We report the observation of a universal scaling of the Nernst coefficient over a wide intermediate temperature range in heavy fermion materials, including the superconductors CeCu$_2$Si$_2$, CeCoIn$_5$, and Ce$_2$PdIn$_8$, the ferromagnetic Kondo lattice Ce$_3$RhSi$_3$, the nonmagnetic CeRu$_2$Si$_2$, the intermediate valent YbAl$_3$, and the hidden order compound URu$_2$Si$_2$, that cover a broad spectrum of heavy fermion materials with different crystal, valence and ground state properties. The scaling formula follows exactly the magnetic susceptibility of emergent heavy quasiparticles as predicted in the two-fluid model. We give a tentative explanation of the scaling based on the skew scattering mechanism and the Boltzmann picture and argue that the Nernst effect is produced by the asymmetry of the quasiparticle density of states rather than that of the scattering rate. In URu$_2$Si$_2$, the giant Nernst signal in the hidden order phase is also found to follow the predicted scaling, indicating the potential involvement of hybridization physics. Our work suggests a candidate unified scenario for the Nernst effect in heavy fermion materials.
A large, strongly temperature-dependent Nernst coefficient, $ν$, is observed between $T$ = 2 K and 300 K for CeCu$_2$Si$_2$ and Ce$_{0.8}$La$_{0.2}$Cu$_2$Si$_2$. The enhanced $ν(T)$ is determined by the asymmetry of the on-site Kondo (conduction electron$-4f$ electron) scattering rate. Taking into account the measured Hall mobility, $μ_H$, the highly unusual thermopower, $S$, of these systems can be semiquantitatively described by $S(T)$ $=$ $-$$ν(T)/μ_H(T)$, which explicitly demonstrates that the thermopower originates from the local Kondo scattering process over a wide temperature range from…
The derivation for the transport coefficients of an electron system in the presence of temperature gradient and the electric and magnetic fields are presented. The Nernst conductivity and the transverse thermoelectric power of the Dirac fermions in graphene under charged impurity scatterings and weak magnetic field are calculated on basis of the self-consistent Born approximation. The result is compared with so far the available experimental data.
We report the study of Nernst effect in quasi-low dimensional tungsten bronze P4W12O44 showing a sequence of Peierls instabilities. We demonstrate that both condensation of the electronic carriers in the CDW state and the existence of high-mobility electrons and holes originating from the small pockets remaining in the incompletely nested Fermi surface give rise to a Nernst effect of a magnitude similar to that observed in heavy fermion compounds.
Giant anomalous Hall and Nernst effects in a heavy fermion ferromagnet
International Center for Quantum Materials, School of Physics, Peking University（北京大学量子材料科学中心物理学院）；Department of Physics, Southern University of Science and Technology（南方科技大学物理系）；Wuhan National High Magnetic Field Center and School of Physics, Huazhong University of Science and Technology（华中科技大学物理学院武汉国家高磁场实验室）；Department of Physics, School of Science, Tianjin University（天津大学理学院物理系）；Interdisciplinary Institute of Light-Element Quantum Materials and Research Center for Light-Element Advanced Materials, Peking University（北京大学轻元素量子材料交叉研究中心及轻元素先进材料研究中心）；Hefei National Laboratory（合肥国家实验室）
A liquid of superconducting vortices generates a transverse thermoelectric response. This Nernst signal has a tail deep in the normal state due to superconducting fluctuations. Here, we present a study of the Nernst effect in two-dimensional hetero-structures of Nb-doped strontium titanate (STO) and in amorphous MoGe. The Nernst signal generated by ephemeral Cooper pairs above the critical temperature has the magnitude expected by theory in STO. On the other hand, the peak amplitude of the vortex Nernst signal below $T_c$ is comparable in both and in numerous other superconductors despite the …
We report a systematic study of the transport properties in the series of Eu(Fe1-xCox)2As2 single crystals with x = 0, 0.15, 0.20 and 0.30. Spin-density-wave order is observed in the undoped and the least doped samples (x = 0, 0.15), while for x = 0.15 and 0.20 Eu(Fe1-xCox)2As2 becomes a superconductor. We found the properties of the parent EuFe2As2 compound well described by the Dirac fermions model, whereas cobalt doping caused an evolution of the system toward a regular metallic state. The antiferromagnetic ordering of the Eu2+ ions at T_N ~ 20 K has only minor influence on the measured qua…
The Nernst effect is known to be a sensitive probe of the scattering mechanisms. Large Nernst effects, a decade ago a topic mainly in vortex dynamics in superconductors, have recently attracted interest in correlated systems like cuprate metals and heavy fermion systems. However, it has been found that these ``giant" Nernst signals stay within one order of magnitude of the classical Sondheimer formula for a Fermi liquid. It therefore seems that a large Nernst effect neither relies on nor is sensitive to strong correlations. This might, however, be different in some recently studied supposedly …
The lead chalcogenides (Pb,Sn)Te and (Pb,Sn)Se are the first examples of topological crystalline insulators (TCI) predicted \cite{Fu,Hsieh} (and confirmed \cite{Hasan,Story,Takahashi}) to display topological surface Dirac states (SDS) that are protected by mirror symmetry. A starting premise \cite{Hsieh} is that the SDS arise from bulk states describable as massive Dirac states \cite{Wallis,Svane}, but this assumption is untested. Here we show that the thermoelectric response of the bulk states display features specific to the Dirac spectrum. We show that, in the quantum limit, the lowest Land…
We present a study of Nernst and Seebeck coefficients in the heavy-fermion compound URu$_{2}$Si$_{2}$, which hosts a phase transition of unsettled origin. A giant Nernst signal of unprecedented magnitude was found to emerge in the ordered state. Moreover, our analysis of the Seebeck and Hall data indicates that the ordering leads to a sudden increase in the entropy per itinerant electron and to a drastic decrease in the scattering rate.
The discovery of topological quantum materials represents a striking innovation in modern condensed matter physics with remarkable fundamental and technological implications. Their classification has been recently extended to topological Weyl semimetals, i.e., solid state systems which exhibit the elusive Weyl fermions as low-energy excitations. Here we show that the Nernst effect can be exploited as a sensitive probe for determining key parameters of the Weyl physics, applying it to the non-collinear antiferromagnet Mn$_3$Ge. This compound exhibits anomalous thermoelectric transport due to en…
We reveal a novel source of giant Nernst response exhibiting strong non-linear temperature and magnetic field dependence including the mysterious tilted-hill temperature profile observed in a pleiad of materials. The phenomenon results directly from the formation of a chiral ground state, e.g. a chiral d-density wave, which is compatible with the eventual observation of diamagnetism and is distinctly different from the usual quasiparticle and vortex Nernst mechanisms. Our picture provides a unified understanding of the anomalous thermoelectricity observed in materials as diverse as hole doped …
We present a study of Nernst and Seebeck coefficients of the heavy-fermion superconductor CeCoIn$_{5}$. Below 18 K, concomitant with a field-dependent Seebeck coefficient, a large sub-linear Nernst signal emerges with a magnitude drastically exceeding what is expected for a multi-band Fermi-liquid metal. In the mixed state, in contrast with all other superconductors studied before, this signal overwhelms the one associated with the motion of superconducting vortices. The results point to a hitherto unknown source of transverse thermoelectricity in strongly interacting electrons.
We report the Nernst effect (v) and thermoelectric power (S) data for the Ce2PdIn8 heavy-fermion compound. Both S and v behave anomalously at low temperatures: the thermopower shows a Kondo-like maximum at T = 37 K, while the Nernst coefficient becomes greatly enhanced and field dependent below T ~ 30 K. In the zero-T limit S/T and v/T diverge logarithmically, what is related to occurrence of the quantum critical point (QCP). Presented results suggest that the antiferromagnetic spin-density-wave scenario may be applicable to QCP in Ce2PdIn8.
We develop a theory of transverse thermoelectric (Peltier) conductivity, α_{xy}, in finite magnetic field -- this particular conductivity is often the most important contribution to the Nernst thermopower. We demonstrate that α_{xy} of a free electron gas can be expressed purely and exactly as the entropy per carrier irrespective of temperature (which agrees with seminal Hall bar result of Girvin and Jonson). In two dimensions we prove the universality of this result in the presence of disorder which allows explicit demonstration of a number features of interest to experiments on graphene and …
When a superconductor is warmed above its critical temperature $T_c$, long range order is destroyed by fluctuations in the order parameter. These fluctuations can be probed by measurements of conductivity, diamagnetism, and of the Nernst effect. Here, we study a regime where superconductivity is destroyed by phase fluctuations arising from a dilute liquid of mobile vortices. We find that the Nernst effect and diamagnetic response differ significantly from Gaussian fluctuations -- in particular, a much sharper decay with temperature is obtained. We predict a rapid onset of Nernst signal at a te…
The strange-metal state is a crucial problem in condensed matter physics highlighted by its ubiquity in almost all major correlated systems[1-7]. Its understanding could provide important insight into high-Tc superconductivity[2] and quantum criticality[8]. However, with the Fermi liquid theory failing in strange metals, understanding the highly unconventional behaviors has been a long-standing challenge. Fundamental aspects of strange metals remain elusive, including the nature of their charge carriers[1]. Here, we report the observation of a giant Nernst response in the strange-metal state i…
Very recently large Nernst effect and Seebeck effect were observed above the superconducting transition temperature 2.3K in a heavy fermion superconductor CeCoIn_5. We shall interpret this large Nernst effect in terms of unconventional density wave (UDW), which appears around T=18K. Also the temperature dependence of the Seebeck coefficient below T=18K is described in terms of UDW. Another hallmark for UDW is the angular dependent magnetoresistance, which should be readily accessible experimentally.
We present a study of transport properties of the heavy fermion URu$_2$Si$_2$ in pulsed magnetic field. The large Nernst response of the hidden order state is found to be suppressed when the magnetic field exceeds 35 T. The combination of resistivity, Hall and Nernst data outlines the reconstruction of the Fermi surface in the temperature-field phase diagram. The zero-field ground state is a compensated heavy-electron semi-metal, which is destroyed by magnetic field through a cascade of field-induced transitions. Above 40 T, URu$_2$Si$_2$ appears to be a polarized heavy fermions metal with a l…
The first heavy fermion superconductor CeCu$_2$Si$_2$ has not revealed all its striking mysteries yet. At high pressures, superconductivity is supposed to be mediated by valence fluctuations, in contrast to ambient pressure, where spin fluctuations most likely act as pairing glue. We have carried out a multiprobe (electric transport, thermopower, ac specific heat, Hall and Nernst effects) experiment up to $7 \text{GPa}$ on a high quality CeCu$_2$Si$_2$ single crystal. Reliable resistivity data reveal for the first time a scaling behavior close to the supposed valence transition, and allow to l…
When a superconductor is heated above its critical temperature $T_c$, macroscopic coherence vanishes, leaving behind droplets of thermally fluctuating Cooper pair. This superconducting fluctuation effect above $T_c$ has been investigated for many decades and its influence on the transport, thermoelectric and thermodynamic quantities in most superconductors is well understood by the standard Gaussian fluctuation theories. The transverse thermoelectric (Nernst) effect is particularly sensitive to the fluctuations, and the large Nernst signal found in the pseudogap regime of the underdoped high-$…
We present a general hydrodynamic theory of transport in the vicinity of superfluid-insulator transitions in two spatial dimensions described by "Lorentz"-invariant quantum critical points. We allow for a weak impurity scattering rate, a magnetic field B, and a deviation in the density, ρ, from that of the insulator. We show that the frequency-dependent thermal and electric linear response functions, including the Nernst coefficient, are fully determined by a single transport coefficient (a universal electrical conductivity), the impurity scattering rate, and a few thermodynamic state variable…
In our mini-review, we address manifestations of $T/B$ scaling behavior of heavy-fermion (HF) compounds, where $T$ and $B$ are respectively temperature and magnetic field. Using experimental data and the fermion condensation theory, we show that this scaling behavior is typical of HF compounds including HF metals, quasicrystals, and quantum spin liquids. We demonstrate that such scaling behavior holds down to the lowest temperature and field values, so that $T/B$ varies in a wide range, provided the HF compound is located near the topological fermion condensation quantum phase transition (FCQP…
Recent experimental and numerical evidence suggest an intriguing universal relationship between the Fermi surface anisotropy of the non-interacting parent two-dimensional electron gas and the strongly correlated composite Fermi liquid formed in a strong magnetic field close to half-filing. Inspired by these observations, we explore more generally the question of anisotropy renormalization in interacting 2D Fermi systems. Using a recently developed non-perturbative and numerically-exact projective quantum Monte Carlo simulation as well as other numerical and analytic techniques, only for Dirac …
We discuss the relation between the T^{2}-coefficient of electrical resistivity $A$ and the T-linear specific-heat coefficient $γ$ for heavy-fermion systems with general $N$, where $N$ is the degeneracy of quasi-particles. A set of experimental data reveals that the Kadowaki-Woods relation; $A/γ^{2} = 1*10^{-5} {μΩ}(K mol/mJ)^{2}$, collapses remarkably for large-N systems, although this relation has been regarded to be commonly applicable to the Fermi-liquids. Instead, based on the Fermi-liquid theory we propose a new relation; $\tilde{A}/\tildeγ^2=1\times10^{-5}$ with $\tilde{A} = A/(1/2)N(N-…
Dynamical conductivity spectra s(w) have been measured for a diverse range of heavy-fermion (HF) Ce and Yb compounds. A characteristic excitation peak has been observed in the mid-infrared region of s(w) for all the compounds, and has been analyzed in terms of a simple model based on conduction (c)-f electron hybridized band. A universal scaling is found between the observed peak energies and the estimated c-f hybridization strengths of these HF compounds. This scaling demonstrates that the model of c-f hybridized band can generally and quantitatively describe the charge excitation spectra of …
The single-particle hopping between two chains is investigated by exact-diagonalizations techniques supplemented by finite-size scaling analysis. In the case of two coupled strongly-correlated chains of spinless fermions, the Taylor expansion of the expectation value of the single-particle interchain hopping operator of an electron at momentum k_F in powers of the interchain hopping t_perp is shown to become unstable in the thermodynamic limit. In the regime alpha<alpha_{tp} (alpha_{tp} simeq 0.41) where transverse two-particle hopping is less relevant than single-particle hopping, the finite-…
We report a systematic study of temperature- and field-dependent charge ($\boldsymbolρ$) and entropy ($\mathbf{S}$) transport in the heavy-fermion superconductor CeIrIn$_5$. Its large positive thermopower $S_{xx}$ is typical of Ce-based Kondo lattice systems, and strong electronic correlations play an important role in enhancing the Nernst signal $S_{xy}$. By separating the off-diagonal Peltier coefficient $α_{xy}$ from $S_{xy}$, we find that $α_{xy}$ becomes positive and greatly enhanced at temperatures well above the bulk $T_c$. Compared with the non-magnetic analog LaIrIn$_5$, these results…
The recent discoveries of strikingly large zero-field Hall and Nernst effects in antiferromagnets Mn$_3$$X$, ($X$ = Sn, Ge) have brought the study of magnetic topological states to the forefront of condensed matter research and technological innovation. These effects are considered fingerprints of Weyl nodes residing near the Fermi energy, promoting Mn$_3$$X$, ($X$ = Sn, Ge) as a fascinating platform to explore the elusive magnetic Weyl fermions. In this review, we provide recent updates on the insights drawn from experimental and theoretical studies of Mn$_3$$X$, ($X$ = Sn, Ge) by combining p…
We demonstrate, that the main universal features of the low temperature experimental $H-T$ phase diagram of CeCoIn5 and other heavy-fermion metals can be well explained using Landau paradigm of quasiparticles. The main point of our theory is that above quasiparticles form so-called fermion-condensate state, achieved by a fermion condensation quantum phase transition (FCQPT). When a heavy fermion liquid undergoes FCQPT, the fluctuations accompanying above quantum critical point are strongly suppressed and cannot destroy the quasiparticles. The comparison of our theoretical results with experime…
We show that Popov-Fedotov trick of mapping spin-1/2 lattice systems on two-component fermions with imaginary chemical potential readily generalizes to bosons with a fixed (but not limited) maximal site occupation number, as well as to fermionic Hamiltonians with various constraints on the site Fock states. In a general case, the mapping---fermionization---is on multi-component fermions with many-body non-Hermitian interactions. Additionally, the fermionization approach allows one to convert large many-body couplings into single-particle energies, rendering the diagrammatic series free of larg…
A new universality class of quantum criticality emerging in itinerant electron systems with strong local electron correlations is discussed. The quantum criticality of a Ce- or Yb-valence transition gives us a unified explanation for unconventional criticality commonly observed in heavy fermion metals such as YbRh2Si2 and β-YbAlB4, YbCu5-xAlx, and CeIrIn5. The key origin is due to the locality of the critical valence fluctuation mode emerging near the quantum critical end point of the first-order valence transition, which is caused by strong electron correlations for f electrons. Wider relevan…
The symmetry of the order parameter is the defining property of a superconductor and a strong clue to its pairing mechanism. While d-wave symmetry is firmly established in high-Tc superconductors, in no heavy-fermion superconductor is the symmetry known definitively. One way to elucidate the order parameter is to locate the symmetry-imposed nodes in the energy gap by measuring the heat carried by the zero-energy quasiparticles associated with those nodes as a function of direction. As verified in high-Tc superconductors a line of nodes yields universal heat transport independent of impurity sc…
The nonlinear conductance of semiconductor heterostructures and single molecule devices exhibiting Kondo physics has recently attracted attention. We address the observed sample dependence of the measured steady state transport coefficients by considering additional electronic contributions in the effective low-energy model underlying these experiments that are absent in particle-hole symmetric setups. A novel version of the superperturbation theory of Hafermann et al. in terms of dual fermions is developed, which correctly captures the low-temperature behavior. We compare our results with the…
In the present work we propose that two-time correlations of Majorana edge localized fermions constitute a novel and versatile toolbox for assessing the topological phases of 1D open lattices. Using analytical and numerical calculations on the Kitaev model, we uncover universal relationships between the decay of the short-time correlations and a particular family of out-of-time-ordered correlators, which provide direct experimental alternatives to the quantitative analysis of the system regime, either normal or topological. Furthermore we show that the saturation of two-time correlations posse…
We have found solution to a model of tunneling between a multi-channel Fermi liquid reservoir and an edge of the principal fractional quantum Hall liquid (FQHL) in the strong coupling limit. The solution explains how the absence of the time-reversal symmetry at high energies due to chiral edge propagation makes the universal two-terminal conductance of the FQHL fractionally quantized and different from that of a 1D Tomonaga-Luttinger liquid wire, where a similar model but preserving the time-reversal symmetry predicts unsuppressed free-electron conductance.
A previous scaling analysis of pressure experiments in heavy fermion is reviewed and enlarged. We show that the critical exponents obtained from this analysis indicate that a one-parameter scaling describes these experiments. We obtain explicitly the enhancemente factors showing that these systems are indeed near criticality and that the scaling approach is appropriate. The physics responsible for the one-parameter scaling and breakdown of hyperscaling is clarified. We discuss a microsocopic theory that is in agreement with the experiments. The scaling theory is generalized for the case the sh…
We verify signatures of antiferromagnetic (AF) correlations in the double occupancy D [Gorelik et al., PRL 105, 065301 (2010)] and study their dimensional dependence using direct quantum Monte Carlo in dimensions d=2,3 and Bethe Ansatz in d=1. We find quantitative agreement with dynamical mean-field theory (DMFT) in the cubic case and qualitative agreement down to d=1. As a function of entropy s=S/(N k_B), D is nearly universal with respect to d; the minimum in D(s) approaches s=log(2) at strong coupling, as predicted by DMFT. Long-range order appears hardly relevant for the current search of …
Many-body fermion systems are important in many branches of physics, including condensed matter, nuclear, and now cold atom physics. In many cases, the interactions between fermions can be approximated by a contact interaction. A recent theoretical advance in the study of these systems is the derivation of a number of exact universal relations that are predicted to be valid for all interaction strengths, temperatures, and spin compositions. These equations, referred to as the Tan relations, relate a microscopic quantity, namely, the amplitude of the high-momentum tail of the fermion momentum d…
Majorana-fermionic quantum computation (MFQC) was proposed by Bravyi and Kitaev (See Ref.\cite{Kitaev}), in which a fault-torrent (non-topological) quantum computer built from Majorana fermions may be more efficient than that built from distinguishable two-state systems. However, till now people don't know how to realize a MFQC in a physical system. In this paper we proposed a possible realization of MFQC. We find that the end of a line-defect of p-wave superconductor or superfluid on a honeycomb lattice will trap a Majorana zero mode, which will become the starting point of MFQC. Then we show…
Non-unitary evolution can give rise to novel steady states classified by their entanglement properties. In this work, we aim to understand its interplay with long-range hopping that decays with $r^{-α}$ in free-fermion systems. We first study two solvable Brownian models with long-range non-unitary dynamics: a large-$N$ SYK$_2$ chain and a single-flavor fermion chain and we show that they share the same phase diagram. When $α>0.5$, we observe two critical phases with subvolume entanglement scaling: (i) $α>1.5$, a logarithmic phase with dynamical exponent $z=1$ and logarithmic subsystem entangl…
