arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2001.08953physics.opticscond-mat.mes-hallphysics.comp-ph
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表面粗糙度对纳米间隙等离子体系统的影响

Impact of surface roughness in nanogap plasmonic systems

Cristian Ciracì, Ferran Vidal-Codina, Daehan Yoo, Jaime Peraire, Sang-Hyun Oh, David R. Smith

摘要:

最近的结果表明,前所未有的控制两个金属元素之间的间隔距离数百纳米的大小,在中红外波长的自由电子非局部响应的影响。然而,由于制造引起的表面粗糙度,大多数金属系统仍然遭受一定程度的不均匀性。这种系统中的纳米级粗糙度可能会阻碍对微观相互作用作用的理解。在这里,我们调查的同轴纳米孔共振在中红外频率的表面粗糙度的影响。我们发现,虽然随机粗糙度以不可预测的方式改变了共振,但仍然可以清楚地观察到非局部效应的影响。粗糙度引起的扰动的峰值共振的系统显示出很强的相关性与有效的间隙大小的个别样品。然后,可以通过对结构系综进行测量来抑制由于制造缺陷引起的波动,其中对大量样本进行平均提供了对理想系统的光学特性的精确测量。

英文摘要:

Recent results have shown unprecedented control over separation distances between two metallic elements hundreds of nanometers in size, underlying the effects of free-electron nonlocal response also at mid-infrared wavelengths. Most of metallic systems however, still suffer from some degree of inhomogeneity due to fabrication-induced surface roughness. Nanoscale roughness in such systems might hinder the understanding of the role of microscopic interactions. Here we investigate the effect of surface roughness in coaxial nanoapertures resonating at mid-infrared frequencies. We show that although random roughness shifts the resonances in an unpredictable way, the impact of nonlocal effects can still be clearly observed. Roughness-induced perturbation on the peak resonance of the system shows a strong correlation with the effective gap size of the individual samples. Fluctuations due to fabrication imperfections then can be suppressed by performing measurements on structure ensembles in which averaging over a large number of samples provides a precise measure of the ideal system's optical properties.

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