6+4 pages, 3+2 figures. This is a preprint of an article published in npj Quantum Mater. The final authenticated version is available online at: https://doi.org/10.1038/s41535-020-00285-3
The bond-disordered Kitaev model attracts much attention due to the experimental relevance in $α$-RuCl$_3$ and $A_3$LiIr$_2$O$_6$ ($A=$ H, D, Ag, $\textit{etc.}$). Applying a magnetic field to break the time-reversal symmetry leads to a strong modulation in mass terms for Dirac cones. Because of the smallness of the flux gap of the Kitaev model, a small bond disorder can have large influence on itinerant Majorana fermions, and Majorana fermions will be in the Anderson localization state immediately. We call this immobile liquid state Anderson-Kitaev liquid state with two localized Majorana fermions, one frozen by gauge fluctuations and the other localized by disordered mass terms. The quantization of the thermal Hall conductivity $κ/T$ disappears by a quantum Hall transition induced by a small disorder, and $κ/T$ shows a rapid crossover into the Anderson-Kitaev liquid with a negligible Hall current. Especially, the critical disorder strength $δJ_{c1} \sim 0.05$ in the unit of the Kitaev interaction would have many implications for the stability of Kitaev spin liquids.
While phase transitions between magnetic analogs of three states of matter --- a long-range ordered state, paramagnet, and spin liquid --- have been extensively studied, the possibility of "liquid-liquid" transitions, namely, between different spin liquids, remains elusive. By introducing the additional Ising coupling into the honeycomb Kitaev model with bond asymmetry, we discover that the Kitaev spin liquid turns into a spin-nematic quantum paramagnet before a magnetic order is established by the Ising coupling. The quantum phase transition between the two liquid states accompanies a topolog…
The periodic Anderson model is a classic theoretical model for understanding novel physics in heavy fermion systems. Here, we modify it with the Sachdev-Ye-Kitaev interaction, (random all-to-all interaction) thus the resultant model admits an exact solution at large-$N$ (e.g. spin flavor) limit. By analytical field theory arguments and numerical calculations, we establish that the system supports a low-temperature (heavy) Fermi liquid and more interesting a non-Fermi liquid solution at elevated temperature/energy. For physical observable, the latter one contributes a sharp peak at Fermi energy…
We point out that the Kitaev materials may not necessarily support Kitaev spin liquid. It is well-known that having a Kitaev term in the spin interaction is not the sufficient condition for the Kitaev spin liquid ground state. Many other spin liquids may be stabilized by the competing spin interactions of the systems. We thus explore the possibilities of non-Kitaev spin liquids in the honeycomb Kitaev materials. We carry out a systematic classification of gapped $\mathbb{Z}_2$ spin liquids using the Schwinger boson representation for the spin variables. The presence of strong spin-orbit coupli…
We investigate a modified Anderson model at the large-$N$ limit, where Coulomb interaction is replaced by Sachdev-Ye-Kitaev random interaction. The resistivity of conduction electron $ρ_{c}$ has a minimum value around temperature $\widetilde{T}_{K}$, which is similar to the Kondo system, but the impurity electron's density of state $A_{d}(ω)$ elucidates no sharp-peak like Kondo resonance around the Fermi surface. The impurity electron's entropy $S_{d}$ and specific heat capacity $C_{\textrm{v}}$ illustrate a crossover from Fermi liquid to the non-Fermi liquid. The system is a non-Fermi liquid …
Motivated by the recent surge of field-driven phenomena discussed for Kitaev materials, in particular the experimental observation of a finite thermal Hall effect and theoretical proposals for the emergence of additional spin liquid phases beyond the conventional Kitaev spin liquid, we develop a theoretical understanding of the thermal Hall effect in honeycomb Kitaev materials in magnetic fields. Our focus is on gapless U(1) spin liquids with a spinon Fermi surface, which have been shown to arise as field-induced phases. We demonstrate that in the presence of symmetry-allowed, second-neighbor …
Kitaev's honeycomb lattice spin model is a remarkable exactly solvable model, which has a particular type of spin liquid (Kitaev spin liquid) as the ground state. Although its possible realization in iridates and $α$-RuCl$_3$ has been vigorously discussed recently, these materials have substantial non-Kitaev direct exchange interactions and do not have a spin liquid ground state. We propose metal-organic frameworks (MOFs) with Ru$^{3+}$ (or Os$^{3+}$) forming the honeycomb lattice as promising candidates for a more ideal realization of Kitaev-type spin models where the direct exchange interact…
Higher-order topological insulators are distinguished by the existence of topologically protected modes with codimension two or higher. Here, we report the manifestation of a second-order topological insulator in a two dimensional frustrated quantum magnet, which exhibits topological corner modes. Our exactly-solvable model is a generalization of the Kitaev honeycomb model to the Shastry-Sutherland lattice that, besides a chiral spin liquid phase, exhibits a gapped spin liquid with Majorana corner modes, which are protected by two mirror symmetries. This second-order Kitaev spin liquid remains…
Magnetoelastic interaction couples spin and lattice degrees of freedom and plays a key role in thermal transport properties of magnetic insulators. In the Kitaev quantum spin liquid, the low energy excitations are charge neutral Majorana fermions, which transform the magnetoelasctic interaction into Majorana-phonon scattering. Motivated by anomalous thermal properties of the Kitaev quantum spin liquid candidate RuCl$_3$, in this letter, we combine meV resolution inelastic x-ray scattering and theoretical calculation to examine the Majorana-phonon scattering. We analytically derive the velocity…
A projective symmetry group (PSG) has been regarded as a classification theory of spin liquids. However, it does not include a symmetry-protected topological order of fermionic spinon excitations, and thus the classification of gapped spin liquids is incomplete. We demonstrate the classification beyond PSG by utilizing the Kitaev model on the squareoctagon lattice, where two gapped spin liquids are distinguished by a topological $Z_2$ invariant. This $Z_2$ invariant can be defined solely by the time-reversal and translation symmetries on condition that the time-reversal symmetry is implemented…
The Kitaev model is a fascinating example of an exactly solvable model displaying a spin-liquid ground state in two dimensions. However, deviations from the original Kitaev model are expected to appear in real materials. In this Letter, we investigate the fate of Kitaev's spin liquid in the presence of disorder -- bond defects or vacancies -- for an extended version of the model. Considering static flux backgrounds, we observe a power-law divergence in the low-energy limit of the density of states with a nonuniversal exponent. We link this power-law distribution of energy scales to weakly coup…
In this paper, we study the lightly doped Kitaev spin liquid (DKSL) and find it to be a Fermi liquid state. The DKSL has a closed Fermi surface around the center of the Brillouin zone with the quantized volume determined by the Luttinger's theorem. It has well-defined quasiparticles near the Fermi surface and can be detected in the angle-resolved photoemission spectroscopy. The DKSL has the topological Kitaev spin liquid (KSL) as its neutral background. It violates the Wiedemann-Franz law and has a large Wilson ration. These results has the potential experimental test in the iridates upon dopi…
In the Kitaev honeycomb model, the quantum spin fractionalizes into itinerant Majorana and gauge flux spontaneously upon cooling, leading to rich experimental ramifications at finite temperature and an upsurge of research interest. In this work, we employ the exponential tensor renormalization group approach to explore the Kitaev model under various perturbations, including the external fields, Heisenberg, and the off-diagonal couplings that are common in the Kitaev materials. Through large-scale manybody calculations, we find a Kitaev fractional liquid at intermediate temperature that is robu…
Elementary excitations in highly entangled states such as quantum spin liquids may exhibit exotic statistics, different from those obeyed by fundamental bosons and fermions. Excitations called non-Abelian anyons are predicted to exist in a Kitaev spin liquid - the ground state of an exactly solvable model proposed by Kitaev almost a decade ago. A smoking-gun signature of such non-Abelian anyons, namely a half-integer quantized thermal Hall conductivity, was recently reported in $α$-RuCl$_3$. While fascinating, a microscopic theory for this phenomenon in $α$-RuCl$_3$ remains elusive because the…
$α$-RuCl$_3$ is a promising candidate material for the Kitaev spin liquid state where the half quantization of the thermal Hall effect, suggesting a topological character, has been observed. However, its relation to the existence of chiral Majorana fermions, which is predicted from the theory of the Kitaev model, is still under debate. Here we propose a more direct signature of a chiral Majorana edge mode which emerges in a universal scaling of the Drude weight of the edge spin Seebeck effect in the Kitaev model. Moreover, the absence of backscatterings in the chiral edge mode results in the g…
The ruthenium halide $α$-RuCl$_{3}$ is a promising candidate for a Kitaev spin liquid. However, the microscopic model describing $α$-RuCl$_{3}$ is still debated partly because of a lack of analogue materials for $α$-RuCl$_{3}$, which prevents tracking of electronic properties as functions of controlled interaction parameters. Here, we report a successful synthesis of RuBr$_{3}$. The material RuBr$_{3}$~possesses BiI$_3$-type structure (space group: $R\overline{3}$) where Ru$^{3+}$ form an ideal honeycomb lattice. Although RuBr$_{3}$ has a negative Weiss temperature, it undergoes a zigzag antif…
The Raman scattering with local optical excitation from the Majorana edge modes of Kitaev spin liquids and topological superconductors is studied theoretically. Although the effective one-dimensional model is common between these two cases, the coupling to the electromagnetic field is different. It is found that the Raman spectrum at low energy scales with $ω^3$ in Kitaev spin liquids while it shows the gap in topological superconductors. This is in sharp contrast to the infrared absorption, where the spectrum shows the gap in Kitaev spin liquids, while it behaves as $\sim ω^2$ in topological …
Recent proposals for spin-1 Kitaev materials, such as honeycomb Ni oxides with heavy elements of Bi and Sb, have shown that these compounds naturally give rise to antiferromagnetic (AFM) Kitaev couplings. Conceptual interest in such AFM Kitaev systems has been sparked by the observation of a transition to a gapless $U(1)$ spin liquid at intermediate field strengths in the AFM spin-1/2 Kitaev model. However, all hitherto known spin-1/2 Kitaev materials exhibit ferromagnetic bond-directional exchanges. Here we discuss the physics of the spin-1 Kitaev model in a magnetic field and show, by extens…
Frustrated magnetic systems exhibit many fascinating phases. Prime among them are quantum spin liquids, where the magnetic moments do not order even at zero temperature. A subclass of quantum spin liquids called Kitaev spin liquids are particularly interesting, because they are exactly solvable, can be realized in certain materials, and show a large variety of gapless and gapped phases. Here, we show that non-symmorphic symmetries can enrich spin liquid phases, such that the low-energy spinon degrees of freedom form three-dimensional Dirac cones or nodal chains. In addition, we suggest how suc…
We investigate the ground state properties of the spin S=1 Kitaev honeycomb model under a magnetic field based on the density matrix renormalization group (DMRG) calculation. With the time reversal symmetry breaking due to the magnetic field, a gapped Kitaev spin liquid is identified for both ferromagnetic (FM) and antiferromagnetic (AFM) Kitaev couplings. The topological nature of such Kitaev spin liquid is manifested by the nearly quantized Wilson loop, degeneracy in the entanglement spectra and existence of edge modes. While the FM Kitaev spin liquid is destroyed by a weaker magnetic field …
Quantum spin liquids (QSLs) form an extremely unusual magnetic state in which the spins are highly correlated and fluctuate coherently down to the lowest temperatures, but without symmetry breaking and without the formation of any static long-range-ordered magnetism. Such intriguing phenomena are not only of great fundamental relevance in themselves, but also hold the promise for quantum computing and quantum information. Among different types of QSLs, the exactly solvable Kitaev model is attracting much attention, with most proposed candidate materials, e.g., RuCl$_3$ and Na$_2$IrO$_3$, havin…
Ultracold atoms and molecules trapped in optical lattices are expected to serve as simulators of strongly correlated systems and topological states of matter. A fascinating example is to realize the Kitaev quantum spin liquid by using ultracold polar molecules. However, although experimental implementation of the Kitaev-type interaction was proposed, the stability of the Kitaev quantum spin liquid has not been fully investigated thus far. Here we study a quantum spin model with long-range angle-dependent Kitaev-type interactions proposed for the polar molecules, by the pseudofermion functional…
We study the stability of Kitaev quasiparticles in the presence of a perturbing Heisenberg interaction as a Fock space localization phenomenon. We identify parameter regimes where Kitaev states are localized, fractal or delocalized in the Fock space of exact eigenstates, with the first two implying quasiparticle stability. Finite temperature calculations show that a vison gap, and a nonzero plaquette Wilson loop at low temperatures, both characteristic of the deconfined Kitaev spin liquid phase, persist far into the neighboring phase that has a concomitant stripy spin-density wave (SDW) order.…
Recently there has been a great interest in understanding quantum spin liquid phases with varying spin magnitude, partly due to possible material realizations. A number of recent numerical computations suggest that the ground state of the S=1 Kitaev model may be a quantum spin liquid in analogy to the renowned $S$=$1/2$ model. On the other hand, the nature of the ground state remains elusive since the $S$=$1$ model is not exactly solvable in contrast to the $S$=$1/2$ model. In this work, we construct a tensor network ground state wavefunction for the S=1 Kitaev model, which is explicitly writt…
Kitaev's honeycomb-lattice compass model describes a spin liquid with emergent fractionalized excitations. Here we study the physics of isolated magnetic impurities coupled to the Kitaev spin-liquid host. We reformulate this Kondo-type problem in terms of a many-state quantum impurity coupled to a multichannel bath of Majorana fermions and present the numerically exact solution using Wilson's numerical renormalization group technique. Quantum phase transitions occur as a function of Kondo coupling and locally applied field. At zero field, the impurity moment is partially screened only when it …
We explore with exact diagonalization the propagation of a single hole in four magnetic phases of the t-J-like Kitaev-Heisenberg model on a honeycomb lattice: the Neel antiferromagnetic, stripe, zigzag and Kitaev spin-liquid phase. We find coherent propagation of spin-polaron quasiparticles in the antiferromagnetic phase by a similar mechanism as in the $t$-$J$ model for high-$T_c$ cuprates. In the stripe and zigzag phases clear quasiparticles features appear in spectral functions of those propagators where holes are created and annihilated on one sublattice, while they remain largely {\it hid…
This paper reviews the current progress on searching the Kitaev spin liquid state in 3d electron systems. Honeycomb cobaltates were recently proposed as promising candidates to realize the Kitaev spin liquid state, due to the more localized wave functions of 3d ions compared with that of 4d and 5d ions, and also the easy tunability of the exchange Hamiltonian in favor of Kitaev interaction. Several key parameters that have large impacts on the exchange constants, such as the charge-transfer gap and the trigonal crystal field, are identified and discussed. Specifically, tuning crystal field eff…
Due to the combination of a substantial spin-orbit coupling and correlation effects, iridium oxides hold a prominent place in the search for novel quantum states of matter, including, e.g., Kitaev spin liquids and topological Weyl states. We establish the promise of the very recently synthesized hyper-honeycomb iridate $β$-Li2IrO3 in this regard. A detailed theoretical analysis reveals the presence of large ferromagnetic first-neighbor Kitaev interactions, while a second-neighbor antiferromagnetic Heisenberg exchange drives the ground state from ferro to zigzag order via a three-dimensional Ki…
Emergence of quantum spin liquid and spin-flop phase in Kitaev antiferromagnets in a [111] magnetic field
College of Physics, Nanjing University of Aeronautics and Astronautics(南京航空航天大学物理学院);Key Laboratory of Aerospace Information Materials and Physics (NUAA), MIIT(工业和信息化部航空航天信息材料与物理重点实验室(南航));School of Physics and Institute for Advanced Study in Physics, Zhejiang University(浙江大学物理学院与高等研究院)
Quantum spin liquids are highly fascinating quantum liquids in which the spin degrees of freedom fractionalize. An interesting class of spin liquids are the exactly solvable, three-dimensional Kitaev spin liquids. Their fractionalized excitations are Majonara fermions, which may exhibit a variety of topological band structures --- ranging from topologically protected Weyl semi-metals over nodal semi-metals to systems with Majorana Fermi surfaces. We study the entanglement spectrum of such Kitaev spin liquids and verify that it is closely related to the topologically protected edge spectrum. Mo…
We study the exchange interactions and resulting magnetic phases in the honeycomb cobaltates. For a broad range of trigonal crystal fields acting on Co2+ ions, the low-energy pseudospin-1/2 Hamiltonian is dominated by bond-dependent Ising couplings that constitute the Kitaev model. The non-Kitaev terms nearly vanish at small values of trigonal field Δ, resulting in spin liquid ground state. Considering Na3Co2SbO6 as an example, we find that this compound is proximate to a Kitaev spin liquid phase, and can be driven into it by slightly reducing Δby \sim 20 meV, e.g., via strain or pressure cont…
Fractionalization is a hallmark of spin-liquid behavior; it typically leads to response functions consisting of continua instead of sharp modes. However, microscopic processes can enable the formation of short-distance bound states of fractionalized excitations, despite asymptotic deconfinement. Here we study such bound-state formation for the $Z_2$ spin liquid realized in Kitaev's honeycomb compass model, supplemented by a kekule distortion of the lattice. Bound states between flux pairs and Majorana fermions form in the Majorana band gaps. We calculate the dynamic spin susceptibility and sho…
We investigate how the Kitaev spin liquid state described by Majorana fermions coupled with $Z_2$ gauge fields is affected by non-Kitaev interactions which exist in real candidate materials of the Kitaev magnet. It is found that the off-diagonal exchange interaction referred to as the $Γ'$ term dramatically changes the Majorana band structure in the case of the antiferromagnetic Kitaev interaction, and gives rise to a topological phase transition from a non-Abelian topological phase with the Chern number equal to $\pm 1$ to an Abelian phase with the Chern number equal to $\pm 2$, in which the …
Anyonic excitations emerging from a Kitaev spin liquid can form a basis for quantum computers. Searching for such excitations motivated intense research on the honeycomb iridate materials. However, access to a spin liquid ground state has been hindered by magnetic ordering. Cu2IrO3 is a new honeycomb iridate without thermodynamic signatures of a long-range order. Here, we use muon spin relaxation to uncover the magnetic ground state of Cu2IrO3. We find a two-component depolarization with slow and fast relaxation rates corresponding to distinct regions with dynamic and static magnetism, respect…
We study quantum disordered ground states of the two dimensional Heisenberg-Kitaev model on the triangular lattice using a Schwinger boson approach. Our aim is to identify and characterize potential gapped quantum spin liquid phases that are stabilized by anisotropic Kitaev interactions. For antiferromagnetic Heisenberg- and Kitaev couplings and sufficiently small spin $S$ we find three different symmetric $Z_2$ spin liquid phases, separated by two continuous quantum phase transitions. Interestingly, the gap of elementary excitations remains finite throughout the transitions. The first spin li…
Mott insulators under sufficiently strong spin-orbit coupling can display quantum spin liquid phases with topological order and fractional excitations. Quantum magnets with pure Kitaev spin exchange interactions can host a gapped quantum spin liquid with a single Majorana edge mode propagating in the counter-clockwise direction when a small positive magnetic field is applied. Here, we show how under a sufficiently strong positive magnetic field a topological transition into a gapped quantum spin liquid with two Majorana edge modes propagating in the clockwise direction occurs. The Dzyaloshinsk…
University of Munich(慕尼黑大学);Munich Center for Quantum Science and Technology(慕尼黑量子科学与技术中心);Shanghai Jiao Tong University(上海交通大学)
Kitaev materials are promising materials for hosting quantum spin liquids and investigating the interplay of topological and symmetry-breaking phases. We use an unsupervised and interpretable machine-learning method, the tensorial-kernel support vector machine, to study the honeycomb Kitaev-$Γ$ model in a magnetic field. Our machine learns the global classical phase diagram and the associated analytical order parameters, including several distinct spin liquids, two exotic $S_3$ magnets, and two modulated $S_3 \times Z_3$ magnets. We find that the extension of Kitaev spin liquids and a field-in…
Material realizations of the bond-dependent Kitaev interactions with $S$=1/2 local moments have vitalized the research in quantum spin liquids. Recently, it has been proposed that higher-spin analogues of the Kitaev interactions may also occur in a number of materials with strong spin-orbit coupling. In contrast to the celebrated $S$=1/2 Kitaev model on the honeycomb lattice, the higher-spin Kitaev models are not exactly solvable. Hence, the existence of quantum spin liquids in these systems remains an outstanding question. In this work, we use the density matrix renormalization group (DMRG) m…
Tuning the Chern number of Kitaev quantum spin liquid
The University of Tokyo(东京大学);Department of Physics and Natural Science Research Institute, University of Seoul(首尔大学物理与自然科学研究所);Department of Applied Physics, Kyung Hee University(庆熙大学应用物理系);School of Physics, Korea Institute for Advanced Study(韩国高等科学研究院物理学院)
The quantum spin liquid (QSL) state has been searched intensively in Kitaev-like materials, such as the Iridium oxides $A_2$IrO$_3$ and $α$-RuCl$_3$. The half-filled Kitaev-Hubbard model with bond dependent hopping terms is used to describe the Kitaev-like materials, which is calculated using the state-of-the-art fermionic projected entangled pair states (fPEPS) method. We find a QSL phase near the Mott insulator transition, which has a strong first-order transition to the semi-metal phase with the decrease of Hubbard $U$. We suggest that a promising routine to find the QSL is to find the Irid…
We study the extent of the spin liquid phases in the Kitaev-Heisenberg model using infinite Projected Entangled-Pair States tensor network ansatz wave functions directly in the thermodynamic limit. To assess the accuracy of the ansatz wave functions we perform benchmarks against exact results for the Kitaev model and find very good agreement for various observables. In the case of the Kitaev-Heisenberg model we confirm the existence of 6 different phases: Néel, stripy, ferromagnetic, zigzag and two spin liquid phases. We find finite extents for both spin liquid phases and discontinuous phase t…
Motivated by the recent experimental observation of the half-quantized thermal Hall conductivity for the candidate material of the Kitaev spin liquid, $α$-RuCl$_3$[ Y. Kasahara et al., Nature 559, 227 (2018)], we investigate effects of non-Kitaev exchange interactions, which exist in the real material, on the gapped chiral spin liquid state realized in the case with an applied magnetic field. It is found that off-diagonal exchange interactions enhance significantly the mass gap of Majorana fermions. This result provides a possible explanation for robust quantization of the thermal Hall conduct…
Relativistic Mott insulators known as 'Kitaev materials' potentially realize spin liquids hosting non-Abelian anyons. Motivated by fault-tolerant quantum-computing applications in this setting, we introduce a dynamical anyon-generation protocol that exploits universal edge physics. The setup features holes in the spin liquid, which define energetically cheap locations for non-Abelian anyons, connected by a narrow bridge that can be tuned between spin liquid and topologically trivial phases. We show that modulating the bridge from trivial to spin liquid over intermediate time scales -- quantifi…
Fractionalized Fermi liquids (FL$^\ast$) have been introduced as non-Fermi-liquid metallic phases, characterized by coexisting electron-like charge carriers and local moments which itself form a fractionalized spin liquid. Here we investigate a Kondo lattice model on the honeycomb lattice with compass interactions among the local moments, a concrete model hosting FL$^\ast$ phases based on Kitaev's $\mathbb{Z}_2$ spin liquid. We characterize the FL$^\ast$ phases via perturbation theory, and we employ a Majorana-fermion mean-field theory to map out the full phase diagram. Most remarkably we find…
Quantum spin liquids realize massive entanglement and fractional quasiparticles from localized spins, proposed as an avenue for quantum science and technology. In particular, topological quantum computations are suggested in the non-abelian phase of Kitaev quantum spin liquid with Majorana fermions, and detection of Majorana fermions is one of the most outstanding problems in modern condensed matter physics. Here, we propose a concrete way to identify the non-abelian Kitaev quantum spin liquid by magnetic field angle dependence. Topologically protected critical lines exist on a plane of magnet…
We propose that resonant inelastic X-ray scattering (RIXS) is an effective probe of the fractionalized excitations in three-dimensional (3D) Kitaev spin liquids. While the non-spin-conserving RIXS responses are dominated by the gauge-flux excitations and reproduce the inelastic-neutron-scattering response, the spin-conserving (SC) RIXS response picks up the Majorana-fermion excitations and detects whether they are gapless at Weyl points, nodal lines, or Fermi surfaces. As a signature of symmetry fractionalization, the SC RIXS response is suppressed around the $Γ$ point. On a technical level, w…
We investigate the generic features of the low energy dynamical spin structure factor of the Kitaev honeycomb quantum spin liquid perturbed away from its exact soluble limit by generic symmetry-allowed exchange couplings. We find that the spin gap persists in the Kitaev-Heisenberg model, but generally vanishes provided more generic symmetry-allowed interactions exist. We formulate the generic expansion of the spin operator in terms of fractionalized Majorana fermion operators according to the symmetry enriched topological order of the Kitaev spin liquid, described by its projective symmetry gr…
Quantum spin liquid is an exotic quantum state of matter in magnets. This state is a spin analogue of the liquid helium which does not solidify down to the lowest temperature due to strong quantum fluctuations. In conventional fluids, liquid and gas possess the same symmetry and adiabatically connect to each other by bypassing the critical end point. We find that the situation is qualitatively different in quantum spin liquids realizing in a three-dimensional Kitaev model; both gapless and gapped quantum spin liquid phases at low temperatures are always distinguished from the high-temperature …
We present the electron tunneling transport and spectroscopic characters of a superconducting {\it Josephson} junction with a barrier of single anisotropic Kitaev quantum spin liquid (QSL) layer. We find that the dynamical spin correlation features are well reflected in the direct-current differential conductance $dI^{c}/dV$ of the single-particle tunneling, including the unique spin gap and dressed itinerant Majorana dispersive band, in addition to an energy shift $2Δ$ of two-lead superconducting gaps. From the spectral characters, we identify different topological quantum phases of the aniso…