We study the anomalous Josephson effect, as well as the dependence on the direction of the critical Josephson current, in an S/N/S junction, where the normal part is realized by alternating spin-orbit coupled and ferromagnetic layers. We show that to observe these effects it is sufficient to break spin rotation and time reversal symmetry in spatially separated regions of the junction. Moreover, we discuss how to further improve these effects by engineering multilayers structures with more that one couple of alternating layers.
Measurement of multiple Andreev reflection (MAR) in a Josephson junction made from an InAs heterostructure with epitaxial aluminum is used to quantify the highly transparent semiconductor-superconductor interface, indicating near-unity transmission. The observed temperature dependence of MAR does not follow a conventional BCS form, but instead agrees with a model in which the density of states in the quantum well acquires an effective induced gap, in our case 180 μeV, close to that of the epitaxial superconductor. Carrier density dependence of MAR is investigated using a depletion gate, reveal…
We investigate the Josephson radiation of nanowire (NW)-based Josephson junctions in a parallel magnetic field. The Josephson junction made of an InAs NW with superconducting Al leads shows the emission spectra which follow the Josephson frequency $f_{J}$ over the range 4-8 GHz at zero magnetic field. We observe an apparent deviation of the emission spectra from the Josephson frequency which is accompanied by a strong enhancement of the switching current above a magnetic field of $\sim 300$ mT. The observed modulations can be understood to reflect trivial changes in the superconducting circuit…
We combine electron beam lithography and masked anodization of epitaxial aluminium to define tunnel junctions via selective oxidation, alleviating the need for wet-etch processing or direct deposition of dielectric materials. Applying this technique to define Josephson junctions in proximity induced superconducting Al-InAs heterostructures, we observe multiple Andreev reflections in transport experiments, indicative of a high quality junction. We further compare the mobility and density of Hall-bars defined via wet etching and anodization. These results may find utility in uncovering new fabri…
When two superconductors are connected across a ferromagnet, the spin configuration of the transferred Cooper pairs can be modulated due to magnetic exchange interaction. The resulting supercurrent can reverse its sign across the Josephson junction (JJ) [1-4]. Here we demonstrate Josephson phase modulation in van der Waals heterostructures when Cooper pairs from superconducting NbSe$_2$ tunnel through atomically thin magnetic insulator (MI) Cr$_2$Ge$_2$Te$_6$. Employing a superconducting quantum interference device based on MI JJs, we probe a doubly degenerate non-trivial JJ phase ($ϕ$) origin…
It is shown that the anomalous elasticity of membranes affects the profile and thermodynamics of a bubble in van der Waals heterostructures. Our theory generalizes the non-linear plate theory as well as membrane theory of the pressurised blister test to incorporate the power-law scale dependence of the bending rigidity and Young's modulus of a two-dimensional crystalline membrane. This scale dependence caused by long-ranged interaction of relevant thermal fluctuations (flexural phonons), is responsible for the anomalous Hooke's law observed recently in graphene. It is shown that this anomalous…
In this paper, we study topological properties and Hall conductivities in PbC/MnSe heterostructure under the illumination of a circularly polarized light. At high frequency regime, energy gap, Chern numbers, and Hall conductivities are studied based on the Floquet theory and Green's function formalism, respectively. The interplay between spin orbit coupling and light leads to topological phase transition between anomalous Hall states and spin Hall states, which is related to the emission and absorption of two virtual photons. The anomalous Hall conductivities are dependent on polarization of l…
Based on ab initio calculations, we predict that a monolayer of Cr-doped (Bi,Sb)2Te3 and GdI2 heterostructure is a quantum anomalous Hall insulator with a non-trivial band gap up to 38 meV. The principle behind our prediction is that the band inversion between two topologically trivial ferromagnetic insulators can result in a non-zero Chern number, which offers a better way to realize the quantum anomalous Hall state without random magnetic doping. In addition, a simple effective model is presented to describe the basic mechanism of spin polarized band inversion in this system. Moreover, we pr…
We numerically study the general valley polarization and anomalous Hall effect in van der Waals (vdW) heterostructures based on monolayer jacutingaite family materials Pt$_{2}$AX$_{3}$ (A = Hg, Cd, Zn; X = S, Se, Te). We perform a systematic study on the atomic, electronic, and topological properties of vdW heterostructures composed of monolayer Pt$_{2}$AX$_{3}$ and two-dimensional ferromagnetic insulators. We show that four kinds of vdW heterostructures exhibit valley-polarized quantum anomalous Hall phase, i.e., Pt$_{2}$HgS$_{3}$/NiBr$_{2}$, Pt$_{2}$HgSe$_{3}$/CoBr$_{2}$, Pt$_{2}$HgSe$_{3}$/…
Hall effect of two-dimensional holes that are spin-polarized by a strong parallel magnetic field was explored with a small tilt angle. The Hall resistivity increases nonlinearly with the magnetic field and exhibits negative corrections. The anomalous negative corrections increase with the perpendicular magnetization of the two-dimensional hole system. We attribute this to the anomalous Hall effect of spin-polarized carriers in a nonmagnetic system. The anomalous corrections to the conductivity exhibit non-monotonic dependence on the magnetic field.
Semiconductor-based Josephson junctions provide a platform for studying proximity effect due to the possibility of tuning junction properties by gate voltage and large-scale fabrication of complex Josephson circuits. Recently Josephson junctions using InAs weak link with epitaxial aluminum contact have improved the product of normal resistance and critical current, $I_cR_N$, in addition to fabrication process reliability. Here we study similar devices with epitaxial contact and find large supercurrent and substantial product of $I_cR_N$ in our junctions. However we find a striking difference w…
Monolayer transition metal dichalcogenides(2D) and zero dimensional quantum dots(QD) are known to have unique optical properties in their individual limit such as high binding energy of excitons. The combination of these two systems is of particular interest in understanding various aspects of energy transfer, charge transfer, dynamics of excitons, etc. In this manuscript, we report the anomalous photoluminescence(PL) emission in one such heterostructure MoS2-CdSe QD. We observe multiple exciton emission peaks of the heterostructure on hBN substrate which are absent on SiO2. Our observation op…
Thermoelectric measurements have the potential to uncover the density of states of low-dimensional materials. Here, we present the anomalous thermoelectric behaviour of mono-layer graphene-nanowire (NW) heterostructures, showing large oscillations as a function of doping concentration. Our devices consist of InAs NW and graphene vertical heterostructures, which are electrically isolated by thin ($\sim$ 10nm) hexagonal boron nitride (hBN) layers. In contrast to conventional thermoelectric measurements, where a heater is placed on one side of a sample, we use the InAs NW (diameter $\sim 50$ nm) …
We demonstrate the van der Waals epitaxy of the topological insulator compound Bi2Te3 on the ferromagnetic insulator Cr2Ge2Te6. The layers are oriented with (001) of Bi2Te3 parallel to (001) of Cr2Ge2Te6 and (110) of Bi2Te3 parallel to (100) of Cr2Ge2Te6. Cross-sectional transmission electron microscopy indicates the formation of a sharp interface. At low temperatures, bilayers consisting of Bi2Te3 on Cr2Ge2Te6 exhibit a large anomalous Hall effect (AHE). Tilted field studies of the AHE indicate that the easy axis lies along the c-axis of the heterostructure, consistent with magnetization meas…
We studied anomalous Josephson effect (AJE) in Josephson trijunctions fabricated on Bi$_2$Se$_3$, and found that the AJE in T-shaped trijunctions significantly alters the Majorana phase diagram of the trijunctions, when an in-plane magnetic field is applied parallel to two of the three single junctions. Such a phenomenon in topological insulator-based Josephson trijunction provides unambiguous evidence for the existence of AJE in the system, and might provide an additional knob for controlling the Majorana bound states in the Fu-Kane scheme of topological quantum computation.
The transparent interface in epitaxial Al-InAs heterostructures provides an excellent platform for potential advances in mesoscopic and topological superconductivity. Semiconductor-based Josephson Junction Field Effect Transistors (JJ-FETs) fabricated on these heterostructures have a metallic gate that tunes the supercurrent. Here we report the fabrication and measurement of gate-tunable Al-InAs JJ-FETs in which the gate dielectric in contact with the InAs is produced by mechanically exfoliated hexagonal boron nitride (h-BN) followed by dry transfer using a van der Waals-mediated pick up proce…
Charge transfer mediated anomalous photoluminescence enhancement in monolayer MoS2 graphene heterostructure via polystyrene assisted wet transfer
Nanomagnetism and Microscopy Laboratory, Department of Physics, Indian Institute of Technology Hyderabad（印度理工学院海得拉巴分校）；Tata Institute of Fundamental Research Hyderabad（塔塔基础研究所海得拉巴分所）
This review discusses the electronic properties and the prospective research directions of superconductor-graphene heterostructures. The basic electronic properties of graphene are introduced to highlight the unique possibility of combining two seemingly unrelated physics, superconductivity and relativity. We then focus on graphene-based Josephson junctions, one of the most versatile superconducting quantum devices. The various theoretical methods that have been developed to describe graphene Josephson junctions are examined, together with their advantages and limitations, followed by a discus…
We study Josephson junctions made of semiconducting nanowires with Rashba spin-orbit coupling, where superconducting correlations are induced by the proximity effect. In the presence of a suitably directed magnetic field, the system displays the anomalous Josephson effect: a nonzero supercurrent in the absence of a phase bias between two superconductors. We show that this anomalous current can be increased significantly by tuning the nanowire into the helical regime. In particular, in a short junction, a large anomalous current is a signature for topologically nontrivial superconductivity in t…
For a general model of a mesoscopic multi-level quantum dot, we determine the necessary conditions for the existence of an anomalous Josephson current with spontaneously broken time-reversal symmetry. They correspond to a finite spin-orbit coupling, a suitably oriented Zeeman field, and the dot being a chiral conductor. We provide analytical expressions for the anomalous supercurrent covering a wide parameter regime.
We calculate the supercurrent through a Josephson junction consisting of a phase-coherent metal particle (quantum dot), weakly coupled to two superconductors. The classical motion in the quantum dot is assumed to be chaotic on time scales greater than the ergodic time $τ_{erg}$, which itself is much smaller than the mean dwell time $τ_{dwell}$. The excitation spectrum of the Josephson junction has a gap $E_{gap}$, which can be less than the gap $Δ$ in the bulk superconductors. The average supercurrent is computed in the ergodic regime $τ_{erg} \ll \hbar/Δ$, using random-matrix theory, and in t…
The search of novel topological phases, such as the quantum anomalous Hall insulator (QAHI) or the axion insulator, has motivated different schemes to introduce magnetism into topological insulators. One scheme is to introduce ferromagnetic dopants in topological insulators. However, it is generally challenging and requires carefully engineered growth/heterostructures or relatively low temperatures to observe the QAHI due to issues such as the added disorder with ferromagnetic dopants. Another promising scheme is using the magnetic proximity effect with a magnetic insulator to magnetize the to…
We propose a setup involving Majorana bound states (MBS) hosted by a vortex on a superconducting surface of a 3D Topological Insulator (TI). We consider a narrow channel drilled across a TI slab with both sides covered by s-wave superconductor. In the presence of a vortex pinned to such a channel, it acts as a ballistic nanowire connecting the superconducting surfaces, with a pair of MBS localized in it. The energies of the MBS possess a 4π-periodic dependence on the superconductive phase difference ϕbetween the surfaces. It results in the appearence of an anomalous term in the current-phase r…
We use magnetotransport in dual-gated magnetic topological insulator heterostructures to map out a phase diagram of the topological Hall and quantum anomalous Hall effects as a function of the chemical potential (primarily determined by the back gate voltage) and the asymmetric potential (primarily determined by the top gate voltage). A theoretical model that includes both surface states and valence band quantum well states allows the evaluation of the variation of the Dzyaloshinskii-Moriya interaction and carrier density with gate voltages. The qualitative agreement between experiment and the…
A superconductor-semiconducting nanowire-superconductor heterostructure in the presence of spin orbit coupling and magnetic field can support a supercurrent even in the absence of phase difference between the superconducting electrodes. We investigate this phenomenon, the anomalous Josephson effect, employing a model capable of describing many bands in the normal region. We discuss geometrical and symmetry conditions required to have finite anomalous supercurrent and in particular we show that this phenomenon is enhanced when the Fermi level is located close to a band opening in the normal reg…
Local and nonlocal differential resistance measurements on Hall bars defined in AlO$_x$/KTaO$_3$ heterostructures show anomalous behavior that depends on the crystal orientation and the applied back gate voltage. The local differential resistance is asymmetric in the dc bias current, with an antisymmetric component that grows with decreasing gate voltage. More surprisingly, a large nonlocal differential resistance is observed that extends between measurement probes that are separated by 100s of microns. The potential source of this anomalous behavior is discussed.
Two-dimensional systems that host one-dimensional helical states are exciting from the perspective of scalable topological quantum computation when coupled with a superconductor. Graphene is particularly promising for its high electronic quality, versatility in van der Waals heterostructures and its electron and hole-like degenerate 0$th$ Landau level. Here, we study a compact double layer graphene SQUID (superconducting quantum interference device), where the superconducting loop is reduced to the superconducting contacts, connecting two parallel graphene Josephson junctions. Despite the smal…
Half-quantized anomalous Hall conductance in topological insulator/ferromagnet van der Waals heterostructures
Linnaeus University（林奈大学）；Nordita, KTH Royal Institute of Technology and Stockholm University（北欧原子理论中心，皇家理工学院和斯德哥尔摩大学）；University of Connecticut（康涅狄格大学）；University of Texas at El Paso（德克萨斯大学埃尔帕索分校）；University of Texas at Austin（德克萨斯大学奥斯汀分校）
The anomalous proximity effect in dirty superconducting junctions is one of most striking phenomena highlighting the profound nature of Majorana bound states and odd-frequency Cooper pairs in topological superconductors. Motivated by the recent experimental realization of planar topological Josephson junctions, we describe the anomalous proximity effect in a superconductor/semiconductor hybrid, where an additional dirty normal-metal segment is extended from a topological Josephson junction. The topological phase transition in the topological Josephson junction is accompanied by a drastic chang…
The anomalous ground state phase shift in S/AF/S Josephson junctions in the presence of the Rashba SO-coupling is predicted and numerically investigated. It is found to be a consequence of the uncompensated magnetic moment at the S/AF interfaces. The anomalous phase shift exhibits a strong dependence on the value of the SO-coupling and the sublattice magnetization with the simultaneous existence of stable and metastable branches. It depends strongly on the orientation of the Neel vector with respect to the S/AF interfaces via the dependence on the orientation of the interface uncompensated mag…
We theoretically study the Josephson current in a superconductor/quantum anomalous Hall insulator/superconductor junction by using the lattice Green function technique. When an in-plane external Zeeman field is applied to the quantum anomalous Hall insulator, the Josephson current $J$ flows without a phase difference across the junction $θ$. The phase shift $φ$ appealing in the current-phase relationship $J\propto \sin(θ-φ$) is proportional to the amplitude of Zeeman fields and depends on the direction of Zeeman fields. A phenomenological analysis of the Andreev reflection processes explains t…
In this work we probe the third-order non-linear optical property of graphene, hexagonal boron nitride and their heterostructure by the use of coherent anti-Stokes Raman Spectroscopy. When the energy difference of the two input fields match the phonon energy, the anti-Stokes emission intensity is enhanced in h-BN, as usually expected while for graphene a anomalous decrease is observed. This behaviour can be understood in terms of q coupling between the electronic continuum and a discrete phonon state. We have also measured a graphene/h-BN heterostructure and demonstrate that the anomalous effe…
We investigate anomalous Hall effect in a magnet coupled to a triplet superconductor under phase gradient. It is found that the anomalous Hall supercurrent arises from non-trivial structure of the magnetization. The magnetic structure manifested in the Hall supercurrent is characterized by even order terms of the exchange coupling, essentially different from that discussed in the context of anomalous Hall effect, reflecting the disspationless nature of supercurrent. We also discuss a possible candidate for magnetic structure to verify our prediction.
Superconductor-ferromagnet (S-F) interfaces in two-dimensional (2D) heterostructures present a unique opportunity to study the interplay between superconductivity and ferromagnetism. The realization of such nanoscale heterostructures in van der Waals (vdW) crystals remains largely unexplored due to the challenge of making an atomically-sharp interface from their layered structures. Here, we build a vdW ferromagnetic Josephson junction (JJ) by inserting a few-layer ferromagnetic insulator Cr2Ge2Te6 into two layers of superconductor NbSe2. Owing to the remanent magnetic moment of the barrier, th…
Van der Waals heterostructures constitute a platform for investigating intriguing many-body quantum phenomena. In particular, transition-metal dichalcogenide (TMD) hetero-bilayers host long-lived interlayer excitons which exhibit permanent out-of-plane dipole moments. Here, we develop a microscopic theory for interlayer exciton-exciton interactions including both the dipolar nature of interlayer excitons as well as their fermionic substructure, which gives rise to an attractive fermionic exchange. We find that these interactions contribute to a drift force resulting in highly non-linear excito…
Correlated charge inhomogeneity breaks the electron-hole symmetry in two-dimensional (2D) bilayer heterostructures which is responsible for non-zero drag appearing at the charge neutrality point. Here we report Coulomb drag in novel drag systems consisting of a two-dimensional graphene and a one dimensional (1D) InAs nanowire (NW) heterostructure exhibiting distinct results from 2D-2D heterostructures. For monolayer graphene (MLG)-NW heterostructures, we observe an unconventional drag resistance peak near the Dirac point due to the correlated inter-layer charge puddles. The drag signal decreas…
We consider a ballistic Josephson junction with a quantum point contact in a two-dimensional electron gas with Rashba spin-orbit coupling. The point contact acts as a spin filter when embedded in a circuit with normal electrodes. We show that with an in-plane external magnetic field an anomalous supercurrent appears even for zero phase difference between the superconducting electrodes. In addition, the external field induces large critical current asymmetries between the two flow directions, leading to supercurrent rectifying effects.
We have confirmed the k-dependent spin splitting in wurtzite AlxGa1-xN/GaN heterostructures. Anomalous beating pattern in Shubnikov-de Haas measurements arises from the interference of Rashba and Dresselhaus spin-orbit interactions. The dominant mechanism for the k-dependent spin splitting at high values of k is attributed to Dresselhaus term which is enhanced by the Delta C1-Delta C3 coupling of wurtzite band folding effect.
We investigate theoretically the Josephson junction of semiconductor nanowire with strong spin-orbit (SO) interaction in the presence of magnetic field. By using a tight-binding model, the energy levels $E_n$ of Andreev bound states are numerically calculated as a function of phase difference $φ$ between two superconductors in the case of short junctions. The DC Josephson current is evaluated from the Andreev levels. In the absence of SO interaction, a $0$-$π$ transition due to the magnetic field is clearly observed. In the presence of SO interaction, the coexistence of SO interaction and Zeem…
We study Josephson effect of $d$-wave superconductor (DS)/ferromagnet insulator(FI)/DS junctions on a surface of topological insulator (TI). We calculate Josephson current $I\left(φ\right) $ for various orientations of the junctions where $φ$ is the macroscopic phase difference between two DSs. In certain configurations, we find anomalous current-phase relation $I(φ)=-I\left( -φ+π\right)$ with $2π$ periodicity. In the case where the first order Josephson coupling is absent without magnetization in FI, $I(φ)$ can be proportional to $\cos φ$. The magnitude of the obtained Josephson current is en…
Periodically driven Kitaev chains are known to exhibit novel Floquet Majorana fermions and anomalous Floquet end modes. The fact that `quasienergy in Floquet systems is periodic' poses a difficulty in defining the ground state in periodically driven systems. To overcome this problem, we start with the ground state of the undriven Kitaev chain and gradually switch on the periodic driving in chemical potential over a timescale $τ$. The extent to which the single particle eigenstates of the undriven system get distributed among the Floquet states upon driving can be characterized by inverse parti…
We demonstrate the transfer of the superconducting properties of NbTi---a large-gap high-critical-field superconductor---into an InAs heterostructure via a thin intermediate layer of epitaxial Al. Two device geometries, a Josephson junction and a gate-defined quantum point contact, are used to characterize interface transparency and the two-step proximity effect. In the Josephson junction, multiple Andreev reflection reveal near-unity transparency, with an induced gap $Δ^*=0.50~\mathrm{meV}$ and a critical temperature of $7.8~\mathrm{K}$. Tunneling spectroscopy yields a hard induced gap in the…
In a standard Josephson junction the current is zero when the phase difference between the superconducting leads is zero. This condition is protected by parity and time-reversal symmetries. However, the combined presence of spin-orbit coupling and magnetic field breaks these symmetries and can lead to a finite supercurrent even when the phase difference is zero. This is the so called anomalous Josephson effect -- the hallmark effect of superconducting spintronics --and can be characterized by the corresponding anomalous phase shift ($ϕ_0$). We report the observation of a tunable anomalous Jose…
Universal scaling of the Anomalous Hall voltage of magnetic layer with the adjacent conducting layer
State Key Laboratory of Semiconductor Physics and Chip Technologies, Institute of Semiconductors, Chinese Academy of Sciences（中国科学院半导体研究所半导体物理与芯片技术国家重点实验室）；Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences（中国科学院大学材料科学与光电技术学院）
We study the frictional drag between carriers in two bilayer graphene flakes separated by a 2 $-$ 5 nm thick hexagonal boron nitride dielectric. At temperatures ($T$) lower than $\sim$ 10 K, we observe a large anomalous negative drag emerging predominantly near the drag layer charge neutrality. The anomalous drag resistivity increases dramatically with reducing {\it T}, and becomes comparable to the layer resistivity at the lowest {\it T} = 1.5 K. At low $T$ the drag resistivity exhibits a breakdown of layer reciprocity. A comparison of the drag resistivity and the drag layer Peltier coefficie…
We demonstrate advantages of samples made by mechanical stacking of exfoliated van der Waals materials for controlling the topological surface state of a 3-dimensional topological insulator (TI) via interaction with an adjacent magnet layer. We assemble bilayers with pristine interfaces using exfoliated flakes of the TI BiSbTeSe2 and the magnet Cr2Ge2Te6, thereby avoiding problems caused by interdiffusion that can affect interfaces made by top-down deposition methods. The samples exhibit an anomalous Hall effect (AHE) with abrupt hysteretic switching. For the first time in samples composed of …
