Direct current in clean semiconductors and metals was recently shown to obey the laws of hydrodynamics in a broad range of temperatures and sample dimensions. However, the determination of frequency window for hydrodynamic phenomena remains challenging. Here, we reveal a phenomenon being a hallmark of high-frequency hydrodynamic transport, the Cerenkov emission of plasmons by drifting Dirac electrons. The effect appears in hydrodynamic regime only due to reduction of plasmon velocity by electron-electron collisions below the velocity of carrier drift. To characterize the Cerenkov effect quantitatively, we analytically find the high-frequency non-local conductivity of drifting Dirac electrons across the hydrodynamic-to-ballistic crossover. We find the growth rates of hydrodynamic plasmon instabilities in two experimentally relevant setups: parallel graphene layers and graphene covered by subwavelength grating, further showing their absence in ballistic regime. We argue that the possibility of Cerenkov emission is linked to singular structure of non-local conductivity of Dirac materials and is independent on specific dielectric environment.
We present a quantization of the hydrodynamic model to describe the excitation of plasmons in a single-walled carbon nanotube by a fast point charge moving near its surface at an arbitrary angle of incidence. Using a two-dimensional electron gas represented by two interacting fluids, which takes into account the different nature of the sigma and pi electrons, we obtain plasmon energies in near-quantitative agreement with experiment. Further, the implemented quantization procedure allows us to study the probability of exciting various plasmon modes, as well as the stopping force and energy loss…
Direct current in confined two-dimensional (2d) electron systems can become unstable with respect to the excitation of plasmons. Numerous experiments and simulations hint that structural asymmetry somehow promotes plasmon generation, but a constitutive relation between asymmetry and instability has been missing. We provide such relation in the present paper and show that bounded perfect 2d electron fluids in asymmetric structures are unstable under arbitrarily weak drive currents. To this end, we develop a perturbation theory for hydrodynamic plasmons and evaluate corrections to their eigenfre…
Perturbation theory is an indispensable tool in quantum mechanics and electrodynamics that handles weak effects on particle motion or fields. However, its extension to plasmons involving complex motion of {\it both} particles and fields remained challenging. We show that this challenge can be mastered if electron motion obeys the laws of hydrodynamics, as recently confirmed in experiments with ultra-clean heterostructures. We present a unified approach to evaluate corrections to plasmon spectra induced by carrier drift, magnetic field, Berry curvature, scattering, and viscosity. As a first app…
Multiscale plasmonic systems e.g. extended metallic nanostructures with sub-nanometer inter-distances) play a key role in the development of next-generation nano-photonic devices. An accurate modeling of the optical interactions in these systems requires an accurate description of both quantum effects and far-field properties. Classical electromagnetism can only describe the latter, while Time-Dependent Density Functional Theory (TD-DFT) can provide a full first-principles quantum treatment. However, TD-DFT becomes computationally prohibitive for sizes that exceed few nanometers, which are irr…
A great deal of theoretical and experimental efforts have been devoted in the last decades to the study of long-wavelength photodetection mechanisms in field-effect transistors hosting two-dimensional (2D) electron systems. A particularly interesting subclass of these mechanisms is intrinsic and based on the conversion of the incoming electromagnetic radiation into plasmons, which resonantly enhance the photoresponse, and subsequent rectification via hydrodynamic nonlinearities. In this Article we show that such conversion and subsequent rectification occur well beyond the frequency regime in …
Using the hydrodynamic model in the electrostatic approximation, we describe the formation of graphene surface plasmons when a charge is in motion either perpendicular or parallel to a graphene sheet. In the first case, the electron-energy loss (EEL) spectrum of the electron is computed, showing that the resonances in the spectrum are linked to the frequency of the graphene surface plasmons. In the second case, we discuss the formation of plasmonic wakes due to the dragging of the surface plasmons induced by the motion of the charge. This effect is similar to Coulomb drag between two electron …
Using an analytically tractable kinetic model of a two dimensional Fermi liquid of electrons, we characterize the crossovers between zero sound, first sound and plasmons. For experimentally realized Fermi liquids in a hydrodynamic limit, both zero and first sound waves are essentially replaced by plasmons. The plasmon dispersion relation is robust against hydrodynamic effects, up to acquiring the viscous-limited decay rate of a first sound wave in the hydrodynamic limit. We discuss implications for experiments in clean two dimensional electron gases.
We show that a small conducting object, such as a nanosphere or a nanoring, embedded into or placed in the vicinity of the two-dimensional electron liquid (2DEL) and subjected to a circularly polarized electromagnetic radiation induces ``twisted'' plasmonic oscillations in the adjacent 2DEL. The oscillations are rectified due to the hydrodynamic nonlinearities leading to the helicity sensitive circular dc current and to a magnetic moment. This hydrodynamic inverse Faraday effect (HIFE) can be observed at room temperature in different materials. The HIFE is dramatically enhanced in a periodic a…
High-frequency response of a system with drifting electrons in a highly doped graphene and surface polar optical phonons of a polar substrate is considered. For this interacting system, we obtained a dielectric function, frequencies and decrement/increment of cooperative plasmon-optical phonon oscillations. We found, that the response is significantly depends on the degree of nonequilibrium of the electrons. In particular, interaction between drifting plasmons and surface polar optical phonons leads to an instability of the electron subsystem due to Vavilov-Cherenkov effect. We suggest that th…
A hybrid system composed of an isotropic nanoparticle and a semiconductor heterostructure with a quantum well has been considered. The nanoparticle is supposed to be polarizable in an external electric field. A theoretical model of the hybrid system is substantiated and formulated. Exact solutions of the model equations are obtained. The frequencies of charge oscillations in the hybrid system and their damping owing to the dipole--plasmon interaction are found, the damping mechanism being similar to that of Landau damping. The space-time behavior of concentration perturbations in the two-dimen…
Starting from the Dirac equation, the relativistic quantum hydrodynamic equations for Dirac electrons on a surface of a three dimensional-topological insulator (TI) are derived and numerically solved to study the spin plasmons. The surface of the TI is modulated by a perpendicular magnetic field and a pulsed exchange field provided by an array of ferromagnetic insulating (FI) stripes. The collective density and velocity oscillations in the two-dimensional Dirac electron gas are simulated and analyzed. It is shown that in spin plasmons, the collective electron density and momentum are modulated…
Hydrodynamic flow in two-dimensional electron systems has so far been probed only by dc transport and scanning gate microscopy measurements. In this work we discuss theoretically signatures of the hydrodynamic regime in near-field optical microscopy. We analyze the dispersion of acoustic plasmon modes in two-dimensional electron liquids using a non-local conductivity that takes into account the effects of (momentum-conserving) electron-electron collisions, (momentum-relaxing) electron-phonon and electron-impurity collisions, and many-body interactions beyond the celebrated Random Phase Approxi…
The hydrodynamic Drude model known from metal plasmonics also applies to semiconductor structures of sizes in between single-particle quantum confinement and bulk. But contrary to metals, for semiconductors two or more types of plasma may have to be taken into account in order to properly describe their plasmonic properties. In this combined analytical and computational study, we explore predictions of the recently proposed two-fluid hydrodynamic Drude model for the optical properties of plasmonic semiconductor nanowires, in particular for thermally excited InSb nanowires. We focus on the low-…
In a recent paper by Lucas and Das Sarma [Physical Review B 97, 115449 (2018)], a solvable model of collective modes in 2D metals was considered in the hydrodynamic regime. In the current work, we generalize the hydrodynamic theory to 3D metals for which the calculation of sound modes in a strongly-coupled quantum Coulomb plasma can be made explicit. The specific theoretical question of interest is how the usual linearly dispersing hydrodynamic sound mode relates to the well-known gapped 3D plasmon collective mode in the presence of long-range Coulomb interaction. We show analytically that bot…
Plasmonics has attracted much attention not only because it has useful properties such as strong field enhancement, but also because it reveals the quantum nature of matter. To handle quantum plasmonics effects, ab initio packages or empirical Feibelman d-parameters have been used to explore the quantum correction of plasmonic resonances. However, most of these methods are formulated within the quasi-static framework. The self-consistent hydrodynamics model offers a reliable approach to study quantum plasmonics because it can incorporate the quantum effect of the electron gas into classical el…
Spatial separation of electrons and holes in graphene gives rise to existence of plasmon waves confined to the boundary region. Theory of such guided plasmon modes within hydrodynamics of electron-hole liquid is developed. For plasmon wavelengths smaller than the size of charged domains plasmon dispersion is found to be ω~ q^(1/4). Frequency, velocity and direction of propagation of guided plasmon modes can be easily controlled by external electric field. In the presence of magnetic field spectrum of additional gapless magnetoplasmon excitations is obtained. Our findings indicate that graphene…
We identify a possible mechanism of the plasmon instabilities in periodically gated two-dimensional electron systems with a modulated electron density (plasmonic crystals) under direct current. The instability occurs due to the amplified reflection of the small density perturbations from the gated/ungated boundaries under the proper phase matching conditions between the crystal unit cells. Based on the transfer-matrix formalism, we derive the generic dispersion equation for the travelling plasmons in these structures. Its solution in the hydrodynamic limit shows that the threshold drift veloci…
We develop an exactly solvable classical kinetic model of transport in Dirac materials accounting for strong electron-electron (e-e) and electron-hole (e-h) collisions. We use this model to track the evolution of graphene conductivity and properties of its collective excitations across the hydrodynamic-to-ballistic crossover. We find the relaxation rate of electric current by e-e collisions that is possible due to the lack of Galilean invariance, and introduce a universal numerical measure of this non-invariance in arbitrary dimension. We find the two branches of collective excitations in the …
Nonlocal electrodynamics of two-dimensional anisotropic magneto-plasmons
Aeronautics Institute of Technology（航空技术学院）；University of Southern Denmark（南丹麦大学）；Universidade Federal do Ceará（塞阿拉联邦大学）；University of Antwerp（安特卫普大学）；Danish Institute for Advanced Study, University of Southern Denmark（南丹麦大学丹麦高等研究院）；Universidade do Minho（米尼奥大学）
Gapless spectrum of graphene allows easy spatial separation of electrons and holes with an external in-plane electric field. Guided collective plasmon modes can propagate along the separation line, whose amplitude decays with the distance to it. Their spectrum and direction of propagation can be controlled with the strength and direction of in-plane electric field. In case of a bilayer graphene additional control is possible by the perpendicular electric field that opens a gap in the band spectrum of electrons. We investigate guided plasmon spectra in bilayer p-n junctions using hydrodynamics …
The recent demonstrations of viscous hydrodynamic electron flow in two-dimensional electron systems poses serious questions to the validity of existing transport theories, including the ballistic model, the collision-induced and collisionless hydrodynamics. While the theories of transport at hydrodynamic-to-ballistic crossover for free 2d electrons are well established, the same is not true for electrons in magnetic fields. In this work, we develop an analytically solvable model describing the transition from ballistic to hydrodynamic transport with changing the strength of electron-electron c…
The ultraconfined light of plasmonic modes put their effective wavelength close to the mean free path of electrons inside the metal electron gas. The Drude model, which can not take the repulsive interactions of electrons into account, then clearly begins to show its limits. In an intermediate length scale where a full quantum treatment is computationally prohibitive, the semiclassical hydrodynamic model, instrinsically non-local, has proven successful. Here we generalize the expression for the absorption volume density and the reciprocity theorem in the framework of this hydrodynamic model. W…
Plasmonics is a rapid growing field, which has enabled both fundamental science and inventions of various quantum optoelectronic devices. An accurate and efficient method to calculate the optical response of metallic structures with feature size in the nanoscale plays an important role. Quantum hydrodynamic theory (QHT) provides an efficient description of the free-electron gas, where quantum effects of nonlocality and spill-out are taken into account. In this work, we introduce a general QHT that includes diffusion to account for the broadening, which is a key problem in practical application…
Plasmonic nanoparticles provide an ideal environment for the enhancement of fluorescent emission. On the one hand, they locally amplify the electromagnetic fields, increasing the emitter excitation rate, and on the other hand, they provide a high local density of states that accelerates spontaneous emission. However, when the emitter is placed in close proximity to a single metal nanoparticle, the number of nonradiative states increases dramatically, causing the fluorescence to quench. It has been predicted theoretically that, through a judicious placing of the emitter, fluorescence in plasmon…
This manuscript provides a general approach to the investigation of field quantization in high-curvature geometries. The models and calculations can help with understanding the elastic and inelastic scattering of photons and electrons in nanostructures and probe-like metallic domains. The results find important applications in high-resolution photonic and electronic modalities of scanning probe microscopy, nano-optics, plasmonics, and quantum sensing. Quasistatic formulation, leading to nonretarded quantities, is employed and justified on the basis of the nanoscale, here subwavelength, dimensi…
Inspired by recent measurements on individual metallic nanospheres that can not be explained with traditional classical electrodynamics, we theoretically investigate the effects of nonlocal response by metallic nanospheres in three distinct settings: atomic spontaneous emission, electron energy loss spectroscopy, and light scattering. These constitute two near-field and one far-field measurements, with zero-, one-, and two-dimensional excitation sources, respectively. We search for the clearest signatures of hydrodynamic pressure waves in nanospheres. We employ a linearized hydrodynamic model …
Plasmon-exciton polaritons provide exciting possibilities to control light-matter interactions at the nanoscale by enabling closer investigation of quantum optical effects and facilitating novel technologies based, for instance, on Bose-Einstein condensation and polaritonic lasing. Nevertheless, observing and visualising polaritons is challenging, and traditional optical microscopy techniques often lead to ambiguities regarding the emergence and strength of the plasmon-exciton coupling. Electron microscopy offers a more robust means to study and verify the nature of plexcitons, but is still hi…
We investigate field quantization in high-curvature geometries. The models and calculations can help with understanding the elastic and inelastic scattering of photons and electrons in nanostructures and probe-like metallic domains. The results find important applications in high-resolution photonic and electronic modalities of scanning probe microscopy, nano-optics, plasmonics, and quantum sensing. Quasistatic formulation, leading to nonretarded quantities, is employed and justified on the basis of the nanoscale, here subwavelength, dimensions of the considered domains of interest. Within the…
Quantum effects play a significant role in nanometric plasmonic devices, such as small metal clusters and metallic nanoshells. For structures containing a large number of electrons, ab-initio methods such as the time-dependent density functional theory (TD-DFT) are often impractical because of severe computational constraints. Quantum hydrodynamics (QHD) offers a valuable alternative by representing the electron population as a continuous fluid medium evolving under the action of the self-consistent and external fields. Although relatively simple, QHD can incorporate quantum and nonlinear effe…
Excitation of confined bulk plasmons in metallic nanoparticles by penetrating electron beams within a nonlocal analytical approach
University of the Basque Country UPV/EHU（巴斯克国立大学）；Donostia International Physics Center (DIPC)（多诺西亚国际物理中心）；IKERBASQUE, Basque Foundation for Science（伊克尔巴斯基奎，巴斯克科学基金会）；Materials Physics Center, CSIC-UPV/EHU（材料物理中心，西班牙国家研究委员会-巴斯克国立大学）
We investigate an interplay between quantum geometrical effects and surface plasmons through surface plasmonic structures, based on an electron hydrodynamic theory. First we demonstrate that the quantum nonlinear Hall effect can be dramatically enhanced over a very broad range of frequency by utilizing plasmonic resonances and near-field effects of grating gates. Under the resonant condition, the enhancement becomes several orders of magnitude larger than the case without the nanostructures, while the peaks of high-harmonic plasmons expand broadly and emerge under the off-resonant condition, l…
We describe the structure of the time-harmonic electromagnetic field of a vertical Hertzian electric dipole source radiating over an infinite, translation invariant two-dimensional electron system. Our model for the electron flow takes into account the effects of shear and Hall viscosities as well as an external static magnetic field perpendicular to the sheet. We identify two wave modes, namely, a surface plasmon and a diffusive mode. In the presence of an external static magnetic field, the diffusive mode combines the features of both the conventional and Hall diffusion and may exhibit a neg…
We develop the theory of hydrodynamics of an isotropic Fermi liquid of electrons coupled to isotropic acoustic phonons, assuming that umklapp processes may be neglected. At low temperatures, the fluid is approximately Galilean invariant; at high temperatures, the fluid is nearly relativistic; at intermediate temperatures, there are seven additional temperature regimes with unconventional thermodynamic properties and hydrodynamic transport coefficients in a three-dimensional system. We predict qualitative signatures of electron-phonon fluids in incoherent transport coefficients, shear and Hall …
We study the surface plasmon (SP) resonance energy of isolated spherical Ag nanoparticles dispersed on a silicon nitride substrate in the diameter range 3.5-26 nm with monochromated electron energy-loss spectroscopy. A significant blueshift of the SP resonance energy of 0.5 eV is measured when the particle size decreases from 26 down to 3.5 nm. We interpret the observed blueshift using three models for a metallic sphere embedded in homogeneous background material: a classical Drude model with a homogeneous electron density profile in the metal, a semiclassical model corrected for an inhomogene…
Electron beams in two-dimensional systems can provide a useful tool to study energy-momentum relaxation of electrons and to generate microwave radiation stemming from plasma-beam instabilities. Naturally, these two applications cannot coexist: if beam electrons do relax, the beam is stabilized; if instability exists, it strongly distorts the distribution function of beam electrons. In this paper, we study the competition of beam relaxation due to electron-electron (e-e) collisions and development of plasma beam instability in graphene. We find that unstable plasma mode associated with a beam i…
