Developing future quantum communication may rely on the ability to engineer cavity-mediated interactions between photons and solid-state artificial atoms, in a deterministic way. Here, we report a set of technological and experimental developments for the deterministic coupling between the optical mode of a micropillar cavity and a quantum dot trion transition. We first identify a charged transition through in-plane magnetic field spectroscopy, and then tune the optical cavity mode to its energy via in-situ lithography. In addition, we design an asymmetric tunneling barrier to allow the optical trapping of the charge, assisted by a quasi-resonant pumping scheme, in order to control its occupation probability. We evaluate the generation of a positively-charged quantum dot through second order auto-correlation measurements of its resonance fluorescence, and the quality of light-matter interaction for these spin-photon interfaces is assessed by measuring the performance of the device as a single-photon source.
We measure the detuning-dependent dynamics of a quasi-resonantly excited single quantum dot coupled to a micropillar cavity. The system is modeled with the dissipative Jaynes-Cummings model where all experimental parameters are determined by explicit measurements. We observe non-Markovian dynamics when the quantum dot is tuned into resonance with the cavity leading to a non-exponential decay in time. Excellent agreement between experiment and theory is observed with no free parameters providing the first quantitative description of an all-solid-state cavity QED system based on quantum dot emit…
We study the optical properties of coupled quantum dot-microcavity systems with elliptical cross section. First, we develop an analytic model that describes the spectrum of the cavity modes that are split due to the reduced symmetry of the resonator. By coupling the QD emission to the polarized fundamental cavity modes, we observe the vectorial nature of the Purcell enhancement, which depends on the intrinsic polarization of the quantum dot and its relative alignment with respect to the cavity axis. The variable interaction strength of the QD with the polarized cavity modes leads to the observ…
We theoretically describe the quantum Zeno effect in a spin-photon interface represented by a charged quantum dot in a micropillar cavity. The electron spin in this system entangles with the polarization of the transmitted photons, and their continuous detection leads to the slowing of the electron spin precession in external magnetic field and induces the spin relaxation. We obtain a microscopic expression for the spin measurement rate and calculate the second and fourth order correlation functions of the spin noise, which evidence the change of the spin statistics due to the quantum Zeno eff…
We report on the observation of bright emission of single photons under pulsed resonance fluorescence conditions from a single quantum dot (QD) in a micropillar cavity. The brightness of the QD fluorescence is greatly enhanced via the coupling to the fundamental mode of a micropillar, allowing us to determine a single photon extraction efficiency of $(20.7\pm0.8)~\%$ per linear polarization basis. This yields an overall extraction efficiency of $(41.4\pm1.5)~\%$ in our device. We observe the first Rabi-oscillation in a weakly coupled quantum dot-micropillar system under coherent pulsed optical…
We demonstrate a technique to tune the optical properties of micropillar cavities by creating small defects on the sample surface near the cavity region with an intense focused laser beam. Such defects modify strain in the structure, changing the birefringence in a controllable way. We apply the technique to make the fundamental cavity mode polarization-degenerate and to fine tune the overall mode frequencies, as needed for applications in quantum information science.
We present a new micromechanical resonator designed for cavity optomechanics. We have used a micropillar geometry to obtain a high-frequency mechanical resonance with a low effective mass and a very high quality factor. We have coated a 60-$μ$m diameter low-loss dielectric mirror on top of the pillar and are planning to use this micromirror as part of a high-finesse Fabry-Perot cavity, to laser cool the resonator down to its quantum ground state and to monitor its quantum position fluctuations by quantum-limited optical interferometry.
The generation of photon pairs in single quantum dots is based on a process that is, in its nature, deterministic. However, an efficient extraction of these photon pairs from a high-index semiconductor host material requires engineering of the photonic environment. We report on a micropillar-based device featuring an extraction efficiency of 69.4(10)$\%$ that is achieved by harnessing a broadband operation suitable for extraction of photon pairs emitted from a single quantum dot. Opposing the approaches that rely solely on Purcell enhancement to realize the enhancement of the extraction effici…
We report on the spectroscopic investigation of quantum dot - micropillar cavities with unprecedented quality factors. We observe a pronounced dependency of the quality factor on the measurement scheme, and find that significantly larger quality factors can be extracted in photoreflectance compared to photoluminescence measurements. While the photoluminescence spectra of the microcavity resonances feature a Lorentzian lineshape and Q-factors up to 184,000, the reflectance spectra have a Fano-shaped asymmetry and feature significantly higher Q-factors in excess of 250,000 resulting from a full …
Scalable quantum photonic architectures demand highly efficient, high-purity single-photon sources, which can be frequency matched via external tuning. We demonstrate a single-photon source based on an InAs quantum dot embedded in a micropillar resonator, which is frequency tunable via externally-applied stress. Our platform combines the advantages of a Bragg micropillar cavity and the piezo-strain-tuning technique enabling single photon spontaneous emission enhancement via the Purcell effect and quantum dot (QD) with tunable wavelength. Our optomechanical platform has been implemented by inte…
Dynamical decoupling of a quantum dot spin in a micropillar cavity for spin-multiphoton entanglement
Université Paris-Saclay（巴黎萨克雷大学）；Centre de Nanosciences et de Nanotechnologies, CNRS（国家科学研究中心纳米科学和纳米技术研究中心）；Quandela SAS（Quandela公司）；Johns Hopkins Applied Physics Laboratory（约翰斯·霍普金斯大学应用物理实验室）；University of Delaware（特拉华大学）
We report optical positioning single quantum dots (QDs) in planar cavity with an average position uncertainty $<$20 nm using an optimized two-color photoluminescence imaging technique. We create single-photon sources based on these QDs in determined micropillar cavities. The brightness of the QD fluorescence is greatly enhanced on resonance with the fundamental mode of the cavity, leading to an high extraction efficiency of 68%$\pm$6% into a lens with numerical aperture of 0.65, and simultaneously exhibiting low multi-photon probability ($g^{2}(0)$=0.144$\pm$0.012) at this collection efficienc…
The implementation and engineering of bright and coherent solid state quantum light sources is key for the realization of both on chip and remote quantum networks. Despite tremendous efforts for more than 15 years, the combination of these two key prerequisites in a single, potentially scalable device is a major challenge. Here, we report on the observation of bright and coherent single photon emission generated via pulsed, resonance fluorescence conditions from a single quantum dot (QD) deterministically centered in a micropillar cavity device via cryogenic optical lithography. The brightness…
We present here precise measurement of the resonance frequency, lifetime and shape of confined acoustic modes in the tens of GHz regime in GaAs/AlAs superlattice planar and micropillar cavities at low temperature ($\sim 20\,\textrm{K}$). The subharmonic resonant pump-probe technique, where the repetition rate of the pump laser is tuned to a subharmonic of the cavity resonance to maximize the amplitude of the acoustic resonance, in combination with a Sagnac interferometer technique for high sensitivity ($\sim 10 \,\textrm{fm}$) to the surface displacement, has been used. The cavity fundamental …
We have fabricated pillar microcavity samples with Bragg mirrors consisting of alternate layers of GaAs and Aluminium Oxide. Compared to the more widely studied GaAs/AlAs micropillars these mirrors can achieve higher reflectivities with fewer layer repeats and reduce the mode volume. We have studied a number of samples containing a low density of InGaAs/GaAs self assembled quantum dots in a cavity and here report observation of a three fold enhancement in the radiative lifetime of a quantum dot exciton state due to the Purcell effect.
We present detuning-dependent spectral and decay-rate measurements to study the difference between spectral and dynamical properties of single quantum dots embedded in micropillar and photonic-crystal cavities. For the micropillar cavity, the dynamics is well described by the dissipative Jaynes-Cummings model, while systematic deviations are observed for the emission spectra. The discrepancy for the spectra is attributed to coupling of other exciton lines to the cavity and interference of different propagation paths towards the detector of the fields emitted by the quantum dot. In contrast, qu…
The large coupling rate between the acoustic and optical fields confined in GaAs/AlAs superlattice cavities makes them appealing systems for cavity optomechanics. We have developed a mathematical model based on the scattering matrix that allows the acoustic guided modes to be predicted in nano and micropillar superlattice cavities. We demonstrate here that the reflection at the surface boundary considerably modifies the acoustic quality factor and leads to significant confinement at the micropillar center. Our mathematical model also predicts unprecedented acoustic Fano resonances on nanopilla…
In an oxide apertured quantum dot (QD) micropillar cavity-QED system, we found strong QD hysteresis effects and lineshape modifications even at very low intensities corresponding to less than 0.001 intracavity photons. We attribute this to the excitation of charges by the intracavity field; charges that get trapped at the oxide aperture, where they screen the internal electric field and blueshift the QD transition. This in turn strongly modulates light absorption by cavity QED effects, eventually leading to the observed hysteresis and lineshape modifications. The cavity also enables us to obse…
We demonstrate the simultaneous dressing of both vacuum-to-exciton and exciton-to-biexciton transitions of a single semiconductor quantum dot in a high-Q micropillar cavity, using photoluminescence spectroscopy. Resonant two-photon excitation of the biexciton is achieved by spectrally tuning the quantum dot emission with respect to the cavity mode. The cavity couples to both transitions and amplifies the Rabi-frequency of the likewise resonant cw laser, driving the transitions. We observe strong-field splitting of the emission lines, which depend on the driving Rabi field amplitude and the cav…
A quantum mechanical superposition of a long-lived, localized phonon and a matter excitation is described. We identify a realization in strained silicon: a low-lying donor transition (P or Li) driven solely by acoustic phonons at wavelengths where high-Q phonon cavities can be built. This phonon-matter resonance is shown to enter the strongly coupled regime where the "vacuum" Rabi frequency exceeds the spontaneous phonon emission into non-cavity modes, phonon leakage from the cavity, and phonon anharmonicity and scattering. We introduce a micropillar distributed Bragg reflector Si/Ge cavity, w…
A two-level system that is coupled to a high-finesse cavity in the Purcell regime exhibits a giant optical non-linearity due to the saturation of the two-level system at very low intensities, of the order of one photon per lifetime. We perform a detailed analysis of this effect, taking into account the most important practical imperfections. Our conclusion is that an experimental demonstration of the giant non-linearity should be feasible using semiconductor micropillar cavities containing a single quantum dot in resonance with the cavity mode.
Levitated nanospheres in optical cavities open a novel route to study many-body systems out of solution and highly isolated from the environment. We show that properly tuned optical parameters allow for the study of the non-equilibrium dynamics of composite nano-particles with non-isotropic optical friction. We find friction induced ordering and nematic transitions with non-equilibrium analogs to liquid crystal phases for ensembles of dimers.
We demonstrate a technique for achieving spectral resonance between a polarization-degenerate micropillar cavity mode and an embedded quantum dot transition. Our approach is based on a combination of isotropic and anisotropic tensile strain effected by laser-induced surface defects, thereby providing permanent tuning. Such a technique is a prerequisite for the implementation of scalable quantum information schemes based on solid-state cavity quantum electrodynamics.
The key challenge to scalable optical quantum computing, boson sampling, and quantum metrology is sources of single photons with near-unity system efficiency and simultaneously near-perfect indistinguishability in all degrees of freedom (including spectral, temporal, spatial, and polarization). However, previous high-indistinguishability solid-state single-photon sources had to rely on polarization filtering that reduced the system efficiency by at least 50%. Here, we overcome this challenge by developing a new single-photon source based on a coherently driven quantum dot embedded in an ellipt…
Pure and bright single photon sources have recently been obtained by inserting solid-state emitters in photonic nanowires or microcavities. The cavity approach presents the attractive possibility to greatly increase the source operation frequency. However, it is perceived as technologically demanding because the emitter resonance must match the cavity resonance. Here we show that the spectral matching requirement is actually strongly lifted by the intrinsic coupling of the emitter to its environment. A single photon source consisting of a single InGaAs quantum dot inserted in a micropillar cav…
We study a system comprising of a double quantum well embedded in a micropillar optical cavity, where strong coupling between a direct exciton, indirect exciton, and cavity photon is achieved. We show that the resulting hybrid quasiparticles - dipolaritons - can induce strong photon correlations and lead to anti-bunched behaviour of the cavity output field. The origin of the observed single photon emission is attributed to unconventional photon blockade. Moreover, we find that the second-order equal time correlation function $g^{(2)}(0)$ can be tuned over a large range using an electric field …
Giant optical nonlinearity is observed under both continuous-wave and pulsed excitation in a deterministically-coupled quantum dot-micropillar system, in a pronounced strong-coupling regime. Using absolute reflectivity measurements we determine the critical intracavity photon number as well as the input and output coupling efficiencies of the device. Thanks to a near-unity input-coupling efficiency, we demonstrate a record nonlinearity threshold of only 8 incident photons per pulse. The output-coupling efficiency is found to strongly influence this nonlinearity threshold. We show how the funda…
The excitonic fine structure plays a key role for the quantum light generated by semiconductor quantum dots, both for entangled photon pairs and single photons. Controlling the excitonic fine structure has been demonstrated using electric, magnetic, or strain fields, but not for quantum dots in optical cavities, a key requirement to obtain high source efficiency and near-unity photon indistinguishability. Here, we demonstrate the control of the fine structure splitting for quantum dots embedded in micropillar cavities. We propose a scheme based on remote electrical contacts connected to the pi…
The emerging hybrid integrated quantum photonics combines advantages of different functional components into a single chip to meet the stringent requirements for quantum information processing. Despite the tremendous progress in hybrid integrations of III-V quantum emitters with silicon-based photonic circuits and superconducting single-photon detectors, on-chip optical excitations of quantum emitters via miniaturized lasers towards single-photon sources (SPSs) with low power consumptions, small device footprints and excellent coherence properties is highly desirable yet illusive. In this work…
It is usually assumed that when performing a photoluminescence experiment on a microcavity containing an inhomogeneously broadened quantum dots ensemble, the cavity mode appears as a positive peak with a linewidth that reflects the mode quality factor Q. We show in this article that this conclusion is in general not true, and that the measured mode linewidth depends strongly on the excitation power for microcavities having large Purcell factors. We analyze theoretically this effect in the case of the micropillar cavity and we show that the same microcavity can give rise to a large variety of p…
Recently, experiments showed that the spatial-mode states of entangled photons are more robust than their polarization-mode states in quantum communications. Here we construct a complete and deterministic protocol for analyzing the spatial Bell states using the interaction between a photon and an electron spin in a charged quantum dot inside a one-side micropillar microcavity. A quantum nondemolition detector (QND) for checking the parity of a two-photon system can be constructed with the giant optical Faraday rotation in this solid state system. With this parity-check QND, we present a comple…
We discuss the efficiency of single photon sources based on a single quasi-monochromatic emitter (such as a semiconductor quantum dot) inserted in a pillar microcavity. We show that their efficiency, which is in principle excellent thanks to the Purcell effect, can be drastically limited by extrinsic cavity losses, such as those related to the scattering by the sidewalls roughness. We present novel design rules for micropillars in view of this application and show that for the well-mastered GaAs/AlAs system more than 70% of the emission can be concentrated into the collimated emission beam ass…
Spin-to-polarization mapping with a coherent quantum dot-cavity receiver
Université Paris-Saclay（巴黎萨克雷大学）；CNRS（法国国家科学研究中心）；Centre de Nanosciences et de Nanotechnologies（纳米科学与纳米技术中心）；Université Paris Cité（巴黎西岱大学）；ICFO-Institut de Ciencies Fotoniques（光子科学研究所）；The Barcelona Institute of Science and Technology（巴塞罗那科学技术研究所）；Quandela（量子达）
We discuss the fine-tuning of the optical properties of self-assembled quantum dots by the strain perturbation introduced by laser-induced surface defects. We show experimentally that the quantum dot transition red-shifts, independently of the actual position of the defect, and that such frequency shift is about a factor five larger than the corresponding shift of a micropillar cavity mode resonance. We present a simple model that accounts for these experimental findings.
The interaction of a single quantum emitter with its environment is a central theme in quantum optics. When placed in highly confined optical fields, such as those created in optical cavities or plasmonic structures, the optical properties of the emitter can change drastically. In particular, photonic crystal (PC) cavities show high quality factors combined with an extremely small mode volume. Efficiently coupling a single quantum emitter to a PC cavity is challenging because of the required positioning accuracy. Here, we demonstrate deterministic coupling of single Nitrogen-Vacancy (NV) cente…
A high-fidelity source of identical single photons is essential for numerous quantum technologies such as quantum repeaters and optical quantum information processing. Hallmarks thereof are a near-unity single-photon purity, near-unity indistinguishability of consecutively emitted photons, and high brightness through a near-unity number of photons per time bin. In order to embed such sources in quantum networks, optical fiber integration is essential but complicated by cryogenic compatability and noise. Here we demonstrate a resonantly pumped, quantum dot (QD) based, transmission operated, sin…
An electro-optomechanical device capable of microwave-to-optics conversion has recently been demonstrated, with the vision of enabling optical networks of superconducting qubits. Here we present an improved converter design that uses a three-dimensional (3D) microwave cavity for coupling between the microwave transmission line and an integrated LC resonator on the converter chip. The new design simplifies the optical assembly and decouples it from the microwave part of the setup. Experimental demonstrations show that the modular device assembly allows us to flexibly tune the microwave coupling…
In fiber based Fabry-Pérot Cavities (FFPCs), limited spatial mode matching between the cavity mode and input/output modes has been the main hindrance for many applications. We have demonstrated a versatile mode matching method for FFPCs. Our novel design employs an assembly of a graded-index and large core multimode fiber directly spliced to a single mode fiber. This all-fiber assembly transforms the propagating mode of the single mode fiber to match with the mode of a FFPC. As a result, we have measured a mode matching of 90\% for a cavity length of $\sim$400 $μm$. This is a significant impro…
We demonstrate unambiguous entangling operation of a photonic quantum-logic gate driven by an ultrabright solid-state single-photon source. Indistinguishable single photons emitted by a single semiconductor quantum dot in a micropillar optical cavity are used as target and control qubits. For a source brightness of 0.56 collected photons-per-pulse, the measured truth table has an overlap with the ideal case of 68.4%, increasing to 73.0% for a source brightness of 0.17 photons- per-pulse. The gate is entangling: at a source brightness of 0.48, the Bell-state fidelity is above the entangling thr…
We describe an assembly of N Cooper-pair boxes (CPB) contained in a single mode cavity. In the dispersive regime, the correlation between the cavity field and each Cooper-pair box results in an effective interaction between CPBs that can be used to dynamically generate maximally entangled states. With only collective manipulations, we show how to create maximally entangled quantum states and how to use these states to reach the Heisenberg limit in the determination of a spectroscopy frequency. This scheme can be applied to other types of superconducting qubits.
We exploit the nonlinearity arising from the spin-photon interaction in an InAs quantum dot to demonstrate phase shifts of scattered light pulses at the single-photon level. Photon phase shifts of close to 90 degrees are achieved using a charged quantum dot in a micropillar cavity. We also demonstrate a photon phase switch by using a spin-pumping mechanism through Raman transitions in an in-plane magnetic field. The experimental findings are supported by a theoretical model which explores the dynamics of the system. Our results demonstrate the potential of quantum dot-induced nonlinearities fo…
We describe an assembly of N superconducting qubits contained in a single-mode cavity. In the dispersive regime, the correlation between the cavity field and each qubit results in an effective interaction between qubits that can be used to dynamically generate maximally entangled states. With only collective manipulations, we show how to create maximally entangled quantum states and how to use these states to reach the Heisenberg limit in the determination of the qubit bias control parameter (gate charge for charge qubits, external magnetic flux for rf-SQUIDs).
We consider a quantum gas of non-interacting particles confined in the expanding cavity, and investigate the nature of the non-adiabatic force which is generated from the gas and acts on the cavity wall. Firstly, with use of the time-dependent canonical transformation which transforms the expanding cavity to the non-expanding one, we can define the force operator. Secondly, applying the perturbative theory which works when the cavity wall begins to move at time origin, we find that the non-adiabatic force is quadratic in the wall velocity and thereby does not break the time-reversal symmetry, …
Over the past decade, strong interactions of light and matter at the single-photon level have enabled a wide set of scientific advances in quantum optics and quantum information science. This work has been performed principally within the setting of cavity quantum electrodynamics with diverse physical systems, including single atoms in Fabry-Perot resonators, quantum dots coupled to micropillars and photonic bandgap cavities, and Cooper-pairs interacting with superconducting resonators. Experiments with single, localized atoms have been at the forefront of these advances with the use of optica…
We report a system where fixed interactions between non-computational levels make bright the otherwise forbidden two-photon 00 --> 11 transition. The system is formed by hand selection and assembly of two discrete component transmon-style superconducting qubits inside a rectangular microwave cavity. The application of a monochromatic drive tuned to this transition induces two-photon Rabi-like oscillations between the ground and doubly-excited states via the Bell basis. The system therefore allows all-microwave two-qubit universal control with the same techniques and hardware required for singl…
