Manipulation of magnetic domain walls via a helicity-independent laser pulse has recently been experimentally demonstrated and various physical mechanisms leading to domain wall dynamics have been discussed. Spin-dependent superdiffusive transport of hot electrons has been identified as one of the possible ways how to affect a magnetic domain wall. Here, we develop a model based on superdiffusive spin-dependent transport to study the laser-induced transport of hot electrons through a smooth magnetic domain wall. We show that the spin transfer between neighboring domains can enhance ultrafast demagnetization in the domain wall. More importantly, our calculations reveal that when the laser pulse is properly focused on to the vicinity of the domain wall, it can excite sufficiently strong spin currents to generate a spin-transfer torque that can rapidly move the magnetic domain wall by several nanometers in several hundreds of femtoseconds, leading to a huge nonequilibrium domain wall velocity.
Ultrafast demagnetization of magnetic layers pumped by a femtosecond laser pulse is accompanied by a nonthermal spin-polarized current of hot electrons. These spin currents are studied here theoretically in a spin valve with noncollinear magnetizations. To this end, we introduce an extended model of superdiffusive spin transport that enables to treat noncollinear magnetic configurations, and apply it to the perpendicular spin valve geometry. We show how spin-transfer torques arise due to this mechanism and calculate their action on the magnetization present, as well as how the latter depends o…
The spin- and energy-dependent interface reflectivity of a ferromagnetic (FM) film in contact with a nonmagnetic (NM) film is calculated using a first-principles transport method and incorporated into the superdiffusive spin transport model to study the femtosecond laser-induced ultrafast demagnetization of Fe|NM and Ni|NM (NM= Au, Al & Pt) bilayers. By comparing the calculated demagnetization with transparent and real interfaces, we demonstrate that the spin-dependent reflection of hot electrons has a noticeable influence on the ultrafast demagnetization and the associated terahertz electroma…
In magnetic wires with perpendicular anisotropy, moving domain with only current or only circularly polarized light requires a high power. Here, we propose to reduce it by using both short current pulses and femtosecond laser pulses simultaneously. The wires were made out of perpendicularly magnetized film of Pt/Co/Ni/Co/Pt. The displacement of the domain wall is found to be dependent on the laser helicity. Based on a quantitative analysis of the current-induced domain wall motion, the spin orbit torque contribution can be neglected when compared to the spin transfer torque contribution. The e…
We study the emission of femtosecond spin current pulses at Fe/Au interfaces. Using optical second harmonic generation we demonstrate the control of pulse shape and duration by varying the emitter thickness and show that it is determined by the parameters of hot electrons emission and the diffusive transport. Using a simple model of electron emission we develop a description of superdiffusive spin transport in Au allowing to extract electron velocity and scattering rates from the experimental data. The importance of carrier multiplication in Fe is demonstrated.
Using the sensitivity of magneto-induced second harmonic generation to spin currents (SC), we demonstrate in Fe/Au/Fe/MgO(001) pseudo spin valves the generation of 250 fs-long SC pulses. Their temporal profile indicates that superdiffusive hot electron transport across a sub-100~nm Au layer is close to the ballistic limit and the pulse duration is primarily determined by the thermalization time of laser-excited hot carriers in Fe. Considering the calculated spin-dependent Fe/Au interface transmittance we conclude that a non-thermal spin-dependent Seebeck effect is responsible for the generatio…
The injection of spin currents in semiconductors is one of the big challenges of spintronics. Motivated by the ultrafast demagnetisation and spin injection into metals, we propose an alternative femtosecond route based on the laser excitation of superdiffusive spin currents in a ferromagnet such as Ni. Our calculations show that even though only a fraction of the current crosses the Ni-Si interface, the laser-induced creation of strong transient electrical fields at a ferromagnet-semiconductor interface allows for the injection of chargeless spin currents with a record spin polarisations of 80…
Femtosecond laser pulses can induce ultrafast demagnetization as well as generate bursts of hot electron spin currents. In trilayer spin valves consisting of two metallic ferromagnetic layers separated by a nonmagnetic one, hot electron spin currents excited by an ultrashort laser pulse propagate from the first ferromagnetic layer through the spacer reaching the second magnetic layer. When the magnetizations of the two magnetic layers are noncollinear, this spin current exerts a torque on magnetic moments in the second ferromagnet. Since this torque is acting only within the sub-ps timescale, …
Domain wall motion driven by ultra-short laser pulses is a prerequisite for envisaged low-power spintronics combining storage of information in magneto electronic devices with high speed and long distance transmission of information encoded in circularly polarized light. Here we demonstrate the conversion of the circular polarization of incident femtosecond laser pulses into inertial displacement of a domain wall in a ferromagnetic semiconductor. In our study we combine electrical measurements and magneto-optical imaging of the domain wall displacement with micromagnetic simulations. The optic…
Spin-orbit torque provides a powerful means of manipulating domain walls along magnetic wires. However, the current density required for domain wall motion is still too high to realize low power devices. Here we experimentally demonstrate helicity-dependent domain wall motion by combining synchronized femtosecond laser pulses and short current pulses in Co/Ni/Co ultra-thin film wires with perpendicular magnetization. Domain wall can remain pinned under one laser circular helicity while depinned by the opposite circular helicity. Thanks to the all-optical helicity-dependent effect, the threshol…
Three-dimensional nanostructured functional materials are important systems, allowing new means to intricately control electromagnetic properties. A key problem is realising a 3D printing methodology upon the nanoscale that can yield a range of functional materials. In this letter, it is shown that two-photon lithography when combined with femtosecond machining of sacrificial layers, can be used to realise such a vision and produce 3D functional nanomaterials of complex geometry. This is demonstrated by fabricating 3D magnetic nanowires that exhibit controlled domain wall injection and propaga…
Employing femtosecond laser pulses in front and back side pumping of Au/Fe/MgO(001) combined with detection in two-photon photoelectron emission spectroscopy we analyze local relaxation dynamics of excited electrons in buried Fe, injection into Au across the Fe-Au interface, and electron transport across the Au layer at 0.6 to 2.0 eV above the Fermi energy. By analysis as a function of Au film thickness we obtain the electron lifetimes of bulk Au and Fe and distinguish the relaxation in the heterostructure's constituents. We also show that the excited electrons propagate through Au in a superd…
An ultrafast spin current can be induced by femtosecond laser excitation in a ferromagnetic (FM) thin film in contact with a nonmagnetic (NM) metal. The propagation of an ultrafast spin current into NM metal has recently been found in experiments to generate transient spin accumulation. Unlike spin accumulation in equilibrium NM metals that occurs due to spin transport at the Fermi energy, transient spin accumulation involves highly nonequilibrium hot electrons well above the Fermi level. To date, the diffusion and dissipation of this transient spin accumulation has not been well studied. Usin…
One-dimensional nanoscale devices, such as semiconductor nanowires (NWs) and single- walled carbon nanotubes (SWNTs), have been intensively investigated because of their potential application of future high-speed electronic, optoelectronic, and sensing devices. To overcome current limitations on the speed of contemporary devices, investigation of charge carrier dynamics with an ultrashort time scale is one of the primary steps necessary for developing high-speed devices. In the present study, we visualize ultrafast carrier dynamics in nanoscale devices using a combination of scanning photocurr…
We report the transport characteristics of both electrons and holes through narrow constricted crystalline Si "wall-like" long-channels that were surrounded by a thermally grown SiO2 layer. Importantly, as a result of the existence of fixed oxide charges in the thermally grown SiO2 layer and the Si/SiO2 interface, the effective Si cross-sectional wall widths were considerably narrower than the actual physical widths, due the formation of depletion regions from both sides. These nanostructures were configured into a metal-semiconductor-metal device configuration that was isolated from the subst…
Revealing domain wall stability during ultrafast demagnetization
Max Planck Institute for Multidisciplinary Sciences（马克斯·普朗克多学科研究所）；Institute of Physics, University of Augsburg（奥格斯堡大学物理研究所）；School of Electrical Engineering, Tel Aviv University（特拉维夫大学电气工程学院）；th Physical Institute, University of Göttingen（哥廷根大学第四物理研究所）；Radboud University, Institute for Molecules and Materials（拉德堡德大学分子与材料研究所）
The Su, Schrieffer and Heeger (SSH) model, describing the soliton excitations in polyacetylene due to the formation of antiphase domain walls (DW) from the alternating bond pattern, has served as a paradigmatic example of one-dimensional (1D) chiral topological insulators. While the SSH model has been realized in photonic and plasmonic systems, there have been limited analogues in three-dimensional (3D) electronic systems, especially regarding the formation of antiphase DWs. Here, we propose that pristine bulk Bi, in which the dimerization of $(111)$ atomic layers renders alternating covalent …
All-optical switching (AOS) of magnetic materials describes the reversal of the magnetization using short (femtosecond) laser pulses, and has been observed in a variety of materials. In the past decade it received extensive attention due to its high potential for fast and energy-efficient data writing in future spintronic memory applications. Unfortunately, the AOS mechanism in the ferromagnetic multilayers commonly used in spintronics needs multiple pulses for the magnetization reversal, losing its speed and energy efficiency. Here, we experimentally demonstrate `on-the-fly' single-pulse AOS …
We use time-resolved x-ray resonant magnetic scattering (tr-XRMS) at the Co M$_{2,3}$- and Tb O$_1$-edges to study ultrafast demagnetization in an amorphous Co$_{88}$Tb$_{12}$ alloy with stripe domains. Combining the femtosecond temporal with nanometer spatial resolution of our experiment, we demonstrate that the equilibrium spin texture of the thin film remains unaltered by the optical pump-pulse on ultrashort timescales ($<$1 ps). However, after $\simeq$ 4 ps, we observe the onset of a significant domain wall broadening, which we attribute to a reduction of the uniaxial magnetic anisotropy o…
The absence of stray fields, their insensitivity to external magnetic fields, and ultrafast dynamics make antiferromagnets promising candidates for active elements in spintronic devices. Here, we demonstrate manipulation of the Néel vector in the metallic collinear antiferromagnet Mn$_2$Au by combining strain and femtosecond laser excitation. Applying tensile strain along either of the two in-plane easy axes and locally exciting the sample by a train of femtosecond pulses, we align the Néel vector along the direction controlled by the applied strain. The dependence on the laser fluence and str…
Understanding microscopic processes in materials and devices that can be switched by light requires experimental access to dynamics on nanometer length and femtosecond time scales. Here, we introduce ultrafast dark-field electron microscopy, tailored to map the order parameter across a structural phase transition. We track the evolution of charge-density wave domains in 1T-TaS2 after ultrashort laser excitation, elucidating relaxation pathways and domain wall dynamics. The unique benefits of selective contrast enhancement will inspire future beam shaping technology in ultrafast transmission el…
The observed magnetization switching by circularly polarized ultrafast laser pulses has been attributed to the inverse Faraday effect in which the induced non-equilibrium orbital momentum serves as an effective magnetic filed via spin-orbit coupling for magnetization rotation and switching. We critically examine this scenario by explicitly calculating the magnitude of the induced orbital momentum for generic itinerant band. We show that the calculated induced angular momentum is not large enough for reversing the magnetization in one laser pulse with the order of 100 femtosecond duration. Inst…
