Yu Li, Zhonghao Liu, Zhuang Xu, Yu Song, Yaobo Huang, Dawei Shen, Ni Ma, Ang Li, Songxue Chi, Matthias Frontzek, Huibo Cao, Qingzhen Huang, Weiyi Wang, Yaofeng Xie, Yan Rong, David P. Young, J. F. DiTusa, Pengcheng Dai
备注:
9 pages, 12 figures, Supplementary Material available upon request, accepted by Phys. Rev. B
合成了一系列Sr(Co $_{1-x}$ Ni $_x$)$_2$ As $_2$单晶,从而建立了关于场、温度和化学取代的综合相图。我们的中子衍射实验揭示了一个helmagnetic顺序与磁矩铁磁(FM)在$ab$平面和helmagnetic波矢量$q=(0,0,0.56)$为$x$ = 0.1。结合中子衍射和角分辨光电子能谱(ARPES)的测量结果表明,具有$d_{x^2-y^2}$轨道特征的平带的调谐驱动了螺旋磁现象,并表明了量子有序无序机制的可能性。
英文摘要:
A series of Sr(Co$_{1-x}$Ni$_x$)$_2$As$_2$ single crystals was synthesized allowing a comprehensive phase diagram with respect to field, temperature, and chemical substitution to be established. Our neutron diffraction experiments revealed a helimagnetic order with magnetic moments ferromagnetically (FM) aligned in the $ab$ plane and a helimagnetic wavevector of $q=(0,0,0.56)$ for $x$ = 0.1. The combination of neutron diffraction and angle-resolved photoemission spectroscopy (ARPES) measurements show that the tuning of a flat band with $d_{x^2-y^2}$ orbital character drives the helimagnetism and indicates the possibility of a quantum order-by-disorder mechanism.
Canted ferromagnetic order in a distorted triangular-lattice magnet Na$_2$SrCo(VO$_4$)$_2$
School of Physics, Beihang University(北京航空航天大学物理学院);Department of Nuclear Physics, China Institute of Atomic Energy(中国原子能科学研究院核物理研究所);Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所凝聚态物理国家实验室);Spallation Neutron Source Science Center(散裂中子源科学中心);Songshan Lake Materials Laboratory(松山湖材料实验室);State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University(北京大学物理学院介观物理国家重点实验室)
Magnetic order and fluctuations in quasi-two-dimensional planar magnet Sr(Co$_{1-x}$Ni$_x$)$_2$As$_2$
我们利用中子散射研究了Sr(Co $_{1-x}$ Ni $_{x})_2$ As $_2$)的自旋激发,该化合物具有二维(2D)面内铁磁(FM)有序层的$c$轴无公度螺旋结构,是$0.013\leq x \leq 0.25$的一种.通过比较螺旋有序Sr(Co $_{0.9}$ Ni $_{0.1}$)$_2$ As $_2$和顺磁性SrCo $_2$ As $_2$中的波矢和能量相关的自旋激发,我们发现Ni掺杂在增加Sr(Co $_{1-x}$ Ni $_{x})_2$ As $_2$中晶格无序度的同时,增强了准二维FM自旋涨落.然而,我们的带结构计算内的组合密度泛函理论和动态平均场理论(DFT+DMFT)未能产生一个正确的无公度波矢量所观察到的螺旋顺序从嵌套费米表面。由于输运测量显示随着Ni掺杂和相关晶格无序的增加,平面内和$c$轴向电阻率增加,我们得出结论,Sr(Co $_{1-x}$ Ni $_{x})_2$ As $_2$中的螺旋磁序可能是通过巡回电子介导的Ruderman-Kittel-Kasuya-Yosida(RKKY)相互作用从量子有序无序机制产生的。
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所);School of Physical Sciences, University of Chinese Academy of Sciences(中国科学院大学物理科学学院);School of Physics and Technology, Wuhan University(武汉大学物理科学与技术学院);Research Center for Functional Materials, National Institute for Materials Science(国立材料研究所功能材料研究中心);International Center for Materials Nanoarchitectonics, National Institute for Materials Science(国立材料研究所国际纳米材料架构中心);Songshan Lake Materials Laboratory(松山湖材料实验室);Hefei National Laboratory(合肥国家实验室);Institute of Microelectronics, Chinese Academy of Sciences(中国科学院微电子研究所)
Effect of uniaxial stress on helimagnetic phases in the square-lattice itinerant magnet EuAl$_{4}$
Institute for Solid State Physics, University of Tokyo(东京大学固体物理研究所);RIKEN Center for Emergent Matter Science (CEMS)(理化学研究所新兴物质科学中心);Department of Physics, Tokyo Metropolitan University(东京都立大学物理学系);Institute of Materials Structure Science, High Energy Accelerator Research Organization(高能加速器研究机构材料结构科学研究所);Department of Advanced Materials Science, The University of Tokyo(东京大学先进材料科学系);Research Center for Advanced Science and Technology, University of Tokyo(东京大学先进科学技术研究中心);Department of Applied Physics, The University of Tokyo(东京大学应用物理学系)
Competing exchange interactions on the verge of a metal-insulator transition in the two-dimensional spiral magnet Sr$_3$Fe$_2$O$_7$
我们报道了双层钙钛矿结构Sr $_3$ Fe $_2$ O $_7$的磁序和磁动力学的中子散射研究,该结构在340 K下表现出温度驱动的金属-绝缘体转变。我们表明,铁$^{4+}$矩采用非公度螺旋顺序低于$T_\text{N}=115$ K,并提供了一个全面的描述相应的自旋波激发。所观察到的磁序和激发谱可以很好地理解的有效自旋哈密顿与范围内的相互作用,以第三近邻对。结果表明,Sr $_3$ Fe $_2$ O $_7$中的螺旋磁性是铁磁双交换和反铁磁超交换相互作用的竞争结果,在金属-绝缘体相变附近,两种相互作用的强度变得相当.因此,它们证实了几十年的理论预测,并为强相关金属中的磁相关模型提供了坚实的实验基础。
Molecular-field-theory fits to magnetic susceptibilities of antiferromagnetic GdCu2Si2, CuO, LiCrO2, and alpha-CaCr2O4 single crystals below their Neel temperatures