Magnetic proximity and nonreciprocal current switching in a monolayer WTe2 helical edge
Wenjin Zhao, Zaiyao Fei, Tiancheng Song, Han Kyou Choi, Tauno Palomaki, Bosong Sun, Paul Malinowski, Michael A. McGuire, Jiun-Haw Chu, Xiaodong Xu, David H. Cobden
The integration of diverse electronic phenomena, such as magnetism and nontrivial topology, into a single system is normally studied either by seeking materials that contain both ingredients, or by layered growth of contrasting materials. The ability to simply stack very different two dimensional (2D) van der Waals materials in intimate contact permits a different approach. Here we use this approach to couple the helical edges states in a 2D topological insulator, monolayer WTe2, to a 2D layered antiferromagnet, CrI3. We find that the edge conductance is sensitive to the magnetization state of the CrI3, and the coupling can be understood in terms of an exchange field from the nearest and next-nearest CrI3 layers that produces a gap in the helical edge. We also find that the nonlinear edge conductance depends on the magnetization of the nearest CrI3 layer relative to the current direction. At low temperatures this produces an extraordinarily large nonreciprocal current that is switched by changing the antiferromagnetic state of the CrI3.
Topological insulators (TIs) are bulk insulators that possess robust helical conducting states along their interfaces with conventional insulators. A tremendous research effort has recently been devoted to TI-based heterostructures, in which conventional proximity effects give rise to a series of exotic physical phenomena. This paper reviews our recent works on the potential existence of topological proximity effects at the interface between a topological insulator and a normal insulator or other topologically trivial systems. Using first-principles approaches, we have established the tunabili…
We consider the superconducting proximity effect in a helical Luttinger liquid at the edge of a 2D topological insulator, and derive the low-energy Hamiltonian for an edge state tunnel-coupled to a s-wave superconductor. In addition to correlations between the left and right moving modes, the coupling can induce them inside a single mode, as the spin axis of the edge modes is not necessarily constant. This can be induced controllably in HgTe/CdTe quantum wells via the Rashba spin-orbit coupling, and is a consequence of the 2D nature of the edge state wave function. The distinction of these two…
We study supercurrent and proximity vortices in a Josephson junction made of disordered surface states of a three-dimensional topological insulator with a proximity induced in-plane helical magnetization. In a regime where the rotation period of helical magnetization is larger than the junction width, we find supercurrent 0-π crossovers as a function of junction thickness, magnetization strength, and parameters inherent to the helical modulation and surface states. The supercurrent reversals are associated with proximity induced vortices, nucleated along the junction width, where the number of…
Motivated by recent experiments, we investigate the nonreciprocal magnetoelastic interaction between the surface acoustic phonons of dielectric non-magnetic substrates and magnons of proximity nanomagnets. The magnetization dynamics exerts rotating forces at the edges of the nanomagnet that causes the nonreciprocal interaction with surface phonons due to its rotation-momentum locking. This coupling induces the nonreciprocity of the surface phonon transmission and a nearly complete phonon diode effect by several (tens of) magnetic nanowires of high (ordinary) magnetic quality. Phase-sensitive m…
We propose a device based on a topological Josephson junction where the helical edge states of a two-dimensional topological insulator are in close proximity to two superconducting leads. The presence of a magnetic flux through the junction leads to a Doppler shift in the spectrum of Andreev bound states, and affects the quantum interference between proximized edge states. We inspect the emergent features, accessing the density of states through a tunnel-coupled metallic probe, thus realizing a Topological Superconducting Quantum Interference Proximity Transistor (TSQUIPT). We calculate the ex…
We study the effects of spatially localized breakdown of time reversal symmetry on the surface of a topological insulator (TI) due to proximity to a helical spin density wave (HSDW). The HSDW acts like an externally applied one-dimensional periodic(magnetic) potential for the spins on the surface of the TI, rendering the Dirac cone on the TI surface highly anisotropic. The decrease of group velocity along the direction $\hat{x}$ of the applied spin potential is twice as much as that perpendicular to $\hat{x}$. At the Brillouin zone boundaries (BZB) it also gives rise to new semi-Dirac points w…
Non-centrosymmetric superconductors exhibit the magnetoelectric effect which manifests itself in the appearance of the magnetic spin polarization in response to a dissipationless electric current (supercurrent). While much attention has been dedicated to the thermodynamic version of this phenomenon (Edelstein effect), non-equilibrium transport magnetoelectric effects have not been explored yet. We propose the magnetoelectric Andreev effect (MAE) which consists in the generation of spin-polarized triplet Andreev conductance by an electric supercurrent. The MAE stems from the spin polarization o…
The quantum spin Hall (QSH) state was recently demonstrated in monolayers of the transition metal dichalcogenide 1T'-WTe$_2$ and is characterized by a band gap in the two-dimensional (2D) interior and helical one-dimensional (1D) edge states. Inducing superconductivity in the helical edge states would result in a 1D topological superconductor, a highly sought-after state of matter. In the present study, we use a novel dry-transfer flip technique to place atomically-thin layers of WTe$_2$ on a van der Waals superconductor, NbSe$_2$. Using scanning tunneling microscopy and spectroscopy (STM/STS)…
Non-local pairing processes at the edge of a two-dimensional topological insulator in proximity to an $s$-wave superconductor are usually suppressed by helicity. However, additional proximity of a ferromagnetic insulator can substantially influence the helical constraint and therefore open a new conduction channel by allowing for crossed Andreev reflection (CAR) processes. We show a one-to-one correspondence between CAR and the emergence of odd-frequency triplet superconductivity. Hence, non-local transport experiments that identify CAR in helical liquids yield smoking-gun evidence for unconve…
We consider the proximity effect between a singlet s-wave superconductor and the edge of a Quantum Spin Hall (QSH) topological insulator. We establish that Andreev reflection at a QSH edge state/superconductor interface is perfect while nonlocal Andreev processes through the superconductor are totally suppressed. We compute the corresponding conductance and noise.
Recent angle-resolved photoemission experiments have observed a proximity-induced superconducting gap in the helical surface states of a thin film of the 3D topological insulator Bi$_2$Se$_3$ grown on a superconducting NbSe$_2$ substrate. The superconducting coherence peaks in the electronic density of states are strongly suppressed when the topological insulator is doped with magnetic Mn impurities, which was interpreted as the complete destruction of helical superconductivity in the topological surface states. Motivated by these experiments, we explore a different possibility: gapless helica…
The xene family of topological insulators plays a key role in many proposals for topological electronic, spintronic, and valleytronic devices. These proposals rely on applying local perturbations, including electric fields and proximity magnetism, to induce topological phase transitions in xenes. However, these techniques lack control over the geometry of interfaces between topological regions, a critical aspect of engineering topological devices. We propose adatom decoration as a method for engineering atomically precise topological edge modes in xenes. Our first-principles calculations show …
We experimentally investigate spin-polarized electron transport between a permalloy ferromagnet and the edge of a two-dimensional electron system with band inversion, realized in a narrow, 8~nm wide HgTe quantum well. In zero magnetic field, we observe strong asymmetry of the edge potential distribution with respect to the ferromagnetic ground lead. This result indicates, that the helical edge channel, specific for the structures with band inversion even at the conductive bulk, is strongly coupled to the ferromagnetic side contact, possibly due to the effects of proximity magnetization. It all…
Conformation dependent circular current is investigated in a single handed helical geometry in presence of magnetic flux $ϕ$ within a Hartree-Fock mean field approach. The helical model is described by a set of non-planar rings connected by some vertical bonds where each ring is formed by introducing a non-zero hopping between the atoms $a$ and $b$ as shown in Fig.1. By stretching and compressing the geometry, circular current can be regulated significantly and thus the system can be exploited to design current controlled device at the nano-scale level. The proximity effect between the atomic …
Superconducting proximity pairing in helical edge modes, such as those of topological insulators (TI), is predicted to provide a unique platform for realizing Majorana zero modes (MZMs). We use scanning tunneling microscopy measurements to probe the influence of proximity induced superconductivity and magnetism on the helical hinge states of Bi(111) films, grown on a superconducting Nb substrate and decorated with magnetic Fe clusters. Consistent with model calculations, our measurements reveal the emergence of a localized MZM at the interface between the superconducting helical edge channel a…
We theoretically study the magnetic proximity effect in the three dimensional (3D) topological insulator/ferromagnetic insulator (TI/FMI) structures in the context of possibility to manage the Dirac helical state in TI. Within continual approach based on the $\mathbf{kp}$ Hamiltonian we predict that, when 3D TI is brought into contact with 3D FMI, the ordinary bound state arising at the TI/FMI interface becomes spin polarized due to the orbital mixing at the boundary. Whereas the wave function of FMI decays into the TI bulk on the atomic scale, the induced exchange field, which is proportional…
Topological materials with broken inversion symmetry can give rise to nonreciprocal responses, such as the current rectification controlled by magnetic fields via magnetochiral anisotropy. Bulk nonreciprocal responses usually stem from relativistic corrections and are always very small. Here we report our discovery that ZrTe5 crystals in proximity to a topological quantum phase transition present gigantic magnetochiral anisotropy, which is the largest ever observed to date. We argue that a very low carrier density, inhomogeneities, and a torus-shaped Fermi surface induced by breaking of invers…
The appearance of topologically protected states at the surface of an ordinary insulator is a rare occurrence and to date only a handful of materials are known for having this property. An intriguing question concerns the possibility of forming topologically protected interfaces between different materials. Here we propose that a topological phase can be transferred to graphene by proximity with the three-dimensional topological insulator Bi$_2$Se$_3$. By using density functional and transport theory we prove that, at the verge of the chemical bond formation, a hybrid state forms at the graphe…
A two-dimensional time-reversal symmetric topological superconductor is a fully gapped system possessing a helical Majorana mode on the edges. This helical Majorana edge mode (HMEM), which is a Kramer's pair of two chiral Majorana edge modes in the opposite propagating directions, is robust under time-reversal symmetry protection. We propose a feasible setup and accessible measurement to provide the preliminary step of the HMEM realization by studying superconducting antiferromagnetic quantum spin Hall insulators. Since this antiferromagnetic topological insulator hosts a helical electron edge…
Probing the topological protection of edge states in multilayer tungsten ditelluride with the superconducting proximity effect
Université Paris-Saclay（巴黎萨克雷大学）；CNRS（法国国家科学研究中心）；Princeton University（普林斯顿大学）；Indian Institute of Technology Guwahati（印度理工学院古瓦哈提分校）；Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所，北京凝聚态物理国家实验室）；Laboratoire National de Métrologie et d’Essais（国家计量与测试实验室）
The presence of a Majorana bound state in condensed matter systems is often associated to a zero bias peak in conductance measurements. Here, we analyze a system were this paradigm is violated. A Majorana bound state is always present at the interface between a quantum spin Hall system that is magnetically gapped and a quantum spin Hall system gapped by proximity induced s-wave superconductivity. However, the linear conductance could be either zero or nonzero and quantized depending on the energy and length scales of the barriers. The transition between the two values is reminiscent of the top…
Currently, much effort is being put into detecting unconventional p-wave superconductivity in Josephson junctions based on topological insulators (TIs). For that purpose we propose to use superconducting Klein tunneling, i.e. the reflectionless passage of Cooper pairs through a potential barrier in a gated ballistic junction. This phenomenon occurs due to the fact that the supercurrent is carried by helical Andreev bound states (ABSs) characterized by spin-momentum locking similar to the normal-state carriers. We derive the spectrum of the helical ABSs and the corresponding Josephson current f…
The interplay between bulk spin-orbit coupling and electron-electron interactions produces umklapp scattering in the helical edge states of a two-dimensional topological insulator. If the chemical potential is at the Dirac point, umklapp scattering can open a gap in the edge state spectrum even if the system is time-reversal invariant. We determine the zero-energy bound states at the interfaces between a section of a helical liquid which is gapped out by the superconducting proximity effect and a section gapped out by umklapp scattering. We show that these interfaces pin charges which are mult…
It is shown that the spin-orbit and Zeeman interactions result in phase shifts of Andreev-reflected holes in disordered topological insulator, or normal Rashba spin-orbit-coupled wires, which are in a contact with an s-wave superconductor. Due to interference of the holes reflected through different paths in Andreev interferometer the electric current through the contact varies depending on the strength and direction of the Zeeman field. It also depends on mutual orientations of Zeeman fields in different shoulders of the interferometer. Such a nonlocal effect is a result of the long-range coh…
Two-particle backscattering in time-reversal invariant interacting helical electron systems can lead to the formation of quasiparticles with charge $e/2$. We propose a way to detect such states by means of the Josephson effect in the presence of proximity-induced superconductivity. In this case, the existence of $e/2$ charges leads to an $8 π$-periodic component of the Josephson current which can be identified through measurement of Shapiro steps in Josephson junctions. In particular, we show that even when there is weak explicit time-reversal symmetry breaking, which causes the two-particle b…
We experimentally investigate electron transport through the interface between a superconductor and the edge of a two-dimensional electron system with band inversion. The interface is realized as a tunnel NbN side contact to a narrow 8~nm HgTe quantum well. It demonstrates a typical Andreev behavior with finite conductance within the superconducting gap. Surprisingly, the conductance is modulated by a number of equally-spaced oscillations. The oscillations are present only within the superconducting gap and at lowest, below 1~K, temperatures. The oscillations disappear completely in magnetic f…
We study analytically and numerically spin effects in MoS_2 monolayer armchair quantum wires and quantum dots. The interplay between intrinsic and Rashba spin orbit interactions induced by an electric field leads to helical modes, giving rise to spin filtering in time-reversal invariant systems. The Rashba spin orbit interaction can also be generated by spatially varying magnetic fields. In this case, the system can be in a helical regime with nearly perfect spin polarization. If such a quantum wire is brought into proximity to an s-wave superconductor, the system can be tuned into a topologic…
We theoretically study graphene nanoribbons in the presence of spatially varying magnetic fields produced e.g. by nanomagnets. We show both analytically and numerically that an exceptionally large Rashba spin orbit interaction (SOI) of the order of 10 meV can be produced by the non-uniform magnetic field. As a consequence, helical modes exist in armchair nanoribbons that exhibit nearly perfect spin polarization and are robust against boundary defects. This paves the way to realizing spin filter devices in graphene nanoribbons in the temperature regime of a few Kelvins. If a nanoribbon in the h…
Chiral and helical Majorana edge modes are two archetypal gapless excitations of two-dimensional topological superconductors. They belong to superconductors from two different Altland-Zirnbauer symmetry classes characterized by $\mathbb{Z}$ and $\mathbb{Z}_2$ topological invariant respectively. It seems improbable to tune a pair of co-propagating chiral edge modes to counter-propagate without symmetry breaking. Here we show that such a direct topological transition is in fact possible, provided the system possesses an additional symmetry $\mathcal{O}$ which changes the bulk topological invaria…
We present results for asymptotic freedom like behavior for the topological state of the helical spin liquid system with finite proximity induced superconducting gap. We derive two different quantum Berezinskii-Kosterlitz-Thouless (BKT) equations for the two different limit of this model Hamiltonian. The common quantum phase for these two quantum BKT transitions is the helical Luttinger liquid phase where there is no evidence of asymptotic freedom. There is no evidence of superconductor-insulator transition for this asymptotic freedom study. We observe the evidance of asymptotic freedom for th…
We determine the nature of the magnetic order on the surface of a topological insulator (TI) which develops due to hexagonal warping and the resulting Fermi surface (FS) nesting in the presence of a repulsive Hubbard interaction. For this purpose we investigate the spin susceptibility and derive a Landau theory to compare the different accessible phases. For a nearly hexagonal FS and sufficiently strong interaction the magnetic ground state is formed by a skyrmion lattice, i.e., by a superposition of three helical spin density waves which preserves C$_3$ symmetry. The magnetic ground state is …
Superconducting diode effect, in analogy to the nonreciprocal resistive charge transport in semiconducting diode, is a nonreciprocity of dissipationless supercurrent. Such an exotic phenomenon originates from intertwining between symmetry-constrained supercurrent transport and intrinsic quantum functionalities of helical/chiral superconductors. In this article, research progress of superconducting diode effect including fundamental concepts, material aspects, device prospects, and theoretical/experimental development is reviewed. First, fundamental mechanisms to cause superconducting diode eff…
Electrical currents in a quantum spin Hall insulator are confined to the boundary of the system. The charge carriers can be described as massless relativistic particles, whose spin and momentum are coupled to each other. While the helical character of those states is by now well established experimentally, it is a fundamental open question how those edge states interact with each other when brought in spatial proximity. We employ a topological quantum point contact to guide edge channels from opposite sides into a quasi-one-dimensional constriction, based on inverted HgTe quantum wells. Apart …
Nanosculpted 3D helices of a magnetic Weyl semimetal with switchable nonreciprocity
RIKEN Center for Emergent Matter Science (CEMS)（RIKEN 新兴物质科学中心）；Department of Applied Physics, The University of Tokyo（东京大学应用物理系）；RIKEN Fundamental Science Program（RIKEN 基础科学项目）；Tokyo College, The University of Tokyo（东京大学东京学院）
Large Field-Free Superconducting Diode Effect with Nonmonotonic Polarity Reversals in NbSe$_2$/CrBr$_3$ Heterostructures
Southern University of Science and Technology（南方科技大学）；International Quantum Academy, and Shenzhen Branch, Hefei National Laboratory（国际量子科学院，合肥国家实验室深圳分院）；Eastern Institute for Advanced Study, Eastern Institute of Technology（宁波东方理工大学（暂名）先进研究院）；State Key Laboratory of Optoelectronic Materials and Technologies, Sun Yat‑sen University（中山大学光电信息材料与技术国家重点实验室）
We present a comparative study of pair correlations and currents through superconducting-magnetic hybrid systems with a particular emphasis on the tunable Bloch domain wall of an exchange spring. This study of the Gor'kov functions contrasts magnetic systems with domain walls that change at discrete points in the magnetic region with those that change continuously throughout. We present results for misaligned homogeneous magnetic multilayers, including spin valves, for discrete domain walls, as well as exchange springs and helical domain walls --such as Holmium-- for the continuous case. Intro…
