The longitudinal momentum of the electron at the tunneling exit is a useful quantity to make sense of the tunneling ionization process. It was usually assumed to be zero from a classical argument, but recent experiments show that it must be nonzero in order to explain the measured electron momentum distributions. In this article we show that the flow momentum of the probability fluid is a sensible quantum mechanical definition for tunneling-exit momentum, and it can be (and in general is) nonzero at the tunneling exit point where the kinetic energy is zero by definition. We show that this longitudinal momentum is nonzero even in the static or adiabatic limit, and this nonzero momentum is a purely quantum mechanical effect determined by the shape of the wave function in the vicinity of the tunneling exit point. Nonadiabaticity or finite wavelength may increase this momentum substantially, and the detailed value depends on both the atomic and the laser parameters.
Based on the strong-field approximation, we obtain analytical expressions for the initial momentum at the tunnel exit and instantaneous ionization rate of tunneling ionization in elliptically polarized laser fields with arbitrary ellipticity. The tunneling electron reveals a nonzero offset of the initial momentum at the tunnel exit in the elliptically polarized laser field. We find that the transverse and longitudinal components of this momentum offset with respect to the instantaneous field direction are directly related to the time derivatives of the instantaneous laser electric field along …
Laser-induced electron tunneling underlies numerous emerging spectroscopic techniques to probe attosecond electron dynamics in atoms and molecules. The improvement of those techniques requires an accurate knowledge of the exit momentum for the tunneling wave packet. Here we demonstrate a photoelectron interferometric scheme to probe the electron momentum longitudinal to the tunnel direction at the tunnel exit by measuring the photoelectron holographic pattern in an orthogonally polarized two-color laser pulse. In this scheme, we use a perturbative 400-nm laser field to modulate the photoelectr…
Recent attoclock experiments and theoretical studies regarding the strong-field ionization of atoms by few-cycle infrared pulses revealed new features that have attracted much attention. Here we investigate tunneling ionization and the dynamics of the electron probability using Bohmian Mechanics. We consider a one-dimensional problem to illustrate the underlying mechanisms of the ionization process. It is revealed that in the major part of the below-the-barrier ionization regime, in an intense and short infrared pulse, the electron does not tunnel \through" the entire barrier, but rather alrea…
We investigate the liberation of an atomic electron by a linearly polarized single-cycle near-infrared laser pulse having a peak intensity that ensures tunneling. Based on phase space analysis and energy distribution in the instantaneous potential, we reveal the importance of quantum interference between tunneling and over-the-barrier pathways of escape. Tunneling is blurred both in space and time, and the contribution of tunneling at the mean energy is almost negligible. We suggest and justify improved initial conditions for a classical particle approximation of strong-field ionization, based…
Tunnel ionization belongs to the fundamental processes of atomic physics. The so-called two-step model, which describes the ionization as instantaneous tunneling at the electric field maximum and classical motion afterwards with zero exit momentum, is commonly employed to describe tunnel ionization in adiabatic regimes. In this contribution, we show by solving numerically the time-dependent Schrödinger equation in one dimension and employing a virtual detector at the tunnel exit that there is a nonvanishing positive time delay between the electric field maximum and the instant of ionization. M…
We unravel the out-of-equilibrium quantum dynamics of a few interacting bosonic clouds in a two-dimensional asymmetric double-well potential at the resonant tunneling scenario. At the single-particle level of resonant tunneling, particles tunnel under the barrier from, typically, the ground-state in the left well to an excited state in the right well, i.e., states of different shapes and properties are coupled when their one-particle energies coincide. In two spatial dimensions, two types of resonant tunneling processes are possible, to which we refer to as longitudinal and transversal resonan…
Tunneling times in atomic ionization are studied theoretically by a virtual detector approach. A virtual detector is a hypothetical device that allows one to monitor the wave function's density with spatial and temporal resolution during the ionization process. With this theoretical approach, it becomes possible to define unique moments when the electron enters and leaves with highest probability the classically forbidden region from first principles and a tunneling time can be specified unambiguously. It is shown that neither the moment when the electron enters the tunneling barrier nor when …
The problem of time delay in tunneling ionization is revisited. The origin of time delay at the tunnel exit is analysed, underlining the two faces of the concept of the tunnelling time delay: the time delay around the tunnel exit and the asymptotic time delay at a detector. We show that the former time delay, in the sense of a delay in the peak of the wavefunction, exists as a matter of principle and arises due to the sub-barrier interference of the reflected and transmitted components of the tunneling electronic wavepacket. We exemplify this by describing the tunnelling ionization of an elect…
Statistical Characteristics of Tunneling States in Strong-Field Atomic Ionization
College of Physics and Information Technology and Quantum Materials and Devices Key Laboratory of Shaanxi Province’s High Education Institution, Shaanxi Normal University（陕西师范大学物理与信息工程学院、陕西省高校量子材料与器件重点实验室）；College of Physics and Hebei Key Laboratory of Photophysics Research and Application, Physics Postdoctoral Research Station, Hebei Normal University（河北师范大学物理学院、河北省光物理研究与应用重点实验室、物理学博士后科研流动站）；Hebei Key Laboratory of Optoelectronic Information and Geo-detection Technology, School of Mathematics and Science, Hebei GEO University（河北地质大学数理学院、河北省光电信息与地质探测技术重点实验室）；College of Physics, Henan Normal University（河南师范大学物理学院）
We study ionization of atoms in strong two-dimensional (2D) laser fields with various forms, numerically and analytically. We focus on the local most-probable tunneling routes (some specific electron trajectories) which are corresponding to the local maxima of photoelectron momentum distributions (PMDs). By making classic-quantum correspondence, we obtain a condition for these routes characterized by the electron position at the tunnel exit. With comparing the identified routes with the classical limit and the partial-decoupling approximation where it is assumed that tunneling is dominated by …
The response time of the electron to light in photoemission is difficult to define and measure. Tunneling ionization of atoms, a strong-laser-induced photoemission process, provides a semiclassical case for visiting the problem. Here, we show that the response time can be determined at the boundary between quantum and classic. Specifically, tunneling is instantaneous but a finite response time (about 100 attoseconds) is needed for the state of the tunneling electron to evolve into the ionized state around tunnel exit. This time can be well described with a compact expression related to some ba…
Multipassage Landau-Zener tunneling oscillations in transverse/longitudinal dual dressing of atomic qubits
INO-CNR（意大利国家研究委员会光学研究所）；Dipartimento di Scienze Fisiche, della Terra e dell’Ambiente, Università degli Studi di Siena（锡耶纳大学地球与环境科学系）；Dipartimento di Fisica E. Fermi, Università of Pisa（比萨大学E.费米物理系）；NEST, Istituto Nanoscienze CNR（纳米科学研究所）；Technische Universität Berlin（柏林工业大学）；Department of Mathematical, Physical and Computer Sciences, University of Parma（帕尔马大学数学、物理与计算机科学系）；National Institute for Nuclear Physics (INFN), Milano Bicocca Section, Parma Group（意大利国家核物理研究所米兰比可卡分部帕尔马组）
Interaction of a strong laser pulse with matter transfers not only energy but also linear momentum of the photons. Recent experimental advances have made it possible to detect the small amount of linear momentum delivered to the photoelectrons in strong-field ionization of atoms. Linear momentum transfer is a unique signature of the laser-atom interaction beyond its dipolar limit. Here, we present a decomposition of the subcycle time-resolved linear momentum transfer in term of its multipolar components. We show that the magnetic dipole contribution dominates the linear momentum transfer durin…
The electron nondipole dynamics in tunneling ionization in an elliptically polarized laser field is investigated theoretically using a relativistic Coulomb-corrected strong-field approximation (SFA) based on the eikonal approximation of the Klein-Gordon equation. We calculate attoclock angle-resolved light-front momentum distributions at different ellipticities of the laser field in quasistatic and nonadiabatic regimes and analyze them with an improved Simpleman model. The nondipole correlations between longitudinal and transverse momentum components are examined. Deviations of the photoelectr…
Tunneling of a particle through a potential barrier remains one of the most remarkable quantum phenomena. Owing to advances in laser technology, electric fields comparable to those electrons experience in atoms are readily generated and open opportunities to dynamically investigate the process of electron tunneling through the potential barrier formed by the superposition of both laser and atomic fields. Attosecond-time and angstrom-space resolution of the strong laser-field technique allow to address fundamental questions related to tunneling, which are still open and debated: Which time is s…
We analyze the two-dimensional photoelectrons momentum distribution of Ar atom ionized by midinfrared laser pulses and mainly concentrate on the energy range below 2Up. By using a generalized quantum trajectory Monte Carlo (GQTMC) simulation and comparing with the numerical solution of time-dependent Schrodinger equation (TDSE), we show that in the deep tunneling regime, the rescattered electron trajectories plays unimportant role and the interplay between the intracycle and inter-cycle results in a ring-like interference pattern. The ring-like interference pattern will mask the holographic in…
