We present and analyze a toolbox for the controlled manipulation of ultracold polar molecules, consisting of detection of molecules, atom-molecule entanglement, and engineering of dissipative dynamics. Our setup is based on fast chemical reactions between molecules and atoms leading to a quantum Zeno-based collisional blockade in the system. We demonstrate that the experimental parameters for achieving high fidelities can be found using a straightforward numerical optimization. We exemplify our approach for a system comprised of NaK molecules and Na atoms and we discuss the consequences of residual imperfections such as a finite strength of the quantum Zeno blockade.
We demonstrate the control of quantum tunneling in an ultracold lattice gas by the measurement backaction imposed by an imaging process. A {\em in situ} imaging technique is used to acquire repeated images of an ultracold gas confined in a shallow optical lattice. The backaction induced by these position measurements modifies the coherent quantum tunneling of atoms within the lattice. By smoothly varying the rate at which spatial information is extracted from the atomic ensemble, we observe the continuous crossover from the 'weak measurement regime' where position measurements have little infl…
We study a one-dimensional system of interacting spinless fermions subject to a localized loss, where the interplay of gapless quantum fluctuations and particle interactions leads to an incarnation of the quantum Zeno effect of genuine many-body nature. This model constitutes a non-equilibrium counterpart of the paradigmatic Kane-Fisher potential barrier problem, and it exhibits strong interaction effects due to the gapless nature of the system. As a central result, we show that the loss probability is strongly renormalized near the Fermi momentum as a realization of the quantum Zeno effect, r…
We show that the quantum Zeno effect gives rise to the Hall effect by tailoring the Hilbert space of a two-dimensional lattice system into a single Bloch band with a nontrivial Berry curvature. Consequently, a wave packet undergoes transverse motion in response to a potential gradient -- a phenomenon we call the Zeno Hall effect to highlight its quantum Zeno origin. The Zeno Hall effect leads to retroreflection at the edge of the system due to an interplay between the band flatness and the nontrivial Berry curvature. We propose an experimental implementation of this effect with ultracold atoms…
We investigate theoretically the suppression of two-body losses when the on-site loss rate is larger than all other energy scales in a lattice. This work quantitatively explains the recently observed suppression of chemical reactions between two rotational states of fermionic KRb molecules confined in one-dimensional tubes with a weak lattice along the tubes [Yan et al., Nature 501, 521-525 (2013)]. New loss rate measurements performed for different lattice parameters but under controlled initial conditions allow us to show that the loss suppression is a consequence of the combined effects of …
Quantum optics and ultracold gases are established fields, but they almost do not overlap: the quantum nature of light is typically neglected in works on ultracold atoms. In our work the quantumness of both light and ultracold matter plays a key role. First, we show that light is a quantum nondemolition (QND) probe of many-body phases: they can be distinguished by correlations and full distribution functions (we consider bosons, fermions, and dipolar molecules). Light is not only sensitive to densities, but also to the matter-field interference. Second, we prove that the measurement backaction…
The interplay between measurement and quantum correlations in many-body systems can lead to novel types of collective phenomena which are not accessible in isolated systems. In this work, we merge the Zeno-paradigm of quantum measurement theory with the concept of polarons in condensed-matter physics. The resulting quantum-Zeno Fermi-polaron is a quasi-particle which emerges for lossy impurities interacting with a quantum-degenerate bath of fermions. For loss rates of the order of the impurity-fermion binding energy the quasi-particle is short lived. However, we show that in the strongly dissi…
Measurement is one of the most counter-intuitive aspects of quantum physics. Frequent measurements of a quantum system lead to quantum Zeno dynamics where time evolution becomes confined to a subspace defined by the projections. However, weak measurement performed at a finite rate is also capable of locking the system into such a Zeno subspace in an unconventional way: by Raman-like transitions via virtual intermediate states outside this subspace, which are not forbidden. Here, we extend this concept into the realm of non-Hermitian dynamics by showing that the stochastic competition between m…
We study the dynamics of counterflowing bosonic and fermionic lithium atoms. First, by tuning the interaction strength we measure the critical velocity vc of the system in the BEC-BCS crossover in the low temperature regime and we compare it to the recent prediction of Castin et al., Comptes Rendus Physique, 16, 241 (2015). Second, raising the temperature of the mixture slightly above the superfluid transitions reveals an unexpected phase-locking of the oscillations of the clouds. We interpret this observation as resulting from a Zeno-like effect induced by dissipation.
Recent studies of quantum circuit models have theoretically shown that frequent measurements induce a transition in a quantum many-body system, which is characterized by the change of the scaling law of the entanglement entropy from a volume law to an area law. In order to propose a way for experimentally observing this measurement-induced transition, we present numerical analyses using matrix-product states on quench dynamics of a dissipative Bose-Hubbard model with controllable two-body losses, which has been realized in recent experiments with ultracold atoms. We find that when the strength…
In this review, we discuss the properties of a few impurity atoms immersed in a gas of ultracold fermions, the so-called Fermi polaron problem. On one side, this many-body system is appealing because it can be described almost exactly with simple diagrammatic and/or variational theoretical approaches. On the other, it provides quantitatively reliable insight into the phase diagram of strongly interacting population imbalanced quantum mixtures. In particular, we show that the polaron problem can be applied to study itinerant ferromagnetism, a long standing problem in quantum mechanics.
The coupling of internal electronic excitations to vibrational modes of the external motion of ultracold atoms in an optical lattice is studied here in using a perturbation expansion in small atomic displacements. In the Mott insulator case with one atom per site, the resonance dipole-dipole coupling between neighboring sites can induce emission and absorption of vibrational quanta. Within a cavity in the strong exciton-photon coupling regime such coupling results in polariton-vibration interactions, which create a significant thermalization mechanism for polaritons toward their minimum energy…
We investigate the use of microwave radiation to produce a repulsive shield between pairs of ultracold polar molecules and prevent collisional losses that occur when molecular pairs reach short range. We carry out coupled-channels calculations on RbCs+RbCs and CaF+CaF collisions in microwave fields. We show that effective shielding requires predominantly circular polarization, but can still be achieved with elliptical polarization that is around 90% circular.
We present a unified formalism for describing chemical reaction rates of trapped, ultracold molecules. This formalism reduces the scattering to its essential features, namely, a propagation of the reactant molecules through a gauntlet of long-range forces before they ultimately encounter one another, followed by a probability for the reaction to occur once they do. In this way, the electric-field dependence should be readily parametrized in terms of a pair of fitting parameters (along with a $C_6$ coefficient) for each asymptotic value of partial wave quantum numbers $|L,M \rangle$. From this,…
We present an architecture for the quantum simulation of many-body spin interactions based on ultracold polar molecules trapped in optical lattices. Our approach employs digital quantum simulation, i.e., the dynamics of the simulated system is reproduced by the quantum simulator in a stroboscopic pattern, and allows to simulate both coherent and dissipative dynamics. We discuss the realization of Kitaev's toric code Hamiltonian, a paradigmatic model involving four-body interactions, and we analyze the requirements for an experimental implementation.
Analytic expressions describe universal elastic and reactive rates of quasi-two-dimensional and quasi-one-dimensional collisions of highly reactive ultracold molecules interacting by a van der Waals potential. Exact and approximate calculations for the example species of KRb show that stability and evaporative cooling can be realized for spin-polarized fermions at moderate dipole and trapping strength, whereas bosons or unlike fermions require significantly higher dipole or trapping strengths.
We report the measurement of the anisotropic AC polarizability of ultracold polar $^{40}$K$^{87}$Rb molecules in the ground and first rotationally excited states. Theoretical analysis of the polarizability agrees well with experimental findings. Although the polarizability can vary by more than 30%, a "magic" angle between the laser polarization and the quantization axis is found where the polarizability of the $|N=0,m_N=0>$ and the $|N=1,m_N=0>$ states match. At this angle, rotational decoherence due to the mismatch in trapping potentials is eliminated, and we observe a sharp increase in the …
Heteronuclear alkali-metal dimers represent the class of molecules of choice for creating samples of ultracold molecules exhibiting an intrinsic large permanent electric dipole moment. Among them, the KCs molecule, with a permanent dipole moment of 1.92~Debye still remains to be observed in ultracold conditions. Based on spectroscopic studies available in the literature completed by accurate quantum chemistry calculations, we propose several optical coherent schemes to create ultracold bosonic and fermionic KCs molecules in their absolute rovibrational ground level, starting from a weakly boun…
We present a novel approach to precisely synthesize arbitrary polarization states of light with a high modulation bandwidth. Our approach consists of superimposing two laser light fields with the same wavelength, but with opposite circular polarizations, where the phase and the amplitude of each light field are individually controlled. We find that the polarization-synthesized beam reaches a degree of polarization of 99.99%, which is mainly limited by static spatial variations of the polarization state over the beam profile. We also find that the depolarization caused by temporal fluctuations …
We demonstrate a scheme for direct absorption imaging of an ultracold ground-state polar molecular gas near quantum degeneracy. A challenge in imaging molecules is the lack of closed optical cycling transitions. Our technique relies on photon shot-noise limited absorption imaging on a strong bound-bound molecular transition. We present a systematic characterization of this imaging technique. Using this technique combined with time-of-flight (TOF) expansion, we demonstrate the capability to determine momentum and spatial distributions for the molecular gas. We anticipate that this imaging techn…
We employ radio-frequency spectroscopy to investigate a polarized spin-mixture of ultracold ${}^6$Li atoms close to a broad Feshbach scattering resonance. Focusing on the regime of strong repulsive interactions, we observe well-defined coherent quasiparticles even for unitarity-limited interactions. We characterize the many-body system by extracting the key properties of repulsive Fermi polarons: the energy $E_+$, the effective mass $m^*$, the residue $Z$ and the decay rate $Γ$. Above a critical interaction, $E_+$ is found to exceed the Fermi energy of the bath while $m^*$ diverges and even tu…
Ultracold molecules trapped in optical tweezers show great promise for the implementation of quantum technologies and precision measurements. We study a prototypical scenario where two interacting polar molecules placed in separate traps are controlled using an external electric field. This, for instance, enables a quantum computing scheme in which the rotational structure is used to encode the qubit states. We estimate the typical operation timescales needed for state engineering to be in the range of few microseconds. We further underline the important role of the spatial structure of the tw…
We design dipolar quantum many-body Hamiltonians that will facilitate the realization of exotic quantum phases under current experimental conditions achieved for polar molecules. The main idea is to modulate both single-body potential barriers and two-body dipolar interactions on a spatial scale of tens of nanometers to strongly enhance energy scales and, therefore, relax temperature requirements for observing new quantum phases of engineered many-body systems. We consider and compare two approaches. In the first, nanoscale barriers are generated with standing wave optical light fields exploit…
We study the growth dynamics of ordered structures of strongly interacting polar molecules in optical lattices. Using dipole blockade of microwave excitations, we map the system onto an interacting spin-1/2 model possessing ground states with crystalline order, and describe a way to prepare these states by non-adiabatically driving the transitions between molecular rotational levels. The proposed technique bypasses the need to cross a phase transition and allows for the creation of ordered domains of considerably larger size compared to approaches relying on adiabatic preparation.
We present a technique for engineering quantum magnets via ultracold polar molecules in optical lattices and explore exotic interplay between its spin superfluidity and solidity. The molecular ground and first excited rotational states are resonantly coupled by a linearly polarized microwave field. The spin-up (spin-down) states are presented by molecular rotational states of electric dipole moment along (against) the coupling field. By controlling the angle between the lattice direction and the coupling field, the inter-site interaction can be tuned from antiferromagnetic to ferromagnetic. Fu…
In contrast to the fully projective limit of strong quantum measurement, where the evolution is locked to a small subspace (quantum Zeno dynamics), or even frozen completely (quantum Zeno effect), the weak non-projective measurement can effectively compete with standard unitary dynamics leading to nontrivial effects. Here we consider global weak measurement addressing collective variables, thus preserving quantum superpositions due to the lack of which path information. While for certainty we focus on ultracold atoms, the idea can be generalized to other multimode quantum systems, including va…
Recent theory has indicated how to emulate tunable models of quantum magnetism with ultracold polar molecules. Here we show that present molecule optical lattice experiments can accomplish three crucial goals for quantum emulation, despite currently being well below unit filling and not quantum degenerate. The first is to verify and benchmark the models proposed to describe these systems. The second is to prepare correlated and possibly useful states in well-understood regimes. The third is to explore many-body physics inaccessible to existing theoretical techniques. Our proposal relies on a n…
We report measurements of the ac polarizabilities of ultracold ground-state $^{23}\rm{Na}^{87}\rm{Rb}$ molecules. While the polarizability of the ground rotational state $J = 0$ is isotropic, that of the first excited rotational state $J = 1$ is anisotropic and depends strongly on the light polarization angle. We obtain both polarizabilities precisely by combining trap oscillation frequency measurement and high resolution rotational spectroscopy driven by microwave. With the optimized light polarization angle and intensity combination, the nonuniformity of the differential ac Stark shift betwe…
Scattering resonances are an essential tool for controlling interactions of ultracold atoms and molecules. However, conventional Feshbach scattering resonances, which have been extensively studied in various platforms, are not expected to exist in most ultracold polar molecules due to the fast loss that occurs when two molecules approach at a close distance. Here, we demonstrate a new type of scattering resonances that is universal for a wide range of polar molecules. The so-called field-linked resonances occur in the scattering of microwave-dressed molecules due to stable macroscopic tetramer…
Quantum states with long-lived coherence are essential for quantum computation, simulation and metrology. The nuclear spin states of ultracold molecules prepared in the singlet rovibrational ground state are an excellent candidate for encoding and storing quantum information. However, it is important to understand all sources of decoherence for these qubits, and then eliminate them, in order to reach the longest possible coherence times. Here, we fully characterise the dominant mechanisms for decoherence of a storage qubit in an optically trapped ultracold gas of RbCs molecules using high-reso…
The dynamics of a bilayer system of ultracold dipolar molecules exhibits classical and quantum glassy behavior, characterized by long tails in the relaxation time and dynamical heterogeneity. In the proposed setup, quantum fluctuations are of the order of thermal fluctuations and the degree of frustration can tuned by the interlayer distance. We present experimental accessible order parameters based on marker molecules, distinguished by properly chosen internal levels, and find quantum features of dynamical heterogeneity.
We explore repulsive Fermi polarons in one-dimensional harmonically trapped few-body mixtures of ultracold atoms using as a case example a $^6$Li-$^{40}$K mixture. A characterization of these quasiparticle-like states, whose appearance is signalled in the impurity's radiofrequency spectrum, is achieved by extracting their lifetime and residua. Increasing the number of $^{40}$K impurities leads to the occurrence of both single and multiple polarons that are entangled with their environment. An interaction-dependent broadening of the spectral lines is observed suggesting the presence of induced …
We explore the feasibility of optically forming long-range tetratomic and larger polyatomic molecules in their ground electronic state from ultracold pairs of polar molecules aligned by external fields. Depending on the relative orientation of the interacting diatomic molecules, we find that a tetratomic can be formed either as a weakly bound complex in a very extended halo state or as a pure long-range molecule composed of collinear or nearly-collinear diatomic molecules. The latter is a novel type of tetratomic molecule comprised of two diatomic molecules bound at long intermolecular range a…
Recent work on ultracold polar molecules, governed by a generalization of the t-J Hamiltonian, suggests that molecules may be better suited than atoms for studying d-wave superfluidity due to stronger interactions and larger tunability of the system. We compute the phase diagram for polar molecules in a checkerboard lattice consisting of weakly coupled square plaquettes. In the simplest experimentally realizable case where there is only tunneling and an XX-type spin-spin interaction, we identify the parameter regime where d-wave superfluidity occurs. We also find that the inclusion of a densit…
Trapping ultracold atoms in optical lattices enabled numerous breakthroughs uniting several disciplines. Coupling these systems to quantized light leads to a plethora of new phenomena and has opened up a new field of study. Here we introduce a physically novel source of competition in a many-body strongly correlated system: We prove that quantum backaction of global measurement is able to efficiently compete with intrinsic short-range dynamics of an atomic system. The competition becomes possible due to the ability to change the spatial profile of a global measurement at a microscopic scale co…
We investigate the effect of far-off-resonant trapping light on ultracold bosonic RbCs molecules. We use kHz-precision microwave spectroscopy to measure the differential AC Stark shifts between the ground and first excited rotational levels of the molecule with hyperfine-state resolution. We demonstrate through both experiment and theory that coupling between neighboring hyperfine states manifests in rich structure with many avoided crossings. This coupling may be tuned by rotating the polarization of the linearly polarized trapping light. A combination of spectroscopic and parametric heating …
In this article we address the general approach for calculating dynamical dipole polarizabilities of small quantum systems, based on a sum-over-states formula involving in principle the entire energy spectrum of the system. We complement this method by a few-parameter model involving a limited number of effective transitions, allowing for a compact and accurate representation of both the isotropic and anisotropic components of the polarizability. We apply the method to the series of ten heteronuclear molecules composed of two of ($^7$Li,$^{23}$Na,$^{39}$K,$^{87}$Rb,$^{133}$Cs) alkali-metal ato…
We study the checkerboard supersolid of the hard-core Bose-Hubbard model with the dipole-dipole interaction. This supersolid is different from all other supersolids found in lattice models in the sense that superflow paths through which interstitials or vacancies can hop freely are absent in the crystal. By focusing on repulsive interactions between interstitials, we reveal that the long-range tail of the dipole-dipole interaction have the role of increasing the energy cost of domain wall formations. This effect produces the supersolid by the second-order hopping process of defects. We also pe…
Ultracold atoms and molecules trapped in optical lattices are expected to serve as simulators of strongly correlated systems and topological states of matter. A fascinating example is to realize the Kitaev quantum spin liquid by using ultracold polar molecules. However, although experimental implementation of the Kitaev-type interaction was proposed, the stability of the Kitaev quantum spin liquid has not been fully investigated thus far. Here we study a quantum spin model with long-range angle-dependent Kitaev-type interactions proposed for the polar molecules, by the pseudofermion functional…
The system of ultracold atoms with hyperfine spin $F=3/2$ might be unstable against the formation of quintet pairs if the interaction is attractive in the quintet channel. We have investigated the behavior of correlation functions in a model including only s-wave interactions at quarter filling by large-scale density-matrix renormalization-group simulations. We show that the correlations of quintet pairs become quasi-long-ranged, when the system is partially polarized, leading to the emergence of various mixed superfluid phases in which BCS-like pairs carrying different magnetic moment coexist…
Ultracold polar molecules (UPMs) are emerging as a novel and powerful platform for fundamental applications in quantum science. Here, we report characterization of the coherence between nuclear spin levels of ultracold ground-state sodium-rubidium molecules loaded into a 3D optical lattice with a nearly photon scattering limited trapping lifetime of 9(1) seconds. After identifying and compensating the main sources of decoherence, we achieve a maximum nuclear spin coherence time of $T_2^* = 3.3(6)$~s with two-photon Ramsey spectroscopy. Furthermore, based on the understanding of the main factor…
We show that single-component fermionic polar molecules confined to a 2D geometry and dressed by a microwave field, may acquire an attractive $1/r^3$ dipole-dipole interaction leading to superfluid p-wave pairing at sufficiently low temperatures even in the BCS regime. The emerging state is the topological $p_x+ip_y$ phase promising for topologically protected quantum information processing. The main decay channel is via collisional transitions to dressed states with lower energies and is rather slow, setting a lifetime of the order of seconds at 2D densities $\sim 10^8$ cm$^{-2}$.
By selecting two dressed rotational states of ultracold polar molecules in an optical lattice, we obtain a highly tunable generalization of the t-J model, which we refer to as the t-J-V-W model. In addition to XXZ spin exchange, the model features density-density interactions and novel density-spin interactions; all interactions are dipolar. We show that full control of all interaction parameters in both magnitude and sign can be achieved independently of each other and of the tunneling. As a first step towards demonstrating the potential of the system, we apply the density matrix renormalizat…
Mobile impurity atoms immersed in Bose-Einstein condensates provide a new platform for exploring Bose polarons. Recent experimental advances in the field of ultracold atoms make it possible to realize such systems with highly tunable microscopic parameters and to explore equilibrium and dynamical properties of polarons using a rich toolbox of atomic physics. In this paper we present a detailed theoretical analysis of Bose polarons in one dimensional systems of ultracold atoms. By combining a non-perturbative renormalization group approach with numerically exact diffusion Monte Carlo calculatio…
We present a quantitative, near-term experimental blueprint for the quantum simulation of topological insulators using lattice-trapped ultracold polar molecules. In particular, we focus on the so-called Hopf insulator, which represents a three-dimensional topological state of matter existing outside the conventional tenfold way and crystalline-symmetry-based classifications of topological insulators. Its topology is protected by a \emph{linking number} invariant, which necessitates long-range spin-orbit coupled hoppings for its realization. While these ingredients have so far precluded its rea…
This paper reviews recent advances in the study of strongly interacting systems of dipolar molecules. Heteronuclear molecules feature large and tunable electric dipole moments, which give rise to long-range and anisotropic dipole-dipole interactions. Ultracold samples of dipolar molecules with long-range interactions offer a unique platform for quantum simulations and the study of correlated many-body physics. We provide an introduction to the physics of dipolar quantum gases, both electric and magnetic, and summarize the multipronged efforts to bring dipolar molecules into the quantum regime.…
The field of ultracold quantum matter has burgeoned over the last few decades, thanks to the growing capabilities for atomic systems to be probed and manipulated with exquisite control. Researchers can now precisely create and study quantum many-body states that are effectively isolated from the external environment. Much of the work in ultracold matter has focused on systems of alkali or alkaline-earth atoms, mainly due to their ease of cooling. Extending this precise control to molecules has seen rapidly increasing interest and activity, as molecules possess additional degrees of freedom tha…
We have investigated Feshbach resonances in collisions of high-spin atoms such as Er and Dy with closed-shell atoms such as Sr and Yb, using coupled-channel scattering and bound-state calculations. We consider both low-anisotropy and high-anisotropy limits. In both regimes we find many resonances with a wide variety of widths. The wider resonances are suitable for tuning interatomic interactions, while some of the narrower resonances are highly suitable for magnetoassociation to form high-spin molecules. These molecules might be transferred to short-range states, where they would have large ma…
