We study the low-energy properties and, in particular, the magnetization process of a spin-1/2 Heisenberg $J_1-J_2$ sawtooth and frustrated chain (also known as zig-zag ladder) with a spatially anisotropic $g$-factor. We treat the problem both analytically and numerically while keeping the $J_2/J_1$ ratio generic. Numerically, we use complete and Lanczos diagonalization as well as the infinite time-evolving block decimation (iTEBD) method. Analytically we employ (non-)Abelian bosonization. Additionally for the sawtooth chain, we provide an analytical description in terms of flat bands and localized magnons. By considering a specific pattern for the $g$-factor anisotropy for both models, we show that a small anisotropy significantly enhances a magnetization plateau at half saturation. For the magnetization of the frustrated chain, we show the destruction of the $1/3$ of the full saturation plateau in favor of the creation of a plateau at half-saturation. For large anisotropies, the existence of an additional plateau at zero magnetization is possible. Here and at higher magnetic fields, the system is locked in the half-saturation plateau, never reaching full saturation.
A simple model consisting of three distinct dimer sublattices is proposed to describe the magnetism of NH4CuCl3. It explains the occurrence of magnetization plateaus only at 1/4 and 3/4 of the saturation magnetization. The field dependence of the excitation modes observed by ESR measurements is also explained by the model. The model predicts that the magnetization plateaus should disappear under high pressure.
The dimer-plaquette chain undergoes a first order transition driven by frustration to an orthogonal dimer ground state. We analyze the magnetization curve in this orthogonal dimer regime. Besides of the recently found magnetization plateaus at m=1/4 and the m=1/2 we find an infinite sequence of plateaus between m=1/4 and m=1/2. These additional plateaus belong to magnetizations m(n)=n/(2n+2), where n is a positive integer number.
The low temperature magnetization process of antiferromagnetic spin-S chains doped with mobile spin-(S-1/2) carriers is studied in an exactly solvable model. For sufficiently high magnetic fields the system is in a metallic phase with a finite gap for magnetic excitations. In this phase which exists for a large range of carrier concentrations x the zero temperature magnetization is determined by x alone. This leads to plateaus in the magnetization curve at a tunable fraction of the saturation magnetization. The critical behaviour at the edges of these plateaus is studied in detail.
We study the magnetization process of the $S=1$ Heisenberg model on a two-leg ladder with farther neighbor spin-exchange interaction. We consider the interaction that couples up to the next-nearest neighbor rungs and find an exactly solvable regime where the ground states become product states. The next-nearest neighbor interaction tends to stabilize magnetization plateaus at multiples of 1/6. In most of the exactly solvable regime, a single magnetization curve shows two series of plateaus with different periodicities.
The phenomenon of magnetization plateaus in antiferromagnets under magnetic field has always been an important topic in magnetism. We propose to probe the elusive physics of plateaus in 2-d by considering hole-doped antiferromagnet and studying the signatures of magnetization plateaus in terms of the properties of holes, coupled to an effective gauge field generated by the spin sector. The latter mediates interaction between the holes, found to be algebraically decaying long-ranged with both Coulombic and dipolar forms outside plateau and short-ranged (local) inside plateau. The resulting hole…
Magnetization plateaus in quantum spin systems emerges in two-dimensional frustrated systems such as kagome lattice. The spin-1/2 antiferromagnetic Heisenberg model on square-kagome lattice is also appropriate for the study of magnetization plateau. Motivated by recent experimental finding of such a square-kagome lattice with nonequivalent three bonds, we investigate the phase diagrams and magnetization plateaus of the lattice by the exact diagonalization method. In addition to previously reported the 1/3 and 2/3 plateaus in the model with two equivalent bonds, we find a new 2/3 plateau whose …
We show that the critical fields of the magnetization plateaus of the Shastry-Sutherland model decrease significantly upon increasing the ratio of inter- to intra-dimer coupling, and accordingly that the magnetization plateaus of SrCu_2(BO_3)_2 shift to lower field under pressure, making the first two plateaus at 1/8 and 2/15 potentially accessible to neutron scattering experiments. These conclusions are based on the derivation of an effective classical model of interacting pinwheel-shaped spin-2 bound states using a combination of perturbative and graph-based continuous unitary transformation…
Magnetic susceptibility and the magnetization process have been measured in \green polycrystal. In this compound, the magnetic manganese ion exists as Mn$^{5+}$ in a tetrahedral environment, and thus the magnetic interaction can be described by an S=1 Heisenberg model. The ground state was found to be a spin singlet with an excitation gap $Δ/k_{\rm B}=11.2$ K. Magnetization plateaus were observed at zero and at half of the saturation magnetization. These results indicate that the present system can be represented by a coupled antiferromagnetic dimer model.
Magnetization plateaus are some of the most striking manifestations of frustration in low-dimensional spin systems. We present numerical studies of magnetization plateaus in the fascinating spin-1/2 skewed ladder system obtained by alternately fusing five- and seven-membered rings. This system exhibits three significant plateaus at $m = 1/4$, $1/2$ and $3/4$, consistent with the Oshikawa-Yamanaka-Affleck condition. Our numerical as well as perturbative analysis shows that the ground state can be approximated by three weakly coupled singlet dimers and two free spins, in the absence of a magneti…
The two-dimensional spin-gap system ${\rm SrCu_2(BO_3)_2}$ shows unique physical properties due to the low-dimensionality character and the strong quantum fluctuations. Experimentally, 1/8-, 1/4-, and 1/3-plateaus have been observed in the magnetization curve under magnetic fields up to 70 Tesla, and the 1/2-plateau is expected to be stabilized at higher magnetic fields. We argue that spin-lattice effects are necessary to describe the superstructures at the plateaus, and we propose a simple microscopic model of spins interacting adiabatically with the lattice to reproduce the main features of …
We present a unified approach to the problem of degeneracy lifting in geometrically frustrated magnets with and without an external field. The method treats fluctuations around a classical spin configuration in terms of a real-space perturbation expansion. We calculate two lowest-order contributions for the Heisenberg spin Hamiltonian and use them to study the magnetization processes of spin-$S$ triangular and kagomé antiferromagnets.
We study an anisotropic Heisenberg antiferromagnet with ferromagnetic transverse spin exchange using exact quantum Monte Carlo methods. Such a model is relevant to a class of rare earth tetraboride materials that display a range of magnetization plateaus under applied magnetic field. The layered arrangement of magnetic ions in these materials is topologically equivalent to the Shastry-Sutherland lattice. In this frustrated geometry, we study the interplay of next-nearest neighbor interactions in stabilizing a plateau at half the saturation magnetization (or 1/2 plateau). We also show hysteresi…
Magnetization plateaus in the Shastry-Sutherland model for ${\rm SrCu_2(BO_3)_2}$ are studied by the perturbation expansion method. The fourth-order effective Hamiltonian which describes the dynamics of triplet dimers (TD's) with $S^{\rm tot}_z=1$ in the singlet sea is derived and then partially diagonalized for the space that consists of the TD configurations with the lowest second-order energy. The fourth-order terms are treated within a low-density approximation. Our procedure makes clear how TD interactions are responsible for the formation of magnetization plateaus. Particularly, the 1/4-…
We discuss zero-temperature quantum spin chains in a uniform magnetic field, with axial symmetry. For integer or half-integer spin, $S$, the magnetization curve can have plateaus and we argue that the magnetization per site $m$ is topologically quantized as $q (S - m)= integer$ at the plateaus, where $q$ is the period of the groundstate. We also discuss conditions for the presence of the plateau at those quantized values. For $S=3/2$ and $m=1/2$, we study several models and find two distinct types of massive phases at the plateau. One of them is argued to be a ``Haldane gap phase'' for half-in…
We study the one-dimensional spin-1/2 model with nearest and next-to-nearest-neighbor couplings exposed to a homogeneous magnetic field $h_{3}$ and a dimer field with period $q$ and strength $δ$. The latter generates a magnetization plateau at $M=(1-q/π)/2$, which evolves with strength $δ$ of the perturbation as $δ^ε$, where $ε=ε(h_{3},α)$ is related to the $η$-exponent which describes the critical behavior of the dimer structure factor, if the perturbation is switched of ($δ=0$). We also discuss the appearance of magnetization plateaus in ladder systems with $l$ legs.
We show the importance of both strong frustration and spin-lattice coupling for the stabilization of magnetization plateaus in translationally invariant two-dimensional systems. We consider a frustrated spin-1/2 Heisenberg model coupled to adiabatic phonons under an external magnetic field. At zero magnetization, simple structures with two or at most four spins per unit cell are stabilized, forming dimers or $2 \times 2$ plaquettes, respectively. A much richer scenario is found in the case of magnetization $m=1/2$, where larger unit cells are formed with non-trivial spin textures and an analog…
Using infinite projected entangled-pair states (iPEPS), we show that the Shastry-Sutherland model in an external magnetic field has low-magnetization plateaus which, in contrast to previous predictions, correspond to crystals of bound states of triplets, and {\it not} to crystals of triplets. The first sizable plateaus appear at magnetization 1/8, 2/15 and 1/6, in agreement with experiments on the orthogonal-dimer antiferromagnet SrCu$_2$(BO$_3$)$_2$, and they can be naturally understood as regular patterns of bound states, including the intriguing 2/15 one. We also show that, even in a confin…
Spin-1/2 Heisenberg model on kagome lattice is a typical frustrated quantum spin system. A basic structure of kagome lattice is also present in kagome-strip lattice in one dimension, where a similar type of frustration is expected. We thus study the magnetization plateaus of the spin-1/2 Heisenberg model on a kagome-strip chain with three-independent antiferromagnetic exchange interactions by the density-matrix renormalization group method. In a certain range of exchange parameters, we find twelve kinds of magnetization plateaus, nine of which have magnetic structures breaking either translati…
A spin-1/2 Heisenberg model on honeycomb lattice is investigated by doing triplon analysis and quantum Monte Carlo calculations. This model, inspired by Cu$_2$(pymca)$_3$(ClO$_4$), has three different antiferromagnetic exchange interactions ($J_A$, $J_B$, $J_C$) on three different sets of nearest-neighbour bonds which form a kagome superlattice. While the model is bipartite and unfrustrated, its quantum phase diagram is found to be dominated by a quantum paramagnetic phase that is best described as a spin-gapped hexagonal-singlet state. The Néel antiferromagnetic order survives only in a small…
We present a single-crystal neutron diffraction study on the Shastry-Sutherland lattice system TbB$_4$ at zero magnetic field and under pulsed high magnetic fields up to 35 T applied along the crystallographic $c$ axis. While our results confirm the magnetic structures at zero-field as well as those at the half- and full-magnetization plateaus, they offer new insight into the $\frac{2}{9}$- and $\frac{1}{3}$-magnetization plateaus observed in this system. A stripe model of polarized 4-spin-plaquettes whose stripe density proportionally increases with the macroscopic magnetization is in full ag…
The magnetization of two spin-1/2 kagome antiferromagnets, volborthite and vesignieite, has been measured in pulsed magnetic fields up to 68 T. A magnetization plateau is observed for each compound near the highest magnetic field. Magnetizations at saturation are approximately equal to 0.40Ms for both compounds, where Ms is the fully saturated magnetization, irrespective of a difference in the distortion of the kagome lattice between the two compounds. It should be noted that these values of magnetizations are significantly larger than Ms/3 predicted theoretically for the one-third magnetizati…
I study a spin system consisting of strongly coupled dimers which are in turn weakly coupled in a plane by zigzag interactions. The model can be viewed as the strong-coupling limit of a two-dimensional zigzag chain structure typical, e.g., for the $(ac)$-planes of KCuCl_3. It is shown that the magnetization curve in this model has plateaus at 1/3 and 2/3 of the saturation magnetization, and an additional plateau at 1/2 can appear in a certain range of the model parameters; the critical fields are calculated perturbatively. It is argued that for the three-dimensional lattice structure of the KC…
Pinwheel-shaped bound triplet pairs in the magnetization plateaus of SrCu$_2$(BO$_3$)$_2$
Laboratoire National des Champs Magnétiques Intenses, LNCMI-CNRS(法国国家强磁场实验室);University of Amsterdam(阿姆斯特丹大学);École Polytechnique Fédérale de Lausanne (EPFL)(洛桑联邦理工学院);Kyoto University(京都大学);University of Tokyo(东京大学)
We study the ground state of $S = 1/2$ Heisenberg model on the checkerboard lattice in a magnetic field by the density matrix renormalization group (DMRG) method with the sine-square deformation. We obtain magnetization plateaus at $M/M_{\rm sat}=$0, 1/4, 3/8, 1/2, and 3/4 where $M_{\rm sat}$ is the saturated magnetization. The obtained 3/4 plateau state is consistent with the exact result, and the 1/2 plateau is found to have a four-spin resonating loop structure similar to the six-spin loop structure of the 1/3 plateau of the kagome lattice. Different four-spin loop structures are obtained i…
We generalize a class of Heisenberg antiferromagnets in one, two and three dimensions, which have been shown to exhibit magnetization plateaus for spin-1/2. In a certain parameter range of the general model, which is formally defined in D dimensions, we obtain the exact ground state(s) in the presence of an external magnetic field for arbitrary values of spin. In this range, the magnetization remains a constant as a function of the external field, except at some special values of the field where there is a jump from one plateau to the next. The plateaus are formed at certain specific fractions…
We study the spin-3/2 Heisenberg model including easy-plane and exchange anisotropies in one and two dimensions. In the Ising limit, when the off-diagonal exchange interaction J is zero, the phase diagram in magnetic field is characterized by magnetization plateaus that are either translationally invariant or have a two-sublattice order, with phase boundaries that are macroscopically degenerate. Using a site factorized variational wave function and perturbational expansion around the Ising limit, we find that superfluid and supersolid phases emerge between the plateaus for small finite values …
Despite the absence of an apparent triangular pattern in the crystal structure, we observe unusually well pronounced 1/3 magnetization plateaus in the quasi one-dimensional Ising spin chain compound CoGeO$_3$ which belongs to the class of pyroxene minerals. We succeeded in uncovering the detailed microscopic spin structure of the 1/3 magnetization plateau phase by means of neutron diffraction. We observed changes of the initial antiferromagnetic zero-field spin structure that are resembling a regular formation of antiferromagnetic "domain wall boundaries", resulting in a kind of modulated magn…
Unconventional features of the magnetization curve at zero temperature such as plateaus or jumps are a hallmark of frustrated spin systems. Very little is known about their behavior at non-zero temperatures. Here we investigate the temperature dependence of the magnetization curve of the kagome lattice antiferromagnet in particular at 1/3 of the saturation magnetization for large lattice sizes of up to N=48 spins. We discuss the phenomenon of asymmetric melting and trace it back to a combined effect of unbalanced magnetization steps on either side of the investigated plateau as well as on the …
We study kagome lattice antiferromagnets where the effects of easy axis single-ion anisotropy ($D$) dominates over the Heisenberg exchange $J$. For $S \ge 3/2$, virtual quantum fluctuations help lift the extensive classical degeneracy. We demonstrate the presence of a one-third magnetization plateau for a broad range of magnetic fields $J^3/D^2 \lesssim B \lesssim JS$ along the easy axis. The fully equilibriated system at low temperature on this plateau develops an unusual {\em nematic} order that breaks sublattice rotation symmetry but not translation symmetry--however, extremely slow dynamic…
Using the density matrix renormalization group technique we investigate the low-energy properties and the magnetization plateau behavior in a 2-leg mixed spin ladder consisting of a spin-1/2 chain coupled with a spin-1 chain. The calculated results show that the system is in the same universality class as the spin-3/2 chain when the interchain coupling is strongly ferromagnetic, but the similarity between the two systems is less clear under other coupling conditions. We have identified two types of magnetization plateau phases. The calculation of the magnetization distribution on the spin-1/2 …
We investigate the properties in finite magnetic field of an extended anisotropic XXZ spin-1/2 model on the Kagome lattice, originally introduced by Balents, Fisher, and Girvin [Phys. Rev. B, 65, 224412 (2002)]. The magnetization curve displays plateaus at magnetization m=1/6 and 1/3 when the anisotropy is large. Using low-energy effective constrained models (quantum loop and quantum dimer models), we discuss the nature of the plateau phases, found to be crystals that break discrete rotation and/or translation symmetries. Large-scale quantum Monte-Carlo simulations were carried out in particul…
We unveil nontrivial topological properties of zero-temperature magnetization plateau states in periodically modulated quantum spin chains under a uniform magnetic field. As positions of plateaus are uniquely determined by the modulation period of exchange couplings, we find that the topologically nontrivial plateau state can be characterized by a nonzero integer Chern number and has nontrivial edge excitations. Our study clarifies the topological origin of the well-known phenomena of quantized magnetization plateaus in one-dimensional quantum spin systems and relates the plateau state to the …
Variational study of the magnetization plateaus in the spin-1/2 kagome Heisenberg antiferromagnet: An approach from vision transformer neural quantum states
Université de Toulouse, CNRS, Laboratoire de Physique Théorique(图卢兹大学,法国国家科学研究中心,理论物理实验室)
We study the magnetization process in two-dimensional S=1/2 spin systems, to discuss the appearance of a plateau structure. The following three cases are considered: (1) the Heisenberg antiferromagnet and multiple-spin exchange model on the triangular lattice, (2) Shastry-Sutherland type lattice, [which is a possible model for SrCu2(BO3)2,] (3) 1/5-depleted lattice (for CaV4O9). We find in these systems that magnetization plateaus can appear owing to a transition from superfluid to a Mott insulator of magnetic excitations. The plateau states have CDW order of the excitations. The magnetization…
We investigate the effect of spin-lattice coupling (SLC) on the magnetic properties of the classical kagome-lattice Heisenberg antiferromagnet (KHAF) using improved Monte Carlo updates. The lattice modes are represented by Einstein site phonons, which introduce effective further-neighbor spin interactions in addition to the nearest-neighbor biquadratic interactions. In the weak SLC, the macroscopically degenerate coplanar ground state remains at zero field, while a $\sqrt{3} \times \sqrt{3}$ ordered phase accompanied by a 1/3-magnetization plateau appears in external magnetic fields. In the st…
Uncovering topologically nontrivial states in nature is an intriguing and important issue in recent years. While most studies are based on the topological band insulators, the topological state in strongly correlated low-dimensional systems has not been extensively explored due to the failure of direct explanation from the topological band insulator theory on such systems and the origin of the topological property is unclear. Here we report the theoretical discovery of strongly correlated topological states in quasi-periodic Heisenberg spin chain systems corresponding to a series of incommensu…
We study the behavior of magnetization curve as a function of magnetic field in the immediate vicinity of the magnetization plateaus of 1D electron systems within the bosonization formalism. First we discuss the plateau that is formed at the saturation magnetization of 1D electron system. Interactions between electrons we treat in the lowest order of perturbation. We show that for isolated systems, where total number of electrons is not allowed to vary, magnetic susceptibility stays always finite away of half filling. Similar statement holds for many other magnetization plateaus supporting non…
The antiferromagnetic Heisenberg model on the frustrated Shastry-Sutherland lattice is studied by a mapping onto spinless fermions carrying one quantum of statistical flux. Using a mean-field approximation these fermions populate the bands of a generalized Hofstadter problem. Their filling leads to the magnetization curve. For SrCu_2(BO_3)_2 we reproduce plateaus at 1/3 and 1/4 of the saturation moment and predict a new one at 1/2. Gaussian fluctuations are shown to be massive at these plateau values.
Ground-state phase diagrams and magnetization curves of a spin-1 Heisenberg diamond cluster with two different coupling constants and uniaxial single-ion anisotropy are investigated in a presence of the external magnetic field with the help of exact diagonalization methods. It is shown that the spin-1 Heisenberg diamond cluster exhibits several remarkable quantum ground states, which are manifested in zero- and low-temperature magnetization curves as intermediate plateaus at one-quarter, one-half and three-quarters of the saturation magnetization. It is found that the width of the fractional m…
We investigate the phase diagram of TmB4, an Ising magnet on a frustrated Shastry-Sutherland lattice by neutron diffraction and magnetization experiments. At low temperature we find Neel order at low field, ferrimagnetic order at high field and an intermediate phase with magnetization plateaus at fractional values M/Msat = 1/7, 1/8, 1/9 ... and spatial stripe structures. Using an effective S = 1/2 model and its equivalent two-dimensional (2D) fermion gas we suggest that the magnetic properties of TmB4 are related to the fractional quantum Hall effect of a 2D electron gas.
A coupled spin-electron chain composed of localized Ising spins and mobile electrons is exactly solved in an external magnetic field within the transfer-matrix method. The ground-state phase diagram involves in total seven different ground states, which differ in the number of mobile electrons per unit cell and the respective spin arrangements. A rigorous analysis of the low-temperature magnetization process reveals doping-dependent magnetization plateaus, which may be tuned through the density of mobile electrons. It is demonstrated that the fractional value of the electron density is respons…
Plateaus can be observed in the zero-temperature magnetization curve of quantum spin systems at rational values of the magnetization. In one dimension, the appearance of a plateau is controlled by a quantization condition for the magnetization which involves the length of the local spin and the volume of a translational unit cell of the ground state. We discuss examples of geometrically frustrated quantum spin systems with large (in general unbounded) periodicities of spontaneous breaking of translational symmetry in the ground state. In two dimensions, we discuss the square, triangular and Ka…
This short note documents some of the pyrochlore magnetization plateaus resulting from the arguments of Pal & Lal that were not mentioned in arxiv:1902.06475v1. These are (layered) "Kagome"-like plateaus that are commensurate with the pyrochlore lattice, including an exact wavefunction for the $\frac{m}{m_s} = \frac{5}{6}$ plateau state.
We present a simple model for a description of magnetization processes in rare-earth tetraborides. The model is based on the coexistence of two subsystems, and namely, the spin subsystem described by the Ising model and the electronic subsystem described by the Falicov-Kimball model on the Shastry-Sutherland lattice (SSL). Moreover, both subsystems are coupled by the anisotropic spin-dependent interaction of the Ising type. We have found, that the switching on the spin-dependent interaction ($J_z$) between the electron and spin subsystems and taking into account the electron hopping on the nea…
$α$-CoV$_{2}$O$_{6}$ consists of $j_{\mathrm{eff}}={1 \over 2}$ Ising spins located on an anisotropic triangular motif with magnetization plateaus in an applied field. We combine neutron diffraction with low temperature magnetization to investigate the magnetic periodicity in the vicinity of these plateaus. We find these steps to be characterized by metastable and spatially short-range ($ξ\sim$ 10 $Å$) magnetic correlations with antiphase boundaries defining a local periodicity of $\langle \hat{T}^{2} \rangle =\ \uparrow \downarrow$ to $\langle \hat{T}^{3} \rangle =\ \uparrow \uparrow \downarr…
We examine the general features of the non-commutativity of the magnetization operator and Hamiltonian for the small quantum spin clusters. The source of this non-commutativity can be a difference in the Landé g-factors for different spins in the cluster, XY-anisotropy in the exchange interaction and the presence of the Dzyaloshinskii-Moriya term in the direction different for the direction of the magnetic field. As a result, a zero-temperature magnetization curve for the small spin clusters mimics that for the macroscopic systems with the band(s) of magnetic excitations, i.e. for the given ei…
We consider insulating states of spin-one bosons in optical lattices in the presence of a weak magnetic field. For the states with more than one atom per lattice site we find a series of quantum phase transitions between states with fixed magnetization and a canted nematic phase. In the presence of a global confining potential, this unusual phase diagram leads to several novel phenomena, including formation of magnetization plateaus. We discuss how these effects can be observed using spatially resolved density measurements.
We study the Heisenberg antiferromagnet on the Shastry-Sutherland lattice under magnetic fields, to clarify the magnetic properties of SrCu_2(BO_3)_2. Treating magnetic excitations promoted by the field as Bose particles and using strong coupling expansion, we derive an effective Hamiltonian for the effective magnetic particles. Anisotropic repulsive interactions between effective particles induce `insulating' states with a stripe SDW structure at magnetization m/m_{sat}=1/3 and a checkerboard structure at 1/2, and thereby form magnetization plateaus. Supersolid phases appear around insulating…
The magnetic phase diagram of a plaquette dimerized antiferromagnetic system is studied by using a combination of numerical and analytical techniques. For the strongly frustrated regime, series expansions and bond operators techniques are employed to analyze zero magnetization plateau, whereas low energy effective models are used to study the complete magnetization process. The interplay between frustration and dimerization gives rise to a rich plateaus structure that is captured by effective models and corroborated by numerical density matrix renormalization group simulations, in particular t…
A complete and exact solution of the ground-state problem for the Ising model on the Shastry-Sutherland lattice in the applied magnetic field is found. The magnetization plateau at the one third of the saturation value is shown to be the only possible fractional plateau in this model. However, stripe magnetic structures with magnetization 1/2 and $1/n$ ($n > 3$), observed in the rare-earth tetraborides RB$_4$, occur at the boundaries of the three-dimensional regions of the ground-state phase diagram. These structures give rise to new magnetization plateaus if interactions of longer ranges are …