We present a theory of radio-frequency spectroscopy of impurities interacting with a quantum gas at finite temperature. By working in the canonical ensemble of a single impurity, we show that the impurity spectral response is directly connected to the finite-temperature equation of state (free energy) of the impurity. We consider two different response protocols: "injection", where the impurity is introduced into the medium from an initially non-interacting state; and "ejection", where the impurity is ejected from an initially interacting state with the medium. We show that there is a simple mapping between injection and ejection spectra, which is connected to the detailed balance condition in thermal equilibrium. To illustrate the power of our approach, we specialize to the case of the Fermi polaron, corresponding to an impurity atom that is immersed in a non-interacting Fermi gas. For a mobile impurity with a mass equal to the fermion mass, we employ a finite-temperature variational approach to obtain the impurity spectral response. We find a striking non-monotonic dependence on temperature in the impurity free energy, the contact, and the radio-frequency spectra. For the case of an infinitely heavy Fermi polaron, we derive exact results for the finite-temperature free energy, thus generalizing Fumi's theorem to arbitrary temperature. We also determine the exact dynamics of the contact after a quench of the impurity-fermion interactions. Finally, we show that the injection and ejection spectra obtained from the variational approach compare well with the exact spectra, thus demonstrating the accuracy of our approximate method.
By using two-fluid model the effect of impurities on the transition temperature of a dipolar trapped Bose gas is investigated. By treating Gaussian spatial correlation for impurities from the interaction modified spectra of the system, the formula for the shift of transition temperature is derived. The shift of the transition temperature contains essentially three contributions due to contact, dipole-dipole and impurity interactions. Applying our results to Dipolar Bose gases show that the shift of the transition temperature due to impurities could be measured for isotropic trap (dipole-dipole…
We propose a minimal model to study the real-time dynamics of a $\mathbb{Z}_2$ lattice gauge theory coupled to fermionic matter in a cold atom quantum simulator setup. We show that dynamical correlators of the gauge fields can be measured in experiments studying the time-evolution of two pairs of impurities, and suggest the protocol for implementing the model in cold atom experiments. Further, we discuss a number of unexpected features found in the integrable limit of the model, as well as its extensions to a non-integrable case. A potential experimental implementation of our model in the latt…
We scrutinize the hydrodynamic approach for calculating dynamical correlations in one-dimensional superfluids near integrability and calculate the characteristic time scale τ beyond which this approach is valid. For time scales shorter than τ hydrodynamics fails and we develop an approach based on kinetics of fermionic quasiparticles described as mobile impurities. New universal results for the dynamical structure factor relevant to experiments in ultracold atomic gases are obtained.
We theoretically study the normal phase properties of strongly interacting two-component Fermi gases in two spatial dimensions. In the limit of weak attraction, we find that the gas can be described in terms of effective polarons. As the attraction between fermions increases, we find a crossover from a gas of non-interacting polarons to a pseudogap regime. We investigate how this crossover is manifested in the radio-frequency (rf) spectroscopy. Our findings qualitatively explain the differences in the recent rf spectroscopy measurements of two-dimensional Fermi gases [Sommer et al., Phys. Rev.…
We propose to use the energy absorption spectroscopy to measure the kinetic coefficients of unitary Fermi gases in a uniform potential. We show that in our scheme, the energy absorption spectrum is proportional to the dynamic structure factor of the system. The profile of the spectrum depends on the shear viscosity $η$, the thermal conductivity $κ$ and the superfluid bulk viscosity $ξ_3$. We show that extraction of these coefficients from the spectrum is achievable in present experiments.
We present a semiclassical treatment of a fermionic impurity coupled to Bogolyubov modes of a BEC. In the lowest order approximation we find a full solution of an initial value problem, which turns out to behave differently in the sub- and supersonic regimes. While in the former case no impurity deceleration is observed, in the latter case non-Markovian dissipation effects kick in resulting in slowing down of the fermion. Although this scenario is compatible with the one offered by an elementary field theoretical picture at weak coupling, the details of the dynamics turn out to be completely d…
We study a one-dimensional interacting quantum liquid hosting a pair of mobile impurities causing backscattering. We determine the effective retarded interaction between the two impurities mediated by the liquid. We show that for strong backscattering this interaction gives rise to resonances and antiresonances in the finite-frequency mobility of the impurity pair. At the antiresonances, the two impurities remain at rest even when driven by a (small) external force. At the resonances, their synchronous motion follows the external drive in phase and reaches maximum amplitude. Using a perturbati…
In several settings of physics and chemistry one has to deal with molecules interacting with some kind of an external environment, be it a gas, a solution, or a crystal surface. Understanding molecular processes in the presence of such a many-particle bath is inherently challenging, and usually requires large-scale numerical computations. Here, we present an alternative approach to the problem - that based on the notion of the angulon quasiparticle. We show that molecules rotating inside superfluid helium nanodroplets and Bose-Einstein Condensates form angulons, and therefore can be described …
We investigate theoretically momentum-resolved radio-frequency (rf) spectroscopy of a noninteracting atomic Fermi gas in a spin-orbit coupled lattice. This lattice configuration has been recently created at MIT [Cheuk et al., arXiv:1205.3483] for 6Li atoms, by coupling the two hyperfine spin-states with a pair of Raman laser beams and additional rf coupling. Here, we show that momentum-resolved rf spectroscopy can measure single-particle energies and eigenstates and therefore resolve the band structure of the spin-orbit coupled lattice. In our calculations, we take into account the effects of …
A few years ago, flow equations were introduced as a technique for calculating the ground-state energies of cold Bose gases with and without impurities. In this paper, we extend this approach to compute observables other than the energy. As an example, we calculate the densities, and phase fluctuations of one-dimensional Bose gases with one and two impurities. For a single mobile impurity, we use flow equations to validate the mean-field results obtained upon the Lee-Low-Pines transformation. We show that the mean-field approximation is accurate for all values of the boson-impurity interaction…
This article provides a brief review of how various spectroscopies have been used to investitage many-body quantum phenomena in the context of ultracold Fermi gases. In particular, work done with RF spectroscopy, Bragg spectroscopy and lattice modulation spectroscopy is considered. The theoretical basis of these spectroscopies, namely linear response theory in the many-body quantum physics context is briefly presented. Experiments related to the BCS-BEC crossover, imbalanced Fermi gases, polarons, possible pseudogap and Fermi liquid behaviour and measuring the contact are discussed. Remaining …
Quantum Impurities as Probes of Finite-Temperature Fluctuations in Two-Dimensional Bose Gases
International School for Advanced Studies (SISSA)（高等研究院）；CINECA Consorzio Interuniversitario（意大利大学联合中心）；School of Science and Technology, Physics Division, Università di Camerino（卡梅里诺大学理学院物理系）；Pitaevskii BEC Center, CNR-INO, Trento（特伦托CNR-INO皮塔耶夫斯基玻色-爱因斯坦凝聚中心）；INFN, Sezione di Perugia（佩鲁贾国家核物理研究所）；School of Pharmacy, Physics Unit, University of Camerino（卡梅里诺大学药学院物理组）；Dipartimento di Fisica, Università di Trieste（的里雅斯特大学物理系）；Istituto Nazionale di Fisica Nucleare (INFN), Trieste Section（的里雅斯特国家核物理研究所）
Motivated by the recent efforts in creating the flat band in ultracold atomic systems, we investigate how to probe the flat band in an optically-trapped spin-orbital coupled Bose-Einstein condensate using Bragg spectroscopy. We have found that the excitation spectrum and the dynamic structure factor of the condensate alter dramatically, when the band structure exhibits various level of flatness. In particular, when the band exhibits perfect flatness around the band minima corresponding to a near infinite effective mass, a quadratic dispersion emerges in the low-energy excitation spectrum; in s…
The fastest possible collective response of a quantum many-body system is related to its excitations at the highest possible energy. In condensed-matter systems, the corresponding timescale is typically set by the Fermi energy. Taking advantage of fast and precise control of interactions between ultracold atoms, we report on the observation of ultrafast dynamics of impurities coupled to an atomic Fermi sea. Our interferometric measurements track the non-perturbative quantum evolution of a fermionic many-body system, revealing in real time the formation dynamics of quasiparticles and the quantu…
We investigate the system of a heavy impurity immersed in a degenerated Fermi gas, where the impurity's internal degree of freedom (pseudospin) is manipulated by a series of radiofrequency (RF) pulses at several different times. Applying the functional determinant approach, we carry out an essentially exact calculation of the Ramsey-interference-type responses to the RF pulses. These responses are universal functions of the multiple time intervals between the pulses for all time and can be regarded as multidimensional (MD) spectroscopy of the system in the time domain. A Fourier transformation…
The weak coupling many-polaron formalism is applied to the case of the polaronic system consisting of impurities in a Bose-Einstein condensate. This allows to investigate the groundstate properties and the response of the system to Bragg spectroscopy. This theory is then applied to the system of spin-polarized fermionic lithium-6 impurities in a sodium condensate. The Bragg spectrum reveals a peak which corresponds to the emission of Bogoliubov excitations. Both ground state properties and the response spectrum show that the polaronic effect vanishes at large densities. We also look at two pos…
We suggest pump-probe spectroscopy to study pair correlations that determine the many-body dynamics in weakly interacting, dilute ultracold gases. A suitably chosen, short laser pulse depletes the pair density locally, creating a 'hole' in the electronic ground state. The dynamics of this non-stationary pair density is monitored by a time-delayed probe pulse. The resulting transient signal allows to spectrally decompose the 'hole' and to map out the pair correlation functions.
The response of cold atom gases to small periodic phase modulation of an optical lattice is discussed. For bosonic gases, the energy absorption rate is given, within linear response theory, by imaginary part of the current correlation function. For fermionic gases in a strong lattice potential, the same correlation function can be probed via the production rate double occupancy. The phase modulation gives thus direct access to the conductivity of the system, as function of the modulation frequency. We give an example of application in the case of one dimensional bosons at zero temperature and …
We investigate a momentum-resolved Raman spectroscopy technique which is able to probe the one-body spectral function and the quasi-particle states of a gas of strongly interacting ultracold atoms. This technique is inspired by Angle-Resolved Photo-Emission Spectroscopy, a powerful experimental probe of electronic states in solid-state systems. Quantitative examples of experimentally accessible spectra are given for the most significant regimes along the BEC-BCS crossover. When the theory is specialized to RF spectroscopy, agreement is found with recent experimental data. The main advantages o…
We demonstrate a photon-counting technique for detecting Bragg excitation of an ultracold gas of atoms. By measuring the response of the light field to the atoms, we derive a signal independent of traditional time-of-flight atom-imaging techniques. With heterodyne detection we achieve photon shot-noise limited detection of the amplification or depletion of one of the Bragg laser beams. Photon counting for Bragg spectroscopy will be useful for strongly interacting gases where atom-imaging detection fails. In addition, this technique provides the ability to resolve the evolution of excitations a…
We investigate theoretically radio-frequency spectroscopy of weakly bound molecules in an ultracold spin-orbit-coupled atomic Fermi gas. We consider two cases with either equal Rashba and Dresselhaus coupling or pure Rashba coupling. The former system has been realized very recently at Shanxi University [Wang et al., arXiv:1204.1887] and MIT [Cheuk et al., arXiv:1205.3483]. We predict realistic radio-frequency signals for revealing the unique properties of anisotropic molecules formed by spin-orbit coupling.
Alkali-earth atoms have a long-lived electronic excited state, which can be localized in the Fermi sea of ground state atoms by an external potential and serve as magnetic impurities, due to the spin-exchange interaction between the excited and the ground state atoms. This can give rise to the Kondo effect. However, in order to achieve this effect in current atomic gas experiment, it requires the Kondo temperature to be increased to a sizable portion of the Fermi temperature. In this letter we propose that the spin-exchange interaction can be strongly enhanced by utilizing the confinement-indu…
Two-dimensional (2D) spectroscopy uses multiple electromagnetic pulses to infer the properties of a complex system. A paradigmatic class of target systems are molecular aggregates, for which one can obtain information on the eigenstates, various types of static and dynamic disorder and on relaxation processes. However, two-dimensional spectra can be difficult to interpret without precise knowledge of how the signal components relate to microscopic Hamiltonian parameters and system-bath interactions. Here we show that two-dimensional spectroscopy can be mapped in the microwave domain to highly …
We propose and investigate a pump-probe spectroscopy scheme to unveil the time-resolved dynamics of fermionic or bosonic impurities immersed in a harmonically trapped Bose-Einstein condensate. In this scheme a pump pulse initially transfers the impurities from a noninteracting to a resonantly interacting spin-state and, after a finite time in which the system evolves freely, the probe pulse reverses this transition. This directly allows to monitor the nonequilibrium dynamics of the impurities as the dynamical formation of coherent attractive or repulsive Bose polarons and signatures of their i…
Bose polarons, quasi-particles composed of mobile impurities surrounded by cold Bose gas, can experience strong interactions mediated by the many-body environment and form bipolaron bound states. Here we present a detailed study of heavy polarons in a one-dimensional Bose gas by formulating a non-perturbative theory and complementing it with exact numerical simulations. We develop an analytic approach for weak boson-boson interactions and arbitrarily strong impurity-boson couplings. Our approach is based on a mean-field theory that accounts for deformations of the superfluid by the impurities …
We demonstrate the possibility of drastically reducing the velocity of phonons in quasi one-dimensional Bose-Einstein condensates. Our scheme consists of a dilute dark-soliton "gas" that provide the trapping for the impurities that surround the condensate. We tune the interaction between the impurities and the condensate particles in such a way that the dark solitons result in an array of {\it qutrits} (three-level structures). We compute the phonon-soliton coupling and investigate the decay rates of these three-level qutrits inside the condensate. As such, we are able to reproduce the phenome…
We address recent momentum resolved radio frequency (RF) experiments on ultracold trapped Fermi gases of $^{40}$K. We show that momentum resolved RF probes provide measurements of the centrally important fermionic spectral function. They also serve to remove ambiguity plaguing the interpretation of momentum integrated RF experiments by establishing a clear dispersion signature of pairing. We find that the temperature dependence of the spectral function is dramatic at unitarity, and, importantly, smooth from above to below $T_c$ throughout BCS-BEC crossover. This should be tested experimentally…
We investigate the radio-frequency spectroscopy of impurities interacting with a quantum gas at finite temperature. In the limit of a single impurity, we show using Fermi's golden rule that introducing (or injecting) an impurity into the medium is equivalent to ejecting an impurity that is initially interacting with the medium, since the "injection" and "ejection" spectral responses are simply related to each other by an exponential function of frequency. Thus, the full spectral information for the quantum impurity is contained in the injection spectral response, which can be determined using …
We demonstrate that identical impurities immersed in a two-dimensional many-particle bath can be viewed as flux-tube-charged-particle composites described by fractional statistics. In particular, we find that the bath manifests itself as an external magnetic flux tube with respect to the impurities, and hence the time-reversal symmetry is broken for the effective Hamiltonian describing the impurities. The emerging flux tube acts as a statistical gauge field after a certain critical coupling. This critical coupling corresponds to the intersection point between the quasiparticle state and the ph…
We present a systematic characterization of the radio frequency (RF) spectra of homogeneous, paired atomic Fermi gases at finite temperatures, $T$, in the presence of final state interactions. The spectra, consisting of possible bound states and positive as well as negative detuning ($ν$) continua, satisfy exactly the zeroth- and first-moment sum rules at all $T$. We show how to detect the $ν< 0$ continuum arising from thermally excited quasiparticles, which has not yet been seen experimentally. We explain semi-quantitatively recent RF experiments on "bound-bound" transitions and, thereby, pre…
Motivated by recent experiments, we address, in a fully self consistent fashion, the behavior and evolution of radio frequency (RF) spectra as temperature and polarization are varied in population imbalanced Fermi gases. We discuss a series of scenarios for the experimentally observed zero temperature pseudogap phase and show how present and future RF experiments may help in its elucidation. We conclude that the MIT experiments at the lowest $T$ may well reflect ground state properties, but take issue with their claim that the pairing gap survives up to temperatures of the order of the degener…
Mobile impurities in cold atomic gases constitute a new platform for investigating polaron physics. Here we show that when impurity atoms interact with a two-dimensional Fermi gas with quadratic band touching the polaron picture may either hold or break down depending on the particle-hole asymmetry of the band structure. If the hole band has a smaller effective mass than the particle band, the quasiparticle is stable and its diffusion coefficient varies with temperature as $D(T) \propto \ln^2 T$. If the hole band has larger mass, the quasiparticle weight vanishes at low energies due to an emer…
We present a theoretical interpretation of radio-frequency (RF) pairing gap experiments in trapped atomic Fermi gases, over the entire range of the BCS-BEC crossover, for temperatures above and below $T_c$. Our calculated RF excitation spectra, as well as the density profiles on which they are based, are in semi-quantitative agreement with experiment. We provide a detailed analysis of the physical origin of the two different peak features seen in RF spectra, one associated with nearly free atoms at the edge of the trap, and the other with (quasi-)bound fermion pairs.
Lattice modulation spectroscopy is a powerful tool for probing low-energy excitations of interacting many-body systems. By means of bosonization we analyze the absorbed power in a one dimensional interacting quantum gas of bosons or fermions, subjected to a periodic drive of the optical lattice. For these Tomonaga Luttinger liquids we find a universal $ω^3$ scaling of the absorbed power, that at very low-frequency turns into an $ω^2$ scaling when scattering processes at the boundary of the system are taken into account. We confirm this behavior numerically by simulations based on time-dependen…
We study the effect of impurities in a supersolid phase in comparison to the behavior in the solid and superfluid phases. A supersolid phase has been established for interacting hardcore bosons on a triangular lattice which may be realizable by ultracold atomic gases. Static vacancies are considered in this model which always lower the magnitude of the order parameter in the solid or superfluid phases. In the supersolid phase, however, the impurities directly affect both order parameters simultaneously and thereby reveal an interesting interplay between them. In particular the solid order may …
We describe how microwave spectroscopy of cold fermions in quasi-1D traps can be used to detect, manipulate, and entangle exotic non-local qbits associated with "Majorana" edge modes. We present different approaches to generate the p-wave superfluidity which is responsible for these topological zero-energy edge modes. We find that the edge modes have clear signatures in the microwave spectrum, and that the line shape distinguishes between the degenerate states of a qbit encoded in these edge modes. Moreover, the microwaves rotate the system in its degenerate ground-state manifold. We use these…
We use Rabi spectroscopy to explore the low-energy excitation spectrum of a finite-temperature Bose gas of rubidium atoms across the phase transition to a Bose-Einstein condensate (BEC). To record this spectrum, we coherently drive the atomic population between two spin states. A small relative displacement of the spin-specific trapping potentials enables sideband transitions between different motional states. The intrinsic non-linearity of the motional spectrum, mainly originating from two-body interactions, makes it possible to resolve and address individual excitation lines. Together with s…
In this paper we present an overview of radio frequency (RF) spectroscopy in the atomic Fermi superfluids. An ultimate goal is to suggest new directions in the cold gas research agenda from the condensed matter perspective.Our focus is on the experimental and theoretical literature of cold gases and photoemission spectroscopy of the cuprates particularly as it pertains to areas of overlap. This paper contains a systematic overview of the theory of RF spectroscopy, both momentum integrated and momentum resolved. We discuss the effects of traps, population imbalance, final state interactions ove…
The advent of the quantum gas microscope allowed for the in situ probing of ultracold gaseous matter on an unprecedented level of spatial resolution. The study of phenomena on ever smaller length scales as well as the probing of three-dimensional systems is, however, fundamentally limited by the wavelength of the imaging light, for all techniques based on linear optics. Here we report on a high-resolution ion microscope as a versatile and powerful experimental tool to investigate quantum gases. The instrument clearly resolves atoms in an optical lattice with a spacing of $532\,\text{nm}$ over …
The precise measurement of low temperatures is a challenging, important and fundamental task for quantum science. In particular, in-situ thermometry is highly desirable for cold atomic systems due to their potential for quantum simulation. Here we demonstrate that the temperature of a non-interacting Fermi gas can be accurately inferred from the non-equilibrium dynamics of impurities immersed within it, using an interferometric protocol and established experimental methods. Adopting tools from the theory of quantum parameter estimation, we show that our proposed scheme achieves optimal precisi…
We present a systematic investigation of the effects of "nonmagnetic" impurities on the $s$-wave BCS-BEC crossover in atomic Fermi gases within a pairing fluctuation theory. Both pairing and impurity scattering $T$-matrices are treated self-consistently at the same time. While the system is less sensitive to impurity scattering in the Born limit, for strong impurity scatterers, both the frequency and the gap function are highly renormalized, leading to significant suppression of the superfluid $T_c$, the order parameter and the superfluid density. We also find the formation of impurity bands a…
ARC Centre of Excellence for Quantum-Atom Optics, Centre for Atom Optics and Ultrafast Spectroscopy, Swinburne University of Technology, Melbourne 3122, Australia
The effects of impurities in spin-1/2 Heisenberg chains are recently experiencing a renewed interest due to experimental realizations in solid state systems and ultra-cold gases. The impurities effectively cut the chains into finite segments with a discrete spectrum and characteristic correlations, which have a distinct effect on the dynamic structure factor. Using bosonization and the numerical Density Matrix Renormalization Group we provide detailed quantitative predictions for the momentum and energy resolved structure factor in doped systems. Due to the impurities, spectral weight is shift…
Polaron quasiparticles are formed when a mobile impurity is coupled to the elementary excitations of a many-particle background. In the field of ultracold atoms, the study of the associated impurity problem has attracted a growing interest over the last fifteen years. Polaron quasiparticle properties are essential to our understanding of a variety of paradigmatic quantum many-body systems realized in ultracold atomic gases and in the solid state, from imbalanced Bose-Fermi and Fermi-Fermi mixtures to fermionic Hubbard models. In this topical review, we focus on the so-called repulsive polaron …
The existence of a self-localization transition in the polaron problem has been under an active debate ever since Landau suggested it 83 years ago. Here we reveal the self-localization transition for the rotational analogue of the polaron -- the angulon quasiparticle. We show that, unlike for the polarons, self-localization of angulons occurs at finite impurity-bath coupling already at the mean-field level. The transition is accompanied by the spherical-symmetry breaking of the angulon ground state and a discontinuity in the first derivative of the ground-state energy. Moreover, the type of th…
One of the hallmarks of quantum statistics, tightly entwined with the concept of topological phases of matter, is the prediction of anyons. Although anyons are predicted to be realized in certain fractional quantum Hall systems, they have not yet been unambiguously detected in experiment. Here we introduce a simple quantum impurity model, where bosonic or fermionic impurities turn into anyons as a consequence of their interaction with the surrounding many-particle bath. A cloud of phonons dresses each impurity in such a way that it effectively attaches fluxes/vortices to it and thereby convert…
