Magnetic skyrmions are promising candidates for future storage devices with a large data density. A great variety of materials have been found that host skyrmions up to the room-temperature regime. Lorentz microscopy, usually performed in a transmission electron microscope (TEM), is one of the most important tools for characterizing skyrmion samples in real space. Using numerical calculations, this work relates the phase contrast in a TEM to the actual magnetization profile of an isolated Neel or Bloch skyrmion, the two most common skyrmion types. Within the framework of the used skyrmion model, the results are independent of skyrmion size and wall width and scale with sample thickness for purely magnetic specimens. Simple rules are provided to extract the actual skyrmion configuration of pure Bloch or Neel skyrmions without the need of simulations. Furthermore, first differential phase contrast (DPC) measurements on Neel skyrmions that meet experimental expectations are presented and showcase the described principles. The work is relevant for material sciences where it enables the engineering of skyrmion profiles via convenient characterization.
Magnetic skyrmions are intriguing topological spin textures that promise future high-density spintronic devices. The creation of magnetic skyrmions has been understood based on the energetics of skyrmions, but the detailed dynamic process of the skyrmion creation remains unclear. Here topological evolution in conversion from uneven domains to Néel-skyrmions is investigated using micromagnetic simulations. We find that, rather than the overall topological charge, annihilation of novel topological defects, i.e., recently suggested domain wall skyrmions, dominantly govern the skyrmion creation pr…
Increasing amounts of information force the continuous improvement of information storage and processing technologies, further device miniaturization, and their efficiency increase. Magnetic skyrmions, topological quasiparticles, and the smallest stable magnetic textures possess intriguing properties and potential for data storage applications. Hybrid nanostructures with elements of different magnetization orientations can offer additional advantages for developing skyrmion-based spintronic and magnonic devices. We show that an Néel-type skyrmion confined within a nanodot placed on top of a fe…
The promise of high-density and low-energy-consumption devices motivates the search for layered structures that stabilize chiral spin textures such as topologically protected skyrmions. At the same time, layered structures provide a new platform for the discovery of new physics and effects. Recently discovered long-range intrinsic magnetic orders in the two-dimensional van der Waals materials offer new opportunities. Here we demonstrate the Dzyaloshinskii-Moriya interaction and Néel-type skyrmions are induced at the WTe2/Fe3GeTe2 interface. Fe3GeTe2 is a ferromagnetic material with strong perp…
We present a mechanism for deterministic control of the Bloch chirality in magnetic domain walls and skyrmions, originating from the interplay between an interfacial Dzyaloshinskii$-$Moriya interaction (DMI) and a perpendicular magnetic field. Although conventional interfacial DMI favors chiral Néel skyrmions, it does not break the energetic symmetry of the two Bloch chiralities in mixed Bloch$-$Néel skyrmions. However, the energy barrier to switching between Bloch chiralities does depend on the sense of rotation, which is dictated by the direction of the driving field. Our analytical and micr…
Spin-polarized scanning tunneling microscopy (SPSTM) was used to directly image nanoscale Néel skyrmions in a SrIrO3 / SrRuO3 bilayer system that are among the smallest reported to date in any system. Off-axis magnetron sputtering was used to cap epitaxial films of the oxide ferromagnet SRO with 2 unit cells of SrIrO3, intended to provide interfacial spin orbit coupling. Atomic resolution STM imaging and tunneling spectroscopy were used to identify island-like SrIrO3 grains and small regions of bare SrRuO3. Isolated skyrmions were only observed in SrIrO3-covered regions of the film, and exhibi…
The 212 species of structural phase transitions which break macroscopic symmetry are analyzed with respect to the occurrence of time-reversal invariant vector and bidirector order parameters. The possibility of discerning the orientational domain states of the low-symmetry phase by these `vectorlike' physical properties has been derived using a computer algorithm exploiting the concept of polar, axial, chiral and neutral dipoles. It is argued that for species 32 > 3, 422 > 4 and 622 > 6, Bogdanov-Yablonskii phenomenological theory for a ferromagnetic Bloch Skyrmions applies also to the ferroel…
Magnetic skyrmions are topologically protected spin textures that exhibit many fascinating features. As compared to the well-studied cryogenic Bloch skyrmions in bulk materials, we focus on the room-temperature Néel skyrmions in thin-film systems with an interfacial broken inversion symmetry in this article. Specifically, we show the stabilization, the creation, and the implementation of Néel skyrmions that are enabled by the electrical current-induced spin-orbit torques. Towards the nanoscale Néel skyrmions, we further discuss the challenges from both material optimization and imaging charact…
Theoretical investigation demonstrates that the composite bilayer (i.e., chiral-magnetic/ferroelectric bilayer) offers the possibility of electric-induced magnetic Skyrmions [Phys. Rev. B \textbf{94}, 014311 (2016)]. In this Article, we propose a micromagnetic model to physically manipulate magnetic Bloch Skyrmions propagating in a chiral-magnetic thin film with a polarized ferroelectric essential to drive the system through the converse magnetoelectric effect. Effects caused by different velocities of the propagation, sizes of the thin film, and strength of the magnetoelectric couplings stron…
We study spin-wave excitations in a circular ferromagnetic nanodot in different inhomogeneous, topologically non-trivial magnetization states, specifically, vortex and skyrmion states. Gradual change in the strength of the out-of-plane magnetic anisotropy and the Dzyaloshinskii-Moriya exchange interaction leads to continuous phase transitions between different stable magnetic configurations and allows for mapping of dynamic spin modes in and between the vortex, Bloch-type skyrmion and Néel-type skyrmion states. Our study elucidates the connections between gyrotropic modes, azimuthal spin waves…
We investigate a mechanical method to manipulate magnetic Bloch Skyrmions by applying an electric field in a composite chiral-magnetic (CM)/ferroelectric (FE) bilayer. The magnetoelectric coupling at the interface allows the electric field to stimulate magnetic ordering. Therefore it offers the possibility to generate Skyrmions [Phys. Rev. B 94, 014311 (2016)]. Here, we design a movable and localized electric field source to drive skyrmion transport along the bilayer. A traveling velocity of the electric field source must be carefully chosen to show the stability and effciency of this process.…
An analytical expression for the energy of Néel skyrmions in ultra-thin nanodots considering exchange, uniaxial anisotropy, Dzyaloshinskii-Moriya, and dipolar contributions has been obtained. In particular, we have proposed for the Néel skyrmion, a general ansatz for the component of the magnetization perpendicular to the dot, given by $m_z(r) = [1-(r/R_s)^n]/[1 + (r/R_s)^n]$, where $R_s$ is the radius of the skyrmion and $n$ is an integer and even number. As proof of concept, we calculate the energy of a Néel skyrmion in an ultra-thin Co/Pt dot, and we find that the dipolar contribution canno…
Magnetic skyrmions are nanoscale spin structures recently discovered at room temperature (RT) in multilayer films. Employing their novel topological properties towards exciting technological prospects requires a mechanistic understanding of the excitation and relaxation mechanisms governing their stability and dynamics. Here we report on the magnetization dynamics of RT Néel skyrmions in Ir/Fe/Co/Pt multilayer films. We observe a ubiquitous excitation mode in the microwave absorption spectrum, arising from the gyrotropic resonance of topological skyrmions, and robust over a wide range of tempe…
We investigate the dependence of the Néel skyrmion size and stability on perpendicular magnetic field in ultrathin circular magnetic dots with out-of-plane anisotropy and interfacial Dzyaloshinskii-Moriya exchange interaction. Our results show the existence of two distinct dependencies of the skyrmion radius on the applied field and dot size. In the case of skyrmions stable at zero field, their radius strongly increases with the field applied parallel to the skyrmion core until skyrmion reaches the metastability region and this dependence slows down. More common metastable skyrmions demonstrat…
Magnetic skyrmions are topologically protected nanoscale spin textures exhibiting fascinating physical behaviors. Recent observations of room temperature Néel-type skyrmions in magnetic multilayer films are an important step towards their use in ultra-low power devices. We have investigated the magnetization reversal in a [Pt/Co/Ta]11 multilayer sample under a tilted magnetic field using the in-situ Lorentz tunneling electron microscopy. On decreasing the magnetic field individual skyrmions appear that subsequently evolve into snake-like structures growing in the direction opposite to the in-p…
Recent advances on the stabilization and manipulation of chiral magnetization configurations in systems consisting in alternating atomic layers of ferromagnetic and non-magnetic materials hold promise of innovation in spintronics technology. The low dimensionality of the systems promotes spin orbit driven interfacial effects like antisymmetric Dzyaloshinskii-Moriya interactions (DMI) and surface magnetic anisotropy, whose relative strengths may be tuned to achieve stable nanometer sized magnetic objects with fixed chirality. While in most of the cases this is obtained by engineering complex mu…
The static and dynamic states of Néel skyrmions in ultrathin ferromagnetic films with interfacial Dzyaloshinskii-Moriya interaction (DMI) have been micromagnetically simulated as functions of the interfacial DMI strength and applied static magnetic field. Findings reveal that while the breathing, counterclockwise (CCW) and clockwise (CW) rotational eigenmodes exist in the skyrmion lattice (SkL) phase, only the first two modes are present in the isolated skyrmion (ISk) phase. Additionally, the eigenfrequency of the CCW mode is insensitive to the magnetic-field driven SkL-ISk phase transition, a…
The orientation of Néel-type skyrmions in the lacunar spinels GaV$_4$S$_8$ and GaV$_4$Se$_8$ is tied to the polar axes of their underlying crystal structure through the Dzyaloshinskii-Moriya interaction. In these crystals, the skyrmion lattice phase exists for externally applied magnetic fields parallel to these axes and withstands oblique magnetic fields up to some critical angle. Here, we map out the stability of the skyrmion lattice phase in both crystals as a function of field angle and magnitude using dynamic cantilever magnetometry. The measured phase diagrams reproduce the major feature…
Skyrmions are nanoscale spin configurations with topological properties that hold great promise for spintronic devices. Here, we establish their Néel texture, helicity, and size in Ir/Fe/Co/Pt multilayer films by constructing a multipole expansion to model their stray field signatures and applying it to magnetic force microscopy (MFM) images. Furthermore, the demonstrated sensitivity to inhomogeneity in skyrmion properties, coupled with a unique capability to estimate the pinning force governing dynamics, portends broad applicability in the burgeoning field of topological spin textures.
A detailed analytic and numerical analysis of the interaction between two bubble skyrmions has been carried out. Results from micromagnetic calculations show a strong dependence of the parameters of the skyrmion magnetic profile as a function of the magnetostatic interaction. The magnetic core and edge-width sizes of the skyrmion increase or decrease depending on the relative position between the skyrmions and the uniaxial perpendicular anisotropy. In particular, when a magnetic disk is over another, there is a transition from a Bloch-like skyrmion configuration to a Néel-like skyrmion configu…
Observation by SANS and PNR of pure Néel-type domain wall profiles and skyrmion suppression below room temperature in magnetic [Pt/CoFeB/Ru]$_{10}$ multilayers
The presence of interfacial Dzyaloshinskii-Moriya interaction (DMI) may lead to the appearance of Néel skyrmions in ferromagnetic films. These topologically protected structures, whose diameter is as small as a few nanometers, can be nowadays stabilized at room temperature and have been proposed for the realization of artificial magnonic crystals and new spintronic devices, such as racetrack memories. In this perspective, it is of utmost importance to analyze their dynamical properties in the GHz range, i.e. in the operation range of current communication devices. Here we exploited the softwar…
A path method is implemented in order to precisely and generally describe the collapse of isolated skyrmions in a Co/Pt(111) monolayer, on the basis of atomic scale simulations. Two collapse mechanisms with different energy barriers are found. The most obvious path, featuring a homogeneous shrinking gives the largest energy, whereas the lowest energy barrier is shown to comply with the outcome of Langevin dynamics under a destabilizing field of 0.25 T, with a lifetime of 20~ns at around 80~K. For this lowest energy barrier path, skyrmion destabilization occurs much before any topology change, …
We study azimuthal spin-wave (SW) excitations in a circular ferromagnetic nanodot in different inhomogeneous, topologically non-trivial magnetization states, specifically, vortex, Bloch-type skyrmion and Néel-type skyrmion states. Continuous mapping of the SW spectrum between these states is realized with gradual change of the out-of-plane magnetic anisotropy and Dzyaloshinskii-Moriya exchange interaction (DMI). Our study shows lifting of the SW frequencies degeneracy and change in systematics of the frequency levels. The change is induced by a geometrical Berry phase, that is present for the …
Magnetic skyrmions are particle-like chiral spin textures found in a magnetic film with out-of-planeanisotropy and are considered to be potential candidates as information carriers in next generationdata storage devices. Despite intense research into the nature of skyrmions and their dynamic prop-erties, there are several key challenges that still need to be addressed. In particular, the outstandingissues are the reproducible generation, stabilization and confinement of skyrmions at room tempera-ture. Here, we present a method for the capture of nanometer sized magnetic skyrmions in an arrayof…
We resolve the domain-wall structure of the model antiferromagnet $\text{Cr}_2\text{O}_3$ using nanoscale scanning diamond magnetometry and second-harmonic-generation microscopy. We find that the 180$^\circ$ domain walls are predominantly Bloch-like, and can co-exist with Néel walls in crystals with significant in-plane anisotropy. In the latter case, Néel walls that run perpendicular to a magnetic easy axis acquire a well-defined chirality. We further report quantitative measurement of the domain-wall width and surface magnetization. Our results provide fundamental input and an experimental m…
The recent discovery of tunable Dzyaloshinskii-Moriya interactions in layered magnetic materials with perpendicular magnetic anisotropy makes them promising candidates for stabilization and manipulation of skyrmions at elevated temperatures. In this article, we use Monte Carlo simulations to investigate the robustness of skyrmions in these materials against thermal fluctuations and finite-size effects. We find that in confined geometries and at finite temperatures skyrmions are present in a large part of the phase diagram. Moreover, we find that the confined geometry favors the skyrmion over t…
Magnetic skyrmions are knot-like quasiparticles. They are candidates for non-volatile data storage in which information is moved between fixed read and write terminals. Read-out operation of skyrmion-based spintronic devices will rely upon electrical detection of a single magnetic skyrmion within a nanostructure. Here, we present Pt/Co/Ir nanodiscs which support skyrmions at room temperature. We measured the Hall resistivity whilst simultaneously imaging the spin texture using magnetic scanning transmission x-ray microscopy (STXM). The Hall resistivity is correlated to both the presence and si…
Ferromagnets in contact with a topological insulator have become appealing candidates for spintronics due to the presence of Dirac surface states with spin-momentum locking. Because of this bilayer Bi$_2$Se$_3$-EuS structures, for instance, show a finite magnetization at the interface at temperatures well exceeding the Curie temperature of bulk EuS. Here we determine theoretically the effective magnetic interactions at a topological insulator-ferromagnet interface {\it above} the magnetic ordering temperature. We show that by integrating out the Dirac fermion fluctuations an effective Dzyalosh…
Magnetic skyrmions formed at temperatures around room temperature in square-based parallelepiped magnetic FePt nanoparticles with perpendicular magnetocrystalline anisotropy (MCA) were studied during the magnetization reversal using micromagnetic simulations. Finite Differences (FD) method were used for the solution of the Landau-Lifshitz-Gilbert equation. Magnetic configurations exhibiting Néel skyrmionic formations were detected. The magnetic skyrmions can be created in different systems generated by the variation of external field, side length and width of the squared-based parallelepiped m…
Magnetic D-brane solitons: skyrmion strings ending on a Néel wall in chiral magnets
Institute of Contemporary Mathematics, School of Mathematics and Statistics, Henan University（河南大学数学与统计学院当代数学研究所）；Department of Physics, Chemistry and Pharmacy, University of Southern Denmark（南丹麦大学物理、化学与药学系）；International Institute for Sustainability with Knotted Chiral Meta Matter (WPI-SKCM 2 ), Hiroshima University（广岛大学缠绕手性超材料可持续国际研究所）
Recently, magnetic skyrmion has emerged as an active topic of fundamental study and applications in magnetic materials research. Magnetic skyrmions are vortex-like spin excitations with topological protection and therefore are more robust to pinning compared with magnetic domain walls. We employ atomistic simulations to create room-temperature ultra-small Neel skyrmions in amorphous ferrimagnet. The fast propagation and low-dissipation dynamics of ultra-small ferrimagnetic skyrmions make them attractive for utilization as an alternative to domain walls in spin-based memory and logic devices.
Magnetic multilayers are promising tuneable systems for hosting magnetic skyrmions at/above room temperature. Revealing their intriguing switching mechanisms and associated inherent electrical responses are prerequisites for developing skyrmionic devices. In this work, we theoretically demonstrate the annihilation of single skyrmions occurring through a multilayer structure, which is mediated by hopping dynamics of topological hedgehog singularities known as Bloch points. The emerging intralayer dynamics of Bloch points are dominated by the Dzyaloshinskii-Moriya interaction, and their propagat…
It is well established that the spin-orbit interaction in heavy metal/ferromagnet heterostructures leads to a significant interfacial Dzyaloshinskii-Moriya Interaction (DMI) that modifies the internal structure of magnetic domain walls (DWs) to favor Néel over Bloch type configurations. However, the impact of such a transition on the structure and stability of internal DW defects (e.g., vertical Bloch lines) has not yet been explored. We present a combination of analytical and micromagnetic calculations to describe a new type of topological excitation called a DW Skyrmion characterized by a $3…
Bias-field control of the Neel skyrmion nonlinearity in a confined nanostructure
Kotel’nikov Institute of Radio-Engineering and Electronics of RAS（俄罗斯科学院科捷利尼科夫无线电电子研究所）；Moscow Institute of Physics and Technology (National Research University)（莫斯科物理技术学院（国立大学））；Bauman Moscow State Technical University（鲍曼莫斯科国立技术大学）；National Research University Moscow Power Engineering Institute（莫斯科动力学院国立研究大学）
In this letter we calculate the energies corresponding to the different magnetic phases present in a ferromagnetic cylinder by means of analytical calculations. From the comparison of these energies, it is possible to construct magnetic phase diagrams as a function of the uniaxial anisotropy of the sample and the external magnetic field applied. As proof of concept, we analyzed the magnetic phase diagrams for a cobalt dot of 240 nm in diameter and 70 nm in length, with an easy axis parallel to the dot axis, and with a magnetic field applied towards or perpendicular to this axis. From these dia…
Magnetic skyrmionium can be used as a nanometer-scale non-volatile information carrier, which shows no skyrmion Hall effect due to its special structure carrying zero topological charge. Here, we report the static and dynamic properties of an isolated nanoscale skyrmionium in a frustrated magnetic monolayer, where the skyrmionium is stabilized by competing interactions. The frustrated skyrmionium has a size of about $10$ nm, which can be further reduced by tuning perpendicular magnetic anisotropy or magnetic field. It is found that the nanoscale skyrmionium driven by the damping-like spin-orbi…
Skyrmionic textures are being extensively investigated due to the occurrence of novel topological magnetic phenomena and their promising applications in a new generation of spintronic devices that take advantage of the robust topological stability of their spin structures. The development of practical devices relies on a detailed understanding of how skyrmionic structures can be formed, transferred, detected and annihilated. In this work, our considerations go beyond static skyrmions and theoretically show that the formation/annihilation of both skyrmions and antiskyrmions is enabled by the tr…
We investigate the stability of Néel skyrmions against tilted magnetic fields, in polar magnets with uniaxial anisotropy ranging from easy-plane to easy-axis type. We construct the corresponding phase diagrams and investigate the internal structure of skewed skyrmions with displaced cores. We find that moderate easy-plane anisotropy increases the stability range of Néel skyrmions for fields along the symmetry axis, while moderate easy-axis anisotropy enhances their robustness against tilted magnetic fields. We stress that the direction, along which the skyrmion cores are shifted, depends on th…
Magnetic storage based on racetrack memory is very promising for the design of ultra-dense, low-cost and low-power storage technology. Information can be coded in a magnetic region between two domain walls or, as predicted recently, in topological magnetic objects known as skyrmions. Here, we show the technological advantages and limitations of using Bloch and Neel skyrmions manipulated by spin current generated within the ferromagnet or via the spin-Hall effect arising from a non-magnetic heavy metal underlayer. We found that the Neel skyrmion moved by the spin-Hall effect is a very promising…
The intrinsic spin Hall effect (SHE) originates from the topology of the Bloch bands in momentum space. The duality between real space and momentum space calls for a spin Hall effect induced from a real space topology in analogy to the topological Hall effect (THE) of skyrmions. We theoretically demonstrate the topological spin Hall effect (TSHE) in which a pure transverse spin current is generated from a skyrmion spin texture.
Rare earth Fe B permanent magnets are usually used because of their excellent magnetic performance at room temperature. The high price of these elements pushes some researchers to find new alternatives. From rare earth elements cerium (Ce) is considered as the most abundant and cheap, therefore, the interest was focused to study the properties of alloys based on this element in recent years. In this work, we investigate the magnetization behavior of CeFeB nanodisks in presence of Dzyaloshinskii Moriya interaction. We show that topological structures, Neel skyrmions, in particular, could be nuc…
Twisted skyrmions, whose helicity angles are different from that of Bloch skyrmions and Néel skyrmions, have already been demonstrated in experiments recently. In this work, we first contrast the magnetic structure and origin of the twisted skyrmion with other three types of skyrmion including Bloch skyrmion, Néel skyrmion and antiskyrmion. Following, we investigate the dynamics of twisted skyrmions driven by the spin transfer toque (STT) and the spin Hall effect (SHE) by using micromagnetic simulations. It is found that the spin Hall angle of the twisted skyrmion is related to the dissipative…
We consider a magnetic skyrmion crystal formed at the surface of a topological insulator. Incorporating the exchange interaction between the helical Dirac surface states and the periodic Néel or Bloch skyrmion texture, we obtain the resulting electronic band structure and discuss the constraints that symmetries impose on the energies and Berry curvature. We find substantive qualitative differences between the Néel and Bloch cases, with the latter generically permitting a multiband low energy tight-binding representation whose parameters are tightly constrained by symmetries. We explicitly comp…
Magnetic skyrmions are topologically non-trivial spin textures of potential interest for future information storage applications, and for such purposes, the control and understanding of single skyrmion creation is required. A scheme is analyzed to create single Néel-type and Bloch-type skyrmions in helimagnetic thin films utilizing the dynamical excitations induced by the Oersted field and the spin transfer torque given by a vertically injected spin-polarized current. A topological charge analysis using a lattice version of the topological charge provides insight into the locally triggered tra…
When magnetic skyrmions move under spin orbit torque in magnetic nanowires, they experience a skyrmion Hall effect, which pushes them towards the nanowire edge where they risk being annihilated; this puts an upper limit on how fast they can be driven. However, the same magnetic multilayer harboring skyrmions can sustain a Néel-type strip domain wall along the nanowire length, potentially keeping the skyrmions separated from the edge. Here we study the interplay between current driven skyrmions and domain walls and find that they increase the annihilation current and allow the skyrmions to move…
Chiral spin textures are fundamentally interesting, with promise for device applications. Stabilizing chirality is conventionally achieved by introducing Dzyaloshinskii-Moriya interaction (DMI) in asymmetric multilayers where the thickness of each layer is at least a few monolayers. Here we report an ultrasensitive chirality switching in (Ni/Co)n multilayer induced by capping with only 0.22 monolayer of Pd. Using spin-polarized low-energy electron microscopy, we monitor the gradual evolution of domain walls from left-handed to right-handed Neel walls and quantify the DMI induced by the Pd capp…
We study the quench dynamics of non-Hermitian topological models with non-Hermitian skin effects. Adopting the non-Bloch band theory and projecting quench dynamics onto the generalized Brillouin zone, we find that emergent topological structures, in the form of dynamic skyrmions, exist in the generalized momentum-time domain, and are correlated with the non-Bloch topological invariants of the static Hamiltonians. The skyrmion structures anchor on the fixed points of dynamics whose existence are conditional on the coincidence of generalized Brillouin zones of the pre- and post-quench Hamiltonia…
