the atomic interferometer. This requires a fast change of the optical frequencies over a few GHz. The number of required independent laser sources is then only 3, which enables the construction of the whole laser system on a single transportable optical bench. Recent results obtained with this optical setup are also presented.
We present a diode laser system optimized for laser cooling and atom interferometry with ultra-cold rubidium atoms aboard sounding rockets as an important milestone towards space-borne quantum sensors. Design, assembly and qualification of the system, combing micro-integrated distributed feedback (DFB) diode laser modules and free space optical bench technology is presented in the context of the MAIUS (Matter-wave Interferometry in Microgravity) mission. This laser system, with a volume of 21 liters and total mass of 27 kg, passed all qualification tests for operation on sounding rockets and i…
A frequency doubled I/Q modulator based optical single-sideband (OSSB) laser system is demonstrated for atomic physics research, specifically for atom interferometry where the presence of additional sidebands causes parasitic transitions. The performance of the OSSB technique and the spectrum after second harmonic generation are measured and analyzed. The additional sidebands are removed with better than 20 dB suppression, and the influence of parasitic transitions upon stimulated Raman transitions at varying spatial positions is shown to be removed beneath experimental noise. This technique w…
The laser-like coherent emission at 391nm from N$_2$ gas irradiated by strong 800nm pump laser and weak 400nm seed laser is theoretically investigated. Recent experimental observations are well simulated, including temporal profile, optical gain and periodic modulation of the 391nm signal from N$_2^+$. Our calculation sheds light on the long standing controversy on whether population inversion is indispensable for the optical gain. We demonstrate the Ramsey interference fringes of the emission intensity at 391nm formed by additionally injecting another 800nm pump or 400nm seed, which are well …
We present a new electro-optic modulation technique that enables a single laser diode to realize a cold-atom source and a quantum inertial sensor based on matter-wave interferometry. Using carrier-suppressed dual single-sideband modulation, an IQ modulator generates two optical sidebands from separate radio-frequency (rf) signals. These sidebands are controlled independently in frequency, phase, and power using standard rf components. Our laser source exhibits improved rejection of parasitic sidebands compared to those based on phase modulators, which generate large systematic shifts in atom i…
We demonstrate single-photon time-domain interference in a new realm. We observe interferences in the photon counting statistics with two separate mode-locked femtosecond lasers of slightly different repetition frequencies, each emitting a comb of evenly spaced spectral lines over a wide spectral span. We exploit the interference pattern for spectroscopic diagnostics over a broad spectral range. An experimental proof-of-concept shows that the emerging technique of high-resolution dual-comb Fourier transform spectroscopy can be performed at light powers that are a billion-fold weaker than those…
This paper reports on a detailed performance characterization of a recently developed optical single-sideband (OSSB) laser system based on an IQ modulator and second-harmonic generation for rubidium atom interferometry experiments. The measured performance is used to evaluate the noise contributions of this OSSB laser system when it is applied to drive stimulated Raman transitions in $^{87}$Rb for precision measurements of gravitational acceleration. The laser system suppresses unwanted sideband components, but additional phase shift compensation needs to be applied when performing frequency c…
We present a general theory for laser-free entangling gates with trapped-ion hyperfine qubits, using either static or oscillating magnetic-field gradients combined with a pair of uniform microwave fields symmetrically detuned about the qubit frequency. By transforming into a `bichromatic' interaction picture, we show that either ${\hatσ_ϕ\otimes\hatσ_ϕ}$ or ${\hatσ_{z}\otimes\hatσ_{z}}$ geometric phase gates can be performed. The gate basis is determined by selecting the microwave detuning. The driving parameters can be tuned to provide intrinsic dynamical decoupling from qubit frequency fluct…
Atom interferometry using stimulated Raman transitions in a retroreflected configuration is the first choice in high precision measurements because it provides low phase noise, high quality Raman wavefront and simple experimental setup. However, it cannot be used for atoms at zero velocity because two pairs of Raman lasers are simultaneously resonant. Here we report a method which allows to lift this degeneracy by using a frequency chirp on the Raman lasers. Using this technique, we realize a Mach-Zehnder atom interferometer hybridized with a force balanced accelerometer which provides horizon…
We propose a scheme for ultrafast real-time imaging of laser-induced collective electron oscillations (Mie plasmons) in gas phase metal clusters by interferometrically stable scanning of two intense few-cycle optical laser pulses. The feasibility of our nonlinear spectral interferometry method with experimentally accessible observables is tested in a theoretical case study on simple-metal clusters (Na$_{147}$). The results show that the plasmon period and lifetime as well as the phase and relative amplitude of the collective electron motion can be extracted with sub-fs resolution. The access t…
Any slight variations in the fundamental constants of Nature, which may be induced by dark matter or some yet-to-be-discovered cosmic field, would characteristically alter the phase of a light beam inside an interferometer, which can be measured extremely precisely. Laser and maser interferometry may be applied to searches for the linear-in-time drift of the fundamental constants, detection of topological defect dark matter through transient-in-time effects and for a relic, coherently oscillating condensate, which consists of scalar dark matter fields, through oscillating effects. Our proposed…
We report a simple technique for stabilization of a laser frequency at the wings of an atomic resonance. The reference signal used for stabilization issues from interference effects obtained in a low-quality cavity filled with a resonant atomic vapour. For a frequency detuned at 2.6 GHz from the $^{133}$Cs D$_2$ 6S$_{1/2}$ F=4 to 6P$_{3/2}$ F'= 5 transition, the fractional frequency Allan deviation is $10^{-8}$ for averaging times of 300 s, corresponding to a frequency deviation of 4 MHz. Adequate choice of the atomic density and of the cell thickness allows locking the laser at detunings larg…
We present an innovative fiber laser system for both cesium and rubidium manipulation. The architecture is based on frequency conversion of two lasers at 1560 nm and 1878 nm. By taking advantage of existing fiber components at these wavelengths, we demonstrate an all fiber laser system delivering 350 mW at 780 nm for rubidium and 210 mW at 852 nm for cesium. This result highlights the promising nature of such laser system especially for Cs manipulation for which no fiber laser system has been reported. It offers new perspectives for the development of atomic instruments dedicated to onboard ap…
We present a modular rack-mounted laser system for the cooling and manipulation of neutral rubidium atoms which has been developed for a portable gravimeter based on atom interferometry that will be capable of performing high precision gravity measurements directly at sites of geophysical interest. This laser system is constructed in a compact and mobile design so that it can be transported to different locations, yet it still offers improvements over many conventional laboratory-based laser systems. Our system is contained in a standard 19" rack and emits light at five different frequencies s…
We present results on a free-space atom interferometer operating on the first order magnetically insensitive |F=1,mF=0> -> |F=2,mF=0> transition of Bose-condensed 87Rb atoms. A pulsed atom laser is output-coupled from a Bose-Einstein condensate and propagates through a sequence of two internal state beam splitters, realized via coherent Raman transitions between the two interfering states. We observe Ramsey fringes with a visibility close to 100% and determine the current and the potentially achievable interferometric phase sensitivity. This system is well suited to testing recent proposals fo…
We demonstrate matterwave interference in a warm vapor of rubidium atoms. Established approaches to light pulse atom interferometry rely on laser cooling to concentrate a large ensemble of atoms into a velocity class resonant with the atom optical light pulse. In our experiment, we show that clear interference signals may be obtained without laser cooling. This effect relies on the Doppler selectivity of the atom interferometer resonance. This interferometer may be configured to measure accelerations, and we demonstrate that multiple interferometers may be operated simultaneously by addressing…
Atom interferometry is the most successful technique for precision metrology. However, current interferometers using ultracold atoms allows one to probe the interference pattern only momentarily and has finite duty cycle, resulting in an aliasing effect and a low-bandwidth measurement -- also known as Dick effect. Interferometry with a continuous-wave atom laser shows promise in overcoming these limitations due a continuous monitoring of the interference pattern. In this work, we demonstrate a key step towards such an interferometry by demonstrating a diffraction of an `atom laser' in the Rama…
A Ramsey-type interferometer is suggested, employing a cold trapped ion and two time-delayed off-resonant femtosecond laser pulses. The laser light couples to the molecular polarization anisotropy, inducing rotational wavepacket dynamics. An interferogram is obtained from the delay dependent populations of the final field-free rotational states. Current experimental capabilities for cooling and preparation of the initial state are found to yield an interferogram visibility of more than 80\%. The interferograms can be used to determine the polarizability anisotropy with an accuracy of about $\p…
We present a local measurement of gravity combining Bloch oscillations and atom interferometry. With a falling distance of 0.8 mm, we achieve a sensitivity of 2x10-7 g with an integration time of 300 s. No bias associated with the Bloch oscillations has been measured. A contrast decay with Bloch oscillations has been observed and attributed to the spatial quality of the laser beams. A simple experimental configuration has been adopted where a single retro-reflected laser beam is performing atoms launch, stimulated Raman transitions and Bloch oscillations. The combination of Bloch oscillations …
The interaction of intense mid-infrared laser fields with atoms and molecules leads to a range of new opportunities, from the production of bright, coherent radiation in the soft x-ray range to imaging molecular structures and dynamics with attosecond temporal and sub-angstrom spatial resolution. However, all these effects, which rely on laser-driven recollision of an electron removed by the strong laser field and the parent ion, suffer from the rapidly increasing role of the magnetic field component of the driving pulse: the associated Lorentz force pushes the electrons off course in their ex…
Continuum-electron interferometry for enhancement of photoelectron circular dichroism and measurement of bound, free, and mixed contributions to chiral response
We here present a high sensitivity gravity-gradiometer based on atom interferometry. In our apparatus, two clouds of laser-cooled rubidium atoms are launched in fountain configuration and interrogated by a Raman interferometry sequence to probe the gradient of gravity field. We recently implemented a high-flux atomic source and a newly designed Raman lasers system in the instrument set-up. We discuss the applications towards a precise determination of the Newtonian gravitational constant G. The long-term stability of the instrument and the signal-to-noise ratio demonstrated here open interesti…
Using the frequency-domain theory, the high-order above threshold ionization (HATI) of a molecule is treated as a two-step transition: an above threshold ionization (ATI) followed by a laser-assisted collision (LAC). It is found that the HATI spectrum carries three pieces of information: the fingerprint of the molecular wave function lying in the ATI transition, the geometry structure of the molecule lying in the potential scattering between two plane waves, and the interaction between the ionized electron and the laser field lying in a phase factor in the LAC transition, where the phase facto…
The Matter-Wave laser Interferometer Gravitation Antenna, MIGA, will be a hybrid instrument composed of a network of atom interferometers horizontally aligned and interrogated by the resonant field of an optical cavity. This detector will provide measurements of sub Hertz variations of the gravitational strain tensor. MIGA will bring new methods for geophysics for the characterization of spatial and temporal variations of the local gravity field and will also be a demonstrator for future low frequency Gravitational Wave (GW) detections. MIGA will enable a better understanding of the coupling a…
We propose a two-dimensional interferometry based on electron wave packet interference with a cycle-shaped orthogonally polarized two-color laser field. With such method, sub-cycle and inter-cycle interferences can be disentangled into different direction in the measured photoelectron momentum spectra. With the cycle-shaped laser field, the Coulomb influence can be minimized and the overlapping of interference fringes with the complicate low-energy structures can be avoided as well. The contributions of excitation effect and long-range Coulomb potential can be traced in the Fourier domain of t…
A new class of atomic interferences using ultra-narrow optical transitions are pushing quantum engineering control to a very high level of precision for a next generation of sensors and quantum gate operations. In such context, we propose a new quantum engineering approach to Ramsey-Bordé interferometry introducing multiple composite laser pulses with tailored pulse duration, Rabi field amplitude, frequency detuning and laser phase-step. We explore quantum metrology with hyper-Ramsey and hyper-Hahn-Ramsey clocks below the $10^-18$ level of fractional accuracy by a fine tuning control of light …
Light-pulse atom interferometers rely on the wave nature of matter and its manipulation with coherent laser pulses. They are used for precise gravimetry and inertial sensing as well as for accurate measurements of fundamental constants. Reaching higher precision requires longer interferometer times which are naturally encountered in microgravity environments such as drop-tower facilities, sounding rockets and dedicated satellite missions aiming at fundamental quantum physics in space. In all those cases, it is necessary to consider arbitrary trajectories and varying orientations of the interfe…
Echo atom interferometers have emerged as interesting alternatives to Raman interferometers for the realization of precise measurements of the gravitational acceleration $g$ and the determination of the atomic fine structure through measurements of the atomic recoil frequency $ω_q$. Here we review the development of different configurations of echo interferometers that are best suited to achieve these goals. We describe experiments that utilize near-resonant excitation of laser-cooled rubidium atoms by a sequence of standing wave pulses to measure $ω_q$ with a statistical uncertainty of 37 par…
Atom interferometry on optical clock transitions is being pursued for numerous long-baseline experiments both terrestrially and for future space missions. Crucial to meeting these experiments' required sensitivities is the implementation of large momentum transfer ($>$10$^3\hbar k$). Here we show that to sequentially apply such a large momentum via $π$ pulses places stringent requirements on the frequency noise of the interferometry laser, finding that the linewidth is required to be considerably lower than has previously been suggested. This is due to imperfect pulse fidelity in the presence …
Laser-induced electron tunneling underlies numerous emerging spectroscopic techniques to probe attosecond electron dynamics in atoms and molecules. The improvement of those techniques requires an accurate knowledge of the exit momentum for the tunneling wave packet. Here we demonstrate a photoelectron interferometric scheme to probe the electron momentum longitudinal to the tunnel direction at the tunnel exit by measuring the photoelectron holographic pattern in an orthogonally polarized two-color laser pulse. In this scheme, we use a perturbative 400-nm laser field to modulate the photoelectr…
Photoelectron interferometry with spectrally shaped polychromatic infrared pulses
Lund University（隆德大学）；Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, LCPMR（索邦大学，法国国家科学研究中心，物理化学物质与辐射实验室）；Institute of Atomic and Molecular Physics, Jilin University（吉林大学原子与分子物理研究所）；Albert-Ludwigs-Universität Freiburg（弗赖堡大学）；EUCOR Centre for Quantum Science and Quantum Computing, Albert-Ludwigs-Universität Freiburg（弗赖堡大学 EUCOR 量子科学与量子计算中心）；University of Gothenburg（哥德堡大学）
