The trilayer nickelate Nd$_4$Ni$_3$O$_{10-δ}$ ($δ\approx$ 0.15) was investigated by the measurements of x-ray diffraction, electrical resistivity, magnetic susceptibility, and heat capacity. The crystal structure data suggest a higher Ni valence in the inner perovskite-like layer. At ambient pressure the resistivity shows a jump at 162 K, indicating a metal-to-metal transition (MMT). The MMT is also characterized by a magnetic susceptibility drop, a sharp specific-heat peak, and an isotropic lattice contraction. Below $\sim$ 50 K, a resistivity upturn with a log$T$ dependence shows up, accompanying with a negative thermal expansion. External hydrostatic pressure suppresses the resistivity jump progressively, coincident with the diminution of the log$T$ behavior. The low-temperature electronic specific-heat coefficient is extracted to be $\sim$ 150 mJ K$^{-2}$ mol-fu$^{-1}$, equivalent to $\sim$ 50 mJ K$^{-2}$ mol-Ni$^{-1}$, indicating an unusual heavy-electron correlated state. The novel heavy-electron state as well as the logarithmic temperature dependence of resistivity is explained in terms of the Ni$^{3+}$ centered Kondo effect in the inner layer of the (NdNiO$_3$)$_3$ trilayers.
A tunnelling conductivity between a heavy fermion metal and a simple metallic point is considered. We show that at low temperatures this conductivity can be noticeably dissymmetrical with respect to the change of voltage bias. The dissymmetry can be observed in experiments on the heavy fermion metals whose electronic system has undergone the fermion condensation quantum phase transition.
A theoretical study has been undertaken of the Peltier effect in normal metal - insulator - heavy fermion metal junctions. The results indicate that, at temperatures below the Kondo temperature, such junctions can be used as electronic microrefrigerators to cool the normal metal electrode and are several times more efficient in cooling than the normal metal - heavy fermion metal junctions.
Low-temperature thermodynamic properties of strongly interacting Fermi liquids with fermion condensate are investigated. We demonstrate that the spin susceptibility of these systems exhibits the Curie-Weiss law, and the entropy contains a temperature-independent term. The excessive entropy is released at the superconducting transition, enhancing the specific heat jump Delta C and rendering it proportional to the effective Curie constant. The theoretical results are favorably compared with the experimental data on the heavy fermion metal CeCoIn5, as well as He-3 films.
Our previous point-contact Andreev reflection studies of the heavy-fermion superconductor CeCoIn$_5$ using Au tips have shown two clear features: reduced Andreev signal and asymmetric background conductance [1]. To explore their physical origins, we have extended our measurements to point-contact junctions between single crystalline heavy-fermion metals and superconducting Nb tips. Differential conductance spectra are taken on junctions with three heavy-fermion metals, CeCoIn$_5$, CeRhIn$_5$, and YbAl$_3$, each with different electron mass. In contrast with Au/CeCoIn$_5$ junctions, Andreev sig…
We demonstrate, that the main universal features of the low temperature experimental $H-T$ phase diagram of CeCoIn5 and other heavy-fermion metals can be well explained using Landau paradigm of quasiparticles. The main point of our theory is that above quasiparticles form so-called fermion-condensate state, achieved by a fermion condensation quantum phase transition (FCQPT). When a heavy fermion liquid undergoes FCQPT, the fluctuations accompanying above quantum critical point are strongly suppressed and cannot destroy the quasiparticles. The comparison of our theoretical results with experime…
Symmetry breaking beyond a global U(1) phase is the key signature of unconventional superconductors. As prototypical strongly correlated materials, heavy-fermion metals provide ideal platforms for realizing unconventional superconductivity. In this article, we review heavy-fermion superconductivity, with a focus on those materials with multiple superconducting phases. In this context, we highlight the role of orbital-selective (matrix) pairing functions, which are defined as matrices in the space of effective orbital degrees of freedom such as electronic orbitals and sublattices as well as equ…
High-temperature superconductors (HTSC) and heavy-fermion (HF) metals exhibit extraordinary properties. They are so unusual that the traditional Landau paradigm of quasiparticles does not apply. It is widely believed that utterly new concepts are required to describe the underlying physics. There is a fundamental question: how many concepts do we need to describe the above physical mechanisms? This cannot be answered on purely experimental or theoretical grounds. Rather, we have to use both of them. Recently, in HTSC, the new and exciting measurements have been performed, demonstrating a puzzl…
We present a comprehensive analysis of the low temperature experimental H-T phase diagram of CeCoIn5. The main universal features of the diagram can be explained within the Fermi-liquid theory provided that quasiparticles form so called fermion-condensate state. We show that in this case the fluctuations accompanying an ordinary quantum critical point are strongly suppressed and cannot destroy the quasiparticles. Analyzing the phase diagram and giving predictions, we demonstrate that the electronic system of CeCoIn5 provides a unique opportunity to study the relationship between quasiparticles…
We have shown that the Landau paradigm based upon both the quasiparticle concept and the notion of the order parameter can be used to explain the anomalous behavior of heavy fermion metals. Exploiting this paradigm and the fermion condensation quantum phase transition (FCQPT) we show that this anomalous behavior is universal and can be used to capture the essential aspects of recent experiments on the heavy-fermion metals at low temperatures. Behind FCQPT a tunneling conductivity between a heavy fermion metal and a simple metallic point can be noticeably dissymmetrical with respect to the chan…
The interface between a heavy electron coherent metallic phase and an incoherent normal metal phase is discussed. The Fermi momentum mismatch between the two phases causes the carriers to scatter at the interface. The interface conductance is a monotonous increasing function of conduction electron density, n_c, and is less than 60% of that of a clean heavy fermion metal at half-filling ($n_c=1$) and can be measured experimentally. Interface experiments can be used as probe of the nature of the homogenous heavy-fermion state and provide important information on the effects of inhomogeneities in…
An explanation of paradoxical behavior of the residual resistivity rho_0 of the heavy-fermion metal CeCoIn5 in magnetic fields and under pressure is developed. The source of this behavior is identified as a flattening of the single-particle spectrum, which exerts profound effects on the specific heat, thermal expansion coefficient, and magnetic susceptibility in the normal state, the specific heat jump at the point of superconducting phase transition, and other properties of strongly correlated electron systems in solids. It is shown that application of a magnetic field or pressure to a system…
Unusual properties of strongly correlated liquid observed in the high-$T_c$ superconductors and heavy-fermion (HF) metals are determined by quantum phase transitions taking place at their critical points. Therefore, direct experimental studies of these transitions and critical points are of crucial importance for understanding the physics of high-$T_c$ superconductors and HF metals. In case of high-$T_c$ superconductors such direct experimental studies are absent since at low temperatures corresponding critical points are occupied by the superconductivity. Recent experimental data on the behav…
We study the quantum phase transition from an antiferromagnetic metal to a heavy fermion metal in the Kondo lattice model. Based on the strong coupling approach we {\it first} diagonalize the Kondo coupling term. Since this strong coupling approach makes the resulting Kondo term {\it relevant}, the Kondo hybridization persists even in the antiferromagnetic metal, indicating that fluctuations of Kondo singlets are not critical in the phase transition. We find that the quantum transition in our strong coupling approach results from {\it softening of antiferromagnetic spin fluctuations of localiz…
Low energy nuclear reactions in the neighborhood of metallic hydride surfaces may be induced by ultra-low momentum neutrons. Heavy electrons are absorbed by protons or deuterons producing ultra low momentum neutrons and neutrinos. The required electron mass renormalization is provided by the interaction between surface electron plasma oscillations and surface proton oscillations. The resulting neutron catalyzed low energy nuclear reactions emit copious prompt gamma radiation. The heavy electrons which induce the initially produced neutrons also strongly absorb the prompt nuclear gamma radiatio…
Strongly correlated electron systems at the border of magnetism are of active current interest, particularly because the accompanying quantum criticality provides a route towards both strange-metal non-Fermi liquid behavior and unconventional superconductivity. Among the many important questions is whether the magnetism acts simply as a source of fluctuations in the textbook Landau framework, or instead serves as a proxy for some unexpected new physics. We put into this general context the recent developments on quantum phase transitions in antiferromagnetic heavy fermion metals. Among these a…
The importance of taking into account inter-site $f-f$ hybridization in electron structure calculations for Ce metal and cerium heavy fermion compounds was studied. We demonstrate that for heavy-fermion systems such as cerium compound CeCu$_2$Si$_2$ $f-f$ hybridization can be neglected and Anderson model application is well justified. On another hand for cerium metal $f-f$ hybridization is strong enough to provide the contribution to hybridization function comparable to hybridization between $4f$ and itinerant electrons. We argue that in the case of Ce only the most general Hamiltonian combini…
The perovskite-like transition-metal oxide Gd$_{1-x}$Sr$_x$TiO$_3$ is investigated by measurements of resistivity, specific-heat, and electron paramagnetic resonance (EPR). Approaching the metal-to-insulator transition from the metallic regime ($x \geq 0.2$), the Sommerfeld coefficient $γ$ of the specific heat becomes strongly enhanced and the resistivity increases quadratically at low temperatures, which both are fingerprints of strong electronic correlations. The temperature dependence of the dynamic susceptibility, as determined from the Gd$^{3+}$-EPR linewidth, signals the importance of st…
We propose a two-stage spin quenching scenario for the unusual heavy fermion state realized in the mixed valent metal LiV$_2$O$_4$. In this theory, local valence fluctuations are responsible for the formation of partially quenched, spin 1/2 moments below room temperature. Frustration of the intersite spin couplings then drives the system to produce the heavy Fermi liquid seen at low temperatures. The anomalous resistivity and the sign change of the Hall constant can be understood naturally within this model, which also predicts a unique symmetry for the heavy quasiparticle bands that may be ob…
We report magnetic and calorimetric measurements down to T = 1 mK on the canonical heavy-electron metal YbRh2Si2. The data reveal the development of nuclear antiferromagnetic order slightly above 2 mK. The latter weakens the primary electronic antiferromagnetism, thereby paving the way for heavy-electron superconductivity below Tc = 2 mK. Our results demonstrate that superconductivity driven by quantum criticality is a general phenomenon.
It is shown that the Landau paradigm based upon both the quasiparticle concept and the notion of the order parameter is valid and can be used to explain the anomalous behavior of the heavy fermion metals near quantum critical points. The understanding of this phenomenon has been problematic largely because of the absence of theoretical guidance. Exploiting this paradigm and the fermion condensation quantum phase transition, we investigate the anomalous behavior of the heavy electron liquid near its critical point at different temperatures and applied magnetic fields. We show that this anomalou…
The quantum spin liquid candidate NaYbSe$_2$ was recently reported to exhibit a Mott transition under pressure. Superconductivity was observed in the high-pressure metallic phase, raising the question concerning its relation with the low-pressure quantum spin liquid ground state. Here we combine the density functional theory and the dynamical mean-field theory to explore the underlying mechanism of the insulator-to-metal transition and superconductivity and establish an overall picture of its electronic phases under pressure. Our results suggest that NaYbSe$_2$ is a charge-transfer insulator a…
The two-fluid model is a phenomenological description of the gradual change of the itinerant and local characters of the f-electrons with temperature and other tuning parameters and has been quite successful in explaining many unusual and puzzling experimental observations in heavy electron materials. We review some of these results and discuss possible implications of the two-fluid model in understanding the microscopic origin of heavy electron physics.
Quantum criticality describes the collective fluctuations of matter undergoing a second-order phase transition at zero temperature. Heavy fermion metals have in recent years emerged as prototypical systems to study quantum critical points. There have been considerable efforts, both experimental and theoretical, which use these magnetic systems to address problems that are central to the broad understanding of strongly correlated quantum matter. Here, we summarize some of the basic issues, including i) the extent to which the quantum criticality in heavy fermion metals goes beyond the standard …
A Zeeman field affects the metallic heavy fermion ground state in two ways: (i) it splits the spin-degerenate conduction sea, leaving spin up and spin down Fermi surfaces with different band curvature; (ii) it competes with the Kondo effect and thus suppresses the mass enhancement. Taking these two effects into account, we compute the quasiparticle effective mass as a function of applied field strength within hybridization mean field theory. We also derive an expression for the optical conductivity, which is relevant to infrared spectroscopy measurements.
We have shown the existence of localized crystal-field states in conducting magnetic materials coexisting with conduction electrons in CeAl3, UPd2Al3 and YbRh2Si2. We point out that the magnetism is strongly correlated with the very detailed local atomic-scale crystal structure.
Using a combination of density functional theory, tight-binding models, and Hartree-Fock theory, we predict topological phases with and without time-reversal symmetry breaking in oxide heterostructures. We consider both heterostructures containing light transition metal ions, and those containing heavy transition metal ions. We find the (111) growth direction naturally leads to favorable conditions for topological phases in both perovskite structures and pyrochlore structures. For the case of light transition metal elements, Hartree-Fock theory predicts the spin-orbit coupling is effectively e…
Optical conductivity [$σ(ω)$] of YbS has been measured under pressure up to 20 GPa. Below 8 GPa, $σ(ω)$ is low since YbS is an insulator with an energy gap between fully occupied 4$f$ state and unoccupied conduction ($c$) band. Above 8 GPa, however, $σ(ω)$ increases dramatically, developing a Drude component due to heavy carriers and characteristic infrared peaks. It is shown that increasing pressure has caused an energy overlap and hybridization between the $c$ band and 4$f$ state, thus driving the initially ionic and insulating YbS into a correlated metal with heavy carriers.
The heavy fermion metal β-YbAlB4 exhibits a bulk room temperature conduction electron ESR signal which evolves into an Ising-anisotropic f-electron signal exhibiting hyperfine features at low temperatures. We develop a theory for this phenomenon based on the development of resonant scattering off a periodic array of Kondo centers. We show that the hyperfine structure arises from the scattering off the Yb atoms with non zero nuclear spin, while the constancy of the ESR intensity is a consequence of the presence of CEF excitations of the order of the hybridization strength.
Spin fluctuations were studied over a wide momentum ($\hbar Q$) and energy ($E$) space in the frustrated $d$-electron heavy-fermion metal LiV$_2$O$_4$ by time-of-flight inelastic neutron scattering. We observed the overall $Q$$-$$E$ evolutions near the characteristic $Q=0.6$ Å$^{-1}$ peak and found another weak broad magnetic peak around 2.4 Å$^{-1}$. The data are described by a simple response function, a highly itinerant magnetic form factor, and antiferromagnetic short-range spatial correlations, indicating that heavy-fermion formation is attributable to spin-orbit fluctuations with orbital…
We report measured dipolar asymmetry ratios at the LIII edges of the heavy rare earth metals. The results are compared with a first principles calculation and excellent agreement is found. A simple model of the scattering is developed, enabling us to re-interpret the resonant x-ray scattering in these materials and to identify the peaks in the asymmetry ratios with features in the spin and orbital moment densities.
Ubiquity of unconventional phenomena observed in a series of heavy fermion metals is discussed on the basis of an idea of critical valence fluctuations. After surveying experimental aspects of these unconventional behaviors in prototypical compounds, CeCu_2(Si,Ge)_2, under pressure, we propose that sharp valence crossover phenomena are realized in CeCu_6, CeRhIn_5, and Ce(Ir,Rh)Si_3 by tuning the pressure and the magnetic field simultaneously, on the basis of previous results for an extended Anderson lattice model with the Coulomb repulsion U_fc between localized f-electron and itinerant condu…
For some heavy-fermion compounds, it has been suggested that a Fermi-surface-changing Lifshitz transition, which can be driven, e.g., by varying an applied magnetic field, occurs inside the heavy- fermion regime. Here we discuss, based on microscopic calculations, how the location of such a transition can be influenced by carrier doping. Due to strong correlations, a heavy band does not shift rigidly with the chemical potential. Intriguingly, we find that the actual shift is determined by the interplay of heavy and additional light bands crossing the Fermi level: doped carriers tend to populat…
We investigate the electron-spin resonance (ESR) phenomenon in the heavy-fermion metal YbRh2Si2 by applying hydrostatic pressure up to 3 GPa and by inducing internal pressure on the Yb site chemically in Yb(Rh1-xCox)2Si2 samples. We found that the increase in pressure, reducing the hybridization between 4f and conduction electrons, leads to a remarkable change in the temperature dependence of the g factor and broadens the ESR line. We relate the differences between the effect of internal and external pressure on the low temperature ESR parameters to the disorder induced by Co doping. The press…
Motivated by the heavy fermion Fermi liquid (HFFL) features observed at low-$T$ in the pyrochlore $LiV_{2}O_{4}$, we consider a material-specific model that includes aspects of the local quantum chemistry, the geometrically frustrated lattice structure, and strong correlations in a {\it single} approach. In particular, we show how geometrical frustration (GF) gives rise to a crossover scale, $T^{*}<<J$, the intersite (AF) exchange, below which the metallic system shows HFFL features. Our scenario is a specific realization of the importance of GF effects in driving HFFL behavior in $LiV_{2}O_{4…
We study a microscopic derivation and the properties of the Dzyaloshinskii-Moriya interaction (DMI) between local magnetic moments in ferromagnet/heavy metal heterostructures. First, we derive DMI by Ruderman-Kittel-Kasuya-Yosida interaction through electrons in a heavy metal with Rashba spin orbit interaction (SOI). Next, we study the dependences of the DMI on the Rashba SOI, lattice constant, and chemical potential. We find that the DMI amplitude increases linearly when the Rashba SOI is small, has a maximum when the Rashba SOI is comparable to the hopping integral, and decreases when the Ra…
The magnetoresistance (MR) of CeCoIn5 is notably different from that expected for orbital MR due to the Lorentz force and described by Kohler's rule which holds in many conventional metals. We show that a pronounced crossover from negative to positive MR of CeCoIn5 that occurs at elevated temperatures is determined by the dependence of the effective mass M*(B,T) on both magnetic field B and temperature T. Thus, the crossover is regulated by the universal behavior of M*(B,T) observed in heavy-fermion metals. This behavior is exhibited by M*(B,T) when a strongly correlated electron system transi…
We discuss the charge carrier dynamics of the heavy-fermion compound CeCoIn$_5$ in the metallic regime measured by means of quasi-optical THz spectroscopy. The transmittance of electromagnetic radiation through a CeCoIn$_5$ thin film on a dielectric substrate is analyzed in the single-particle Drude framework. We discuss the temperature dependence of the electronic properties, such as the scattering time and dc-conductivity and compare with transport measurements of the sheet resistance. Towards low temperatures, we find an increasing mismatch between the results from transport and Drude-analy…
Extraordinary new materials named quasicrystals and characterized by noncrystallographic rotational symmetry and quasiperiodic translational properties have attracted scrutiny. Study of quasicrystals may shed light on the most basic notions related to the quantum critical state observed in heavy-fermion metals. We show that the electronic system of some quasicrystals is located at the fermion condensation quantum phase transition without tuning. In that case the quasicrystals possess the quantum critical state with the non-Fermi liquid behavior which in magnetic fields transforms into the Land…
Heavy fermion alloys at critical doping typically exhibit non-Fermi-liquid behavior at low temperatures, including a logarithmic or power law rise in the ratio of specific heat to temperature as the temperature is lowered. Anomalous specific heat of this type is also observed in a simple class of gravitational dual models that exhibit anisotropic scaling with dynamical critical exponent z > 1.
Considerable recent theoretical and experimental efforts have been devoted to the study of quantum criticality and novel phases of antiferromagnetic heavy-fermion metals. In particular, quantum phase transitions have been discovered in the compound Yb$_2$Pt$_2$Pb. These developments have motivated us to study the competition between the RKKY and Kondo interactions on the Shastry-Sutherland lattice. We determine the zero-temperature phase diagram as a function of magnetic frustration and Kondo coupling within a slave-fermion approach. Pertinent phases include the Shastry-Sutherland valence bond…
Motivated by the recent discovery of a continuous ferromagnetic quantum phase transition in CeRh$_6$Ge$_4$ and its distinction from other U-based heavy fermion metals such as UGe$_2$, we develop a unified explanation of their different ground state properties based on an anisotropic ferromagnetic Kondo-Heisenberg model. We employ an improved large-$N$ Schwinger boson approach and predict a full phase diagram containing both a continuous ferromagnetic quantum phase transition for large magnetic anisotropy and first-order transitions for relatively small anisotropy. Our calculations reveal three…
Heavy electron metals on the verge of a quantum phase transition to magnetism show a number of unusual non-fermi liquid properties which are poorly understood. This article discusses in a general way various theoretical aspects of this phase transition with an eye toward understanding the non-fermi liquid phenomena. We suggest that the non-Fermi liquid quantum critical state may have a sharp Fermi surface with power law quasiparticles but with a volume not set by the usual Luttinger rule. We also discuss the possibility that the electronic structure change associated with the possible Fermi su…
Heavy fermion metals typically exhibit unconventional quantum critical point or quantum critical phase at zero temperature due to competition of Kondo effect and magnetism. Previous theories were often based on certain local type of assumptions and a fully consistent explanation of experiments has not been achieved. Here we develop an efficient algorithm for the Schwinger boson approach to explore the effect of spatial correlations on the Kondo lattice and introduce the concept of nonlocal Kondo effect in the quantum critical region with deconfined spinons. We predict a global phase diagram co…
We present a detailed theoretical study of the ultrafast quasiparticle relaxation dynamics observed in normal metals and heavy fermion materials with femtosecond time-resolved optical pump-probe spectroscopy. For normal metals, a nonthermal electron distribution gives rise to a temperature (T) independent electron-phonon relaxation time at low temperatures, in contrast to the T^{-3}-divergent behavior predicted by the two-temperature model. For heavy fermion compounds, we find that the blocking of electron-phonon scattering for heavy electrons within the density-of-states peak near the Fermi e…
We present a theory of the dynamic magnetic susceptibility of quantum spin liquid. The obtained results are in good agreement with experimental facts collected on herbertsmithite ZnCu3(OH)6Cl2 and on heavy-fermion metals, and allow us to predict a new scaling in magnetic fields in the dynamic susceptibility. Under the application of strong magnetic fields quantum spin liquid becomes completely polarized. We show that this polarization can be viewed as a manifestation of gapped excitations when investigating the spin-lattice relaxation rate.
The critical theory of the onset of antiferromagnetism in metals, with concomitant Fermi surface reconstruction, has recently been shown to be strongly coupled in two spatial dimensions. The onset of unconventional superconductivity near this critical point is reviewed: it involves a subtle interplay between the breakdown of fermionic quasiparticle excitations on the Fermi surface, and the strong pairing glue provided by the antiferromagnetic fluctuations. The net result is a logarithm-squared enhancement of the pairing vertex for generic Fermi surfaces, with a universal dimensionless co-effic…
The mechanism of strange metal (SM) with unconventional charge transport near magnetic phase transitions has become an outstanding open problem in correlated electron systems. Recently, an exotic quantum critical SM phase was observed in paramagnetic frustrated heavy-fermion materials near Kondo breakdown. We establish a controlled theoretical framework to this issue via a dynamical large-N fermionic multichannel approach to the two-dimensional Kondo-Heisenberg lattice model, where KB transition separates a heavy-Fermi liquid from fermionic spin-liquid state. With Kondo fluctuations being full…
We describe the experimentally revealed by Sichelschmidt et al, Phys. Rev. Lett. 91 (2003) 156401, g tensor, g_perpendicular=3.561 and g_parallel=0.17, at 5 K by means of crystal field interactions of the 4f13 configuration of the Yb3+ ion of YbRh2Si2 in a slightly orthorhombically distorted tetragonal crystal field. We have shown that the temperature dependence of the quadrupolar interactions Q(T) of the Yb nucleous will help to distinguish between Gamma_7 and Gamma_6 ground state. For the Gamma_7 ground state Q(T) is expected to exhibits an anomalous dependence. Keywords: heavy fermion, crys…
Strange metal behavior refers to a linear temperature dependence of the electrical resistivity at temperatures below the Mott-Ioffe-Regel limit. It is seen in numerous strongly correlated electron systems, from the heavy fermion compounds, via transition metal oxides and iron pnictides, to magic angle twisted bi-layer graphene, frequently in connection with unconventional or "high temperature" superconductivity. To achieve a unified understanding of these phenomena across the different materials classes is a central open problem in condensed matter physics. Tests whether the linear-in-temperat…
Slow spin fluctuations ($ν< 10^{12}$ s$^-1$) observed by the muon spin relaxation technique in Y$_{1-x}$Sc$_x$Mn$_2$ exhibits a power law dependence on temperature ($ν\propto T^α$), where the power converges asymptotically to unity ($α\rightarrow 1$) as the system moves away from spin-glass instability with increasing Sc content $x$. This linear $T$ dependence, which is common to that observed in LiV$_2$O$_4$, is in line with the prediction of the "intersecting Hubbard chains" model for a metallic pyrochlore lattice, suggesting that the geometrical constraints to t2g bands specific to the pyro…
We report results of the study of the recently discovered magnetic resonance in the orbitally ordered phase of CeB6 (the orbital ordering resonance) in a wide frequency range 44-360 GHz. It is found that the g-factor for this resonance increases with frequency from g(44 GHz)~1.55 to g(>250 GHz)~1.7. In addition to the orbital ordering resonance for the frequencies exceeding 200 GHz a new magnetic resonance with the g-factor 1.2-1.3 is detected.
The heavy fermion systems present a unique platform in which strong electronic correlations give rise to a host of novel, and often competing, electronic and magnetic ground states. Amongst a number of potential experimental tools at our disposal, measurements of the Hall effect have emerged as a particularly important one in discerning the nature and evolution of the Fermi surfaces of these enigmatic metals. In this article, we present a comprehensive review of Hall effect measurements in the heavy-fermion materials, and examine the success it has had in contributing to our current understand…
We present a Quantum Monte Carlo (QMC) study of the 1D Kondo lattice at non-integer filling, i.e. a one-dimensional version of a heavy electron metal. For this special system the minus-sign problem turns out to be strongly reduced, which allows QMC simulations for temperatures as low as 1% of the conduction electron bandwidth. The single particle Green's function shows and intricate network of low-energy bands at low temperature, with a Fermi surface volume that comprises both c and f-electrons. As temperature increases the system evolves through two distinct crossover temperatures into a very…
We fully support the interpretation of Prof. F. Steglich, reported recently in Phys. Rev. Lett. 91 (2003)156401, that the observed \textit{below} Kondo temperature, Electron Spin Resonance (ESR) in a heavy fermion metal YbRh2Si2 is associated with the Yb3+ moment, more exactly with the strongly-correlated 4f13 configuration. We derived the ground-state eigenfunction Gamma_7^1= 0.803|\pm 3/2>+ 0.595|\mp 5/2> - 0.026|\mp 1/2> - 0.008|\pm 7/2> and crystal field parameters: B20= +14 K, B40= +60 mK, B60= -0.5 mK, B44= -2.23 K and B64= -10 mK with a small orthorhombic distortion B22= +0.23 K, that p…
The electronic structure of the first reported heavy fermion compound without f-electrons LiV_2O_4 was studied by an ab-initio calculation method. In the result of the trigonal splitting and d-d Coulomb interaction one electron of the $d^{1.5}$ configuration of V ion is localized and the rest partially fills a relatively broad conduction band. The effective Anderson impurity model was solved by Non-Crossing-Approximation method, leading to an estimation for the single-site Kondo energy scale T_K. Then, we show how the so-called exhaustion phenomenon of Nozières for the Kondo lattice leads to a…
Recent experiments on quantum criticality in the Ge-substituted heavy-electron material YbRh2Si2 under magnetic field have revealed a possible non-Fermi liquid (NFL) strange metal (SM) state over a finite range of fields at low temperatures, which still remains a puzzle. In the SM region, the zero-field antiferromagnetism is suppressed. Above a critical field, it gives way to a heavy Fermi liquid with Kondo correlation. The T (temperature)-linear resistivity and the T-logarithmic followed by a power-law singularity in the specific heat coefficient at low T, salient NFL behaviours in the SM reg…
