arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 1908.04323physics.opticsnlin.PS

Nonlinear Spectroscopy and All-Optical Switching of Femtosecond Soliton Molecules

Felix Kurtz, Claus Ropers, Georg Herink

英文摘要:

The emergence of confined structures and pattern formation are exceptional manifestations of concurring nonlinear interactions found in a variety of physical, chemical and biological systems[1]. Optical solitons are a hallmark of extreme spatial or temporal confinement enabled by a variety of nonlinearities. Such particle-like structures can assemble in complex stable arrangements, forming "soliton molecules"[2,3]. Recent works revealed oscillatory internal motions of these bound states, akin to molecular vibrations[4-8]. These observations beg the question as to how far the "molecular" analogy reaches, whether further concepts from molecular spectroscopy apply in this scenario, and if such intra-molecular dynamics can be externally driven or manipulated. Here, we probe and control such ultrashort bound-states in an optical oscillator, utilizing real-time spectroscopy and time-dependent external perturbations. We introduce two-dimensional spectroscopy of the linear and nonlinear bound-state response and resolve anharmonicities in the soliton interaction leading to overtone and sub-harmonic generation. Employing a non-perturbative interaction, we demonstrate all-optical switching between distinct states with different binding separation, opening up novel schemes of ultrafast spectroscopy, optical logic operations and all-optical memory.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

↑