We present a method for the simultaneous observation of heteronuclear multi-quantum coherences (up to the 3rd order), which give an additional degree of freedom for ultralow magnetic field (ULF) MR experiments, where the chemical shift is negligible. The nonequilibrium spin state is generated by Signal Amplification By Reversible Exchange (SABRE) and detected at ULF with SQUID-based NMR. We compare the results obtained by the heteronuclei Correlated SpectroscopY (COSY) with a Flip Angle FOurier Series (FAFOS) method. COSY allows a quantitative analysis of homo- and heteronuclei quantum coherences.
Ultralow-power coherent qubit control using AQFP logic at millikelvin temperatures
RIKEN（理化学研究所）；Tokyo University of Science（东京科学大学）；The University of Tokyo（东京大学）；National Institute of Advanced Industrial Science and Technology (AIST)（国立产业技术综合研究所）；Tohoku University（东北大学）；Yokohama National University（横滨国立大学）；Kobe University（神户大学）
We present an algorithm for synchronizing two clocks based on second-order quantum interference between entangled photons generated by parametric down-conversion. The procedure is distinct from the standard Einstein two-way clock synchronization method in that photon correlations are used to define simultaneous events in the frame of reference of a Hong-Ou-Mandel (HOM) interferometer. Once the HOM interferometer is balanced, by use of an adjustable optical delay in one arm, arrival times of simultaneously generated photons are recorded by each clock. Classical information on the arrival times …
We present a direct measurement of the spatiotemporal coherence of parametric down-conversion in the range of negative group-velocity dispersion. In this case, the frequency-angular spectra are ring-shaped and temporal coherence is coupled to spatial coherence. Correspondingly, the lack of coherence due to spatial displacement can be compensated with the introduction of time delay. We show a simple technique, based on a modified Mach-Zehnder interferometer, which allowed us to measure time coherence and near-field space coherence simultaneously, with complete control of both variables. This te…
A new scheme for infrared generation without population inversion between subbands in quantum-well and quantum-dot lasers is presented and documented by detailed calculations. The scheme is based on the simultaneous generation at three frequencies: optical lasing at the two interband transitions which take place simultaneously, in the same active region, and serve as the coherent drive for the IR field. This mechanism for frequency down-conversion does not rely upon any ad hoc assumptions of long-lived coherences in the semiconductor active medium. And it should work efficiently at room temper…
Polarization-sensitive quantum optical coherence tomography (PS-QOCT) makes use of a Type-II twin-photon light source for carrying out optical sectioning with polarization sensitivity. A BBO nonlinear optical crystal pumped by a Ti:sapphire psec-pulsed laser is used to confirm the theoretical underpinnings of this imaging paradigm. PS-QOCT offers even-order dispersion cancellation with simultaneous access to the group-velocity dispersion characteristics of the interstitial medium between the reflecting surfaces of the sample.
We experimentally study two-photon coherence in plasmon-assisted transmission with a two-photon Mach-Zehnder (MZ) interferometer. Two collinear photons of identical or orthogonal polarization are simultaneously incident on one optically thick metal film, perforated with a periodic array of subwavelength holes. The de Broglie wavelength of plasmon-assisted transmitted photons is measured, which shows that two photons are re-eradiated by the plasmons and the quantum coherence of biphoton is preserved in the conversion process of transforming biphoton to plasmons and then back to biphoton.
Nanchang University（南昌大学）；School of Materials Science and Engineering, Nanchang University（南昌大学材料科学与工程学院）；Institute of Modern Physics, Nanchang University（南昌大学现代物理研究所）
In this work, we studied the relaxation dynamics of coherences of different order present in a system of two coupled nuclear spins. We used a previously designed model for intrinsic noise present in such systems which considers the Lindblad master equation for Markovian relaxation. We experimentally created zero-, single- and double- quantum coherences in several two-spin systems and performed a complete state tomography and computed state fidelity. We experimentally measured the decay of zero- and double- quantum coherences in these systems. The experimental data fitted well to a model that c…
We consider the physical situations where the resource theories of coherence and thermodynamics play competing roles. In particular, we study the creation of quantum coherence using unitary operations with limited thermodynamic resources. We first find the maximal coherence that can be created under unitary operations starting from a thermal state and find explicitly the unitary transformation that creates the maximal coherence. Since coherence is created by unitary operations starting from a thermal state, it requires some amount of energy. This motivates us to explore the trade-off between t…
Solid-state electronic spins are extensively studied in quantum information science, as their large magnetic moments offer fast operations for computing and communication, and high sensitivity for sensing. However, electronic spins are more sensitive to magnetic noise, but engineering of their spectroscopic properties, e.g. using clock transitions and isotopic engineering, can yield remarkable spin coherence times, as for electronic spins in GaAs, donors in silicon and vacancy centres in diamond. Here we demonstrate simultaneously induced clock transitions for both microwave and optical domain…
Quantum coherence marks a deviation from classical physics, and has been studied as a resource for metrology and quantum computation. Finding reliable and effective methods for assessing its presence is then highly desirable. Coherence witnesses rely on measuring observables whose outcomes can guarantee that a state is not diagonal in a known reference basis. Here we experimentally measure a novel type of coherence witness that uses pairwise state comparisons to identify superpositions in a basis-independent way. Our experiment uses a single interferometric set-up to simultaneously measure the…
Quantum manipulation of coupled mechanical resonators has become an important research topic in optomechanics because these systems can be used to study the quantum coherence effects involving multiple mechanical modes. A prerequisite for observing macroscopic mechanical coherence is to cool the mechanical resonators to their ground state. Here we propose a theoretical scheme to cool two coupled mechanical resonators by introducing an optomechanical interface. The final mean phonon numbers in the two mechanical resonators are calculated exactly and the results show that the ground-state coolin…
Quantum coherence represented by a superposition of energy eigenstates is, together with energy, an important resource for quantum technology and thermodynamics. Energy and quantum coherence however, can be complementary. The increase of energy can reduce quantum coherence and vice versa. Recently, it was realized that steady-state quantum coherence could be autonomously harnessed from a cold environment. We propose a conditional synthesis of $N$ independent two-level systems (TLS) with partial quantum coherence obtained from an environment to one coherent system using a measurement able to in…
Four-wave mixing in resonant atomic vapors based on maximum coherence induced by Stark-chirped rapid adiabatic passage (SCRAP) is investigated theoretically. We show the advantages of a coupling scheme involving maximum coherence and demonstrate how a large atomic coherence between a ground and an highly excited state can be prepared by SCRAP. Full analytic solutions of the field propagation problem taking into account pump field depletion are derived. The solutions are obtained with the help of an Hamiltonian approach which in the adiabatic limit permits to reduce the full set of Maxwell-Bloc…
Er$^{3+}$$:$Y$_2$SiO$_5$ is a material of particular interest due to its suitability for telecom-band quantum memories and quantum transducers interfacing optical communication with quantum computers working in the microwave regime. Extending the coherence lifetimes of the electron spins and the nuclear spins is essential for implementing efficient quantum information processing based on such hybrid electron-nuclear spin systems. The electron spin coherence time of Er$^{3+}$$:$Y$_2$SiO$_5$ is so far limited to several microseconds, and there are significant challenges in optimizing coherence l…
Quantum computation and quantum information processing are emerging technologies that have potential to overcome the physical limitation of traditional computation systems. Present quantum systems based on photons, atoms and molecules, however, all face challenges such as short coherence time, requirement of ultralow temperature and/or high vacuum, and lack of scalability. We report a new type of molecular qubits and nanoparticle ensembles based on thermally controllable transformation between J-aggregation and monomeric states of molecular chromophores, using pyrrolopyrrole cyanine tethered w…
Multipartite entanglement plays an important role in quantum information processing and quantum metrology. Here, the dressing-energy-level-cascaded (DELC) four-wave mixing (FWM) processes are proposed to generate all-optical controlled multipartite entanglement within a single device. The entanglement characteristics of the produced states of light are characterized by applying the Duan criterion and the positivity under partial transposition criterion. Moreover, by using an internal dressing field to modulate atomic coherence, multiple quantum coherent channels of FWM are simultaneously const…
In relation of observable and quantum state, the entity $I_C$ from previous work quantifies simultaneously coherence, incompatibility and quantumness. In this article its application to quantum correlations in bipartite states is studied. It is shown that Zurek's quantum discord can always be expressed as excess coherence information (global minus local). Strong and weak zero-discord cases are distinguished and investigated in terms of necessary and sufficient and sufficient conditions respectively. A unique string of relevant subsystem observables, each a function of the next, for "interrogat…
The uncertainty principle sets a bound on our ability to predict the measurement outcomes of two incompatible observables which are measured on a quantum particle simultaneously. In quantum information theory, the uncertainty principle can be formulated in terms of the Shannon entropy. Entropic uncertainty bound can be improved by adding a particle which correlates with the measured particle. The added particle acts as a quantum memory. In this work, a method is provided for obtaining the entropic uncertainty relations in the presence of a quantum memory by using quantum coherence. In the meth…
The uncertainty principle sets limit on our ability to predict the values of two incompatible observables measured on a quantum particle simultaneously. This principle can be stated in various forms. In quantum information theory, it is expressed in terms of the entropic measures. Uncertainty bound can be altered by considering a particle as a quantum memory correlating with the primary particle. In this work, we provide a method for converting the entropic uncertainty relation in the absence of quantum memory to that in its presence. It is shown that the lower bounds obtained through the meth…
We report a tunable single-photon source based on a single trapped ion. Employing spontaneous Raman scattering and in-vacuum optics with large numerical aperture, single photons are efficiently created with controlled temporal shape and coherence time. These can be varied between 70 ns and 1.6 $μ$s, as characterized by operating two sources simultaneously in two remote ion traps which reveals mutual and individual coherence through two-photon interference.
We present high-performance megahertz micromechanical oscillators based on freestanding epitaxial AlGaAs distributed Bragg reflectors. Compared with dielectric reflectors, the low mechanical loss of the monocrystalline heterostructure gives rise to significant improvements in the achievable mechanical quality factor Q while simultaneously exhibiting near unity reflectivity. Experimental characterization yields an optical reflectivity exceeding 99.98% and mechanical quality factors up to 20 000 at 4 K. This materials system is not only an interesting candidate for optical coatings with ultralow…
Here, we study a minimal model, the three-level V system coupled to two heat baths, and investigate the role of quantum coherences in heat transport in both the transient regime and in the nonequilibrium steady-state. In our model, energy is exchanged between the baths through two parallel pathways, which can be made distinct through the nondegeneracy of excited levels (energy splitting $Δ$) and a control parameter $α$, which adjusts the strength of one of the arms. Using a nonsecular quantum master equation of Redfield form, we succeed in deriving closed-form expressions for the quantum coher…
The existence of vacuum fluctuations is one of the most important predictions of modern quantum field theory. In the vacuum state, fluctuations occurring at different frequencies are uncorrelated. However, if a parameter in the Lagrangian of the field is modulated by an external pump, vacuum fluctuations stimulate spontaneous downconversion processes, creating squeezing between modes symmetric with respect to half of the frequency of the pump. Here we show that by double parametric pumping of a superconducting microwave cavity, it is possible to generate another fundamental type of correlation…
Based on the second-order quantum interference between frequency entangled photons that are generated by parametric down conversion, a quantum strategic algorithm for synchronizing two spatially separated clocks has been recently presented. In the reference frame of a Hong-Ou-Mandel (HOM) interferometer, photon correlations are used to define simultaneous events. Once the HOM interferometer is balanced by use of an adjustable optical delay in one arm, arrival times of simultaneously generated photons are recorded by each clock. The clock offset is determined by correlation measurement of the r…
We examine quantum statistics of optical photons emitted from atomic ensembles which are classically driven and simultaneously coupled to a two-level atom via microwave photon exchange. Quantum statistics and correlations are analyzed by calculating second order coherence degree, von Neumann entropy, spin squeezing for multi-particle entanglement, as well as genuine two and three-mode entanglement parameters for steady state and non-equilibrium situations. Coherent transfer of population between the radiation modes and quantum state mapping between the two-level atom and the optical modes are …
The introduction of the quantum analogue of a Carnot engine based on a bath comprising of particles with a small amount of coherence initiated an active line of research on the harnessing of different quantum resources for the enhancement of thermal machines beyond the standard reversible limit, with an emphasis on non-thermal baths containing quantum coherence. In our work, we investigate the impact of coherence on the thermodynamic tasks of a collision model which is composed of a system interacting, in the continuous time limit, with a series of coherent ancillas of two baths at different t…
Nitrogen-vacancy centres (NVs) in diamond are attractive for research straddling quantum information science and nanoscale magnetometry and thermometry. While ultrapure bulk diamond NVs sustain the longest spin coherence times among optically accessible spins, nanodiamond NVs display persistently poor spin coherence. Here we introduce high-purity nanodiamonds accommodating record-long NV coherence times, >60 us, observed via universal dynamical decoupling. We show that the main contribution to decoherence comes from nearby nitrogen impurities rather than surface states. We protect the NV spin …
In the endeavour to make quantum computers a reality, integrated superconducting circuits have become a promising architecture. A major challenge of this approach is decoherence originating from spurious atomic tunneling defects at the interfaces of qubit electrodes, which may resonantly absorb energy from the qubit's oscillating electric field and reduce the qubit's energy relaxation time $T_1$. Here, we show that qubit coherence can be improved by tuning dominating defects away from the qubit resonance using an applied DC-electric field. We demonstrate a method that optimizes the applied fie…
Quantum states and measurements exhibit wave-like --- continuous, or particle-like --- discrete, character. Hybrid discrete-continuous photonic systems are key to investigating fundamental quantum phenomena, generating superpositions of macroscopic states, and form essential resources for quantum-enhanced applications, e.g. entanglement distillation and quantum computation, as well as highly efficient optical telecommunications. Realizing the full potential of these hybrid systems requires quantum-optical measurements sensitive to complementary observables such as field quadrature amplitude an…
Optomechanical systems offer new opportunities in quantum information processing and quantum sensing. Many solid-state quantum devices operate at millikelvin temperatures -- however, it has proven challenging to operate nanoscale optomechanical devices at these ultralow temperatures due to their limited thermal conductance and parasitic optical absorption. Here, we demonstrate a two-dimensional optomechanical crystal resonator capable of achieving large cooperativity $C$ and small effective bath occupancy $n_b$, resulting in a quantum cooperativity $C_{\text{eff}}\equiv C/n_b \approx 1.3 > 1$ …
Answering the titular question has become a central motivation in the field of quantum biology, ever since the idea was raised following a series of experiments demonstrating wave-like behavior in photosynthetic complexes. Here, we report a direct evaluation of the effect of quantum coherence on the efficiency of three natural complexes. An open quantum systems approach allows us to simultaneously identify their level of "quantumness" and efficiency, under natural physiological conditions. We show that these systems reside in a mixed quantum-classical regime, characterized by dephasing-assiste…
Estimating phase parameters of a three-level system interacting with two classical monochromatic fields in simultaneous and individual metrological strategies
Gaussian boson sampling exploits squeezed states to provide a highly efficient way to demonstrate quantum computational advantage. We perform experiments with 50 input single-mode squeezed states with high indistinguishability and squeezing parameters, which are fed into a 100-mode ultralow-loss interferometer with full connectivity and random transformation, and sampled using 100 high-efficiency single-photon detectors. The whole optical set-up is phase-locked to maintain a high coherence between the superposition of all photon number states. We observe up to 76 output photon-clicks, which yi…
Electron charge qubits are compelling candidates for solid-state quantum computing because of their inherent simplicity in qubit design, fabrication, control, and readout. However, all existing electron charge qubits, built upon conventional semiconductors and superconductors, suffer from severe charge noise that limits the coherence time to the order of 1 microsecond. Here, we report our experimental realization of ultralong-coherence electron charge qubits, based upon isolated single electrons trapped on an ultraclean solid neon surface in vacuum. Quantum information is encoded in the motion…
