Topological superconductivity, ferromagnetism, and valley-polarized phases in moire systems: Renormalization group analysis for twisted double bilayer graphene
Recent experiments have observed possible spin- and valley-polarized insulators and spin-triplet superconductivity in twisted double bilayer graphene, a moire structure consisting of a pair of Bernal-stacked bilayer graphene. Besides the continuously tunable band widths controlled by an applied displacement field and twist angle, these moire bands also possess van Hove singularities near the Fermi surface and a field-dependent nesting which is far from perfect. Here we carry out a perturbative renormalization group analysis to unbiasedly study the competition among all possible instabilities in twisted double bilayer graphene and related systems with a similar van Hove fermiology in the presence of weak but finite repulsive interactions. Our key finding is that there are several competing magnetic, valley, charge, and superconducting instabilities arising from interactions in twisted double bilayer graphene, which can be tuned by controlling the displacement field and the twist angle. In particular, we show that spin- or valley-polarized uniform instabilities generically dominate under moderate interactions smaller than the band width, whereas $p$-wave spin-triplet topological superconductivity and exotic spin-singlet modulated paired state become important as the interactions decrease. Realization of our findings in general moire systems with a similar van Hove fermiology should open up new opportunities for manipulating topological superconductivity and spin- or valley-polarized states in highly tunable platforms.
Recent experiments have observed correlated insulating and possible superconducting phases in twisted homobilayer transition metal dichalcogenides (TMDs). Besides the spin-valley locked moire bands due to the intrinsic Ising spin-orbit coupling, homobilayer moire TMDs also possess either logarithmic or power-law divergent Van Hove singularities (VHS) near the Fermi surface, controllable by an external displacement field. The former and the latter are dubbed conventional and higher-order VHS, respectively. Here, we perform a perturbative renormalization group (RG) analysis to unbiasedly study t…
Several moiré systems created by various twisted bilayers have manifested magnetism under flatband conditions leading to enhanced interaction effects. We theoretically study stability of moiré flatband ferromagnetism against collective excitations, with a focus on the effects of Bloch band quantum geometry. The spin magnon spectrum is calculated using different approaches, including Bethe-Salpeter equation, single mode approximation, and an analytical theory. One of our main results is an analytical expression for the spin stiffness in terms of the Coulomb interaction potential, the Berry curv…
Chern-Textured Exciton Insulators with Valley Spiral Order in Moiré Materials
Rudolf Peierls Centre for Theoretical Physics（鲁道夫·皮尔斯理论物理中心）；Princeton Center for Theoretical Science, Princeton University（普林斯顿大学理论科学中心）；Department of Physics, University of Zurich（苏黎世大学物理系）；Department of Physics, Ghent University（根特大学物理系）
Moiré heterobilayer transition metal dichalcogenides (TMDs) emerge as an ideal system for simulating the single-band Hubbard model and interesting correlated phases have been observed in these systems. Nevertheless, the moiré bands in heterobilayer TMDs were believed to be topologically trivial. Recently, it was reported that both a quantum valley Hall insulating state at filling $ν=2$ (two holes per moiré unit cell) and a valley-polarized quantum anomalous Hall state at filling $ν=1$ were observed in AB stacked moiré MoTe$_2$/WSe$_2$ heterobilayers. However, how the topologically nontrivial s…
One salient feature of systems with Moiré superlattice is that, Chern number of "minibands" originating from each valley of the original graphene Brillouin zone becomes a well-defined quantized number because the miniband from each valley can be isolated from the rest of the spectrum due to the Moiré potential. Then a Moiré system with a well-defined valley Chern number can become a nonchiral topological insulator with $U(1) \times Z_3 $ symmetry and a $\mathbb{Z}$ classification at the free fermion level. Here we demonstrate that the strongly interacting nature of the Moiré system reduces the…
Twisted van der Waals heterostructures have recently been proposed as a condensed-matter platform for realizing controllable quantum models due to the low-energy moiré bands with specific charge distributions in moiré superlattices. Here, combining angle-resolved photoemission spectroscopy with sub-micron spatial resolution (μ-ARPES) and scanning tunneling microscopy (STM), we performed a systematic investigation on the electronic structure of 5.1° twisted bilayer WSe2 that hosts correlated insulating and zero-resistance states. Interestingly, contrary to one's expectation, moiré bands were ob…
Twisting moiré heterostructures to the flatband regime allows for the formation of strongly correlated quantum states, since the dramatic reduction of the bandwidth can cause the residual electronic interactions to set the principal energy scale. An effective description for such correlated moiré heterostructures, derived in the strong-coupling limit at integer filling, generically leads to spin-valley Heisenberg models. Here we explore the emergence and stability of spin liquid behavior in an SU(2)$^{\mathrm{spin}}\otimes$SU(2)$^{\mathrm{valley}}$ Heisenberg model upon inclusion of Hund's-ind…
Valley polarization of moiré interlayer exciton complexes driven by many-body interactions
Technical University of Munich（慕尼黑工业大学）；Munich Center for Quantum Science and Technology (MCQST)（慕尼黑量子科学与技术中心）；National Institute for Materials Science（物质材料研究机构）；Research Center for Electronic and Optical Materials, National Institute for Materials Science（物质材料研究机构电子光学材料研究中心）；Research Center for Materials Nanoarchitectonics, National Institute for Materials Science（物质材料研究机构材料纳米架构研究中心）
Ferromagnetism from the geometry of localized wavefunctions in moiré systems
Princeton Center for Theoretical Science, Princeton University（普林斯顿大学理论物理中心）；Department of Electrical and Computer Engineering, Princeton University（普林斯顿大学电气与计算机工程系）
Exotic correlated insulating phases emerge in the ABC-stacked trilayer graphene-boron nitride Moire super-lattice at both quarter and half-filling. A single-band minimal model with valley contrasting staggered-flux is proposed to capture the relevant band structure, where the conspiracy of perfect Fermi-surface nesting and van Hove singularity strongly enhance the valley fluctuation, leading to inter-valley spiral (IVS) order at half filling. In this paper, we consider a strong coupling U(1)$_{v}\times $SU(2)$_{s}$ symmetric spin-valley model to obtain the correlated insulating state and the p…
Recent experiment has shown that the ABC-stacked trilayer graphene-boron nitride Moire super-lattice at half-filling is a Mott insulator. Based on symmetry analysis and effective band structure calculation, we propose a valley-contrasting chiral tight-binding model with local Coulomb interaction to describe this Moire super-lattice system. By matching the positions of van Hove points in the low-energy effective bands, the valley-contrasting staggered flux per triangle is determined around $π/2$. When the valence band is half-filled, the Fermi surfaces are found to be perfectly nested between t…
Many graphene moiré superlattices host narrow bands with non-zero valley Chern numbers. We provide analytical and numerical evidence for a robust spin and/or valley polarized insulator at total integer band filling in nearly flat bands of several different moiré materials. In the limit of a perfectly flat band, we present analytical arguments in favor of the ferromagnetic state substantiated by numerical calculations. Further, we numerically evaluate its stability for a finite bandwidth. We provide exact diagonalization results for models appropriate for ABC trilayer graphene aligned with hBN,…
Studies on two-dimensional electron systems in a strong magnetic field first revealed the quantum Hall (QH) effect, a topological state of matter featuring a finite Chern number (C) and chiral edge states. Haldane later theorized that Chern insulators with integer QH effects could appear in lattice models with complex hopping parameters even at zero magnetic field. The ABC-trilayer graphene/hexagonal boron nitride (TLG/hBN) moiré superlattice provides an attractive platform to explore Chern insulators because it features nearly flat moiré minibands with a valley-dependent electrically tunable …
The interplay between strong correlations and non-trivial topology in twisted moiré systems can give rise to a rich landscape of ordered states that intertwine the spin, valley, and charge degrees of freedom. In this paper, we investigate the properties of a system that displays long-range valley-polarized nematic order. Besides breaking the threefold rotational symmetry of the triangular moiré superlattice, this type of order also breaks twofold rotational and time-reversal symmetries, which leads to interesting properties. First, we develop a phenomenological model to describe the onset of t…
The observation of strongly-correlated states in moiré systems has renewed the conceptual interest in magnetic systems with higher SU(4) spin symmetry, e.g. to describe Mott insulators where the local moments are coupled spin-valley degrees of freedom. Here, we discuss a numerical renormalization group scheme to explore the formation of spin-valley ordered and unconventional spin-valley liquid states at zero temperature based on a pseudo-fermion representation. Our generalization of the conventional pseudo-fermion functional renormalization group approach for $\mathfrak{su}$(2) spins is capabl…
We introduce and study a minimum two-orbital Hubbard model on a triangular lattice, which captures the key features of both the trilayer ABC-stacked graphene-boron nitride heterostructure and twisted transition metal dichalcogenides in a broad parameter range. Our model comprises first- and second-nearest neighbor hoppings with valley-contrasting flux that accounts for trigonal warping in the band structure. For the strong-coupling regime with one electron per site, we derive a spin-orbital exchange Hamiltonian and find the semiclassical ground state to be a spin-valley density wave. We show t…
Moiré materials provide fertile ground for the correlated and topological quantum phenomena. Among them, the quantum anomalous Hall (QAH) effect, in which the Hall resistance is quantized even under zero magnetic field, is a direct manifestation of the intrinsic topological properties of a material and an appealing attribute for low-power electronics applications. The QAH effect has been observed in both graphene and transition metal dichalcogenide (TMD) moiré materials. It is thought to arise from the interaction-driven valley polarization of the narrow moiré bands. Here, we show surprisingly…
Motivated by the recent observation of evidences of ferromagnetism in correlated insulating states in systems with Moiré superlattices, we study a two-orbital quantum antiferromagnetic model on the triangular lattice, where the two orbitals physically correspond to the two valleys of the original graphene sheet. For simplicity this model has a SU(2)$^s$$\otimes$SU(2)$^v$ symmetry, where the two SU(2) symmetries correspond to the rotation within the spin and valley space respectively. Through analytical argument, Schwinger boson analysis and also DMRG simulation, we find that even though all th…
Electrons' multiple quantum degrees of freedom can lead to rich physics, including a competition between various exotic ground states, as well as novel applications such as spintronics and valleytronics. Here we report magneto-transport experiments demonstrating how the valley degree of freedom impacts the fractional quantum states (FQHSs), and the related magnetic-flux-electron composite fermions (CFs), at very high magnetic fields in the extreme quantum limit when only the lowest Landau level is occupied. Unlike in other multivalley two-dimensional electron systems such as Si or monolayer gr…
Detecting magnetic order at the nanoscale is of central interest for the study of quantum magnetism in general, and the emerging field of moiré magnets in particular. Here, we analyze the exciton band structure that arises from a periodic modulation of the valley Zeeman effect. Despite long-range electron-hole exchange interactions, we find a sizable splitting in the energy of the bright circularly-polarized exciton Umklapp resonances, which serves as a direct optical probe of magnetic order. We first analyze quantum moiré magnets realized by periodic ordering of electron spins in Mott-Wigner …
Moiré in $Γ$-valley square lattice: Copper- and iron-based superconductor simulation in a single device
International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science（物质纳米结构国际中心（WPI-MANA），国立材料研究所）；Department of Physics, Harvard University（哈佛大学物理系）；Department of Physics, University of Connecticut（康涅狄格大学物理系）；School of Physics, Georgia Institute of Technology（佐治亚理工学院物理学院）
Although evidence of inter-valley attraction-mediated by phonon or topological fluctuations is accumulating, the origin of superconductivity in the flat-band quantum moiré materials remains an open question. Here, instead of attempting to pinpoint the origin of the superconductivity, we aim at identifying universal properties of moiré flat bands that shall emerge in the presence of inter-valley attractions. We show that by matching the interaction strength of inter-valley attraction with intra-valley repulsion, the flat-band limit becomes exactly solvable. Away from the flat-band limit, the sy…
We propose a new mechanism for quantum anomalous Hall (QAH) effect in the AB stacked MoTe$_2$/WSe$_2$ system. Based on the observation that the inter-layer tunneling is suppressed in the AB stacking, we consider a model with two layers coupled through the Coulomb interaction. The moiré lattices of the two layers are shifted to form a honeycomb lattice together. Initially, the system is in a layer-polarized Mott insulator at $ν_T=1$. But with a displacement field, an equal number of holes and electrons are doped into the two layers respectively and they form inter-layer exciton condensation. Th…
We use a lowest Landau level model to study the recent observation of an anomalous Hall effect in twisted bilayer graphene. This effective model is rooted in the occurrence of Chern bands which arise due to the coupling between the graphene device and its encapsulating substrate. Our model exhibits a phase transition from a spin-valley polarized insulator to a partial or fully valley unpolarized metal as the bandwidth is increased relative to the interaction strength, consistent with experimental observations. In sharp contrast to standard quantum Hall ferromagnetism, the Chern number structur…
We predict that in a twisted homobilayer of transition-metal dichalcogenide MoS$_2$, spin-orbit coupling in the conduction band states from $\pm K$ valleys can give rise to moiré flat bands with nonzero Chern numbers in each valley. The nontrivial band topology originates from a unique combination of angular twist and local mirror symmetry breaking in each individual layer, which results in unusual skyrmionic spin textures in momentum space with skyrmion number $\mathcal{S} = \pm 2$. Our Hartree-Fock analysis further suggests that density-density interactions generically drive the system at $1…
Near a magic twist angle, the lowest energy conduction and valence bands of bilayer graphene moiré superlattices become extremely narrow. The band dispersion that remains is sensitive to the moiré's strain pattern, nonlocal tunneling between layers, and filling-factor dependent Hartree and exchange band renormalizations. In this article we analyze the influence of these band-structure details on the pattern of flavor-symmetry-breaking observed in this narrow band system, and on the associated pattern of Fermi surface reconstructions revealed by weak-field-Hall and Schubnikov-de Haas magneto-tr…
We investigate interaction-induced valley domain walls in bilayer graphene in the $ν=0$ quantum Hall state, subject to a perpendicular electric field that is antisymmetric across a line in the sample. Such a state can be realized in a double-gated suspended sample, where the electric field changes sign across a line in the middle. The non-interacting energy spectrum of the ground state is characterized by a sharp domain wall between two valley-polarized regions. Using the Hartree-Fock approximation, we find that the Coulomb interaction opens a gap between the two lowest-lying states near the F…
We investigate few- and many-body states in half-filled maximally symmetric topological insulator flat bands realized by two degenerate Landau levels which experience opposite magnetic fields. This serves as a toy model of flat bands in moiré materials in which valleys have Chern numbers $C= \pm 1$. We argue that although the spontaneously polarized Ising Chern magnet is a natural ground state for repulsive Coulomb interactions, it can be in reasonable energetic competition with correlated states which can be viewed as Laughlin states of excitons when short distance corrections to the interact…
Bilayer Moiré structures are a highly tunable laboratory to investigate the physics of strongly correlated electron systems. Moiré transition metal dichalcogenides at low-energies, in particular, are believed to be described by a single narrow band Hubbard model on a triangular lattice with spin-orbit coupling. Motivated by recent experimental evidence for superconductivity in twisted bilayer materials, we investigate the possible superconducting pairings in a two-dimensional single band Rashba-Hubbard model. Using a random-phase approximation in the presence of nearest and next-nearest neighb…
