测量了12442型KCa $_2$ Fe $_4$ As $_4$ F $_2$单晶在不同磁场下的低温比热。在超导转变温度$T_c$观察到一个明显的SH跳跃,其高度为$ΔC/T|_{T_c}$ = 130 mJ/mol K $^2$.结果表明,电子SH系数$Δγ(H)$在低于3 T的低场区迅速增大,随着场的进一步增大,其增大速度明显减慢,这表明超导体具有较强的各向异性或多能隙特征,在超导能隙中存在一个极小值.与温度相关的SH数据表明存在$T^2$项,该项提供了进一步的信息,并支持具有线节间隙结构的图像。此外,SH转变的起始点在高达9 T的磁场下几乎保持不变,这与在铜酸盐中观察到的相似,并且将该系统置于BCS极限和玻色-爱因斯坦凝聚之间。
英文摘要:
Low-temperature specific heat (SH) is measured for the 12442-type KCa$_2$Fe$_4$As$_4$F$_2$ single crystal under different magnetic fields. A clear SH jump with the height of $ΔC/T|_{T_c}$ = 130 mJ/mol K$^2$ is observed at the superconducting transition temperature $T_c$. It is found that the electronic SH coefficient $Δγ(H)$ quickly increases when the field is in the low-field region below 3 T and then considerably slows down the increase with a further increase in the field, which indicates a rather strong anisotropy or multi-gap feature with a small minimum in the superconducting gap(s). The temperature-dependent SH data indicates the presence of the $T^2$ term, which supplies further information and supports the picture with a line-nodal gap structure. Moreover, the onset point of the SH transition remains almost unchanged under the field as high as 9 T, which is similar to that observed in cuprates, and placed this system in the middle between the BCS limit and the Bose-Einstein condensation.
Anisotropic physical properties and large critical current density in KCa${_2}$Fe${_4}$As${_4}$F${_2}$ single crystal
本文系统地研究了KCa ${_2}$ Fe ${_4}$ As ${_4}$ F ${_2}$单晶的电阻率、霍尔系数、磁光成像、磁化强度和STEM分析。尖锐的抗磁性转变和磁光成像显示单晶的均匀性和突出的豆状穿透的漩涡。电阻率的大的各向异性,其中${ρ_c / ρ_{ab}}$ > 100,和类磁阻${ρ_c}$表明电子态是准二维的。霍尔效应测量表明,KCa ${_2}$ Fe ${_4}$ As ${_4}$ F ${_2}$是一个以空穴为主载流子的多带体系.磁化强度测量结果表明,与其他铁基超导体相比,J $_c$显着更大,J $_c$值取决于磁场的方向。这些J $_c$特性的起源进行了讨论的基础上使用STEM显微结构观察。此外,在重离子辐照方面证明了在KCa ${_2}$ Fe ${_4}$ As ${_4}$ F ${_2}$中J $_c$的进一步增强以用于未来的应用。
Superconductivity in KCa$_2$Fe$_4$As$_4$F$_2$ with Separate Double Fe$_2$As$_2$ Layers
本文报道了五元铁砷氟化物KCa $_2$ Fe $_4$ As $_4$ F $_2$的合成、晶体结构和物理性质。这种新化合物以体心四元晶格(空间群为$I4/mmm$,$a$ = 3.8684(2),c = 31.007(1),$Z$ = 2)结晶,其中含有双Fe $_2$ As $_2$导电层,由绝缘Ca $_2$ F $_2$层隔开。我们的电阻率,直流磁化率和热容量的测量表明,在33 K的KCa $_2$ Fe $_4$作为$_4$ F $_2$的体超导性。
Strong Pauli paramagnetic effect in the upper critical field of KCa$_2$Fe$_4$As$_4$F$_2$
近年来,12442系统铁基超导体由于其独特的双FeAs层结构而引起了人们的广泛关注。在KCa $_2$ Fe $_4$ As $_4$ F $_2$单晶中,在超导转变温度$T_c$附近,观察到面内上临界场随冷却而急剧增加.本文报道了在宽温度范围内对该材料上临界场的高场研究,测量了面外($H\|c$,$H_{c2}^{c}$)和面内($H\|ab$,$H_{c2}^{ab}$)方向。一个次线性的温度依赖性行为观察到的平面外$H_{c2}^{c}$,而强烈的凸曲率与冷却观察到的平面内$H_{c2}^{ab}$。这种行为不能用传统的Werthamer-Helfand-Hohenberg(WHH)模型来描述。基于WHH模型考虑自旋方面的数据分析揭示了大的Maki参数$α=9$,表明面内上临界场受到非常强的泡利顺磁效应的影响。
Spontaneous stoichiometry change in a single crystal of (Ba1-x Kx)Fe2As2 produced by rapid heating method
为了防止Ba_(1-x)K_xFe_2As_2单晶生长过程中K的损失,我们发展了一种快速加热的Sn助熔剂法。获得了最佳超导转变温度TC约为38 K的大单晶,并对其结构、化学和超导性能进行了研究。此外,还研究了不同温度下生长后退火对晶体生长的影响。扫描电子显微镜微探针研究的样品与Ba.25 K.75 Fe 2 As 2的组合物的目标揭示了一个尖锐的分离的两个阶段的组合物,是建议合理的比例的K和Ba含量。
Specific-heat study of superconducting and normal states in FeSe1-xTex (0.6<=x<=1) single crystals: Strong-coupling superconductivity, strong electron-correlation, and inhomogeneity
Multigap nodeless superconductivity in CsCa2Fe4As4F2 probed by heat transport
最近发现了一个新的铁基超导体12442族,对该族的两个成员KCa $_2$ Fe $_4$ As $_4$ F $_2$和CsCa $_2$ Fe $_4$ As $_4$ F $_2$多晶的μ子自旋弛豫($μ$ SR)测量表明,它们都具有$s+d$配对对称的节状超导能隙结构.本文报道了CsCa $_2$ Fe $_4$ As $_4$ F $_2$单晶($T_c$ = 29.3 K)的超低温热导率测量结果。零场下可忽略的剩余线性项$κ_0/T$和$κ_0/T$的场依赖性表明CsCa $_2$ Fe $_4$ As $_4$ F $_2$中存在多个无结超导能隙.这种间隙结构类似于CaKFe $_4$ As $_4$和中等掺杂的Ba $_{1-x}$ K $_x$ Fe $_2$ As $_2$,但与CsCa $_2$ Fe $_4$ As $_4$ F $_2$多晶上的$μ$ SR测量所指示的节状间隙结构相反。
Calorimetric study in single crystal of CsFe$_2$As$_2$
我们测量了用自熔法生长的高质量CsFe $_2$ As $_2$单晶的电阻率和比热。CsFe $_2$ As $_2$晶体在1.8 K时出现了明显的超导转变,转变宽度为0.1 K。急剧的超导转变和比热的显著跳跃表明晶体的高质量。对超导态比热的分析支持CsFe $_2$ As $_2$的非常规配对对称性。
Evolution of crystalline electric field effects, superconductivity, and heavy fermion behavior in the specific heat of Pr(Os$_{1-x}$Ru$_x$)$_4$Sb$_{12}$
Heat transport in RbFe2As2 single crystal: evidence for nodal superconducting gap
测量了铁基超导体RbFe $_2$ As $_2$单晶($T_c \approx$ 2.1 K)的面内热导率,其值可低至100 mK。在零场条件下,观测到一个显著的剩余线性项$κ_0/T$ = 0.65 mW K $^{-2}$ cm $^{-1}$,为结超导能隙提供了明确的证据。$κ_0/T$的场依赖性类似于其姊妹化合物CsFe $_2$ As $_2$的场依赖性,具有相当的剩余电阻率$ρ_0$,并且位于脏的和干净的KFe $_2$ As $_2$之间。这些结果表明,(K,Rb,Cs)Fe $_2$ As $_2$系列超导体具有共同的节隙结构。