We present a 100 MHz repetition rate Yb-fiber-laser-pumped synchronously pumped optical parametric oscillator (SPOPO) delivering tunable frequency combs covering almost the entire visible spectral range. By intracavity doubling both the signal and idler combs and using collinear residual pump light, nearly continuous tuning over the range of 420-700 nm is achieved with only small gaps near the OPO degeneracy condition. Output powers range from 10 mW to 200 mW, depending on wavelength, with pulse durations below 150 fs without external compression. Frequency locking of all three collinearly outcoupled combs (pump, doubled signal, and doubled idler) to a femtosecond enhancement cavity facilitates direct comparison of their optical phase noise and phase modulation transfer functions. In the singly-resonant OPO, optical phase modulation of the pump comb is transferred nearly completely to the non-resonant idler comb. This results in a resonant signal comb with reduced optical phase noise and also enables high-bandwidth modulation on the idler comb via phase modulation of the pump.
We describe two noncollinear optical parametric amplifier (NOPA) systems pumped by either the second (515 nm) or the third (343 nm) harmonic of an Yb:KGW amplifier, respectively. Pulse durations as short as 6.8 fs are readily obtained by compression with commercially available chirped mirrors. The availability of both second and third harmonic for NOPA pumping allows for gap-free tuning from 520 to 980 nm. The use of an intermediate NOPA to generate seed light at 780 nm extends the tuning range of the third-harmonic pumped NOPA towards 450 nm.
We demonstrate a mid-infrared dysprosium-doped fluoride fiber laser with a continuously tunable output range of 573 nm, pumped by a 1.7 μm Raman fiber laser. To the best of our knowledge, this represents the largest tuning range achieved to date from any rare-earth-doped fiber laser and, critically, spans the 2.8-3.4 μm spectral region, which contains absorption resonances of many important functional groups and is uncovered by other rare-earth ions. Output powers up to 170 mW are achieved, with 21% slope efficiency. We also discuss the relative merits of the 1.7 μm pump scheme, including poss…
We demonstrate a broadband mid-infrared (MIR) frequency comb source based on difference frequency generation (DFG) in periodically poled lithium niobate (PPLN) crystal. Mid-infrared radiation is obtained via mixing of the output of a 125 MHz repetition rate Yb-doped fiber laser with Raman-shifted solitons generated from the same source in a highly nonlinear fiber. The resulting idler is tunable in the range of 2.7 - 4.2 μm with average output power reaching 237 mW, and pulses as short as 115 fs. The coherence of the MIR comb is confirmed by spectral interferometry and heterodyne beat measureme…
Gaseous ammonia has previously been demonstrated as a compelling gain medium for a quantum cascade laser pumped molecular laser (QPML), exhibiting good power efficiency but limited tunability. Here we explore the potential of the ammonia QPML to produce powerful, broadly tunable terahertz frequency lasing on rotational and pure inversion transitions. After theoretically predicting possible laser frequencies, pump thresholds, and efficiencies, we experimentally demonstrate unprecedented tunability -- from 0.762 to more than 4.5 THz -- by pumping Q- and R-branch infrared transitions with widely …
By introducing methyl fluoride (CH$_3$F) as a new gain medium for a quantum cascade laser-pumped molecular laser (QPML), we demonstrate continuous-wave lasing from more than 120 discrete transitions spanning the frequency range 0.25 to 1.3 THz. The unprecedented degree of spectral tuning achieved with CH$_3$F also confirms the universality of the QPML concept: for all polar gas molecules, lasing can be induced on any dipole-allowed rotational transition by sufficient pumping of a related roto-vibrational transition using a continuously tunable quantum cascade laser.
We present a tunable, hybrid waveguide-fiber optical parametric oscillator (OPO) synchronously pumped by an ultra-fast fiber laser exploiting four-wave mixing (FWM) generated in silicon nitride waveguides. Parametric oscillation results in a 35 dB enhancement of the idler spectral power density in comparison to spontaneous FWM, with the ability of wide wavelength tuning over 86 nm in the O-band. Measurements of the oscillation threshold and the efficiency of the feedback loop reveal how an integration of the OPO on a single silicon nitride chip can be accomplished at standard repetition rates …
Many fields such as bio-spectroscopy and photochemistry often require sources of vacuum ultraviolet (VUV) pulses featuring a narrow linewidth and tunable over a wide frequency range. However, the majority of available VUV light sources do not simultaneously fulfill those two requirements, and few if any are truly compact, cost-effective and easy to use by non-specialists. Here we introduce a novel approach that goes a long way to meeting this challenge. It is based on hydrogen-filled hollow-core photonic crystal fiber pumped simultaneously by two spectrally distant pulses. Stimulated Raman sca…
We report generation of high harmonics in a gas-jet pumped by pulses self-compressed in a He-filled hollow-core photonic crystal fiber through the soliton effect. The gas-jet is placed directly at the fiber output. As the energy increases the ionization-induced soliton blue-shift is transferred to the high harmonics, leading to a emission bands that are continuously tunable from 17 to 45 eV.
10 μm lasing is studied in a compact CO2-He cell pressurized up to 15 atm when optically pumped by a ~50 mJ Fe:ZnSe laser tunable around 4.3 μm. The optimal pump wavelength and partial pressure of CO2 for generating 10 μm pulses are found to be ~4.4 μm and 0.75 atm, respectively. Without cavity optimization, the optical-to-optical conversion efficiency reached ~10% at a total pressure of 7 atm. The gain lifetime is measured to be ~1 μs at pressures above 10 atm, indicating the feasibility of using high-pressure optically pumped CO2 for the efficient amplification of picosecond 10 μm pulses.
Quantum cascade laser (QCL)-pumped molecular lasers (QPMLs) have recently been introduced as a new source of powerful (>1 mW), tunable (>1 THz), narrow-band (<10 kHz), continuous-wave terahertz radiation. The performance of these lasers depends critically on molecular collision physics, pump saturation, and on the design of the laser cavity. Using a validated three-level model that captures the essential collision and saturation behaviors of the QPML gas nitrous oxide (N2O),we explore how threshold pump power and output terahertz power depend on pump power, gas pressure, as well as on the diam…
A novel method for efficient generation of high power, equalized continuous-wave supercontinuum source in an all conventional silica fiber architecture is demonstrated. Highly nonlinear fiber (HNLF) is pumped in its anomalous dispersion region using a novel, high power, L-band laser. The L-band laser encompasses a 6th order cascaded Raman amplifier which is pumped with a high power Ytterbium doped fiber laser and amplifies a low-power, tunable L-band seed source. The supercontinuum generated 35W of power with ~40% efficiency. The Supercontinuum spectrum was measured to have a high degree of fl…
We report the compact and robust coherent source operating in mid-IR based on Fe:ZnSe chalcogenide gain medium optically pumped by Er:ZBLAN fiber laser. The output power of 2.1 W with 59% slope efficiency with respect to absorbed pump power at liquid nitrogen cooling is achieved. We show that strong re-absorption at high pump power and iron ion doping concentrations leads to the continuous tuning of central wavelength from 4012 to 4198 nm. Robustness of high power Er:ZBLAN fiber laser combined with prominent spectroscopic properties of Fe:ZnSe media pave the way for the development of reliable…
A tunable nanoscale "zipper" laser cavity, formed from two doubly clamped photonic crystal nanobeams, is demonstrated. Pulsed, room temperature, optically pumped lasing action at a wavelength of 1.3 micron is observed for cavities formed in a thin membrane containing InAsP/GaInAsP quantum-wells. Metal electrodes are deposited on the ends of the nanobeams to allow for micro-electro-mechanical actuation. Electrostatic tuning and modulation of the laser wavelength is demonstrated at a rate of 0.25nm/V^2 and a frequency as high as 6.7MHz, respectively.
The bias-pumped gain-switched fiber laser proposed by us is considered a novel pulsed fiber laser based on a new pulsing mechanism. With a certain signal power seeding, synchronization of temporal evolution can be kept between the output signal laser and the pump. The seed laser can be supplied conveniently by a CW pump power which is named bias pump power. A pulsed pump is responsible for shaping the output pulse. Stable pulsed lasers with tunable durations can be achieved under bias pump combined with pulsed pump. In addition, the temporal shape of output pulses can be controllable based on …
We report the first experimental demonstration of efficient and high-power operation of a Ti:sapphire laser pumped by a simple, compact, continuous-wave (cw) fiber-laser-based green source. The pump radiation is obtained by direct single-pass second-harmonic-generation (SHG) of a 33-W, cw Yb-fiber laser in 30-mm-long MgO:sPPLT crystal, providing 11 W of single-frequency green power at 532 nm in TEM00 spatial profile with power and frequency stability better than 3.3% and 32 MHz, respectively, over one hour. The Ti:sapphire laser is continuously tunable across 743-970 nm and can deliver an outp…
We report on a mid-infrared frequency comb source of unprecedented tunability covering the entire 3-10 μm molecular fingerprint region. The system is based on difference frequency generation in a GaSe crystal pumped by a 151 MHz Yb:fiber frequency comb. The process was seeded with Raman shifted solitons generated in a highly nonlinear suspended-core fiber with the same source. Average powers up to 1.5 mW were achieved at 4.7 μm wavelength.
Using a compact optically-pumped silicon nanophotonic chip consisting of coupled silicon microrings, we generate photon pairs in multiple pairs of wavelengths around 1.55 μm. The wavelengths are tunable over several nanometers, demonstrating the capability to generate wavelength division multiplexed photon pairs at freely-chosen telecommunications-band wavelengths.
Graphene, a unique two-dimensional material of carbon in a honeycomb lattice, has brought remarkable breakthroughs across the domains of electronics, mechanics, and thermal transport, driven by the quasiparticle Dirac fermions obeying a linear dispersion. Here we demonstrate a counter-pumped all-optical difference frequency process to coherently generate and control THz plasmons in atomic layer graphene with an octave tunability and high efficiency. We leverage the inherent surface asymmetry of graphene for a strong second-order nonlinear polarizability chi(2), which together with tight plasmo…
We theoretically and experimentally investigate the chaotic regime of optical frequency combs generated in nonlinear ring microresonators pumped with continuous wave light. We show that the chaotic regime reveals itself, in an apparently counter-intuitive way, by a flat top symmetric envelope of the frequency spectrum, when observed by means of an optical spectrum analyzer. The comb demodulated on a fast photodiode produces a noisy radio frequency signal with an spectral width significantly exceeding the linear bandwidth of the microresonator mode.
Liquid dye lasers have long been considered as ideal tunable laser sources in the visible range but are bulky, expensive, and require a complex system for dye circulation. Here, we present a system that relies on a low-cost blue laser diode as the pump source and a sealed dye cell with no flowing circuitry, resulting in a device that combines the convenience and size of a solid-state device with the stability of a liquid organic laser. A very high photo-stability is obtained (up to 1.2 x 10$^9$ pulses or 12 days at 1 kHz), which is five orders of magnitude higher than a solid-state dye laser o…
One notable feature of dye doped cholesteric liquid crystal is the variation of pitch and refractive index as the incidence angle of the pumping light shifts. Based on this feature, this paper studies the effects of pumping light's incidence angle on emission properties of the dye doped cholesteric liquid crystal tunable laser. First, we investigated the relationship among the concentration of chiral reagent, the incidence angle of the pumping light, and the pitch of liquid-crystal display (LCD); then we made a tunable-wavelength laser and pumped the prepared sample with 532nm laser outputted …
Much progress, both experimentally and theoretically, has recently been made towards optical frequency comb generation from continuously pumped second-order nonlinear systems. Here, we present the first observations towards finding an integrated solution for such a system, using a titanium indiffused lithium niobate waveguide resonator. These results are compared to recently developed theory for equivalent systems. The system is seen to exhibit strong instabilities, which require further investigation in order to fully determine the suitability of this platform for stable optical frequency com…
Optical frequency comb generation by continuous-wave-pumped cascaded quadratic nonlinearities (CQN) appears a promising alternative to well-established modelocked lasers, especially if access to the mid-infrared spectral region is needed. We report an experimental investigation of spectral properties of a CQN frequency comb, which is based on second-harmonic generation (SHG) and is pumped internally by a continuous-wave optical parametric oscillator. Our study focuses on SHG phase mismatch, which has drawn little attention in the previously reported CQN frequency comb research. The main observ…
Absolute output power optimization and performance of a near- to mid-infrared picosecond optical parametric oscillator (OPO) is studied at two high pump powers using a widely-tunable output coupling (OC) technique which provides 15% to 68% OC. The MgO:PPLN-based OPO is synchronously pumped at 81.1 MHz by an Yb:fiber laser with double-peak spectrum. At 2 W pump power, maximum signal (at 1.46 $μ$m) and idler (at 3.92 $μ$m) power of 670 mW and 270 mW are obtained at 27% OC at 47% total extraction efficiency and 58% pump power depletion where at 15.5 W pump power, 7.4 W signal and 2.7 W idler powe…
We demonstrate a two-crystal mid-infrared dual-wavelength optical parametric oscillator, synchronously pumped by a high power femtosecond Yb:fiber laser. The singly-resonant ring cavity, containing two periodically poled lithium niobate crystals, is capable of generating two synchronized idler wavelengths, independently tunable over 30 THz in the 2.9 - 4.2 μm wavelength region, due to the cascaded quadratic nonlinear effect. The independent tunability of the two idlers makes the optical parametric oscillator a promising source for ultrafast pulse generation towards the THz wavelength region, b…
The recent demonstration of a terahertz (THz) molecular gas laser pumped by a mid-infrared quantum cascade laser (QCL) has opened up new perspectives for this family of sources, traditionally relying on CO2-laser pumping. A so far open question concerning QCL-pumped THz molecular lasers (MLs) is related to their spectral purity. Indeed, assessing their frequency/phase noise is crucial for a number of applications potentially exploiting these sources as local oscillators. Here this question is addressed by reporting the measurement of the frequency noise power spectral density (PSD) of a THz ML…
A study is made of the nonlinear dynamics of dual pumped microresonator Kerr frequency combs described by a driven and damped nonlinear Schrödinger equation, with an additional degree of freedom in the form of the modulation frequency. A truncated four wave model is derived for the pump modes and the dominant sideband pair which is found to be able to describe much of the essential dynamical behaviour of the full equation. The stability of stationary states within the four wave model is investigated and numerical simulations are made to demonstrate that a large range of solutions, including ca…
A watt-level ultrahigh optical signal-to-noise ratio (OSNR) single-longitudinal-mode (SLM) tunable Brillouin fiber laser (BFL) has been demonstrated.By optimizing the length of the single mode fiber (SMF) cavity at 11m and its output ratio at sixty percent, 1.04 W output power, as well as stable SLM operation is obtained at 2.24 W pump power. The single pass cavity BFL has the advantage that Brillouin pump frequency doesn't need to match the cavity mode, thus the stability is greatly improved. As only SMF is used in the cavity, the operate wavelength can be tunable without the restriction from…
We report ultra-low phase-noise microwave generation at a 9.6 GHz carrier frequency from optical frequency combs based on diode-pumped solid-state lasers emitting at telecom wavelength and referenced to a common cavity-stabilized continuous-wave laser. Using a novel fibered polarization-maintaining pulse interleaver, a single-oscillator phase-noise floor of -171 dBc/Hz has been measured with commercial PIN InGaAs photodiodes, constituting a record for this type of detector. Also, a direct optical measurement of the stabilized frequency combs timing jitter was performed using a balanced optical…
An optical parametric chirped pulse amplifier fully based on Yb lasers at 500 kHz is described. Passive optical-synchronization is achieved between a fiber laser-pumped white-light and a 515 nm pump produced with a 200 W picosecond Yb:YAG InnoSlab amplifier. An output power up to 19.7 W with long-term stability of 0.3% is demonstrated for wavelength tunable pulses between 680 nm and 900 nm and spectral stability of 0.2%; 16.5 W can be achieved with a bandwidth supporting 5.4 fs pulses. We demonstrate compression of 30 microjoule pulses to sub-20 fs duration with a prism compressor, suitable fo…
Within a synchronously pumped optical parametric oscillator (SPOPO), the inherent synchronism between the pump and the resonating signal is the magic to partly transfer the coherence property of the pump to the signal. In our demonstration, Vernier effect is observed within a femtosecond SPOPO by simply detuning the FSR of the cavity, generating signal pulses at tunable repetition rate from several GHz to 1 THz with a maximum 22.58 nm full width half maximum (FWHM) bandwidth supporting 160 fs pulses covering the C- and L-bands of the telecom wavelength region. This technique offers a simple me…
We report a 1 um continuous wave pumped supercontinuum which extends short of the pump wavelength to 0.65 um. This is achieved by using a 50 W Yb fibre laser in combination with a photonic crystal fibre with a carefully engineered zero dispersion wavelength. We show that the short wavelength generation is due to a combination of four-wave mixing and dispersive wave trapping by solitons. The evolution and limiting factors of the continuum are discussed.
In this work, we show that the application of a sol-gel coating renders a microbubble whispering gallery resonator into an active device. During the fabrication of the resonator, a thin layer of erbium-doped sol-gel is applied to a tapered microcapillary, then a microbubble with a wall thickness of 1.3 $μ$m is formed with the rare earth diffused into its walls. The doped microbubble is pumped at 980 nm and lasing in the emission band of the Er$^{3+}$ ions with a wavelength of 1535 nm is observed. The laser wavelength can be tuned by aerostatic pressure tuning of the whispering gallery modes of…
We report on the experimental observation of internally-pumped parametric oscillation in a high-Q lithium niobate microresonator under conditions of natural phase-matching. Specifically, launching near-infrared pump light around 1060 nm into a $z$-cut congruent lithium niobate microresonator, we observe the generation of optical sidebands around the input pump under conditions where second-harmonic generation is close to natural phase-matching. We find that a wide range of different sideband frequency shifts can be generated by varying the experimental parameters. Under particular conditions, …
We describe the cavity-enhancement of frequency combs over a wide tuning range of 450-700 nm (> 7900 cm$^{-1}$), covering nearly the entire visible spectrum. Tunable visible frequency combs from a synchronously-pumped optical parametric oscillator are coupled into a 4-mirror, dispersion-managed cavity with a finesse of 600 to 1400. An intracavity absorption path length enhancement greater than 190 is obtained over the entire tuning range, while preserving intracavity spectral bandwidths capable of supporting sub-200 fs pulse durations. These tunable cavity-enhanced frequency combs can find man…
Continuously pumped passive nonlinear cavities can be harnessed for the creation of novel optical frequency combs. While most research has focused on third-order "Kerr" nonlinear interactions, recent studies have shown that frequency comb formation can also occur via second-order nonlinear effects. Here, we report on the formation of quadratic combs in optical parametric oscillator (OPO) configurations. Specifically, we demonstrate that optical frequency combs can be generated in the parametric region around half of the pump frequency in a continuously-driven OPO. We also model the OPO dynamic…
Kerr microresonators driven in the normal dispersion regime typically require the presence of localized dispersion perturbations, such as those induced by avoided mode crossings, to initiate the formation of optical frequency combs. In this work, we experimentally demonstrate that this requirement can be lifted by driving the resonator with a pulsed pump source. We also show that controlling the desynchronization between the pump repetition rate and the cavity free-spectral range (FSR) provides a simple mechanism to tune the center frequency of the output comb. Using a fiber mini-resonator wit…
We have developed an angle-resolved photoemission spectrometer with tunable VUV laser as a photon source. The photon source is based on the fourth harmonic generation of a near IR beam from a Ti:sapphire laser pumped by a CW green laser and tunable between 5.3eV and 7eV. The most important part of the set-up is a compact, vacuum enclosed fourth harmonic generator based on KBBF crystals, grown hydrothermally in the US. This source can deliver a photon flux of over 10^14 photons/s. We demonstrate that this energy range is sufficient to measure the kz dispersion in an iron arsenic high temperatur…
Ultrafast optical excitation with intense mid-infrared and terahertz pulses has emerged as a new tool to control materials dynamically. As most experiments are performed with femtosecond pulse excitation, typical lifetimes of most light-induced phenomena in solids are of only few picoseconds. Yet, many scientific applications require longer drive pulses and lifetimes. Here, we describe a mid-infrared pump - terahertz-probe setup based on a CO$\mathrm{_2}$ laser seeded with 10.6 $\mathrmμ$m wavelength pulses from an optical parametric amplifier, itself pumped by a Ti:Al$\mathrm{_2}$O$\mathrm{_3…
We report the generation of a purely vibrational Raman comb, extending from the vacuum ultraviolet (184 nm) to the visible (478 nm), in hydrogen-filled kagomé-style photonic crystal fiber pumped at 266 nm. Stimulated Raman scattering and molecular modulation processes are enhanced by higher Raman gain in the ultraviolet. Owing to the pressure-tunable normal dispersion landscape of the fiber-gas system in the ultraviolet, higher-order anti-Stokes bands are generated preferentially in higher-order fiber modes. The results pave the way towards tunable fiber-based sources of deep- and vacuum ultra…
We show that both the power and repetition rate of a frequency comb generated in a nonlinear ring resonator, pumped with continuous wave (cw) coherent light, are modulated. The modulation is brought about by the interaction of the cw background with optical pulses excited in the resonator, and occurs in resonators with nonzero high-order chromatic dispersion and wavelength-dependent quality factor. The modulation frequency corresponds to the detuning of the pump frequency from the eigenfrequency of the pumped mode in the resonator.
Dissipative Kerr solitons (DKSs) intrinsically exhibit two degrees of freedom through their group and phase rotation velocity. Periodic extraction of the DKS into a waveguide produces a pulse train and yields the resulting optical frequency comb's repetition rate and carrier-envelope offset, respectively. Here, we demonstrate that it is possible to create a system with a single repetition rate but two different phase velocities by employing dual driving forces. By recasting these phase velocities into frequencies, we demonstrate, experimentally and theoretically, that they can mix and create n…
We describe a novel method for making microbottle-shaped lasers by using a CO$_2$ laser to melt Er:Yb glass onto silica microcapillaries or fibres. This is realised by the fact that the two glasses have different melting points. The CO$_2$ laser power is controlled to flow the doped glass around the silica cylinder. In the case of a capillary, the resulting geometry is a hollow, microbottle-shaped resonator. This is a simple method for fabricating a number of glass WGM lasers with a wide range of sizes on a single, micron-scale structure. The Er:Yb doped glass outer layer is pumped at 980 nm v…
We report a few-cycle, broadband, singly-resonant optical parametric oscillator (OPO) for the mid-infrared based on MgO-doped periodically-poled LiNbO3 (MgO:PPLN), synchronously pumped by a 20-fs Ti:sapphire laser. By using crystal interaction lengths as short as 250 um, and careful dispersion management of input pump pulses and the OPO resonator, near-transform-limited, few-cycle idler pulses tunable across the mid-infrared have been generated, with as few as 3.7 optical cycles at 2682 nm. The OPO can be continuously tuned over 2179-3732 nm by cavity delay tuning, providing up to 33 mW of out…
Space-division multiplexing (SDM), whereby multiple spatial channels in multimode and multicore optical fibers are used to increase the total transmission capacity per fiber, is being investigated to avert a data capacity crunch and reduce the cost per transmitted bit. With the number of channels employed in SDM transmission experiments continuing to rise, there is a requirement for integrated SDM components that are scalable. Here, we demonstrate a cladding-pumped SDM erbium-doped fiber amplifier (EDFA) that consists of six uncoupled multimode erbium-doped cores. Each core supports three spat…
Optical parametric oscillation (OPO) with far-shifted frequency sidebands has attracted significant interests in precision spectroscopy and quantum information processing. Microresonator based OPO sources hold the advantages of miniaturized footprint and versatile dispersion engineering. Here we demonstrate large-frequency-shifted $χ^{(3)}$-based OPO from crystalline aluminum nitride microrings pumped at $\sim$2 $μ$m in the normal dispersion regime. OPO in the telecom and mid-infrared bands with a frequency separation of 65.5 THz is achieved. The OPO frequency can be agilely tuned in the range…
We propose and analyze an active mirror structure that uses a subwavelength grating reflector combined with optical gain. The structure is designed to be directly bonded to a thermal substrate (such as diamond) for efficient heat removal. We present optical wave propagation and thermal transport analysis and show that such a structure is well suited for power scaling of optically pumped semiconductor disk lasers to multi-kilowatt CW power operation.
