The phase diagram of the cuprate superconductors has posed a formidable scientific challenge for more than three decades. This challenge is perhaps best exemplified by the need to understand the normal-state charge transport as the system evolves from Mott insulator to Fermi-liquid metal with doping. Here we report a detailed analysis of the temperature (T) and doping (p) dependence of the planar resistivity of simple-tetragonal HgBa$_2$CuO$_{4+δ}$ (Hg1201), the single-CuO$_2$-layer cuprate with the highest optimal $T_c$. The data allow us to test a recently proposed phenomenological model for the cuprate phase diagram that combines a universal transport scattering rate with spatially inhomogeneous (de)localization of the Mott-localized hole. We find that the model provides an excellent description of the data. We then extend this analysis to prior transport results for several other cuprates, including the Hall number in the overdoped part of the phase diagram, and find little compound-to-compound variation in (de)localization gap scale. The results point to a robust, universal structural origin of the inherent gap inhomogeneity that is unrelated to doping-related disorder. They are inconsistent with the notion that much of the phase diagram is controlled by a quantum critical point, and instead indicate that the unusual electronic properties exhibited by the cuprates are fundamentally related to strong nonlinearities associated with subtle nanoscale inhomogeneity.
We report the observation of resistivity saturation in lightly doped ($x\sim 0.10)$ as-grown samples of the electron-doped cuprate La$_{2-x}$Ce$_x$CuO$_4$ (LCCO). The saturation occurs at resistivity values roughly consistent with the phenomenological Mott-Ioffe-Regel criterion once the low effective carrier density of these materials is included in the analysis. These results imply that, at least for light doping, the high-temperature metallic phase of these materials is not necessarily strange and may be understood as simply a low-density metal.
A common origin for the resistivity of Cd$_2$Re$_2$O$_7$, the cuprates, and Sr$_2$RuO$_4$?
我们提出了一个解释的电阻率的温度依赖性的Cd $_2$ Re $_2$ O $_7$,包括以上的结构相变在$T$ =200 $^o$ K的制度。所涉及的机制依赖于一个强大的范霍夫奇点接近费米面的存在,这是证明了相关的能带结构计算。同样的机制已经成功地描述了$T$ -铜酸盐和Sr $_2$ RuO $_4$的线性电阻率,以及前一种材料中的单粒子散射率,如最近的实验所证实的。我们描述了Cd $_2$ Re $_2$ O $_7$和Cd $_2$ O $_2$ O $_7$的一些预测。
Planar normal state resistivity data taken from three families of cuprate superconductors are compared with theoretical calculations from the recent extremely correlated Fermi liquid theory (ECFL). The two hole doped cuprate materials $LSCO$ and $BSLCO$ and the electron doped material $LCCO$ have yielded rich data sets at several densities $δ$ and temperatures T, thereby enabling a systematic comparison with theory. The recent ECFL resistivity calculations for the highly correlated $t$-$t'$-$J$ model by us give the resistivity for a wide set of model parameters. After using X-ray diffraction a…
We show that the resistivity in each phase of the High-Tc cuprates is a special case of a general expression derived from the Kubo formula. We obtain, in particular, the T-linear behavior in the strange metal (SM) and upper pseudogap (PG) phases, the pure $T^2$, Fermi liquid (FL) behavior observed in the strongly overdoped regime as well as the $T^{1+δ}$ behavior that interpolates both in the crossover. We calculate the coefficients: a) of $T$ in the linear regime and show that it is proportional to the PG temperature $T^*(x)$; b) of the $T^2$-term in the FL regime, without adjusting any param…
Recent analysis has confirmed earlier general arguments that the Kerr response vanishes in any time-reversal invariant system which satisfies the Onsager relations. Thus, the widely cited relation between natural optical activity (gyrotropy) and the Kerr response, employed in Hosur \textit{et al}, Phys. Rev. B \textbf{87}, 115116 (2013), is incorrect. However, there is increasingly clear experimental evidence that, as argued in our paper, the onset of an observable Kerr-signal in the cuprates reflects point-group symmetry rather than time-reversal symmetry breaking.
A key unexplained feature of cuprate superconductors is the upturn in their normal state electrical resistivity $ρ(T)$ seen at low temperature inside the pseudogap phase. We examined this issue via measurements of the thermal conductivity $κ(T)$ down to 50 mK and in fields up to 17 T on the cuprate La$_{2-x}$Sr$_x$CuO$_4$ at dopings $p = 0.13$, 0.136, 0.143 and 0.18. At $p$ = 0.136, 0.143, and 0.18, we observe an initial increase of the electronic thermal conductivity $κ_0/T$ as a function of field, as expected in a $d$-wave superconductor. For $p$ = 0.136 and 0.143, further increasing the fie…
One of the prime manifestations of an anisotropic electronic state in underdoped cuprates is the in-plane resistivity anisotropy $Δρ\equiv(ρ_{a}-ρ_{b})/ρ_{b}$. Here we use a Boltzmann-equation approach to compute the contribution to $Δρ$ arising from scattering by anisotropic charge and spin fluctuations, which have been recently observed experimentally. While the anisotropy in the charge fluctuations is manifested in the correlation length, the anisotropy in the spin fluctuations emerges only in the structure factor. As a result, we find that spin fluctuations favor $Δρ>0$, whereas charge flu…
Resistivity in the quantum-critical fluctuation region of several metallic compounds such as the cuprates, the heavy-fermions, Fe-chalogenides and pnictides, twisted bi-layer graphene and WSe$_2$, is linear in temperature $T$ as well as in a magnetic field $H$. Scattering of fermions by the excitations of a time-reversal odd polar vector field ${\bf Ω}$ characterizing loop-current fluctuations has been shown to give a linear in T resistivity and other anomalous properties in the cuprates. An extension of this theory to an applied magnetic field is presented. Magnetic field is shown to generate…
We report extensive resistivity, Hall, and magnetoresistance measurements on thin films of the electron-doped cuprate \PCCO~(PCCO), as a function of doping, temperature and magnetic field. The doping dependence of the resistivity and Hall number at low temperatures are characteristic of a system near a quantum phase transition or a Fermi Surface Reconstruction (FSR) point. The spin magnetoresistance drops to zero near the critical point. The data presented in this paper were compiled during the 2004-2007 period but were never published in this comprehensive form. Because of the recent interest…
Correlation between the strength of low-temperature T-linear normal-state resistivity and $T_{\rm c}$ in overdoped electron-doped cuprate superconductors
本文在动能驱动超导框架内,揭示了过掺杂电子掺杂型铜氧化物超导体中由自旋激发同时介导的电子umklapp散射与电子配对,自然导致了低温T线性正常态电阻率强度与超导转变温度$T_{\ m c}$之间的内在关联。
The highly anisotropic and qualitatively different nature of in- and out-of-plane charge dynamics in high-Tc cuprates cannot be accommodated within the conventional Boltzmann transport theory. The variation of in- and out-of-plane resistivities with temperature and hole content are also anomalous and cannot be explained by Fermi-liquid theory. In this study we have proposed a simple phenomenological model for the dc resistivity of cuprates by incorporating two firmly established generic features of all hole doped cuprate superconductors- (1) the pseudogap in the quasiparticle energy spectrum a…
Starting from a recently proposed comprehensive theory for the high-Tc superconductivity in cuprates, we derive a general analytic expression for the planar resistivity, in the presence of an applied external magnetic field $\textbf{H}$ and explore its consequences in the different phases of these materials. As an initial probe of our result, we show it compares very well with experimental data for the resistivity of LSCO at different values of the applied field. We also apply our result to Bi2201 and show that the magnetoresistivity in the strange metal phase of this material, exhibits the $H…
Systematic analysis of the planar resistivity, Hall effect and cotangent of the Hall angle for the electron-doped cuprates reveals underlying Fermi-liquid behavior even deep in the antiferromagnetic part of the phase diagram. The transport scattering rate exhibits a quadratic temperature dependence, and is nearly independent of doping, compound and carrier type (electrons vs. holes), and hence universal. Our analysis moreover indicates that the material-specific resistivity upturn at low temperatures and low doping has the same origin in both electron- and hole-doped cuprates.
In cuprate superconductors, high magnetic fields have been used extensively to suppress superconductivity and expose the underlying normal state. Early measurements revealed insulating-like behavior in underdoped material versus temperature $T$, in which resistivity increases on cooling with a puzzling $\log(1/T)$ form. We instead use microwave measurements of flux-flow resistivity in YBa$_2$Cu$_3$O$_{6+y}$ and Tl$_2$Ba$_2$CuO$_{6+δ}$ to study charge transport deep inside the superconducting phase, in the low temperature and low field regime. Here, the transition from metallic low-temperature …
An understanding of the normal state in the high-temperature superconducting cuprates is crucial to the ultimate understanding of the long-standing problem of the origin of the superconductivity itself. This so-called strange metal state is thought to be associated with a quantum critical point (QCP) hidden beneath the superconductivity(1,2). In electron-doped cuprates in contrast to hole-doped cuprates it is possible to access the normal state at very low temperatures and low magnetic fields to study this putative QCP and to probe the T~0 K state of these materials(3,4). We report measurement…
Superconductivity in cuprates peaks in the doping regime between a metal at high p and an insulator at low p. Understanding how the material evolves from metal to insulator is a fundamental and open question. Early studies in high magnetic fields revealed that below some critical doping an insulator-like upturn appears in the resistivity of cuprates at low temperature, but its origin has remained a puzzle. Here we propose that this 'metal-to-insulator crossover' is due to a drop in carrier density n associated with the onset of the pseudogap phase at a critical doping p*. We use high-field res…
Among all experimental observations of cuprate physics, the metal-insulator-crossover (MIC), seen in the pseudogap (PG) region of the temperature-doping phase diagram of copper-oxides under a strong magnetic field, when the superconductivity is suppressed, is most likely the most intriguing one. Since it was expected that the PG-normal state for these materials, as for conventional superconductors, is conducting. This MIC, revealed in such phenomena as heat conductivity downturn, anomalous Lorentz ratio, insulator resistivity boundary, nonlinear entropy, resistivity temperature upturn, insulat…
A one band Hubbard model with intermediate coupling is shown to describe the two most important unusual features of a normal state: linear resistivity strange metal and the pseudogap. Both the spectroscopic and transport properties of the cuprates are considered on the same footing by employing a relatively simple postgaussian approximation valid for the intermediate couplings $U/t=1.5-4$ in relevant temperatures $T>100{\rm K}.$ In the doping range $\ p=0.1-0.3$, the value of $U$ is smaller than that in the parent material. For a smaller doping, especially in the Mott insulator phase, the coup…
c-Axis Phase Coherence and Spin Fluctuations in Cuprates
铜酸盐的超导电性(SC)是二维的,这是一个共识。人们普遍认为,由于SC CuO_{2}(二、三、.)层次。最近的T_{c}和T12212中的电阻率测量作为施加压力的函数(Salvetat J. P.等人,欧罗巴信件:52(2000)584)表明,层间约瑟夫森耦合机制不符合数据。在这里,我们分析Andreev反射,中子散射,微波,μ子自旋弛豫,隧道和电阻率测量不同的铜氧化物,主要是,YBCO,Bi 2212和LSCO上获得的数据。分析结果表明,铜氧化物的长程相位相干性与沿c轴的反铁磁相互作用密切相关。同时,SC的面内机制似乎与沿c轴的磁相互作用没有或几乎没有关系。
We report magnetoresistance and Hall Effect results for electron-doped films of the high-temperature superconductor La$_{2-x}$Ce$_x$CuO$_4$ (LCCO) for temperatures from 0.7 to 45 K and magnetic fields up to 65 T. For x = 0.12 and 0.13, just below the Fermi surface reconstruction (FSR), the normal state in-plane resistivity exhibits a well-known upturn at low temperature. Our new results show that this resistivity upturn is eliminated at high magnetic field and the resistivity becomes linear-in-temperature from $\sim$ 40 K down to 0.7 K. The magnitude of the linear coefficient scales with Tc an…
There is considerable recent interest in the phenomenon of anisotropic electroresistivity of correlated metals. While some interesting work has been done on the iron-based superconducting systems, not much is known for the cuprate materials. Here we study the anisotropy of elastoresistivity for cuprates in the normal state. We present theoretical results for the effect of strain on resistivity, and additionally on the optical weight and local density of states. We use the recently developed extremely strongly correlated Fermi liquid theory in two dimensions, which accounts quantitatively for t…