The ultraconfined light of plasmonic modes put their effective wavelength close to the mean free path of electrons inside the metal electron gas. The Drude model, which can not take the repulsive interactions of electrons into account, then clearly begins to show its limits. In an intermediate length scale where a full quantum treatment is computationally prohibitive, the semiclassical hydrodynamic model, instrinsically non-local, has proven successful. Here we generalize the expression for the absorption volume density and the reciprocity theorem in the framework of this hydrodynamic model. We validate numerically these generalized theorems and show that using classical expressions instead leads to large discrepancies.
Quantum theory of surface plasmons is very important for studying the interactions between light and different metal nanostructures in nanoplasmonics. In this work, using the canonical quantization method, the SPPs on nanowires and their orbital and spin angular momentum are investigated. The results show that the SPPs on nanowire carry both orbital and spin momentum during propagation. Later, the result is applied on the plasmonic nanowire waveguide to show the agreement of the theory. The study is helpful for the nano wire based plasmonic interactions and the quantum information based optica…
Nonlinear metasurfaces based on coupling a locally enhanced plasmonic response to intersubband transitions of n-doped multi-quantum-wells (MQWs) have recently provided second-order susceptibilities orders of magnitude larger than any other nonlinear flat structure measured so far. Here, we present a comprehensive theory to characterize the electromagnetic response of nonlinear processes occurring in ultrathin MQW-based plasmonic metasurfaces, providing a homogeneous model that takes phase-matching at the unit-cell level and the influence of saturation and losses into account. In addition, the …
A chiral near field with a highly contorted electromagnetic field builds a bridge to match the chiral molecules and light wavelengths with large size differences. It significantly enhances the circular dichroism of chiral molecules and has great prospects in chirality sensing, detection, trapping, and other chirality-related applications. Surface plasmons feature outstanding light-trapping and electromagnetic-field-concentrating abilities. Plasmonic chiral nanostructures facilitate light manipulation to generate superchiral near fields. Meanwhile, the nanophotonic structures have attracted sig…
This work is focussed on the role of the angle of incidence of an incoming electromagnetic wave in its transmission through a subwavelength nano-hole in a thin semiconductor plasmonic layer. Fully detailed calculations and results are exhibited for $ p$- and $s$-polarizations of the incident wave for a variety of incident angles in the near, middle and far zones of the transmitted radiation. Our dyadic Green's function formulation includes both (1) the electromagnetic field transmitted directly through the $ 2D $ plasmonic layer superposed with (2) the radiation emanating from the nano-hole. I…
We introduce two types of toroidal metamaterials which are invisible to surface plasmon polaritons (SPPs) propagating on a metal surface. The former is a toroidal handlebody bridging remote holes on the metal surface: It works as a kind of plasmonic counterpart of electromagnetic wormholes. The latter is a toroidal ring lying on the metal surface: This bridges two disconnected metal surfaces i.e. It connects a thin metal cylinder to a flat metal surface with a hole. Full-wave numerical simulations demonstrate that an electromagnetic field propagating inside these metamaterials does not disturb…
Electromagnetic absorbers have drawn increasing attention in many areas. A series of plasmonic and metamaterial structures can work as efficient narrow band absorbers due to the excitation of plasmonic or photonic resonances, providing a great potential for applications in designing selective thermal emitters, bio-sensing, etc. In other applications such as solar energy harvesting and photonic detection, the bandwidth of light absorbers is required to be quite broad. Under such a background, a variety of mechanisms of broadband/multiband absorption have been proposed, such as mixing multiple r…
This paper presents high-order (HO) electromagnetic modeling of plasmonic nanostructures based on the Locally Corrected Nystrom (LCN) method. Advanced nanophotonic and nanoplasmonic structures involve electrically large electromagnetic structures that are very complex in both geometry and material composition. Hence, advanced analysis and design tools are required in order to predict the performance of such structures and optimize the geometrical parameters prior to costly prototype development. In this perspective, the LCN is exploited to solve the electromagnetic scattering of plasmonic nano…
A tri-layer metamaterial perfect absorber of light, consisting of (Al/ZnS/Al) films with the top aluminium layer patterned as an array of circular disk nanoantennas, is investigated for resonantly enhancing Raman scattering from C-60 fullerene molecules deposited on the metamaterial. The metamaterial is designed to have resonant bands due to plasmonic and electromagnetic resonances at the Raman pump frequency (725 nm) as well as Stokes emission bands. The Raman scattering from C60 on the metamaterial with resonantly matched bands is measured to be enhanced by an order of magnitude more than fr…
We consider a simple configuration for realizing one-dimensional slow-light metamaterials with large bandwidth-delay products using stub-shaped Fabry-Perot resonators as building blocks. Each metaatom gives rise to large group indices due to a classical analog of the dressed-state picture of electromagnetically-induced transparency. By connecting up to eight metaatoms, we find bandwidth-delay products over unity and group indices approaching 100. Our approach is quite general and can be applied to any type of Fabry-Perot resonators and tuned to different operating wavelengths.
Plasmons in two-dimensional electron systems (2DES) feature ultra-strong confinement and are expected to efficiently mediate the interactions between light and charge carriers. Despite these expectations, the electromagnetic detectors exploiting 2d plasmon resonance have been so far inferior to their non-resonant counterparts. Here, we theoretically analyse the origin of these failures, and suggest a proper niche for 2d plasmonics in electromagnetic wave detection. We find that a confined 2DES supporting plasmon resonance has an upper limit of absorption cross-section, which is identical to th…
Nanoscale localization of electromagnetic fields near metallic nanostructures underpins the fundamentals and applications of plasmonics. The unavoidable energy loss from plasmon decay, initially seen as a detriment, has now expanded the scope of plasmonic applications to exploit the generated hot carriers. However, quantitative understanding of the spatial localization of these hot carriers, akin to electromagnetic near-field maps, has been elusive. Here we spatially map hot-electron-driven reduction chemistry with 15 nanometre resolution as a function of time and electromagnetic field polariz…
A giant thermal magnetoresistance is predicted for the electromagnetic transport of heat in magneto-optical plasmonic structures. In chains of InSb-Ag nanoparticles at room temperature, we found that the resistance can be increased by almost a factor of 2 with magnetic fields of 2 T. We show that this important change results from the strong spectral dependence of localized surface waves on the magnitude of the magnetic field.
This paper is concerned with the analysis of time-harmonic electromagnetic scattering from plasmonic inclusions in the finite frequency regime beyond the quasi-static approximation. The electric permittivity and magnetic permeability in the inclusions are allowed to be negative-valued. Using layer potential techniques for the full Maxwell system, the scattering problem is reformulated into a system of integral equations. We derive the complete eigensystem of the involved matrix-valued integral operator within spherical geometry. As applications, we construct two types of plasmonic structures s…
Perturbation theory of mesoscale plasmonic waveguide with an analytical treatment of nonclassical electromagnetic boundary condition
Institute of Modern Optics, College of Electronic Information and Optical Engineering, Nankai University（南开大学电子信息与光学工程学院现代光学研究所）；National Key Laboratory of Semiconductor Laser（半导体激光国家重点实验室）
Considerations for Electromagnetic Simulations for a Quantitative Correlation of Optical Spectroscopy and Electron Tomography of Plasmonic Nanoparticles
Plasmonic nano antennas are highly attractive at optical frequencies due to their strong resonances - even when their size is smaller than the wavelength - and because of their potential of extreme field enhancement. Such antennas may be applied for sensing of biological nano particles as well as for single molecule detection. Because of considerable material losses and strong dispersion of metals at optical frequencies, the numerical analysis of plasmonic antennas is very demanding. An additional difficulty is caused when very narrow gaps between nano particles are utilized for increasing the…
The coupled light-matter modes supported by plasmonic metasurfaces can be combined with topological principles to yield subwavelength topological valley states of light. We give a systematic presentation of the topological valley states available for lattices of metallic nanoparticles: All possible lattices with hexagonal symmetry are considered, as well as valley states emerging on a square lattice. Several unique effects which have yet to be explored in plasmonics are identified, such as robust guiding, filtering and splitting of modes, as well as dual-band effects. We demonstrate these by m…
Focusing electromagnetic energy to sub-wavelength dimensions has become an increasingly active field of research for a variety of applications such as Heat Assisted Magnetic Recording (HAMR), nanolithography, and nanoscale optical characterization of biological cells and single molecules using near-field scanning optical microscopy (NSOM) technique. Double-sided surface plasmons in a metal-insulator-metal (MIM) geometry have been shown to have very small wavelengths for dielectric of thickness of less than 10 nm. A tapered dielectric structure sandwiched between metal, can be used to efficient…
The interaction of electromagnetic waves with metallic nanostructures generates resonant oscillations of the conduction-band electrons at the metal surface. These resonances can lead to large enhancements of the incident field and to the confinement of light to small regions, typically several orders of magnitude smaller than the incident wavelength. The accurate prediction of these resonances entails several challenges. Small geometric variations in the plasmonic structure may lead to large variations in the electromagnetic field responses. Furthermore, the material parameters that characteri…
Quantum-statistical effects occur during the propagation of electromagnetic (EM) waves inside the dielectric media or metamaterials, which include a large class of nanophotonic and plasmonic waveguides with dissipation and noise. Exploiting the formal analogy between the Schrodinger equation and the Maxwell equations for dielectric linear media, we rigorously derive the effective Hamiltonian operator which describes such propagation. This operator turns out to be essentially non-Hermitian in general, and pseudo-Hermitian in some special cases. Using the density operator approach for general no…
Herein we report on our studies of radiative and non-radiative interaction between an individual quantum emitter and an anisotropic plasmonic nanostructure: a gold nanotriangle. Our theoretical and three-dimensional electromagnetic simulation studies highlight an interesting connection between: dipole-orientation of the quantum emitter, anisotropy of the plasmonic nanostructure and, radiative and non-radiative energy transfer processes between the emitter and the plasmonic geometry. For the out of plane orientation of quantum emitter, the total decay rate and non-radiative decay rate was found…
We develop an analytic circuit model for coupled plasmonic dimers separated by small gaps that provides a complete account of the optical resonance wavelength. Using a suitable equivalent circuit, it shows how partially conducting links can be treated and provides quantitative agreement with both experiment and full electromagnetic simulations. The model highlights how in the conducting regime, the kinetic inductance of the linkers set the spectral blue-shifts of the coupled plasmon.
Nonreciprocity is important for optical information processing, full-duplex communications, and protection of sensitive laser equipment from unwanted reflections. However, it is very challenging to obtain strong nonreciprocal response in optical frequencies, especially when nanoscale configurations are considered. In this work, we solve this problem by demonstrating a compact bifacial plasmonic metasurface that acts as a new ultrathin nonreciprocal transmission filter at near-infrared frequencies. The proposed nanostructure is simple to be practically implemented, since it is composed of two s…
The emerging field of plasmonics can lead to enhanced light matter interactions at extremely nanoscale regions. Plasmonic (metallic) devices promise to efficiently control both classical and quantum properties of light. Plasmonic waveguides are usually used to excite confined electromagnetic modes at the nanoscale that can strongly interact with matter. The analysis of these nanowaveguides exhibits similarities with their low frequency microwave counterparts. In this article, we review ways to study plasmonic nanostructures coupled to quantum optical emitters from a classical electromagnetic p…
We measured a change in the current transport of an antenna-coupled, multi-gate, GaAs/AlGaAs field-effect transistor when terahertz electromagnetic waves irradiated the transistor and attribute the change to bolometric heating of the electrons in the two-dimensional electron channel. The observed terahertz absorption spectrum indicates coherence between plasmons excited under adjacent biased device gates. The experimental results agree quantitatively with a theoretical model we developed that is based on a generalized plasmonic transmission line formalism and describes an evolution of the plas…
Electrically-driven optical antennas can serve as compact sources of electromagnetic radiation operating at optical frequencies. In the most widely explored configurations, the radiation is generated by electrons tunneling between metallic parts of the structure when a bias voltage is applied across the tunneling gap. Rather than relying on an inherently inefficient inelastic light emission in the gap, we suggest to use a ballistic nanoconstriction as the feed element of an optical antenna supporting plasmonic modes. We discuss the underlying mechanisms responsible for the optical emission, an…
Coupling between tuneable broadband modes of an array of plasmonic metamolecules and a vibrational mode of carbonyl bond of poly(methyl methacrylate) is shown experimentally to produce a Fano resonance, which can be tuned in situ by varying the polarization of incident light. The interaction between the plasmon modes and the molecular resonance is investigated using both rigorous electromagnetic calculations and a quantum mechanical model describing the quantum interference between a discrete state and two continua. The predictions of the quantum mechanical model are in good agreement with the…
Plasmonic nanojunctions, consisting of adjacent metal structures with nanometre gaps, can support localised plasmon resonances that boost light matter interactions and concentrate electromagnetic fields at the nanoscale. In this regime, the optical response of the system is governed by poorly understood dynamical phenomena at the frontier between the bulk, molecular and atomic scales. Here, we report ubiquitous spectral fluctuations in the intrinsic light emission from photo-excited gold nanojunctions, which we attribute to the light-induced formation of domain boundaries and quantum-confined …
Plasmon resonance, with strong coupling of light to electrons at a metal-dielectric interface, allows light confinement and control at subwavelength scale. It's fundamentally limited by the inherent mobility of the electrons, leading to the corresponding non-locality of the electromagnetic response. We report that this non-locality also results in the formation of a hyperbolic layer near the metal-dielectric interface, with a strong anisotropy of its electromagnetic response. While the resulting "hyperbolic blockade" leads to the suppression of the conventional plasmon resonance, the hyperboli…
We present a rigorous electromagnetic method based on Green's second identity for studying the plasmonic response of graphene-coated wires of arbitrary shape. The wire is illuminated perpendicular to its axis by a monochromatic electromagnetic wave and the wire substrate is homogeneous and isotropic. The field is expressed everywhere in terms of two unknown source functions evaluated on the graphene coating which can be obtained from the numerical solution of a coupled pair of inhomogeneous integral equations. To assess the validity of the Green formulation, the scattering and absorption effic…
Electromagnetic surface waves supported by an isotropic chiral material were investigated via the associated canonical boundary-value problem. Specifically, two scenarios were considered: surface waves guided by the planar interface of an isotropic chiral material and (a) an isotropic dielectric material and (b) a uniaxial dielectric (or plasmonic) material. Both plasmonic and non-plasmonic achiral partnering materials were investigated. In scenario (a) surface waves akin to surface-plasmon-polariton (SPP) waves were excited, while in scenario (b) surface waves akin to Dyakonov waves and akin …
The optical response of a coupled nanowire dimer is studied using a fully quantum mechanical approach. The translational invariance of the system allows to apply the time--dependent density functional theory for the plasmonic dimer with the largest size considered so far in quantum calculations. Detailed comparisons with results from classical electromagnetic calculations based on local and non local hydrodynamic response, as well as with results of the recently developed quantum corrected model is performed. We show that electron tunneling and dynamical screening are the major nonlocal quantu…
Plasmonic nanoparticles provide an ideal environment for the enhancement of fluorescent emission. On the one hand, they locally amplify the electromagnetic fields, increasing the emitter excitation rate, and on the other hand, they provide a high local density of states that accelerates spontaneous emission. However, when the emitter is placed in close proximity to a single metal nanoparticle, the number of nonradiative states increases dramatically, causing the fluorescence to quench. It has been predicted theoretically that, through a judicious placing of the emitter, fluorescence in plasmon…
Nanoparticle (NP) arrays of noble metals strongly absorb light in the visible to infrared wavelengths through resonant interactions between the incident electromagnetic field and the metal's free electron plasma. Such plasmonic interfaces enhance light absorption and photocurrent in solar cells. We report a cost effective and scalable room temperature/pressure spin-coating route to fabricate broadband plasmonic interfaces consisting of silver NPs. The NP interface yields photocurrent enhancement (PE) in thin film silicon devices by up to 200% which is significantly greater than previously repo…
We investigate electromagnetic scattering and plasmonic cloaking in a system composed by a dielectric cylinder coated with a magneto-optical shell. In the long-wavelength limit we demonstrate that the application of an external magnetic field can not only switch on and off the cloaking mechanism but also mitigate losses, as the absorption cross-section is shown to be minimal precisely at the cloaking operation frequency band. We also show that the angular distribution of the scattered radiation can be effectively controlled by applying an external magnetic field, allowing for a swift change in…
Plasmonic distributed-feedback lasers based on a two-dimensional periodic array of metallic nanostructures are the main candidate for nanoscale sources of coherent electromagnetic field. Strong localization of the electromagnetic field and the large radiation surface are good opportunities for achieving an ultrashort response time to the external actions and creating beam directionality. At the same time, the investigation of such a system is a challenging problem. In this paper, we present an exhaustive study of the operation of a two-dimensional plasmonic distributed-feedback laser. We show …
Electromagnetic (EM) wave detection over a large spectrum has recently attracted significant amount of attention. Traditional electronic EM wave sensors use large metallic probes which distort the field to be measured and also have strict limitations on the detectable RF bandwidth. To address these problems, integrated photonic EM wave sensors have been developed to provide high sensitivity and broad bandwidth. Previously we demonstrated a compact, broadband, and sensitive integrated photonic EM wave sensor, consisting of an organic electro-optic (EO) polymer refilled silicon slot photonic cry…
The field of plasmonics offers a route to control light fields with metallic nanostructures through the excitation of Surface Plasmon Polaritons (SPPs). These surface waves, bound to a metal dielectric interface, tightly confine electromagnetic energy. Active control over SPPs has potential for applications in sensing, photovoltaics, quantum communication, nano circuitry, metamaterials and super-resolution microscopy. We achieve here a new level of control of plasmonic fields using a digital spatial light modulator. Optimizing the plasmonic phases via feedback we focus SPPs at a freely pre-cho…
While the thermal and electromagnetic properties of plasmonic nanostructures are well understood, nanoscale thermometry still presents an experimental and theoretical challenge. Plasmonic structures can confine electromagnetic energy at the nanoscale, resulting in local, inhomogeneous, controllable heating. But reading out the temperature with nanoscale precision using optical techniques poses a difficult challenge. Here we report on the optical thermometry of individual gold nanorod trimers that exhibit multiple wavelength-dependent plasmon modes resulting in measurably different local temper…
Quantum plasmonics is a rapidly growing field of research that involves the study of the quantum properties of light and its interaction with matter at the nanoscale. Here, surface plasmons - electromagnetic excitations coupled to electron charge density waves on metal-dielectric interfaces or localized on metallic nanostructures - enable the confinement of light to scales far below that of conventional optics. In this article we review recent progress in the experimental and theoretical investigation of the quantum properties of surface plasmons, their role in controlling light-matter interac…
A waveguide structure consisting of a tapered nanofiber on a metal film is proposed and analyzed to support highly localized hybrid plasmonic modes. The hybrid plasmonic mode can be efficiently excited through the in-line tapered fiber based on adiabatic conversion and collected by the same fiber, which is very convenient in the experiment. Due to the ultrasmall mode area of plasmonic mode, the local electromagnetic field is greatly enhanced in this movable waveguide, which is potential for enhanced coherence light emitter interactions, such as waveguide quantum electrodynamics, single emitter…
Surface plasmon polaritons (SPP or SP) are electromagnetic waves propagating along metal dielectric interfaces and existing over a wide range of frequencies. They have become popular because of their sub-wavelength confinement and the possibility to perform ultrasensitive optical measurements. Driven by tremendous progress in nanofabrication techniques and ultrafast laser technologies the applications of SP nanooptics extend beyond the border of nanoplasmonics. Here we review how using novel hybrid multilayer structures combining different functionalities allows to develop active plasmonic dev…
Localized surface plasmon polaritons in conducting structures give rise to enhancements of electromagnetic local fields and extinction efficiencies. Resonant conducting structures are conventionally fabricated with a fixed geometry that determines their plasmonic response. Here, we challenge this conventional approach by demonstrating the photo-generation of plasmonic materials (THz plasmonic antennas) on a flat semiconductor layer by the structured optical illumination through a spatial light modulator. Free charge carriers are photo-excited only on selected areas, which enables the definitio…
We derive general coupled-mode equations describing the nonlinear interaction of electromagnetic modes in media with loss and gain. Our approach is rigorously based on the Lorentz reciprocity theorem, and it can be applied to a broad range of metal-dielectric photonic structures, including plasmonic waveguides and metamaterials. We verify that our general results agree with the previous analysis of particular cases, and predict novel effects on self- and cross-phase modulation in multi-layer nonlinear fishnet metamaterials.
This chapter discusses a hydrodynamics-inspired approach to trap and manipulate light in plasmonic nanostructures, which is based on steering optical powerflow around nano-obstacles. New insights into plasmonic nanofocusing mechanisms are obtained by invoking an analogy of the 'photon fluid' (PF). By proper nanostructure design, PF kinetic energy can be locally increased via convective acceleration and then converted into 'pressure' energy to generate localized areas of high field intensity. In particular, trapped light can be molded into optical vortices -tornado-like areas of circular motion…
The toroidal dipole is an exquisite electromagnetic momentum apart from the classical multipoles family that can be localized and squeezed in an extremely tiny spot. This mode, in optical nanosystems, can be particularly distinguished as a non-radiating charge-current configuration, manifests in a head-to-tail fashion. Here going beyond conventional toroidal dipoles, we explained the possibility of the excitation of directional toroidal dipoles in plasmonic meta-atoms driven by controlling the oblique poloidal fluxes. We showed that the unique structural properties of the proposed asymmetric d…
Strong coupling between a single quantum emitter and an electromagnetic mode is one of the key effects in quantum optics. In the cavity QED approach to plasmonics, strongly coupled systems are usually understood as single-transition emitters resonantly coupled to a single radiative plasmonic mode. However, plasmonic cavities also support non-radiative (or "dark") modes, which offer much higher coupling strengths. On the other hand, realistic quantum emitters often support multiple electronic transitions of various symmetry, which could overlap with higher order plasmonic transitions -- in the …
Over the last few years, optical nanoantennas are continuously attracting interest owing to their ability to efficiently confine, localize resonance, and significantly enhanced electromagnetic fields at subwavelength scale. However, such strong confinement can be further enhanced by using an appropriate combination of optical nanoantenna and Slanted Bound states in the continuum cavities. Here, we propose to synergistically bridge the plasmonic nanoantenna and high optical quality-factor cavities to numerically demonstrate three orders of magnitude local intensity enhancement. The proposed hyb…
We analytically derive a rigorous expression for the relative impedance ratio between two photonic structures based on their electromagnetic interaction. Our approach generalizes the physical meaning of the impedance to a measure for the reciprocity-based overlap of eigenmodes. The consistence with known cases in the radiofrequency and optical domain is shown. The analysis reveals where the applicability of simple circuit parameters ends and how the impedance can be interpreted beyond this point. We illustrate our approach by successfully describing a Bragg reflector that terminates an insulat…
We study the optical properties associated to both the polariton gap and the Bragg gap in periodic resonator-waveguide coupled system, based on the temporal coupled mode theory and the transfer matrix method. By the complex band and the transmission spectrum, it is feasible to tune the interaction between multiple Bragg scattering and the local resonance, which may give rise to analogous phenomena of electromagnetically induced transparency (EIT). We further design a plasmonic slot waveguide side-coupled with local plasmonic resonator to demonstrate the EIT-like effects in the near-infared ban…
We demonstrate that plasmonic helical gratings consisting of metallic nanowires imprinted with helical grooves or ridges can be used efficiently to generate plasmonic vortices with radius much smaller than the operating wavelength. In our proposed approach, these helical surface gratings are designed so that plasmon modes with different azimuthal quantum numbers (topological charge) are phase-matched, thus allowing one to generate optical plasmonic vortices with arbitrary topological charge. The general principles for designing plasmonic helical gratings that facilitate efficient generation of…
