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arXiv 2405.09280cond-mat.str-el
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具有锯齿形自旋链的准一维伊辛磁体$\boldsymbol{TbTi_3Bi_4}$中的1/3及其他磁化平台

1/3 and other magnetization plateaus in a quasi-one-dimensional Ising magnet $\mathbf{TbTi_3Bi_4}$ with zigzag spin chain

Kaizhen Guo, Zeyu Ma, Hongxiong Liu, Ziyang Wu, Junfeng Wang, Youguo Shi, Yuan Li, Shuang Jia

AI总结:

本研究针对新合成的准一维伊辛磁体$TbTi_3Bi_4$单晶,探究其磁学性质,发现其因晶场效应具有强易轴各向异性,在20.4 K下反铁磁有序,沿链向加场会出现1/3等多个磁化平台与变磁转变,还构建了相图明确阻挫引发的复杂磁结构。

摘要:

我们报道了新合成的$\boldsymbol{TbTi_3Bi_4}$单晶的磁学性质,其晶体结构以铽基锯齿链与钛基笼目晶格的堆叠为显著特征。由于晶场效应使$\boldsymbol{Tb^{3+}}$磁矩沿锯齿链方向排列,该化合物表现出极强的易轴磁各向异性。受强单离子各向异性与多重磁相互作用的共同影响,$\boldsymbol{TbTi_3Bi_4}$表现为准一维伊辛磁体,在$T_\boldsymbol{N}$=20.4 K处存在显著的反铁磁有序。当沿锯齿链方向施加磁场时,在1/3磁化平台与其他磁化平台之间会发生多次变磁转变。我们构建了磁场-温度相图,并确定了由阻挫导致的复杂磁结构。

英文摘要:

We report the magnetic properties of newly synthesized, single crystals of $\mathrm{TbTi_3Bi_4}$ whose crystal structure is highlighted by the stacking of terbium-based zigzag chains and titanium-based kagome lattices. This compound demonstrates extreme easy-axis magnetic anisotropy due to the crystalline-electric-field effect which aligns the $\mathrm{Tb^{3+}}$ moments along the zigzag chain direction. As the result of the strong single-ion anisotropy and multiple magnetic interactions, $\mathrm{TbTi_3Bi_4}$ behaves as a quasi-one-dimensional Ising magnet with a remarkable antiferromagnetic ordering at $T_\mathrm{N}$ = 20.4 K. When a magnetic field is applied along the direction of the zigzag chain, multiple meta-magnetic transitions occur between 1/3 and other magnetization plateaus. We have created a field-temperature phase diagram and mapped out the complex magnetic structures resulting from frustration.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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