We investigate theoretically the noise and the full counting statistics of electrons that are emitted from a superconductor into two spatially separated quantum dots by the splitting of Cooper pairs and further on collected in two normal-state electrodes. With negatively-biased drain electrodes and a large superconducting gap, the dynamics of the Cooper pair splitter can be described by a Markovian quantum master equation. Using techniques from full counting statistics, we evaluate the electrical currents, their noise power spectra, and the power-power correlations in the output leads. The current fluctuations can be attributed to the competition between Cooper pair splitting and elastic cotunneling between the quantum dots via the superconductor. In one regime, these processes can be clearly distinguished in the cross-correlation spectrum with peaks and dips appearing at characteristic frequencies associated with elastic cotunneling and Cooper pair splitting, respectively. We corroborate this interpretation by analyzing the charge transport fluctuations in the time domain, specifically by investigating the $g^{(2)}$-function of the output currents. Our work identifies several experimental signatures of the fundamental transport processes involved in Cooper pair splitting and provides specific means to quantify their relative strengths. As such, our results may help guide and interpret future experiments on current fluctuations in Cooper pair splitters.
Cooper pair splitters are promising candidates for generating spin-entangled electrons. However, the splitting of Cooper pairs is a random and noisy process, which hinders further synchronized operations on the entangled electrons. To circumvent this problem, we here propose and analyze a dynamic Cooper pair splitter that produces a noiseless and regular flow of spin-entangled electrons. The Cooper pair splitter is based on a superconductor coupled to quantum dots, whose energy levels are tuned in and out of resonance to control the splitting process. We identify the optimal operating conditio…
Spin-orbit interaction provides a spin filtering effect in carbon nanotube based Cooper pair splitters that allows us to determine spin correlators directly from current measurements. The spin filtering axes are tunable by a global external magnetic field. By a bending of the nanotube the filtering axes on both sides of the Cooper pair splitter become sufficiently different that a test of entanglement of the injected Cooper pairs through the Bell inequality can be implemented. This implementation does not require noise measurements, supports imperfect splitting efficiency and disorder, and doe…
We report an experimental study of Cooper pair splitting in an encapsulated graphene based multiterminal junction in the ballistic transport regime. Our device consists of two transverse junctions, namely the superconductor/graphene/superconductor and the normal metal/graphene/normal metal junctions. In this case, the electronic transport through one junction can be tuned by an applied bias along the other. We observe clear signatures of Cooper pair splitting in the local as well as nonlocal electronic transport measurements. Our experimental data can be very well described by using a modified…
We study the statistics of charge transport in a mesoscopic three-terminal device with one superconducting terminal and two normal-metal terminals. We calculate the full distribution of transmitted charges into the two symmetrically biased normal terminals. In a wide parameter range, we find large positive crosscorrelations between the currents in the two normal arms. We also determine the third cumulant that provides additional information on the statistics not contained in the current noise.
The quantum entanglement between two qubits is crucial for applications in the quantum communication. After the entanglement of photons was experimentally realized, much effort has been taken to exploit the entangled electrons in solid-state systems. Here, we propose a Cooper-pair splitter, which can generate spatially-separated but entangled electrons, in a quantum anomalous Hall insulator proximity-coupled with a superconductor. After coupling with a superconductor, the chiral edge states of the quantum anomalous Hall insulator can still survive, making the backscattering impossible. Thus, t…
We measure the tunneling rates and coupling coefficients for local Andreev, non-local Andreev and elastic cotunneling processes. The non-local Andreev process, giving rise to Cooper pair splitting, exhibits the same coupling coefficient as the elastic co-tunneling whereas the local Andreev process is more than two orders of magnitude stronger than the corresponding non-local one. Theory estimates describe the findings and explain the large difference in the non-local and local coupling arising from competition between electron diffusion in the superconductor and tunnel junction transparency.
We analyze microscopically a Cooper pair splitting device in which a central superconducting lead is connected to two weakly coupled normal leads through a carbon nanotube. We determine the splitting efficiency at resonance in terms of geometrical and material parameters, including the effect of spin-orbit scattering. While the efficiency in the linear regime is limited to 50% and decay exponentially as a function of the width of the superconducting region we show that it can rise up to $\sim 100%$ in the non-linear regime for certain regions of the stability diagram.
A Cooper pair splitter consists of a central superconducting contact, S, from which electrons are injected into two parallel, spatially separated quantum dots (QDs). This geometry and electron interactions can lead to correlated electrical currents due to the spatial separation of spin-singlet Cooper pairs from S. We present experiments on such a device with a series of bottom gates, which allows for spatially resolved tuning of the tunnel couplings between the QDs and the electrical contacts and between the QDs. Our main findings are gate-induced transitions between positive conductance corre…
We investigate the nonlocal thermoelectric transport in a Cooper-pair splitter based on a double-quantum-dot-superconductor three-terminal hybrid structure. We find that the nonlocal coupling between the superconductor and the quantum dots gives rise to nonlocal thermoelectric effects which originate from the nonlocal particle-hole breaking of the system. We show that Cooper-pair splitting induces the generation of a thermo-current in the superconducting lead without any transfer of charge between the two normal metal leads. Conversely, we show that a nonlocal heat exchange between the normal …
Cooper pairs in the superconductor are a natural source of spin entanglement. The existing proposals of the Cooper pair splitter can only realize a low efficiency of entanglement production, and its size is constrained by the superconducting coherence length. Here we show that a long-range Cooper pair splitter can be implemented in a normal metal-superconductor-normal metal (NSN) junction by driving a supercurrent in the S. The supercurrent results in a band gap modification of the S, which significantly enhances the crossed Andreev reflection (CAR) of the NSN junction and simultaneously quenc…
This article discusses how to demonstrate the entanglement of the split Cooper pairs produced in a double-quantum-dot based Cooper pair beam splitter (CPS), by performing the microwave spectroscopy of the CPS. More precisely, one can study the DC current response of such a CPS to two on-phase microwave gate irradiations applied to the two CPS dots. Some of the current peaks caused by the microwaves show a strongly nonmonotonic variation with the amplitude of the irradiation applied individually to one dot. This effect is directly due to a subradiance property caused by the coherence of the spl…
We report on conductance measurements in carbon nanotube based double quantum dots connected to two normal electrodes and a central superconducting finger. By operating our devices as beam splitters, we provide evidence for Crossed Andreev Reflections \textit{tunable in situ}. This opens an avenue to more sophisticated quantum optics-like experiments with spin entangled electrons.
Electron waiting times are an important concept in the analysis of quantum transport in nano-scale conductors. Here we show that the statistics of electron waiting times can be used to characterize Cooper pair splitters that create spatially separated spin-entangled electrons. A short waiting time between electrons tunneling into different leads is associated with the fast emission of a split Cooper pair, while long waiting times are governed by the slow injection of Cooper pairs from a superconductor. Experimentally, the waiting time distributions can be measured using real-time single-electr…
The control of nonlocal entanglement in solid state systems is a crucial ingredient of quantum technologies. We investigate a Cooper-pair splitter based on a double quantum dot realised in a semiconducting nanowire. In the presence of interdot tunnelling the system provides a simple mechanism to develop spatial entanglement even in absence of nonlocal coupling with the superconducting lead. We discuss the possibility to control the symmetry (singlet or triplet) of spatially separated, entangled electron pairs taking advantage of the spin-orbit coupling of the nanowire. We also demonstrate that…
We investigate the Andreev transport through double-quantum-dot Cooper pair splitters with ferromagnetic leads. The analysis is performed with the aid of the real-time diagrammatic technique in the sequential tunneling regime. We study the dependence of the Andreev current, the differential conductance, and the tunnel magnetoresistance on various parameters of the model in both the linear and nonlinear response regimes. In particular, we analyze the spin-resolved transport in the crossed Andreev reflection regime, where a blockade of the current occurs due to enhanced occupation of the triplet…
A Cooper pair splitter consists of two quantum dots side-coupled to a conventional superconductor. Usually, the quantum dots are assumed to have a large charging energy compared to the superconducting gap, in order to suppress processes other than the coherent splitting of Cooper pairs. In this work, in contrast, we investigate the limit in which the charging energy is smaller than the superconducting gap. This allows us, in particular, to study the effect of a Zeeman field comparable to the charging energy. We find analytically that in this parameter regime the superconductor mediates an inte…
The generation of spin-entangled electrons is an important prerequisite for future solid-state quantum technologies. Cooper pairs in a superconductor can be split into separate electrons in a spin-singlet state, however, detecting their entanglement remains an open experimental challenge. Proposals to detect the entanglement by violating a Bell inequality typically require a large number of current cross-correlation measurements, and not all entangled states can be detected in this way. Here, we instead formulate an entanglement witness that can detect the spin-entanglement using only three cr…
Motivated by the recent experiments [Scientific reports 6, 23051 (2016), Phys. Rev. Lett. 114, 096602 (2015)], we theoretically investigate Cooper pair splitting current in a graphene based Cooper pair beam splitter geometry. By considering the graphene based superconductor as an entangler device, instead of normal (2D) BCS superconductor, we show that the Cooper pair splitting current mediated by Crossed Andreev process is amplified compared to its normal superconductor counterpart. This amplification is attributed to the strong suppression of local normal Andreev reflection process (arising …
We analyze a model of double quantum dot Cooper pair splitter coupled to two ferromagnetic detectors, and demonstrate the possibility of determination of spin correlation by current measurements. We use perturbation theory taking account of the exchange interaction with the detectors, which leads to complex spin dynamics in the dots. This affects the measured spin and restricts the use of ferromagnetic detectors to the nonlinear current-voltage characteristic regime at current plateau, where the relevant spin projection is conserved, in contrast to the linear current-voltage characteristic reg…
The Andreev transport properties of double quantum dot based Cooper pair splitters with one superconducting and two normal leads are studied theoretically in the Kondo regime. The influence of the superconducting pairing correlations on the local density of states, Andreev transmission coefficient and Cooper pair splitting efficiency is thoroughly analyzed. It is shown that finite superconducting pairing potential quickly suppresses the SU(2) Kondo effect, which can however reemerge for relatively large values of coupling to superconductor. In the SU(4) Kondo regime, a crossover from the SU(4)…
We consider the sub-gap physics of a hybrid double-quantum dot Cooper-pair splitter with large single-level spacings, in the presence of tunnelling between the dots and finite Coulomb intra- and inter-dot Coulomb repulsion. In the limit of a large superconducting gap, we treat the coupling of the dots to the superconductor exactly. We employ a generalized master-equation method which easily yields currents, noise and cross-correlators. In particular, for finite inter- and intra-dot Coulomb interaction, we investigate how the transport properties are determined by the interplay between local an…
We study adiabatic pumping through a double quantum dot coupled to normal and superconducting leads. For this purpose a perturbation expansion in the tunnel coupling between the dots and the normal leads is performed and processes underlying the pumping current are discussed. Features of crossed Andreev reflection are investigated in the average pumped charge and related to local Andreev reflection in a single quantum dot. In order to distinguish Cooper pair splitting from quasi-particle pumping, we compare the properties of Cooper pair pumping with single-electron pumping in a system with onl…
We investigate the current cross-correlations in a double quantum dot based Cooper pair splitter coupled to one superconducting and two ferromagnetic electrodes. The analysis is performed by assuming a weak coupling between the double dot and ferromagnetic leads, while the coupling to the superconductor is arbitrary. Employing the perturbative real-time diagrammatic technique, we study the Andreev transport properties of the device, focusing on the Andreev current cross-correlations, for various parameters of the model, both in the linear and nonlinear response regimes. Depending on parameters…
We simulated the radiative response of the cavity quantum electrodynamics (QED) coupled to the double quantum dot Cooper pair splitter and analyzed its spectral dependence to get insight into dynamics of the Cooper pair transfers. The model is confined to the energy subspace where two entangled electrons are transferred to two normal electrodes through the inter-dot singlet state on two proximitized quantum dots. Our research is focused on the Andreev scatterings in the subgap regime, for which the local charge susceptibility $Π(ω_p)$ is derived, by means of Keldysh Green functions, in a whole…
New generation of Cooper pair splitters defined on hybrid nanostructures are devices with high tunable coupling parameters. Transport measurements through these devices revealed clear signatures of interference effects and motivated us to introduce a new model, called the 3-sites model. These devices provide an ideal playground to tune the Cooper pair splitting (CPS) efficency on demand, and displays a rich variety of physical phenomena. In the present work we analyze theoretically the conductance of the 3-sites model in the linear and non-linear regimes and characterize the most representativ…
We consider a double quantum dot coupled to two normal leads and one superconducting lead, modeling the Cooper pair beam splitter studied in two recent experiments. Starting from a microscopic Hamiltonian we derive a general expression for the branching current and the noise crossed correlations in terms of single and two-particle Green's function of the dot electrons. We then study numerically how these quantities depend on the energy configuration of the dots and the presence of direct tunneling between them, isolating the various processes which come into play. In absence of direct tunnelin…
We investigate Andreev transport through a quantum dot attached to two external ferromagnetic leads and one superconducting electrode. The transport properties of the system are studied by means of the real-time diagrammatic technique in the sequential tunneling regime. To distinguish various contributions to Andreev current we calculate the current cross-correlations, i.e. correlations between currents flowing through two junctions with normal leads. We analyze dependence of current cross-correlations on various parameters of the considered model, both in linear and nonlinear transport regime…
Cooper pair splitting (CPS) is a process in which the electrons of naturally occurring spin-singlet pairs in a superconductor are spatially separated using two quantum dots. Here we investigate the evolution of the conductance correlations in an InAs CPS device in the presence of an external magnetic field. In our experiments the gate dependence of the signal that depends on both quantum dots continuously evolves from a slightly asymmetric Lorentzian to a strongly asymmetric Fano-type resonance with increasing field. These experiments can be understood in a simple three - site model, which sho…
We propose an approach allowing the computation of currents and their correlations in interacting multiterminal mesoscopic systems involving quantum dots coupled to normal and/or superconducting leads. The formalism relies on the expression of branching currents and noise crossed correlations in terms of one- and two-particle Green's functions for the dots electrons, which are then evaluated self-consistently within a conserving approximation. We then apply this to the Cooper-pair beam-splitter setup recently proposed [L. Hofstetter et al. Nature (London) 461 960 (2009); Phys. Rev. Lett. 107 1…
Thermoelectric effect generating electricity from thermal gradient and vice versa appears in numerous generic applications. Recently, an original prospect of thermoelectricity arising from the nonlocal Cooper pair splitting (CPS) and the elastic co-tunneling (EC) in hybrid normal metal-superconductor-normal metal (NSN) structures was foreseen. Here we demonstrate experimentally the existence of non-local Seebeck effect in a graphene-based CPS device comprising two quantum dots connected to an aluminum superconductor and theoretically validate the observations. This non-local Seebeck effect off…
Exact analytical formulas are derived, by means of Keldysh Green functions, for currents and current correlation functions in a Cooper pair splitter modelled on a double quantum dot system coherently coupled to a superconductor and two normal metallic electrodes. Confining to the subspace with the inter-dot singlet we show perfect entanglement of split electrons in two separated crossed Andreev reflection processes. The studies are focused on the noise power spectrum in a whole bias voltage range. In particular, in the large voltage limit shot noise dominates and its spectrum exhibits two extr…
We theoretically study the spin-resolved subgap transport properties of a Cooper pair splitter based on a triple quantum dot attached to superconducting and ferromagnetic leads. Using the Keldysh Green's function formalism, we analyze the dependence of the Andreev conductance, Cooper pair splitting efficiency, and tunnel magnetoresistance on the gate and bias voltages applied to the system. We show that the system's transport properties are strongly affected by spin dependence of tunneling processes and quantum interference between different local and nonlocal Andreev reflections. We also stud…
We demonstrate high efficiency Cooper pair splitting in a graphene-based device. We utilize a true Y-shape design effectively placing the splitting channels closer together: graphene is used as the central superconducting electrode as well as QD output channels, unlike previous designs where a conventional superconductor was used with tunnel barriers to the quantum dots (QD) of a different material. Superconductivity in graphene is induced via the proximity effect, thus resulting in both a large measured superconducting gap $Δ=0.5$meV, and a long coherence length $ξ=200$nm. The graphene-graphe…
We study the full counting statistics of heterostructures consisting of normal metal parts connected to a superconducting terminal. Assuming that coherent superconducting correlations are suppressed in the normal metals we show, using Keldysh-Nambu Green's functions, that the system can be mapped onto a purely normal system with twice the number of elements. For a superconducting beam splitter with several normal terminals we obtain general results for the counting statistics.
We present a proof-of-principle of how electronic transport measurements permits the observation of the Autler-Townes doublet, an optical property of nanodevices. The quantum physical system consists of one optically pumped quantum dot, a second auxiliary quantum dot, and a superconductor lead which provides an effective coupling between the dots via crossed Andreev reflection. Electrodes, working as source and drain, acts as nonequilibrium electronic reservoirs. Our calculations of the photocurrent at both, transient and stationary regimes, obtained using a density matrix formalism for open q…
We calculate the charge transport in a flux biased dissipative Cooper pair pump using the method of full counting statistics (FCS). This is instead of a more traditional technique of integrating a very small expectation value of the instantaneous current over the pumping period. We show that the rotating wave approximation (RWA), which fails in the traditional technique, produces accurate results within the FCS method.
We study the spin-resolved subgap transport in a triple quantum-dot system coupled to one superconducting and two ferromagnetic leads. We examine the Andreev processes in the parallel and antiparallel alignments of ferromagnets magnetic moments in both the linear and nonlinear response regimes. The emphasis is put on the analysis of the current cross-correlations between the currents flowing through the left and right arms of the device and relevant electron waiting time distributions. We show that both quantities can give an important insight into the subgap transport processes and their anal…
Hybrid nanostructures consisting of two parallel InAs nanowires connected by an epitaxially grown superconductor (SC) shell recently became available. Due to the defect-free SC-semiconductor interface and the two quasi-one-dimensional channels being close by, these novel platforms can be utilized to spatially separate entangled pairs of electrons by using quantum dots (QD) in the so-called Cooper pair splitting (CPS) process. The minimized distance between the QDs overcomes the limitations of single-wire-based geometries and can boost the splitting efficiency. Here we investigate CPS in such a…
The Cooper pair shuttle is a simple model system that combines features of coherent and incoherent transport. We evaluate the full counting statistics (FCS) of charge transfer via the shuttle in the incoherent regime. We describe two limiting cases when the FCS allows for classical interpretation. Generally, the classical interpretation fails yielding negative and imaginary "probabilities". This signals that superconducting coherence survives even in incoherent regime. We evaluate the current noise in some detail.
We investigate non-linear transport in a double quantum dot connected to two normal electrodes and a central superconducting finger. By this means, we perform a transport spectroscopy of such a system which implements a Cooper pair splitter. The non-linear conductance exhibits strong subgap features which can be associated with the coherence of the injected Cooper pairs. Our findings are well accounted for by the recently developed microscopic theory of Cooper pairs splitters made in SWNTs.
Splitting of Cooper pairs has recently been realized experimentally for s-wave Cooper pairs. A split Cooper pair represents an entangled two-electron pair state which has possible application in on-chip quantum computation. Likewise the spin-activity of interfaces in nanoscale tunnel junctions has been investigated theoretically and experimentally in recent years. However, the possible implications of spin-active interfaces in Cooper pair splitters so far have not been investigated. We analyse the current and the cross correlation of currents in a superconductor ferromagnet beamsplitter includ…
The nonlocal conductance and the current cross-correlations are investigated within scattering theory for three-terminal normal metal-superconductor-normal metal (NSN) hybrid structures. The positive cross-correlations at high transparency found by Mélin, Benjamin and Martin [Phys. Rev. B 77, 094512 (2008)] are not due to crossed Andreev reflection. On the other hand, local processes can be enhanced by reflectionless tunneling but this mechanism has little influence on nonlocal processes and on current cross-correlations. Therefore Cooper pair splitting cannot be enhanced by reflectionless tun…
The electrons forming a Cooper pair in a superconductor can be spatially separated preserving their spin entanglement by means of quantum dots coupled to both the superconductor and independent normal leads. We investigate the thermoelectric properties of such a Cooper pair splitter and demonstrate that cooling of a reservoir is an indication of non-local correlations induced by the entangled electron pairs. Moreover, we show that the device can be operated as a non-local thermoelectric heat engine. Both as a refrigerator and as a heat engine, the Cooper pair splitter reaches efficiencies clos…
We investigate transport properties of a double quantum dot based Cooper pair splitter, where the superconducting lead consists of Sr$_2$RuO$_4$. The proposed device can be used to explore the symmetry of the superconducting order parameter in Sr$_2$RuO$_4$ by testing the presence of gapless chiral edge states, which are predicted to exist if the bulk superconductor is described by a chiral $p$--wave state. The odd orbital symmetry of the bulk order parameter ensures that we can realize a regime where the electrons tunneling into the double dot system come from the chiral edge states and there…
This work discusses theoretically the behavior of a microwave cavity and a Cooper pair beam splitter (CPS) coupled non-resonantly. The cavity frequency pull is modified when the CPS is resonant with a microwave excitation. This provides a direct way to probe the coherence of the Cooper pair splitting process. More precisely, the cavity frequency pull displays an anticrossing whose specificities can be attributed unambiguously to coherent Cooper pair injection. This work illustrates that microwave cavities represent a powerful tool to investigate current transport in complex nanocircuits.
We discuss the counting statistics and current noise associated with the double Josephson quasiparticle resonance point in a superconducting single electron transistor. The counting statistics are in general phase-dependent, despite the fact that the average current has no dependence on phase. Focusing on parameter regimes where the counting statistics have no phase-dependence, we use a general relation first derived by MacDonald in 1948 to obtain the full frequency-dependent shot noise directly from the counting statistics, without any further approximations. We comment on problems posed by t…
A Cooper-pair or electron-hole splitter is a device capable of spatially separating entangled fermionic quasiparticles into mesoscopic solid-state systems such as quantum dots or quantum wires. We theoretically study such a splitter based on a pair of helical Luttinger liquids, which arise naturally at the edges of a quantum spin Hall insulator. Equipping each helical liquid with a beam splitter, current-current cross correlations can be used to construct a Bell inequality whose violation would indicate nonlocal orbital entanglement of the injected electrons and/or holes. Due to Luttinger-liqu…
In this paper we derive the Clauser-Horne (CH) inequality for the full electron counting statistics in a mesoscopic multiterminal conductor and we discuss its properties. We first consider the idealized situation in which a flux of entangled electrons is generated by an entangler. Given a certain average number of incoming entangled electrons, the CH inequality can be evaluated for different numbers of transmitted particles. Strong violations occur when the number of transmitted charges on the two terminals is the same ($Q_1=Q_2$), whereas no violation is found for $Q_1\ne Q_2$. We then consid…
We suggest a way to characterize the coherence of the split Cooper pairs emitted by a double-quantum-dot based Cooper pair splitter (CPS), by studying the radiative response of such a CPS inside a microwave cavity. The coherence of the split pairs manifests in a strongly nonmonotonic variation of the emitted radiation as a function of the parameters controlling the coupling of the CPS to the cavity. The idea to probe the coherence of the electronic states using the tools of Cavity Quantum Electrodynamics could be generalized to many other nanoscale circuits.
