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arXiv 1802.08003cond-mat.mes-hall
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倾斜磁场中过渡金属二硫属化合物单层暗激子的强谷塞曼效应

Strong Valley Zeeman Effect of Dark Excitons in Monolayer Transition Metal Dichalcogenides in a Tilted Magnetic Field

M. Van der Donck, M. Zarenia, F. M. Peeters

摘要:

研究了单层过渡金属二硫属化物(TMD)的激子光致发光(PL)谱随外加磁场倾角的变化关系。从一个四带哈密顿量,我们构建了一个理论,定量再现现有的实验PL谱垂直和面内磁场。在存在倾斜磁场的情况下,我们证明了暗激子PL峰由于磁场的面内分量而变亮,并且由于磁场的垂直分量而对于具有不同圆偏振的光分裂。这种分裂是钨基TMD中亮激子峰分裂的两倍多。我们提出了一个实验装置,将允许访问的PL光谱中的暗激子峰的预测分裂。

英文摘要:

The dependence of the excitonic photoluminescence (PL) spectrum of monolayer transition metal dichalcogenides (TMDs) on the tilt angle of an applied magnetic field is studied. Starting from a four-band Hamiltonian we construct a theory which quantitatively reproduces the available experimental PL spectra for perpendicular and in-plane magnetic fields. In the presence of a tilted magnetic field, we demonstrate that the dark exciton PL peaks brighten due to the in-plane component of the magnetic field and split for light with different circular polarization as a consequence of the perpendicular component of the magnetic field. This splitting is more than twice as large as the splitting of the bright exciton peaks in tungsten-based TMDs. We propose an experimental setup that will allow to access the predicted splitting of the dark exciton peaks in the PL spectrum.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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