Nuclear magnetic resonance (NMR) and Knight shift measurements are critical tools in the identification of spin-triplet superconductors. We discuss the effects of spin orbit coupling on the Knight shift and susceptibilities for a variety of spin triplet multi-orbital gap functions with orbital-singlet character and compare their responses to "traditional" single band spin-triplet ($p_x+ip_y$) superconductors. We observe a non-negligible residual spin-susceptibility at low temperature.
The Josephson effect between triplet and singlet superconductors is studied. Josephson current can flow between triplet and singlet superconductors due to the spin-orbit coupling in the spin-triplet superconductor but it is finite only when triplet superconductor has $L_z=-S_z=\pm 1$, where $L_z$ and $S_z$ are the perpendicular components of orbital angular momentum and spin angular momentum of the triplet Cooper pairs, respectively. The recently observed temperature and orientational dependence of the critical current through a Josephson junction between UPt$_3$ and Nb is investigated by cons…
Motivated by the recent experimental realization of a quantum interference transistor based on the superconducting proximity effect, we here demonstrate that the inclusion of a textured ferromagnet both strongly enhances the flux sensitivity of such a device and additionally allows for singlet-triplet switching by tuning a bias voltage. This functionality makes explicit use of the induced spin-triplet correlations due to the magnetic texture. Whereas the existence of such triplet correlations is well-known, our finding demonstrates how spin-triplet superconductivity may be utilized for concret…
Chiral and helical domain walls are generic defects of topological spin-triplet superconductors. We study theoretically the magnetic and transport properties of superconducting singlet-triplet-singlet heterostructure as a function of the phase difference between the singlet leads in the presence of chiral and helical domains inside the spin-triplet region. The local inversion symmetry breaking at the singlet-triplet interface allows the emergence of a static phase-controlled magnetization, and generally yields both spin and charge currents flowing along the edges. The parity of the domain wall…
We propose a phase diagram of quasi-low-dimensional type II superconductors in parallel magnetic fields, when antiferromagnetic fluctuations contribute to the pairing interactions. We point out that pairing interactions mediated by antiferromagnetic fluctuations necessarily include both singlet channels and triplet channels as attractive interactions. Usually, a singlet pairing is favored at zero field, but a triplet pairing occurs at high fields where the singlet pairing is suppressed by the Pauli paramagnetic pair-breaking effect. As a result, the critical field increases divergently at low …
Quantum oscillations in a tilted magnetic field offer the possibility of distinguishing singlet versus triplet order parameters in the particle hole channel provided the measurements reflect a putative ``normal'' state of a density wave obtained by applying by high magnetic field at low temperatures. A theoretical analysis is given that compares spin density wave, a singlet $d$-density wave, and a triplet $d$-density wave. While the existence of a spin zero in the oscillation amplitude is a necessary consequence of a singlet order parameter, a triplet order parameter may or may not exhibit a s…
We study the Andreev bound states in a Josephson junction between a singlet and a triplet superconductors. Because of the mismatch in the spin symmetries of pairing, the energies of the spin up and down quasiparticles are generally different. This results in imbalance of spin populations and net spin accumulation at the junction in equilibrium. This effect can be detected using probes of local magnetic field, such as the scanning SQUID, Hall, and Kerr probes. It may help to identify potential triplet pairing in $\rm(TMTSF)_2X$, $\rm Sr_2RuO_4$, and oxypnictides.
Larkin-Ovchinnikov (LO) states typically have a singlet-gap that vanishes along real-space lines. These real-space nodes lead to Andreev midgap states which can serve as a signature of LO pairing. We show that at these nodes, an odd-parity, spin-triplet component is always induced, leading to a nodeless LO phase. We find the two-dimensional weak coupling, clean limit s-wave phase diagram when this spin-triplet part is included. The triplet component is large and increases the stability of the FFLO phase. We also show that the spin-triplet contribution pushes the midgap states away from zero en…
Quasi-low-dimensional type II superconductors in parallel magnetic fields are studied when singlet pairing interactions and relatively weak triplet pairing interactions coexist. Singlet and triplet components of order parameter are mixed at high fields, and at the same time an inhomogeneous superconducting state called a Fulde-Ferrell-Larkin-Ovchinnikov state occurs. As a result, the triplet pairing interactions enhance the upper critical field of superconductivity remarkably even at temperatures far above the transition temperature of parallel spin pairing. It is found that the enhancement is…
A theoretical study is presented on the odd-frequency spin-singlet pairing that arises in nonuniform even-frequency superconductors as a consequence of broken translation symmetry. The effect of the odd-frequency pairing on the superfluid density and the spin susceptibility is analyzed by using the quasiclassical theory of superconductivity. It is shown that (1) the superfluid density is reduced by the formation of the odd-frequency singlet pairs and (2) the odd-frequency pairing increases the spin susceptibility even though its spin symmetry is singlet. The two unusual phenomena are related t…
Motivated by recent experimental findings, we have developed a theory of the superconducting state for 2D metals without inversion symmetry modeling the geometry of a surface superconducting layer in a field-effect-transistor or near the boundary doped by adsorbed ions. In such systems the two-fold spin degeneracy is lifted by spin-orbit interaction, and singlet and triplet pairings are mixed in the wave function of the Cooper pairs. As a result, spin magnetic susceptibility becomes anisotropic and Knight shift retains finite and rather high value at T=0.
We study the spin susceptibility of the orbital-singlet pairings, including the spin-triplet/orbital-singlet/$s$-wave $E_g$ representation proposed by Suh \textit{et al}., [H.\ G.\ Suh \textit{et al}., Phys.\ Rev.\ Research \textbf{2}, 032023 (2020)], for a three-orbital model of superconducting Sr$_2$RuO$_4$ in three dimensions. For the pseudospin-singlet states represented in the band basis, the spin susceptibility decreases when reducing the temperature, irrespective of the direction of the applied magnetic fields, even if they are spin-triplet/orbital-singlet pairings in the spin-orbital s…
We analyze the magnetization at the interface between singlet and triplet superconductors and show that its direction and dependence on the phase difference across the junction are strongly tied to the structure of the triplet order parameter as well as to the pairing interactions. We consider equal spin helical, opposite spin chiral, and mixed symmetry pairing on the triplet side and show that the magnetization vanishes at $ϕ=0$ only in the first case, follows approximately a $\cosϕ$ behavior for the second, and shows higher harmonics for the last configuration. We trace the origin of the mag…
We study the current-phase relation of a ballistic SIFIT junction, consisting of a spin-singlet superconductor (S), a weak ferromagnetic metal (F), a spin-triplet superconductor (T), and insulating ferromagnetic interfaces (I). We use the generalized quasiclassical formalism developed by A. Millis et al. to compute the current density and the free energy of the junction for arbitrary orientation of the magnetizations of the junction barrier. We investigate in detail the effect of the distribution of magnetization on the various harmonics of the current-phase relation and the transition of the …
One of the key effects which is predicted to arise in superconductors without a centre of inversion is the mixing of singlet and triplet order parameters, which are no longer good quantum numbers on their own due to parity. We have probed the gap structure in the noncentrosymmetric superconductor Ru$_7$B$_3$, through small-angle neutron diffraction from the vortex lattice, in order to search for the proposed mixed order parameter. We find that the measured temperature dependence of the vortex-lattice form factor is well characterised by a model constructed to describe the effects of broken inv…
We theoretically study static and dynamic properties of short Josephson junctions (JJ) with singlet and triplet Josephson coupling. In singlet Josephson weak links, two singlet superconductors S are connected with each other by a normal film (N) or wire. Triplet JJs, which we denote S$_{\text{m}}$/N(F)/S$_{\text{m}}$, are formed by two singlet BCS superconductors covered by a thin layer of a weak ferromagnet F$_{\text{w}}$. These superconductors S$_{\text{m}}$ are separated from the N (or F) layer by spin filters, which pass electrons with only one spin orientation. The triplet Cooper pairs pr…
Have you been lying awake wondering what symmetries determine whether a superconductor is spin singlet, triplet, or both? We show that if BCS theory is supplied with additional degrees of freedom, spin singlet can coexist with spin triplet superconductivity. In the first part, we didactically guide the reader to the most general superconducting state using symmetry arguments. If both singlet and triplet pairing channels are present, a magnetic field can convert between spin singlet and triplet states. In the second part, we discuss two possible singlet-triplet superconductors: CeRh$_2$As$_2$ a…
The increased capabilities of coupling more and more materials through functional interfaces are paving the way to a series of exciting experiments and extremely advanced devices. Here we focus on the capability of magnetically inhomogeneous superconductor/ferromagnet (S/F) interfaces to generate spin-polarized triplet pairs. We build on previous achievements on spin-filter ferromagnetic Josephson junctions (JJs) and find unique correspondence between neat experimental benchmarks in the temperature behavior of the critical current and theoretical modeling based on microscopic calculations, whi…
We report fully momentum dependent, self-consistent calculations of the gap symmetry, Fermi surface (FS) anisotropy and Tc of superconducting (SC) LiFeAs using the experimental band structure and a realistic small-q electron phonon interaction within the framework of Migdal-Eliashberg theory. In the stoichiometric regime, we find the exact s++ gap as reported by ARPES. For slight deviations from stoichiometry towards electron doping, we find that a chiral triplet p_x+ip_y state stabilizes near Tc and that at lower temperatures a transition from the triplet to singlet s+- SC takes place. Furthe…
The symmetry properties of the Cooper pairing problem for multi-component ultra-cold dipolar molecular systems are investigated. The dipolar anisotropy provides a natural and robust mechanism for both triplet and singlet Cooper pairing to first order in the interaction strength. With a purely dipolar interaction, the triplet $p_z$-like polar pairing is the most dominant. A short-range attractive interaction can enhance the singlet pairing to be nearly degenerate with the triplet pairing. We point out that these two pairing channels can mix by developing a relative phase of $\pm\fracπ{2}$, thus…
We show how in principle a coherent coupling between two superconductors of opposite parity can be realized in a three-layer oxide heterostructure. Due to strong intraionic spin-orbit coupling in the middle layer, singlet Cooper pairs are converted into triplet ones and vice versa. This results in a large enhancement of the triplet superconductivity, persisting well above the native triplet critical temperature.
We calculate the diamagnetic susceptibility in zero external magnetic field above the phase transition from ferromagnetic phase to phase of coexistence of ferromagnetic order and unconventional superconductivity. For this aim we use generalized Ginzburg-Landau free energy of unconventional ferromagnetic superconductor with spin-triplet electron pairing. A possible application of the result to some intermetallic compounds is briefly discussed.
In present work the effective singlet-triplet model for CuO2-layer on the grounds of multiband p-d model of strongly correlated electrons is obtained. The resulting Hamiltonian has a form of generalized singlet-triplet t-t'-J model for p-type superconductors and form of usual t-t'-J model for n-type superconductors. In the mean field approximation in X-operator representation we derived equations for Gorkov type Green functions. The symmetry classification of the superconducting order parameter in case of tetragonal lattice resulted in d_{x^2-y^2}- and d_{xy}-types of singlet pairing for both …
An inhomogeneous magnetic exchange field at a superconductor/ferromagnet interface converts spin-singlet Cooper pairs to a spin-aligned (i.e. spin-polarized) triplet state. Although the decay envelope of such triplet pairs within ferromagnetic materials is well studied, little is known about their decay in non-magnetic metals and superconductors, and in particular in the presence of spin-orbit coupling (SOC). Here we investigate devices in which triplet supercurrents are injected into the s-wave superconductor Nb. In the normal state of Nb, triplet supercurrents decay over a distance of 5 nm, …
We propose a theoretical model of quasi-one-dimensional superconductors, with attractive electron-electron interactions dominant in the singlet d-wave channel and sub-dominant in the p-wave channel. We discuss, in the mean field approximation, the effect of a magnetic field applied perpendicularly to the direction of the lowest conductivity. The lowest free energy phase corresponds to a singlet d-wave symmetry in low fields, but to a triplet symmetry in high fields. A first order singlet-triplet phase transition is expected at moderate applied fields of a few teslas. We propose to ascribe the …
Recent experiments in quantum critical heavy fermion metals have pushed to the fore the question about whether antiferromagnetic fluctuations can promote both spin-singlet and spin-triplet superconductivity. Here we address the issue through non-perturbative calculations in antiferromagnetically correlated Kondo systems. We identify Kondo-destruction quantum critical points in both the SU(2) symmetric and Ising-anisotropic cluster Bose-Fermi Anderson models. The spin-singlet pairing correlations are significantly enhanced near the quantum critical point in the SU(2) case; however, with adequat…
We derive gap equations for superconductivity in coexistence with ferromagnetism. We treat singlet states and triplet states with either equal spin pairing (ESP) or opposite spin pairing (OSP) states, and study the behaviour of these states as a function of exchange splitting. For the s-wave singlet state we find that our gap equations correctly reproduce the Clogston--Chandrasekhar limiting behaviour and the phase diagram of the Baltensperger--Sarma equation (excluding the FFLO region). The singlet superconducting order parameter is shown to be independent of exchange splitting at zero temper…
We have investigated the proximity effect in superconductor/ferromagnet junctions in a systematic manner to discuss the relationship between the zero-energy peak (ZEP) of the local density of states (LDOS) and spin-triplet odd-frequency pairing. By exactly solving the nonlinear Usadel equations, we have found that the ZEP is realized in a wide range of geometrical and material parameters in the case of the noncollinear magnetization. This strongly suggests the robustness of the ZEP induced by spin-triplet odd-frequency pairing in such systems. We also found that the crossover from singlet pair…
We study the Coulomb-Fröhlich model on a triangular lattice, looking in particular at states with angular momentum. We examine a simplified model of crab bipolarons with angular momentum by projecting onto the low energy subspace of the Coulomb-Fröhlich model with large phonon frequency. Such a projection is consistent with large long-range electron-phonon coupling and large repulsive Hubbard $U$. Significant differences are found between the band structure of singlet and triplet states: The triplet state (which has a flat band) is found to be significantly heavier than the singlet state (whic…
We propose a two-dimensional exciton model showing the possibility of two-exciton pairing in cuprates, both in singlet and in triplet states. The former is assumed to be responsible for the superconductivity and the latter for the unusual normal state properties. The ground state is found to be a projection of the Bose condensation of N/2 mobile bosons with a ηprojection operator which is a generalization of the Gutzwiller projection operator. The phase diagram of the model shows insulator-superconductivity and superconductivity-metal transitions with doping.
We study a singlet-triplet Josephson junction between a conventional s-wave superconductor and an unconventional p$_{\rm x}$-wave superconductor. The Andreev spectrum of the junction yields a spontaneous magnetization in equilibrium. This allows manipulating the occupation of the Andreev levels using an ac Zeeman field. The induced Rabi oscillations manifest themselves as a resonance in the current-phase relation. For a circularly polarized magnetic field, we find a spin selection rule, yielding Rabi oscillations only in a certain interval of the superconducting phase difference.
We develop a theory which describes hybrid structures consisting out of superconducting and ferromagnetic parts. We give two examples for applications. First, we consider a hybrid structure containing a strong ferromagnet in the ballistic limit. Second, we study for a weak ferromagnet the influence of a domain wall on the superconducting proximity effect. In both cases we account quantitatively for the mixing between singlet and triplet correlations.
We present precise measurements of the upper critical field (Hc2) in the recently discovered cobalt oxide superconductor. We have found that the critical field has an unusual temperature dependence; namely, there is an abrupt change of the slope of Hc2(T) in a weak field regime. In order to explain this result we have derived and solved Gor'kov equations on a triangular lattice. Our experimental results may be interpreted in terms of the field-induced transition from singlet to triplet superconductivity.
We propose a model for a superconductor where both spin-singlet and chiral triplet pairing amplitudes can coexist. By solving the Bogoliubov-de Gennes equations with a general pair potential that accounts for both spin states we study experimental signatures of normal metal and superconductor hybrids. The interplay between the spin-singlet and triplet correlations manifests in the appearance of two effective gaps. When the amplitude of the spin-triplet component is stronger than that of the spin-singlet, a topological phase transition into a non-trivial regime occurs. As a result, the normal m…
We have studied the competition and coexistence of staggered triplet SC with d-wave singlet SC and SDW in the mean-field approximation. Detailed numerical studies demonstrate that particle-hole asymmetry mixes these states and therefore they are simultaneously present. Even more interesting were the results of our study of the influence of a uniform magnetic field. We observe novel transitions that show the characteristics of Fulde-Ferrel phases, yet they concern transitions to different combinations of the above orders. For example, above a given field, in a particle-hole symmetric system we …
We investigate the pair condensation of a two-spin-component Fermi gas in the presence of both Rashba and Dresselhaus spin-orbit couplings. We calculate the condensate fraction in the BCS-BEC crossover both in two and in three dimensions by taking into account singlet and triplet pairings. These quantities are studied by varying the spin-orbit interaction from the case with the only Rashba to the equal-Rashba-Dresselhaus one. We find that, by mixing the two couplings, the singlet pairing decreases while the triplet pairing is suppressed in the BCS regime and increased in the BEC regime, both i…
In the present paper, we propose the parity even,orbital singlet and spin triplet pairing state as the ground state of the newly discovered super-conductor $LaO_{1-x}F_xFeAs$.The pairing mechanism involves both the special shape of the electron fermi surface and the strong ferromagnetic fluctuation induced by Hund's rule coupling.The special behavior of the Bogoliubov quasi-particle spectrum may leads to "Fermi arc" like anisotropy super-conducting gap, which can be detected by angle resolved photo emission(ARPES).The impurity effects are also discussed.
We consider a Josephson junction with an arbitrary transmission coefficient $\mathcal{D}$ between a singlet and a triplet superconductor with the latter order parameter characterized by a d-vector of the form ($k_x\hat{y}-k_y\hat{x}$). Various quantities such as the tunnelling current, spin accumulation, and spin current are calculated via the quasiclassical Green's functions. We also present a symmetry argument on the existence of these quantities and their dependencies on the phase difference across the junction. A physical picture is also given in terms of the Andreev states near the juncti…
Recently, a new pairing state with the mixing between s-wave singlet channel and isotropic d-wave quintet channel induced by centrosymmetric spin-orbit coupling has been theoretically proposed in the superconducting materials with $j=\frac{3}{2}$ electrons. In this work, we derive the expressions of the zero-temperature spin susceptibility, the upper critical field close to the zero-field critical temperature $T_c$ and the critical temperature with weak random non-magnetic disorders for the singlet-quintet mixed state based on the Luttinger model. Our study revealed the following features of t…
This work explores the possibility to transfer the parity law of the singlet-triplet gap established for square ladders (gapped for even number of legs, gapless for odd number of legs) to fused polyacenic 1-D systems, i.e., graphite ribbons. Qualitative arguments are presented in favor of a gapped character when the number $n\_ω$ of benzene rings along the ribbon width is odd. A series of numerical calculations (quantitative mapping on spin 1/2 chains, renormalized excitonic treatments and Quantum Monte Carlo) confirm the parity law and the gapless character of the ribbon for even $n\_ω$.
Employing a spin-parameterized Kleldysh-Usadel technique for the diffusive regime, we demonstrate that even in the low proximity limit, considerable long-ranged triplet supercurrents can be effectively generated by spin-singlet supercurrents flowing \textit{parallel} to the interfaces of uniform double ferromagnet interlayers with noncollinear exchange fields "{\it independent}" of actual junction geometry. The triplet supercurrents are found to be most pronounced when the thicknesses of the ferromagnet strips are unequal. To experimentally verify this generic phenomenon, we propose an accessi…
