We study the superconducting instability in disordered non-centrosymmetric monolayers with intrinsic Ising spin-orbit coupling (SOC) subjected to an in-plane Zeeman magnetic field. The pairing interaction contains the channels allowed by crystal symmetry, such that in general, the pairing state is a mixture of singlet and triplet Cooper pairs. The joint action of SOC and Zeeman field selects a specific in-plane $\mathbf{d}$-vector triplet component to couple with the singlets, which gains robustness against disorder through the coupling. The out-of-plane $\mathbf{d}$-vector component, that in the clean case is immune to both the Zeeman field and SOC is obliterated by a very small impurity scattering rate. We formulate the quasi-classical theory of Ising superconductors and solve the linearized Eilenberger equations to obtain the pair-breaking equations that determine the Zeeman field -- temperature dependence of the continuous superconducting transition. Our discussion emphasizes how the Zeeman field, SOC and disorder affect the different superconducting order parameters, and we show how the spin-fields inevitably induce odd-frequency pairing correlations.
The few-layer transition metal dichalcogenides (TMDs) have been recently suggested as a platform for controlled unconventional superconductivity. We study the manifestations of unconventional triplet pairing in the density of states of a disordered TMD based monolayer. The conventional singlet pairing attraction is assumed to be the dominant pairing interaction. We map the phase diagrams of disordered Ising superconductors in the plane of temperature and the in-plane magnetic field. The latter suppresses singlet and promote triplet correlations. The triplet order parameters of a trivial (non-t…
We theoretically study the electronic transport through a ferromagnet-Ising superconductor junction. A tight-binding Hamiltonian describing the Ising superconductor is presented. Then by combing the non-equilibrium Green's function method, the expressions of Andreev reflection coefficient and conductance are obtained. A strong magnetoanisotropic spin-triplet Andreev reflection is shown, and the magnetoanisotropic period is $π$ instead of $2π$ as in the conventional magnetoanisotropic system. We demonstrate a significant increase of the spin-triplet Andreev reflection for the single-band Ising …
In conventional Bardeen-Cooper-Scrieffer (BCS) superconductors, Cooper pairs of electrons of opposite spin (i.e. singlet structure) form the ground state. Equal spin triplet pairs (ESTPs), as in superfluid $^3$He, are of great interest for superconducting spintronics and topological superconductivity, yet remain elusive. Recently, odd-parity ESTPs were predicted to arise in (few-)monolayer superconducting NbSe$_2$, from the non-colinearity between the out-of-plane Ising spin-orbit field (due to the lack of inversion symmetry in monolayer NbSe$_2$) and an applied in-plane magnetic field. These …
Ising superconductivity, observed experimentally in NbSe$_{2}$ and similar materials, has generated tremendous interest. Recently, attention was called to the possible role that spin fluctuations (SF) play in this phenomenon, in addition to the dominant electron-phonon coupling (EPC); the possibility of a predominantly-triplet state was discussed and led to a conjecture of viable singlet-triplet Leggett oscillations. However, these hypotheses have not been put to a quantitative test. In this paper, we report first principle calculations of the EPC and also estimate coupling with SF, including …
In monolayer transition metal dichalcogenides (TMDs), electrons in opposite $K$ valleys are subject to opposite effective Zeeman fields, which are referred to as Ising spin-orbit coupling (SOC) fields. The Ising SOC, originated from in-plane mirror symmetry breaking pins the electron spins in out-of-plane directions, and results in the newly discovered Ising superconducting states with strongly enhanced upper critical fields. In this work, we show that the Ising SOC generates equal-spin triplet Cooper pairs with spin polarization in the in-plane directions. Importantly, the spin-triplet Cooper…
An in-plane magnetic field applied to an Ising superconductor converts spin-singlet Cooper pairs to spin-triplet ones. In this work, we study a Josephson junction formed by two Ising superconductors that are proximitized by ferromagnetic layers. This leads to highly tunable spin-triplet pairing correlations which allow to modulate the charge and spin supercurrents through the in-plane magnetic exchange fields. For a junction with a nonmagnetic barrier, the charge current is switchable by changing the relative alignment of the in-plane exchange fields, and a $π$-state can be realized. Furthermo…
Recent experiments in quantum critical heavy fermion metals have pushed to the fore the question about whether antiferromagnetic fluctuations can promote both spin-singlet and spin-triplet superconductivity. Here we address the issue through non-perturbative calculations in antiferromagnetically correlated Kondo systems. We identify Kondo-destruction quantum critical points in both the SU(2) symmetric and Ising-anisotropic cluster Bose-Fermi Anderson models. The spin-singlet pairing correlations are significantly enhanced near the quantum critical point in the SU(2) case; however, with adequat…
In the theory of dilute magnetic impurities in superconductors, the effect of all impurity spin-components is expressed via a single magnetic scattering rate $Γ_\mathrm{m}$. In a more realistic setting, magnetic impurities are anisotropic. In this case, the spatial randomness of three spin-components of impurities gives rise to generally different scattering rates $Γ_i$ ($i=1,2,3$). We explore the effects of anisotropic magnetic impurities on the in-plane critical field in 2D superconductors. We discuss singlet, triplet and parity-mixed order parameters allowed in systems without the inversion…
We show that an in-plane Zeeman field applied to non-centrosymmetric Ising superconductors converts singlet $s$-wave Cooper pairs to equal-spin triplet $if$ pairs, leading to an enhancement of the critical transition line beyond expected from Ising spin-orbit coupling. Singlet to triplet conversion relates to a phase transformation due to spin rotation by the Zeeman field and has a geometric origin. The discussion is especially relevant, but not limited to monolayer transition metal dichalcogenides.
Superconductivity is commonly destroyed by a magnetic field due to orbital or Zeeman-induced pair breaking. Surprisingly, the spin-valley locking in a two-dimensional superconductor with spin-orbit interaction makes the superconducting state resilient to large magnetic fields. We investigate the spectral properties of such an Ising superconductor in a magnetic field taking into account disorder. The interplay of the in-plane magnetic field and the Ising spin-orbit coupling leads to noncollinear effective fields. We find that the emerging singlet and triplet pairing correlations manifest themse…
We theoretically study the superconducting properties of multi-band two-dimensional transition metal oxide superconductors by analyzing not only the role played by conventional singlet pairings, but also by the triplet order parameters, favored by the spin-orbit couplings present in these ma- terials. In particular, we focus on the two-dimensional electron gas at the (001) interface between LaAlO3 and SrTiO3 band insulators where the low electron densities and the sizeable spin-orbit couplings affect the superconducting features. Our theoretical study is based on an extended su- perconducting …
We show that Majorana edge modes of two-dimensional spin-triplet topological superconductors have Ising-like spin density whose direction is determined by the d-vector characterizing the spin-triplet pairing symmetry. Exchange coupling between an impurity spin (S=1/2) and Majorana edge modes is thus Ising-type. Under external magnetic field perpendicular to the Ising axis, the system can be mapped to a two-level system with Ohmic dissipation, which is equivalent to the anisotropic Kondo model. The magnetic response of the impurity spin can serve as a local experimental probe for the order para…
Topological Ising superconductivity in two-dimensional p-wave magnet
Asia Pacific Center for Theoretical Physics（亚太理论物理中心）；Pohang University of Science and Technology（浦项科技大学）；The University of Melbourne（墨尔本大学）；Hanyang University（汉阳大学）；Research Institute for Natural Science and High Pressure, Hanyang University（汉阳大学自然科学高压研究所）
In this paper we extend our earlier analysis of the novel Josephson effect in triplet superconductor--ferromagnet--triplet superconductor (TFT) junctions [B. Kastening \emph{et al.}, Phys. Rev. Lett. {\bf{96}}, 047009 (2006)]. In our more general formulation of the TFT junction we allow for potential scattering at the barrier and an arbitrary orientation of the ferromagnetic moment. Several new effects are found upon the inclusion of these extra terms: for example, we find that a Josephson current can flow even when there is vanishing phase difference between the superconducting condensates on…
Nonrelativistic-Ising superconductivity in p-wave magnets
Racah Institute of Physics, Hebrew University of Jerusalem（拉卡物理研究所，耶路撒冷希伯来大学）；Materials Science Division, Argonne National Laboratory（材料科学部，阿贡国家实验室）；Max Planck Institute for the Physics of Complex Systems（马克斯·普朗克复杂系统物理研究所）；Max Planck Institute for Chemical Physics of Solids（马克斯·普朗克固体化学物理研究所）；Institute of Physics, Academy of Sciences of the Czech Republic（捷克科学院物理研究所）；Department of Physics and Astronomy, George Mason University（乔治梅森大学物理与天文学系）；Quantum Science and Engineering Center, George Mason University（乔治梅森大学量子科学与工程中心）
We study the electrodynamics of spin triplet superconductors including dipolar interactions, which give rise to an interplay between the collective spin dynamics of the condensate and orbital Meissner screening currents. Within this theory, we identify a class of spin waves that originate from the coupled dynamics of the spin-symmetry breaking triplet order parameter and the electromagnetic field. In particular, we study magnetostatic spin wave modes that are localized to the sample surface. We show that these surface modes can be excited and detected using experimental techniques such as micr…
We study a mechanism for superconductivity in quasi-one-dimensional materials with Ising anisotropy. In an isolated chain Ising anisotropy opens a spin gap; if inter-chain coupling is sufficiently weak, single particle hopping is suppressed and the physics of coupled chains is controlled by a competition between pair hopping and exchange interaction. Spin density wave and triplet superconductivity phases are found separated by a first order phase transition. For particular parameter values a second order transition described by SO(4) symmetry is found.
Non-equilibrium studies of two-dimensional (2D) superconductors (SCs) with Ising spin-orbit coupling are prerequisite for their successful application to equilibrium spin-triplet Cooper pairs and, potentially, Majorana fermions. By taking advantage of the recent discoveries of 2D SCs and their compatibility with any other materials, we fabricate here non-local magnon devices to examine how such 2D Ising superconductivity affects the conversion efficiency of magnon spin to quasiparticle charge in superconducting flakes of 2H-NbSe2 transferred onto ferrimagnetic insulating Y3Fe5O12. Comparison w…
The interplay between antiferromagnetism and d-wave superconductivity is studied in a mean-field approximation for a generic microscopic Hamiltonian with short-range repulsion and near-neighbor attraction. In the presence of competing microscopic interactions, the phase boundaries of antiferromagnetic and superconducting states are significantly modified in some region of the doping-temperature plane. The transition between superconductivity and antiferromagnetism occurs through a phase where both order parameters coexist with a third, dynamically generated, spin-triplet amplitude. This dynami…
We study the interplay of spin and charge coherence in a single-level quantum dot. A tunnel coupling to a superconducting lead induces superconducting correlations in the dot. With full spin symmetry retained, only even-singlet superconducting correlations are generated. An applied magnetic field or attached ferromagnetic leads partially or fully reduce the spin symmetry, and odd-triplet superconducting correlations are generated as well. For single-level quantum dots, no other superconducting correlations are possible. We analyze, with the help of a diagrammatic real-time technique, the inter…
We present theoretical results on the interplay of magnetic and superconducting orders in diffusive ferromagnet-superconductor-ferromagnet trilayers. The induced triplet superconducting correlations throughout the trilayer lead to an induced spin magnetization. We include self-consistency of the order parameter in the superconducting layer at arbitrary temperatures, arbitrary interface transparency, and any relative orientation of the exchange fields in the two ferromagnets. We propose to use the torque on the trilayer in an external magnetic field as a probe of the presence of triplet correla…
We discuss the possibility of coexistence of spin density wave (antiferromagnetism) and triplet superconductivity as a particular example of a broad class of systems where the interplay of magnetism and superconductivity is important. We focus on the case of quasi-one-dimensional metals, where it is known experimentally that antiferromagnetism is in close proximity to triplet superconductivity in the temperature versus pressure phase diagram. Over a narrow range of pressures, we propose an intermediate non-uniform phase consisting of alternating antiferromagnetic and triplet superconducting st…
Surface-Selective Probe of Spin-Triplet Superconductivity in Rhombohedral Graphene
Institute of Physics, École Polytechnique Fédérale de Lausanne (EPFL)（洛桑联邦理工学院物理研究所）；Department of Applied Physics, Aalto University School of Science（阿尔托大学理学院应用物理系）；Research Center for Functional Materials, National Institute for Materials Science（国立材料科学研究所功能材料研究中心）；International Center for Materials Nanoarchitectonics, National Institute for Materials Science（国立材料科学研究所国际纳米材料组装中心）；Braun Center for Submicron Research, Department of Condensed Matter Physics（雷霍沃特凝聚态物理系布朗亚微米研究中心）；Department of Physics, Florida State University（佛罗里达州立大学物理系）；National High Magnetic Field Laboratory（国家高磁场实验室）；Center for Quantum Science and Engineering (QSE Center), École Polytechnique Fédérale de Lausanne (EPFL)（洛桑联邦理工学院量子科学与工程中心）
We theoretically study the Josephson current in Ising superconductor-half-metal-Ising superconductor junctions. By solving the Bogoliubov-de Gennes equations, the Josephson currents contributed by the discrete Andreev levels and the continuous spectrum are obtained. For very short junctions, because the direct tunneling of the Cooper pair dominates the Josephson current, the current-phase difference relation is independent of the magnetization direction, which is the same as the conventional superconductor-ferromagnet-superconductor junctions. On the other hand, when the length of the half-met…
We discuss the possibility of coexistence of spin density wave (antiferromagnetism) and triplet superconductivity as a particular example of a broad class of systems where the interplay of magnetism and superconductivity is important. We focus on the case of quasi-one-dimensional metals, where it is kown that antiferromagnetism is in close proximity to triplet superconductivity in the pressure versus temperature phase diagram. Over a range of pressures, we propose an intermediate non-uniform phase consisting of antiferromagnetic and triplet superconducting orders. In the coexistence region, we…
Superconductivity found in doped NdNiO$_2$ is puzzling as two local symmetries of doped NiO$_2$ layers compete, with presumably far-reaching implications for the involved mechanism: a cuprate-like regime with Zhang-Rice singlets {\cblue is replaced by local triplet states at realistic values of charge-transfer energy, which would suggest a rather different superconductivity scenario from high-$T_c$ cuprates}. We address this competition by investigating Ni$_4$O$_8$ clusters with periodic boundary conditions in the parameter range relevant for the superconducting nickelates. With increasing val…
We study tunneling currents in a model consisting of two non-unitary ferromagnetic spin-triplet superconductors separated by a thin insulating layer. We find a novel interplay between ferromagnetism and superconductivity, manifested in the Josephson effect. This offers the possibility of tuning dissipationless currents of charge and spin in a well-defined manner by adjusting the magnetization direction on either side of the junction.
This work discusses theoretically the interplay between the superconducting and ferromagnetic proximity effects, in a diffusive normal metal strip in contact with a superconductor and a non-uniformly magnetized ferromagnetic insulator. The quasiparticle density of states of the normal metal shows clear qualitative signatures of triplet correlations with spin one (TCS1). When one goes away from the superconduting contact, TCS1 focus at zero energy under the form of a peak surrounded by dips, which show a typical spatial scaling behavior. This behavior can coexist with a focusing of singlet corr…
Triplet pairing, orbital selectivity and correlations in Iron-based superconductors
University of Cincinnati（辛辛那提大学）；Max-Planck-Institut für Festkörperforschung（马克斯·普朗克固体研究所）；Rutgers University（罗格斯大学）；Royal Holloway, University of London（伦敦大学皇家霍洛威学院）
Pairing-channel reconstruction by Ising spin-orbit coupling in a multiorbital triangular-lattice model
Anhui Provincial Key Laboratory of Low-Energy Quantum Materials and Devices, High Magnetic Field Laboratory, HFIPS, Chinese Academy of Sciences（中国科学院合肥物质科学研究院强磁场科学中心安徽省低能量子材料与器件重点实验室）；Science Island Branch of Graduate School, University of Science and Technology of China（中国科学技术大学研究生院科学岛分院）
Van der Waals heterostructures have risen as a tunable platform to combine different electronic orders, due to the flexibility in stacking different materials with competing symmetry broken states. Among them, van der Waals ferromagnets such as CrI3 and superconductors as NbSe2 provide a natural platform to engineer novel phenomena at ferromagnet-superconductor interfaces. In particular, NbSe2 is well known for hosting strong spin-orbit coupling effects that influence the properties of the superconducting state. Here we put forward a ferromagnet/NbSe2/ferromagnet heterostructure where the inte…
We propose a model for a superconductor where both spin-singlet and chiral triplet pairing amplitudes can coexist. By solving the Bogoliubov-de Gennes equations with a general pair potential that accounts for both spin states we study experimental signatures of normal metal and superconductor hybrids. The interplay between the spin-singlet and triplet correlations manifests in the appearance of two effective gaps. When the amplitude of the spin-triplet component is stronger than that of the spin-singlet, a topological phase transition into a non-trivial regime occurs. As a result, the normal m…
We study tunneling currents in a model consisting of two non-unitary ferromagnetic spin-triplet superconductors separated by a thin insulating layer. We find a novel interplay between ferromagnetism and superconductivity, manifested in the Josephson effect. This offers the possibility of tuning dissipationless currents of charge and spin in a well-defined manner by adjusting the magnetization direction on either side of the junction.
Hybrid Ising superconductor-ferromagnetic insulator heterostructures provide a unique opportunity to explore the interplay between proximity-induced magnetism, spin-orbit coupling and superconductivity. Here we use a combination of first-principles calculations of NbSe$_{2}$/CrBr$_{3}$ heterostructures and an analytical theory of Ising superconductivity to analyze the existing experiments and provide a complete explanation of highly nontrivial and largely counterintuitive effects: an increase in the magnitude of the superconducting gap accompanied by the broadening of the tunneling peaks; hyst…
We investigate the interplay of classical degeneracy and quantum dynamics in a range of periodic frustrated transverse field Ising systems at zero temperature. We find that such dynamics can lead to unusual ordered phases and phase transitions, or to a quantum spin liquid (cooperative paramagnetic) phase as in the triangular and kagome lattice antiferromagnets, respectively. For the latter, we further predict passage to a bond-ordered phase followed by a critical phase as the field is tilted. These systems also provide exact realizations of quantum dimer models introduced in studies of high te…
We address the quantum-critical behavior of a two-dimensional itinerant ferromagnetic systems described by a spin-fermion model in which fermions interact with close to critical bosonic modes. We consider Heisenberg ferromagnets, Ising ferromagnets, and the Ising nematic transition. Mean-field theory close to the quantum critical point predicts a superconducting gap with spin-triplet symmetry for the ferromagnetic systems and a singlet gap for the nematic scenario. Studying fluctuations in this ordered phase using a nonlinear sigma model, we find that these fluctuations are not suppressed by a…
We study spin-half fermions in a one-dimensional extended Hubbard chain at low filling. We identify three triplet and one singlet pairing channels in the system, which are independently tunable as a function of nearest-neighbor charge and spin interactions. In a large-size system with translational invariance, we derive gap equations for the corresponding pairing gaps and obtain a Bogoliubov-de Gennes Hamiltonian with its non-trivial topology determined by the interplay of these gaps. In an open-end system with a fixed number of particles, we compute the exact many-body ground state and identi…
A common path to superconducting spintronics, Majorana fermions, and topologically-protected quantum computing relies on spin-triplet superconductivity. While naturally occurring spin-triplet pairing is elusive and even common spin-triplet candidates, such as Sr$_2$RuO$_4$, support alternative explanations, proximity effects in heterostructures can overcome these limitations. It is expected that robust spin-triplet superconductivity in magnetic junctions should rely on highly spin-polarized magnets or complex magnetic multilayers. Instead, we predict that the interplay of interfacial spin-orbi…
Distinguishing nodal and nonunitary superconductivity in quasiparticle interference of an Ising superconductor with Rashba spin-orbit coupling: an example of NbSe$_2$
Applying the linearized Usadel equations, we consider the nucleation of superconductivity in multiply connected mesoscopic superconductor/ferromagnet (S/F) hybrids such as a thin superconducting ring on a ferromagnet with a uniform in-plane magnetization M and a spin-active S/F interface. We demonstrate that the exchange field in F provokes a switching between superconducting states with different vorticities which may increase the critical temperature ( Tc ) of the superconductor in a magnetic field. We study the interplay between oscillations in Tc due to the Little--Parks effect and oscilla…
We present a theoretical study of a ferromagnet/s-wave superconductor junction to investigate the signatures of induced triplet correlations in the system. We apply the extended BTK-formalism and allow for an arbitrary magnetization strength/direction of the ferromagnet, a spin-active barrier, Fermi-vector mismatch, and different effective masses in the two systems. It is found that the phase associated with the $xy$-components of the magnetization in the ferromagnet couples with the superconducting phase and induces spin-triplet pairing correlations in the superconductor, if the tunneling bar…
We study the interplay between proximity-induced superconductivity and ferromagnetism in graphene by self-consistently solving the Bogoliubov-de Gennes equations on the honeycomb lattice. We find that a strong triplet proximity effect is generated in graphene, leading to odd-frequency pairing correlations. These odd-frequency correlations are clearly manifested in the local density of states of the graphene sheet, which can be probed via STM-measurements. Motivated by recent experiments on S$\mid$N$\mid$S graphene Josephson junctions, we also study the spectrum of Andreev-bound states formed i…
